arXiv subjects

T. R. Kirkpatrick

Publications and source records attributed to T. R. Kirkpatrick.

At least 19 recordsLinked to original sources

arXiv2026

Generic Long-Range Order-Parameter Correlations in Metallic Quantum Magnets

It is shown that in all types of metallic magnets the coupling of the order parameter to the conduction electrons leads to an order-parameter susceptibility that is long-ranged at zero temperature. This is true for all known classes of ferromagnets, and also for antiferromagnets and spin-density wave systems, helimagnets, magnetic nematics, and altermagnets. The consequences for the magnetic quantum phase transition vary between different classes of magnets. In almost all 3-d systems with a homogeneous magnetization, as well as in magnetic nematics and in altermagnets, the long-ranged correlations generically modify the nature of the magnetic quantum phase transition from second order to first order. The only exception are non-centrosymmetric ferromagnets with a strong spin-orbit interaction, where the correlations change the order of the transition in 2-d systems, but not in 3-d ones. In helimagnets, spin-wave systems, and Neel antiferromagnets their effect is even weaker and does not change the order of the transition if the ordering wave number is sufficiently large, except in flat-band systems. In systems with quenched disorder the transition generically is of second order, but the correlations modify the critical behavior. These conclusions are reached by very simple considerations that are based entirely on the single-particle excitations in the nonmagnetic phase and their modifications by a field conjugate to the order parameter, augmented by renormalization-group considerations.

cond-mat.str-el↗

arXiv2026

Comment on "Instability of the ferromagnetic quantum critical point and symmetry of the ferromagnetic ground state in two-dimensional and three-dimensional electron gases with arbitrary spin-orbit splitting"

Metallic quantum ferromagnets in the absence of quenched disorder are known to generically undergo a first-order quantum phase transition, avoiding the quantum critical point that had originally been expected. This is due to soft modes in the underlying Fermi liquid that lead to long-ranged correlations. These correlations in turn yield a nonanalytic dependence of the free energy on the magnetization even at a mean-field level that results in a fluctuation-induced first-order transition. Kirkpatrick and Belitz [Phys. Rev. Lett. {\bf 124}, 147201 (2020)] have pointed out that one notable exception are non-centrosymmetric metals with a strong spin-orbit interaction. In such materials the spin-orbit interaction gives the relevant soft modes a mass, which inhibits the mechanism leading to a first-order transition. Miserev, Loss, and Klinovaja [Phys. Rev. B {\bf 106}, 134417 (2022)] have claimed that this conclusion does not hold if electron-electron interactions in the particle-particle channel, or 2$\kF$ scattering processes, are considered. They concluded that this interaction channel leads to soft modes that are not rendered massive by the spin-orbit interaction and again lead to a first-order quantum phase transition. In this Comment we show that this conclusion is not correct in three-dimensional magnets if the screening of the interaction is properly taken into account.

cond-mat.str-el↗

arXiv2026

In memoriam J. Robert Dorfman

An obituary of J.R. Dorfman. The focus is on his scientific career and on his many important publications.

cond-mat.stat-mech↗

arXiv2024

Collective dynamic length increases monotonically in pinned and unpinned glass forming systems

The Random First Order Transition Theory (RFOT) predicts that transport proceeds by cooperative movement of particles in domains whose sizes increase as a liquid is compressed above a characteristic volume fraction, $\phi_d$. The rounded dynamical transition around $\phi_d$, which signals a crossover to activated transport, is accompanied by a growing correlation length that is predicted to diverge at the thermodynamic glass transition density ($> \phi_d$). Simulations and imaging experiments probed the single particle dynamics of mobile particles in response to pinning all the particles in a semi-infinite space or randomly pinning (RP) a fraction of particles in a liquid at equilibrium. The extracted dynamic length increases non-monotonically with a peak around $\phi_d$, which not only depends on the pinning method but is different from $\phi_d$ of the actual liquid. This finding is at variance with the results obtained using the small wave length limit of a four-point structure factor for unpinned systems. To obtain a consistent picture of the growth of the dynamic length, one that is impervious to the use of RP, we introduce a multi particle structure factor, $S^c_{mp}(q,t)$, that probes collective dynamics. The collective dynamic length, calculated from the small wave vector limit of $S^c_{mp}(q,t)$, increases monotonically as a function of the volume fraction in glass forming binary mixture of charged colloidal particles in both unpinned and pinned systems. This prediction, which also holds in the presence of added monovalent salt, may be validated using imaging experiments.

cond-mat.soft↗

arXiv2024

Diffusion, Long-Time Tails, and Localization in Classical and Quantum Lorentz Models: A Unifying Hydrodynamic Approach

Long-time tails, or algebraic decay of time-correlation functions, have long been known to exist both in many-body systems and in models of non-interacting particles in the presence of quenched disorder that are often referred to as Lorentz models. In the latter, they have been studied extensively by a wide variety of methods, the best known example being what is known as weak-localization effects in disordered systems of non-interacting electrons. This paper provides a unifying, and very simple, approach to all of these effects. We show that simple modifications of the diffusion equation due to either a random diffusion coefficient, or a random scattering potential, accounts for both the decay exponents and the prefactors of the leading long-time tails in the velocity autocorrelation functions of both classical and quantum Lorentz models.

cond-mat.dis-nn↗

arXiv2024

Fluctuation-Response Relation in Non-Equilibrium Systems and Active Matter

We use dynamic equations to derive a relation between correlation functions and response or relaxation functions in many-body systems. The relation is very general and holds both in equilibrium, when the usual fluctuation-dissipation theorem is valid, and to linear order in an expansion about arbitrary non-equilibrium states, when it is not. We illustrate our results by discussing fluids, both in equilibrium and non-equilibrium states, as well as several active-matter systems.

cond-mat.stat-mech↗

arXiv2024

A Fluctuation-Response Relation as a Probe of Long-Range Correlations in Non-Equilibrium Quantum and Classical Fluids

The absence of a simple fluctuation-dissipation theorem is a major obstacle for studying systems that are not in thermodynamic equilibrium. We show that for a fluid in a non-equilibrium steady state characterized by a constant temperature gradient the commutator correlation functions are still related to response functions; however, the relation is to the bilinear response of products of two observables, rather than to a single linear response function as is the case in equilibrium. This modified fluctuation-response relation holds for both quantum and classical systems. It is both motivated and informed by the long-range correlations that exist in such a steady state and allows for probing them via response experiments. This is of particular interest in quantum fluids, where the direct observation of fluctuations by light scattering would be difficult. In classical fluids it is known that the coupling of the temperature gradient to the diffusive shear velocity leads to correlations of various observables, in particular temperature fluctuations, that do not decay as a function of distance, but rather extend over the entire system. We investigate the nature of these correlations in a fermionic quantum fluid and show that the crucial coupling between the temperature gradient and velocity fluctuations is the same as in the classical case. Accordingly, the nature of the long-ranged correlations in the hydrodynamic regime also is the same. However, as one enters the collisionless regime in the low-temperature limit the nature of the velocity fluctuations changes: they become ballistic rather than diffusive. As a result, correlations of the temperature and other observables are still singular in the long-wavelength limit, but the singularity is weaker than in the hydrodynamic regime.

cond-mat.stat-mech↗

arXiv2023

Fluctuation-dissipation relation in a non-equilibrium quantum fluid

There is no simple fluctuation-dissipation theorem (FDT) for nonequilibrium systems. We show that for a fluid in a nonequilibrium steady state (NESS) characterized by a constant temperature gradient there is a generalized FDT that relates commutator correlation functions to the bilinear response of products of observables. This allows for experimental probes of the long-range correlations in such a system, quantum or classical, via response experiments. We also show that the correlations are not tied to thermal fluctuations but are intrinsic to the NESS and reflect a generalized rigidity.

cond-mat.stat-mech↗

arXiv2023

Free volume theory explains the unusual behavior of viscosity in a non-confluent tissue during morphogenesis

A recent experiment on zebrafish blastoderm morphogenesis showed that the viscosity (η) of a non-confluent embryonic tissue grows sharply until a critical cell packing fraction (ϕS). The increase in η up to ϕS is similar to the behavior observed in several glass-forming materials, which suggests that the cell dynamics is sluggish or glass-like. Surprisingly, η is a constant above ϕS. To determine the mechanism of this unusual dependence of η on ϕ, we performed extensive simulations using an agent-based model of a dense non-confluent two-dimensional tissue. We show that polydispersity in the cell size, and the propensity of the cells to deform, results in the saturation of the available free area per cell beyond a critical packing fraction. Saturation in the free space not only explains the viscosity plateau above ϕS but also provides a relationship between equilibrium geometrical packing to the dramatic increase in the relaxation dynamics.

cond-mat.soft↗

arXiv2023

Velocity-Dependent Forces and Non-Hydrodynamic Initial Conditions in Quantum and Classical Fluids

We consider a fermionic fluid in a non-equilibrium steady state where the fluctuation-dissipation theorem is not valid and fields conjugate to the hydrodynamic variables are explicitly required to determine response functions. We identify velocity-dependent forces in the kinetic equation that are equivalent to such fields. They lead to driving terms in the hydrodynamic equations and to corrections to the hydrodynamic initial conditions.

cond-mat.stat-mech↗

arXiv2022

Topological transitions, turbulent-like motion and long-time-tails driven by cell division in biological tissues

The complex spatiotemporal flow patterns in living tissues, driven by active forces, have many of the characteristics associated with inertial turbulence even though the Reynolds number is extremely low. Analyses of experimental data from two-dimensional epithelial monolayers in combination with agent-based simulations show that cell division and apoptosis lead to directed cell motion for hours, resulting in rapid topological transitions in neighboring cells. These transitions in turn generate both long ranged and long lived clockwise and anticlockwise vortices, which gives rise to turbulent-like flows. Both experiments and simulations show that at long wavelengths the wave vector ($k$) dependent energy spectrum $E(k) \approx k^{-5/3}$, coinciding with the Kolmogorov scaling in fully developed inertial turbulence. Using theoretical arguments and simulations, we show that long-lived vortices lead to long-time tails in the velocity auto-correlation function, $C_v(t) \sim t^{-1/2}$, which has the same structure as in classical 2D fluids but with a different scaling exponent.

cond-mat.soft↗

arXiv2022

Thermal Transport and Non-Mechanical Forces in Metals

We discuss contributions to the thermopower in an electron fluid. A simple argument based on Newton's second law with the pressure gradient as the force suggests that the thermopower is given by a thermodynamic derivative, viz., the entropy per particle, rather than being an independent transport coefficient. The resolution is the existence of an entropic force that results from a coupling between the mass current and the heat current in the fluid. We also discuss and clarify some aspects of a recent paper (Phys. Rev. B {\bf 102}, 214306 (2020)) that provided a method for exactly solving electronic transport equations in the low-temperature limit.

cond-mat.stat-mech↗

arXiv2022

Soft modes in Fermi liquids at arbitrary temperatures

We use kinetic-theory methods to analyze Landau Fermi-liquid theory, and in particular to investigate the number and nature of soft modes in Fermi liquids, both in the hydrodynamic and the collisionless regimes. In the hydrodynamic regime we show that Fermi-liquid theory is consistent with Navier-Stokes hydrodynamics at all temperatures. The soft modes are the ones familiar from classical hydrodynamics that are controlled by the five conservation laws; namely, two first-sound modes, two shear diffusion modes, and one heat diffusion mode. These modes have a particle-like spectrum and are soft, or scale invariant, at all temperatures. In the collisionless regime we show that the entire single-particle distribution function is soft with a continuous part of the spectrum. This continuous soft mode, which is well known but often not emphasized, has important physical consequences, e.g., for certain quantum phase transitions. In addition, there are the well known soft zero-sound excitations that describe angular fluctuations of the Fermi surface; their spectra are particle-like. They are unrelated to conservation laws, acquire a mass at any nonzero temperature, and their number depends on the strength of the quasiparticle interaction. We also discuss the fates of these two families of soft modes as the temperature changes. With increasing temperature the size of the collisionless regime shrinks, the damping of the modes grows, and eventually all of the collisionless modes become overdamped. In their stead the five hydrodynamic modes appear in the hydrodynamic regime at asymptotically low frequencies. The two families of soft modes are unrelated and have very different physical origins.In charged Fermi liquids the first-sound modes in the hydrodynamic regime and the l=0 zero-sound modes in the collisionless regime get replaced by plasmons, all other modes remain soft.

cond-mat.stat-mech↗

arXiv2022

Fluctuating Quantum Kinetic Theory

We consider a quantum Langevin kinetic equation for a system of fermions. We first derive the Langevin force noise correlation functions in Landau's Fermi-liquid kinetic theory from general considerations. We then use the resulting equation to calculate the equilibrium dynamic structure factor in the collisionless regime at low temperatures. The result is in agreement with the conventional many-body result. We then use the theory to derive both the fluctuating Navier-Stokes equations for a quantum fluid and the fluctuating hydrodynamic equations for fermions in the presence of quenched disorder. We also discuss the modifications needed for the fluctuating hydrodynamic equations to describe an electron fluid with long-ranged interactions, and we prove an H-theorem for the nonlinear Landau kinetic equation.

cond-mat.stat-mech↗

arXiv2021

Rigidity and Superfast Signal Propagation in Fluids and Solids in Non-Equilibrium Steady States

In the 1980s it was theoretically predicted that correlations of various observables in a fluid in a non-equilibrium steady state (NESS) are extraordinarily long-ranged, extending, in a well-defined sense, over the size of the system. This is to be contrasted with correlations in an equilibrium fluid, whose range is typically just a few particle diameters. These NESS correlations were later confirmed by numerous experimental studies. Unlike long-ranged correlations at critical points, these correlations are generic in the sense that they exist for any temperature as long as the system is in a NESS. In equilibrium systems, generic long-ranged correlations are caused by spontaneously broken continuous symmetries and are associated with a generalized rigidity, which in turn leads to a new propagating excitation or mode. For example, in a solid, spatial rigidity leads to transverse sound waves, while in a superfluid, phase rigidity leads to temperature waves known as second sound at finite temperatures, and phonons at zero temperature. More generally, long-ranged spatial correlations imply rigidity irrespective of their physical origin. This implies that a fluid in a NESS should also display a type of rigidity and related anomalous transport behavior. Here we show that this is indeed the case. For the particular case of a simple fluid in a constant temperature gradient, the anomalous transport behavior takes the form of a super-diffusive spread of a constant-pressure temperature perturbation. We also discuss the case of an elastic solid, where we predict a spread that is faster than ballistic.

cond-mat.stat-mech↗

arXiv2021

Activity induced turbulence in driven active matter

Turbulence in driven stratified active matter is considered. The relevant parameters characterizing the problem are the Reynolds number Re and an active matter Richardson-like number,R. In the mixing limit,Re>>1, R<<1, we show that the standard Kolmogorov energy spectrum 5/3 law is realized. On the other hand, in the stratified limit, Re>>1,R>>1, there is a new turbulence universality class with a 7/5 law. The crossover from one regime to the other is discussed in detail. Experimental predictions and probes are also discussed.

cond-mat.soft↗

arXiv2021

Non-Hydrodynamic Initial Conditions are Not Soon Forgotten

Solutions to hydrodynamic equations, which are used for a vast variety of physical problems, are assumed to be specified by boundary conditions and initial conditions on the hydrodynamic variables only. Initial values of other variables are assumed to be irrelevant for a hydrodynamic description. This assumption is not correct because of the existence of long-time-tail effects that are ubiquitous in systems governed by hydrodynamic equations. We illustrate this breakdown of a hydrodynamic description by means of the simple example of diffusion in a disordered electron system.

cond-mat.stat-mech↗

arXiv2020

RFOT theory for glassy dynamics in a single condensed polymer

The number of compact structures of a single condensed polymer (SCP), with similar free energies, grows exponentially with the degree of polymerization. In analogy with structural glasses (SGs), we expect that at low temperatures chain relaxation should occur by activated transitions between the compact metastable states. By evolving the states of the SCP that is linearly coupled to a reference state, we show that, below a dynamical transition temperature ($T_d$), the SCP is trapped in a metastable state leading to slow dynamics. At a lower temperature, $T_K \ne 0$, the configurational entropy vanishes, resulting in a thermodynamic random first order ideal glass transition. The relaxation time obeys the Vogel-Fulcher-Tamman law, diverging at $T=T_0 \approx T_K$. These findings, accord well with the random first order transition theory, establishing that SCP and SG exhibit similar universal characteristics.

cond-mat.soft↗