arXiv subjects

T. Rauscher

Publications and source records attributed to T. Rauscher.

At least 91 records · Page 5Linked to original sources

arXiv2013

Systematic study of (p,γ) reactions on Ni isotopes

A systematic study of the radiative proton capture reaction for all stable nickel isotopes is presented. The results were obtained using 2.0 - 6.0 MeV protons from the 11 MV tandem Van de Graaff accelerator at the University of Notre Dame. The γ-rays were detected by the NSCL SuN detector utilising the γ-summing technique. The results are compared to a compilation of earlier measurements and discrepancies between the previous data are resolved. The experimental results are also compared to the theoretical predictions obtained using the NON-SMOKER and SMARAGD codes. Based on these comparisons an improved set of astrophysical reaction rates is proposed for the (p,γ) reactions on the stable nickel isotopes as well as for the 56Ni(p,γ)57Cu reaction.

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arXiv2013

Constraining the astrophysical origin of the p-nuclei through nuclear physics and meteoritic data

A small number of naturally occurring, proton-rich nuclides (the p-nuclei) cannot be made in the s- and r-process. Their origin is not well understood. Massive stars can produce p-nuclei through photodisintegration of pre-existing intermediate and heavy nuclei. This so-called gamma-process requires high stellar plasma temperatures and occurs mainly in explosive O/Ne burning during a core-collapse supernova. Although the gamma-process in massive stars has been successful in producing a large range of p-nuclei, significant deficiences remain. An increasing number of processes and sites has been studied in recent years in search of viable alternatives replacing or supplementing the massive star models. A large number of unstable nuclei, however, with only theoretically predicted reaction rates are included in the reaction network and thus the nuclear input may also bear considerable uncertainties. The current status of astrophysical models, nuclear input, and observational constraints is reviewed. After an overview of currently discussed models, the focus is on the possibility to better constrain those models through different means. Meteoritic data not only provide the actual isotopic abundances of the p-nuclei but can also put constraints on the possible contribution of proton-rich nucleosynthesis. The main part of the review focusses on the nuclear uncertainties involved in the determination of the astrophysical reaction rates required for the extended reaction networks used in nucleosynthesis studies. Experimental approaches are discussed together with their necessary connection to theory, which is especially pronounced for reactions with intermediate and heavy nuclei in explosive nuclear burning, even close to stability.

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arXiv2013

Neutron capture cross section of unstable 63Ni: implications for stellar nucleosynthesis

The $^{63}$Ni($n, γ$) cross section has been measured for the first time at the neutron time-of-flight facility n\_TOF at CERN from thermal neutron energies up to 200 keV. In total, capture kernels of 12 (new) resonances were determined. Maxwellian Averaged Cross Sections were calculated for thermal energies from kT = 5 keV to 100 keV with uncertainties around 20%. Stellar model calculations for a 25 M$_\odot$ star show that the new data have a significant effect on the $s$-process production of $^{63}$Cu, $^{64}$Ni, and $^{64}$Zn in massive stars, allowing stronger constraints on the Cu yields from explosive nucleosynthesis in the subsequent supernova.

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arXiv2013

Proton-rich nucleosynthesis and nuclear physics

Although the detailed conditions for explosive nucleosynthesis are derived from astrophysical modeling, nuclear physics determines fundamental patterns in abundance yields, not only for equilibrium processes. Focussing on the nu-p- and the gamma-process, general nucleosynthesis features within the range of astrophysical models, but (mostly) independent of details in the modelling, are presented. Remaining uncertainties due to uncertain Q-values and reaction rates are discussed.

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arXiv2012

General properties of astrophysical reaction rates in explosive nucleosynthesis

Fundamental differences in the prediction of reaction rates with intermediate and heavy target nuclei compared to the ones with light nuclei are discussed, with special emphasis on stellar modifications of the rates. Ground and excited state contributions to the stellar rates are quantified, deriving a linear weighting of excited state contributions despite of a Boltzmann population of the nuclear states. A Coulomb suppression effect of the excited state contributions is identified, acting against the usual Q-value rule in some reactions. The proper inclusion of experimental data in revised stellar rates is shown, containing revised uncertainties. An application to the s-process shows that the actual uncertainties in the neutron capture rates are larger than would be expected from the experimental errors alone. Sensitivities of reaction rates and cross sections are defined and their application in reaction studies is discussed. The conclusion provides a guide to experiment as well as theory on how to best improve the rates used in astrophysical simulations and how to assess their uncertainties.

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arXiv2012

Investigation of the reaction 74Ge(p,gamma)75As using the in-beam method to improve reaction network predictions for p nuclei

A measurement of 74Ge(p,gamma)75As at low proton energies, inside the astrophysically relevant energy region, is important in several respects. The reaction is directly important as it is a bottleneck in the reaction flow which produces the lightest p nucleus 74Se. It is also an important addition to the data set required to test reaction-rate predictions and to allow an improvement in the global p+nucleus optical potential required in such calculations. An in-beam experiment was performed, making it possible to measure in the energy range between 2.1 and 3.7 MeV, which is for the most part inside the astrophysically relevant energy window. Angular distributions of the gamma-ray transitions were measured with high-purity germanium detectors at eight angles relative to the beam axis. In addition to the total cross sections, partial cross sections for the direct population of twelve levels were determined. The resulting cross sections were compared to Hauser-Feshbach calculations using the code SMARAGD. Only a constant renormalization factor of the calculated proton widths allowed a good reproduction of both total and partial cross sections. The accuracy of the calculation made it possible to check the spin assignment of some states in 75As. In the case of the 1075 keV state, a double state with spins and parities of 3/2- and 5/2- is needed to explain the experimental partial cross sections. A change in parity from 5/2+ to 5/2- is required for the state at 401 keV. Furthermore, in the case of 74Ge, studying the combination of total and partial cross sections made it possible to test the gamma width, which is essential in the calculation of the astrophysical 74$As(n,gamma)75As rate.

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arXiv2012

Investigation of alpha-induced reactions on 127I for the astrophysical gamma process

(Shorten version of the PRC abstract) Alpha-induced reactions on 127I have been studied using the activation technique in order to provide cross section data for the modeling of the astrophysical gamma process. The relative intensity of the 536.1 keV gamma transition was measured precisely, its uncertainty was reduced from 13% to 4%. By measuring the yield of the characteristic X-rays, the cross sections of the 127I(alpha,gamma)131Cs reaction have been determined for the first time close to the astrophysically relevant energy region, at energies 9.50 < Ec.m. < 15.15$ MeV. The 127I(alpha,n)130Cs reaction was studied in the range 9.62 < Ec.m. < 15.15 MeV by measuring the yield of the 536.1 keV gamma-ray and at the lower part of this energy range by counting the characteristic X-rays. A comparison of the resulting cross sections to predictions of statistical model calculations confirmed the predictions of the astrophysically relevant averaged alpha width. Nevertheless, the newly derived stellar reaction rates at gamma process temperatures for 127I(alpha,gamma)131$Cs and its reverse reaction are factors 4-10 faster than previous calculations, due to improvements in the reaction model.

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arXiv2012

Astrophysical analysis of the measurement of (alpha,gamma) and (alpha,n) cross sections of 169Tm

Reaction cross sections of 169Tm(alpha,gamma)173Lu and 169Tm(alpha,n)172Lu have been measured in the energy range 12.6<=E_alpha<=17.5 MeV and 11.5<=E_alpha<=17.5 MeV, respectively, using the recently introduced method of combining activation with X-ray counting. Improved shielding allowed to measure the (alpha,gamma) to lower energy than previously possible. The combination of (alpha,gamma) and (alpha,n) data made it possible to study the energy dependence of the alpha width. While absolute value and energy dependence are perfectly reproduced by theory at energies above 14 MeV, the observed change in energy dependence at energies below 14 MeV requires a modification of the predicted alpha width. Using an effective, energy-dependent, local optical alpha+nucleus potential it is possible to reproduce the data but the astrophysical rate is still not well constrained at gamma-process temperatures. The additional uncertainty stemming from a possible modification of the compound formation cross section is discussed. Including the remaining uncertainties, the recommended range of astrophysical reaction rate values at 2 GK is higher than the previously used values by factors of 2-37.

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arXiv2012

Sensitivity of astrophysical reaction rates to nuclear uncertainties

Sensitivities of nuclear reaction rates to a variation of nuclear properties are studied. Target nuclei range from proton- to neutron-dripline for 10<=Z<=83. Reactions considered are nucleon- and alpha-induced reactions mediated by the strong interaction. The contribution of reactions proceeding on the target ground state to the total stellar rate is also given. General dependences on various input quantities are discussed. Additionally, sensitivities of laboratory cross sections of nucleon-, alpha-, and gamma-induced reactions are shown, allowing to estimate the impact of cross section measurements. Finally, recommended procedures to explore and improve reaction rate uncertainties using the present sensitivity data are outlined.

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arXiv2012

Investigation of alpha-induced reactions on 130Ba and 132Ba and their importance for the synthesis of heavy p nuclei

Captures of alpha particles on the proton-richest Barium isotope, 130Ba, have been studied in order to provide cross section data for the modeling of the astrophysical gamma process. The cross sections of the 130Ba(alpha,gamma)134Ce and 130Ba(alpha,n)133Ce reactions have been measured with the activation technique in the center-of mass energy range between 11.6 and 16 MeV, close above the astrophysically relevant energies. As a side result, the cross section of the 132Ba(alpha,n)135Ce reaction has also been measured. The results are compared with the prediction of statistical model calculations, using different input parameters such as alpha+nucleus optical potentials. It is found that the (alpha,n) data can be reproduced employing the standard alpha+nucleus optical potential widely used in astrophysical applications. Assuming its validity also in the astrophysically relevant energy window, we present new stellar reaction rates for 130Ba(alpha,gamma)134Ce and 132Ba(alpha,gamma)136Ce and their inverse reactions calculated with the SMARAGD statistical model code. The highly increased 136Ce(gamma,alpha)132Ba rate implies that the p nucleus 130Ba cannot directly receive contributions from the Ce isotopic chain. Further measurements are required to better constrain this result.

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arXiv2011

Determination of 141Pr(alpha,n)144Pm cross sections at energies of relevance for the astrophysical p-process using the gamma-gamma coincidence method

The reaction 141Pr(alpha,n)144Pm was investigated between E_alpha=11 MeV and 15 MeV with the activation method using the gamma-gamma coincidence method with a segmented clover-type high-purity Germanium (HPGe) detector. Measurements with four other HPGe detectors were additionally made. The comparison proves that the gamma-gamma coincidence method is an excellent tool to investigate cross sections down to the microbarn range. The (alpha,n) reaction at low energy is especially suited to test alpha+nucleus optical-model potentials for application in the astrophysical p-process. The experimentally determined cross sections were compared to Hauser-Feshbach statistical model calculations using different optical potentials and generally an unsatisfactory reproduction of the data was found. A local potential was constructed to improve the description of the data. The consequences of applying the same potential to calculate astrophysical (gamma,alpha) rates for 145Pm and 148Gd were explored. In summary, the data and further results underline the problems in global predictions of alpha+nucleus optical potentials at astrophysically relevant energies.

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arXiv2011

Opportunities to constrain astrophysical reaction rates for the s-process through determination of the ground state cross sections

Modern models of s-process nucleosynthesis in stars require stellar reaction rates with high precision. Most of the neutron capture cross sections in the s-process have been measured and for an increasing number of reactions the required precision is achieved. This does not necessarily mean, however, that the stellar rates are constrained equally well because only capture on the ground state of a target is measured in the laboratory. Captures on excited states can considerably contribute to stellar rates already at typical s-process temperatures. We show that the ground state contribution X to a stellar rate is the relevant measure to identify reactions which are or could be well constrained by experiments and apply it to (n,gamma) reactions in the s-process. It is further shown that the maximally possible reduction in uncertainty of a rate through determination of the g.s. cross section is directly given by X. An error analysis of X is presented and it is found that X is a robust measure with overall small uncertainties. Several specific examples (neutron capture on 79Se, 95Zr, 121Sn, 187Os, and 193Pt) are discussed in detail. The ground state contributions for a set of 411 neutron capture reactions around the s-process path are presented in a table. This allows to identify reactions which may be better constrained by experiments and such which cannot be constrained by only measuring ground state cross sections (and thus require supplementary studies). General trends and implications are discussed.

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arXiv2011

Cross sections for proton-induced reactions on Pd isotopes at energies relevant for the gamma process

Proton-activation reactions on natural and enriched palladium samples were investigated via the activation technique in the energy range of E_p=2.75 MeV to 9 MeV, close to the upper end of the respective Gamow window of the gamma process. We have determined cross sections for 102Pd(p,gamma)103Ag, 104Pd(p,gamma)105Ag, and 105Pd(p,n)105Ag, as well as partial cross sections of 104Pd(p,n)104Ag^g, 105Pd(p,gamma)106Ag^m, 106Pd(p,n)106Ag^m, and 110Pd(p,n)110Ag^m with uncertainties between 3% and 15% for constraining theoretical Hauser-Feshbach rates and for direct use in gamma-process calculations.

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arXiv2011

The Path to Improved Reaction Rates for Astrophysics

This review focuses on nuclear reactions in astrophysics and, more specifically, on reactions with light ions (nucleons and alpha particles) proceeding via the strong interaction. It is intended to present the basic definitions essential for studies in nuclear astrophysics, to point out the differences between nuclear reactions taking place in stars and in a terrestrial laboratory, and to illustrate some of the challenges to be faced in theoretical and experimental studies of those reactions. The discussion revolves around the relevant quantities for astrophysics, which are the astrophysical reaction rates. The sensitivity of the reaction rates to the uncertainties in the prediction of various nuclear properties is explored and some guidelines for experimentalists are also provided.

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arXiv2011

Core-collapse supernova explosions triggered by a quark-hadron phase transition during the early post-bounce phase

We explore explosions of massive stars, which are triggered via the quark-hadron phase transition during the early post bounce phase of core-collapse supernovae. We construct a quark equation of state, based on the bag model for strange quark matter. The transition between the hadronic and the quark phases is constructed applying Gibbs conditions. The resulting quark-hadron hybrid equations of state are used in core-collapse supernova simulations, based on general relativistic radiation hydrodynamics and three flavor Boltzmann neutrino transport in spherical symmetry. The formation of a mixed phase reduces the adiabatic index, which induces the gravitational collapse of the central protoneutron star. The collapse halts in the pure quark phase, where the adiabatic index increases. A strong accretion shock forms, which propagates towards the protoneutron star surface. Due to the density decrease of several orders of magnitude, the accretion shock turns into a dynamic shock with matter outflow. This moment defines the onset of the explosion in supernova models that allow for a quark-hadron phase transition, where otherwise no explosions could be obtained. The shock propagation across the neutrinospheres releases a burst of neutrinos. This serves as a strong observable identification for the structural reconfiguration of the stellar core. The ejected matter expands on a short timescale and remains neutron-rich. These conditions might be suitable for the production of heavy elements via the r-process. The neutron-rich material is followed by proton-rich neutrino-driven ejecta in the later cooling phase of the protoneutron star where the vp-process might occur.

astro-ph.HE↗

arXiv2011

Mass measurements of very neutron-deficient Mo and Tc isotopes and their impact on rp process nucleosynthesis

The masses of ten proton-rich nuclides, including the N=Z+1 nuclides 85-Mo and 87-Tc, were measured with the Penning trap mass spectrometer SHIPTRAP. Compared to the Atomic Mass Evaluation 2003 a systematic shift of the mass surface by up to 1.6 MeV is observed causing significant abundance changes of the ashes of astrophysical X-ray bursts. Surprisingly low alpha-separation energies for neutron-deficient Mo and Tc are found, making the formation of a ZrNb cycle in the rp process possible. Such a cycle would impose an upper temperature limit for the synthesis of elements beyond Nb in the rp process.

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arXiv2010

Origin of the p-Nuclei in Explosive Nucleosynthesis

A number of naturally occurring, proton-rich nuclides (the p-nuclei) cannot be made in the s- and r-process. It has been found that massive stars can produce p-nuclei through photodisintegration of pre-existing intermediate and heavy nuclei. This so-called gamma-process requires sufficiently high temperatures and occurs in pre-explosive or explosive O/Ne burning, depending on the mass of the star. Although the gamma-process has been successful in producing a large range of p-nuclei, two mass regions remain problematic, A<110 and 150<A<165, where a number of p-nuclei are severely underproduced. The origin of the problems is yet to be identified. A large number of unstable nuclei with only theoretically predicted reaction rates are included in the reaction network and thus the nuclear input may involve uncertainties. Deficiencies in charged-particle optical potentials at gamma-process temperatures have been found for nuclei at stability. On the other hand, the gamma-process conditions (temperature profiles, entropy of the O shell, seed composition) also sensitively depend on details of the stellar structure and evolution, as well as on the initial metallicity. Nevertheless, especially the deficient low-mass p-nuclei may call for an additional production process or site, such as production in (subChandrasekhar) type Ia supernovae. Also the (im)possibility of a synthesis in the rp- and nu-p-processes is discussed. Were this the case, the production of p-nuclei would be realized as a superposition of several different processes, not necessarily in the same site.

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arXiv2010

Origin of the Chemical Elements

This review provides the necessary background from astrophysics, nuclear, and particle physics to understand the cosmic origin of the chemical elements. It reflects the year 2009 state of the art in this extremely quickly developing interdisciplinary research direction. The discussion summarizes the nucleosynthetic processes in the course of the evolution of the Universe and the galaxies contained within, including primordial nucleosynthesis, stellar evolution, and explosive nucleosynthesis in single and binary systems.

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