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T. Renstrøm

Publications and source records attributed to T. Renstrøm.

At least 19 recordsLinked to original sources

Photoneutron reactions on $^{165}$Ho and $^{169}$Tm in the giant dipole resonance region

Photoneutron reactions were investigated for the deformed $^{165}$Ho and $^{169}$Tm nuclei from the vicinity of the neutron emission threshold up to $\sim$40~MeV, well above the giant dipole resonance (GDR) region, using quasimonochromatic laser Compton scattering $γ$-ray beams provided at the NewSUBARU facility, Japan. A high-and-flat efficiency moderated array of $^3$He counters was used for the neutron detection and an associated neutron multiplicity sorting method for extracting the $(γ,\,1nX)$, $(γ,\,2nX)$, $(γ,\,3nX)$ and $(γ,\,4nX)$ reaction cross sections and average neutron emission energies. The present $^{165}$Ho cross sections were compared to existing data, revealing discrepancies with the Saclay multiplicity sorting results and an overall 10$\%$ strength difference with the Livermore ones. There are no other data for $^{169}$Tm. GDR parameters based on phenomenological Lorentzian models were extracted by fitting the present $σ(γ,\,Sn)$ data with adjustments for the missing contribution of charged-particle-only reactions not observed experimentally. For both nuclei we observed high energy structures at 20-25~MeV, matching giant quadrupole resonance KMFR predictions. Based on the present centroid energies of the first and second GDR peaks, hydrodynamic model predictions gave intrinsic electric quadrupole moments of +7.00(34)~b and +7.38(28)~b for the ground states of $^{165}$Ho and $^{169}$Tm, respectively. The present experimental excitation functions and photoneutron energies were compared to statistical model calculations. Using the EMPIRE code, we performed a sensitivity test to phenomenological models of photon strength functions and nuclear level densities. The TALYS code was used to reproduce the present experimental $(γ,\,inX)$ cross sections and average neutron energies using microscopic nuclear level density models.

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Statistical and non-statistical $γ$-decay properties of $^{64}$Zn

We present a study on the $γ$-decay properties of $^{64}$Zn using the Oslo method on $^{64}$Zn($p,p^\prime γ$) data combined with $^{64}$Zn$(γ,n)$ cross-section measurements at the NewSUBARU facility. With the Oslo method, we have measured the $γ$-ray strength function ($γ$SF) and the nuclear level density (NLD) below the neutron threshold. We observe that the NLD trend in the quasi-continuum region of $^{64}$Zn is best characterized by a constant-temperature-like model. %with temperature parameter $T_{\rm CT}=1.21(5)$ MeV. Surprisingly, we find that $γ$-ray transitions from the quasi-continuum decaying directly to the $0^+$ ground state seem to be strongly hindered with a hindrance factor of $κ\approx 0.5$, which could be an indication of non-statistical effects in the ground-state decay due to, \textit{e.g.}, differences in nuclear shapes. For $γ$ energies above the neutron separation energy, the NewSUBARU ($γ, n$) data set probes a significant part of the giant dipole resonance. Furthermore, we find that the Oslo-method $γ$SF shows a rather smooth behavior, with a clear low-energy enhancement (LEE) for $E_γ < 4$ MeV.

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Photoneutron reactions on gold in the giant dipole resonance region: reaction cross sections and average kinetic energies of $(γ,\,xn)$ photoneutrons

In this work, we present new data on the $^{197}$Au photoneutron reactions in and above the giant dipole resonance region, obtained by using 8 to 39~MeV quasi-monochromatic $γ$-ray beams produced at the NewSUBARU facility in Japan and a high-and-flat efficiency neutron detection system. We report absolute cross sections and mean photoneutron energies for the $^{197}$Au$(γ,\,inX)$ reactions with $i$~=~1 to 4. The photoabsorption cross section was obtained as the sum of the $(γ,\,inX)$ reaction cross sections. The giant dipole resonance parameter values were obtained by fitting the experimental photoabsorption cross sections. The present photoabsorption cross sections are in good agreement with the Saclay results of Veyssiere~\emph{et al.}. Thus, our study does not support the recommendation of Berman~\emph{et al.} of lowering the Saclay photoabsorption cross sections by 8$\%$. We observed a non-statistical high-energy neutron emission in the $(γ,\,n)$ reaction in the low-energy region between $S_n$ and 10~MeV. The present results are compared with data from the literature and statistical model calculations performed with the TALYS and EMPIRE codes.

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Nuclear level densities and $γ-$ray strength functions of $^{111,112,113}$Sn isotopes studied with the Oslo method

The $^{111,112,113}$Sn isotopes have been studied with ($p,d γ$), ($p,p^{\prime} γ$), and ($d,p γ$) reactions to extract the nuclear level densities (NLDs) and $γ$-ray strength functions (GSFs) of these nuclei below the neutron separation energy by means of the Oslo method. The experimental NLDs for all three nuclei demonstrate a trend compatible with the constant-temperature model below the neutron separation energy while also being in good agreement with the NLDs of neighboring Sn isotopes, obtained previously with the Oslo-type and neutron evaporation experiments. The extracted microcanonical entropies yield $\approx 1.5$ $k_B$ entropy of a valence neutron in both $^{111}$Sn and $^{113}$Sn. Moreover, the deduced microcanonical temperatures indeed suggest a clear constant-temperature behavior above $\approx$ 3 MeV in $^{111,113}$Sn and above $\approx$ 4.5 MeV in $^{112}$Sn. We observe signatures for the first broken neutron pairs between 2 and 4 MeV in all three nuclei. The GSFs obtained with the Oslo method are found to be in good agreement below the neutron threshold with the strengths of $^{112,114}$Sn extracted in the ($p,p^{\prime}$) Coulomb excitation experiments.

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Photoneutron emission cross sections for $^{13}$C

Photoneutron emission cross sections were measured for $^{13}$C below $2n$ threshold using quasi-monochromatic $γ$-ray beams produced in laser Compton-scattering at the NewSUBARU synchrotron radiation facility. The data show fine structures in the low-energy tail of the giant-dipole resonance; the integrated strength of the fine structure below 18~MeV is intermediate among the past measurements with bremsstrahlung and the positron annihilation $γ$ rays. We compare the photoneutron emission data with the {\sf TALYS} statistical model calculation implemented with the simple modified Lorentzian model of $E1$ and $M1$ strengths. We also compare the total photoabsorption cross sections for $^{13}$C with the shell model and antisymmetrized molecular dynamics calculations as well as the statistical model calculation. We further investigate the consistency between the present photoneutron emission and the reverse $^{12}$C(n,$γ$) cross sections through their corresponding astrophysical rate.

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New experimental constraint on the $^{185}$W($n,γ$)$^{186}$W cross section

In this work, we present new data on the $^{182,183,184}$W($γ,n$) cross sections, utilizing a quasi-monochromatic photon beam produced at the NewSUBARU synchrotron radiation facility. Further, we have extracted the nuclear level density and $γ$-ray strength function of $^{186}$W from data on the $^{186}$W($α,α^\primeγ$)$^{186}$W reaction measured at the Oslo Cyclotron Laboratory. Combining previous measurements on the $^{186}$W($γ,n$) cross section with our new $^{182,183,184}$W($γ,n$) and ($α,α^\primeγ$)$^{186}$W data sets, we have deduced the $^{186}$W $γ$-ray strength function in the range of $1 < E_γ< 6$ MeV and $7 < E_γ< 14$ MeV. Our data are used to extract the level density and $γ$-ray strength functions needed as input to the nuclear-reaction code \textsf{TALYS}, providing an indirect, experimental constraint for the $^{185}$W($n,γ$)$^{186}$W cross section and reaction rate. Compared to the recommended Maxwellian-averaged cross section (MACS) in the KADoNiS-1.0 data base, our results are on average lower for the relevant energy range $k_B T \in [5,100]$ keV, and we provide a smaller uncertainty for the MACS. The theoretical values of Bao \textit{et al.} and the cross section experimentally constrained on photoneutron data of Sonnabend \textit{et al.} are significantly higher than our result. The lower value by Mohr \textit{et al.} is in very good agreement with our deduced MACS. Our new results could have implications for the $s$-process and in particular the predicted $s$-process production of $^{186,187}$Os nuclei.

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Evolution of the $γ$-ray strength function in neodymium isotopes

The experimental gamma-ray strength functions (gamma-SFs) of 142,144-151Nd have been studied for gamma-ray energies up to the neutron separation energy. The results represent a unique set of gamma-SFs for an isotopic chain with increasing nuclear deformation. The data reveal how the low-energy enhancement, the scissors mode and the pygmy dipole resonance evolve with nuclear deformation and mass number. The data indicate that the mechanisms behind the low-energy enhancement and the scissors mode are decoupled from each other.

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Statistical properties of the well deformed $^{153,155}$Sm nuclei and the scissors resonance

The Nuclear Level Densities (NLDs) and the $γ$-ray Strength Functions ($γ$SFs) of $^{153,155}$Sm have been extracted from (d,p$γ$) coincidences using the Oslo method. The experimental NLD of $^{153}$Sm is higher than the NLD of $^{155}$Sm, in accordance with microscopic calculations. The $γ$SFs of $^{153,155}$Sm are in fair agreement with QRPA calculations based on the D1M Gogny interaction. An enhancement is observed in the $γ$SF for both $^{153,155}$Sm nuclei around 3 MeV in excitation energy and is attributed to the M1 Scissors Resonance (SR). Their integrated strengths were found to be in the range 1.3 - 2.1 and 4.4 - 6.4 $μ^{2}_{N}$ for $^{153}$Sm and $^{155}$Sm, respectively. The strength of the SR for $^{155}$Sm is comparable to those for deformed even-even Sm isotopes from nuclear resonance fluorescence measurements, while that of $^{153}$Sm is lower than expected.

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Strong enhancement of level densities in the crossover from spherical to deformed neodymium isotopes

Understanding the evolution of level densities in the crossover from spherical to well-deformed nuclei has been a long-standing problem in nuclear physics. We measure nuclear level densities for a chain of neodymium isotopes $^{142,144-151}$Nd which exhibit such a crossover. These results represent to date the most complete data set of nuclear level densities for an isotopic chain between neutron shell-closure and towards mid-shell. We observe a strong increase of the level densities along the chain with an overall increase by a factor of $\approx 170$ at an excitation energy of 7.5 MeV and saturation around mass 150. Level densities calculated by the shell model Monte Carlo (SMMC) are in excellent agreement with these experimental results. Based on our experimental and theoretical findings, we offer an explanation of the observed mass dependence of the level densities in terms of the intrinsic single-particle level density and the collective enhancement.

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The radiative width of the Hoyle state from $γ$-ray spectroscopy

The cascading 3.21 MeV and 4.44 MeV electric quadrupole transitions have been observed from the Hoyle state at 7.65 MeV excitation energy in $^{12}$C, excited by the $^{12}$C(p,p$^{\prime}$) reaction at 10.7 MeV proton energy. From the proton-$γ$-$γ$ triple coincidence data, a value of ${Γ_{\rm rad}}/Γ=6.2(6) \times 10^{-4}$ was obtained for the radiative branching ratio. Using our results, together with ${Γ_π^{E0}}/Γ$ from Eriksen et al., Phys. Rev. C 102, 024320 and the currently adopted $Γ_π(E0)$ values, the radiative width of the Hoyle state is determined as $Γ_{\rm rad}=5.1(6) \times 10^{-3}$ eV. This value is about 34% higher than the currently adopted value and will impact on models of stellar evolution and nucleosynthesis.

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The beta-Oslo method: experimentally constrained ($n,γ$) reaction rates relevant to the $r$-process

Unknown neutron-capture reaction rates remain a significant source of uncertainty in state-of-the-art $r$-process nucleosynthesis reaction network calculations. As the $r$-process involves highly neutron-rich nuclei for which direct ($n,γ$) cross-section measurements are virtually impossible, indirect methods are called for to constrain ($n,γ$) cross sections used as input for the $r$-process nuclear network. Here we discuss the newly developed beta-Oslo method, which is capable of providing experimental input for calculating ($n,γ$) rates of neutron-rich nuclei. The beta-Oslo method represents a first step towards constraining neutron-capture rates of importance to the $r$-process.

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$γ$-ray Strength Function for Barium Isotopes

Photoneutron cross sections were measured for $^{137}$Ba and $^{138}$Ba at energies below two-neutron threshold using quasi-monochromatic $γ$-ray beams produced in laser Compton-scattering at the NewSUBARU synchrotron radiation facility. The photoneutron data are used to constrain the $γ$-ray strength function on the basis of the Hartree-Fock-Bogolyubov plus quasi-particle random phase approximation using the Gogny D1M interaction. Supplementing the experimentally constrained $γ$-ray strength function with the zero-limit E1 and M1 contributions which are unique to the deexcitation mode, we discuss radiative neutron capture cross sections relevant to the s-process nucleosynthesis of barium isotopes in the vicinity of the neutron magic number 82.

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IAEA Photonuclear Data Library 2019

Photo-induced reaction cross section data are of importance for a variety of current or emerging applications, such as radiation shielding design and radiation transport analyses, calculations of absorbed dose in the human body during radiotherapy, physics and technology of fission reactors (influence of photo-reactions on neutron balance) and fusion reactors (plasma diagnostics and shielding), activation analyses, safeguards and inspection technologies, nuclear waste transmutation, medical isotope production and astrophysical applications. Since the release of the IAEA Photonuclear Data Library in 1999 however, new experimental data as well as new methods to assess the reliability of experimental cross sections have become available. Theoretical models and input parameters used to evaluate photo-induced reactions have improved significantly over the years. In addition, new measurements of partial photoneutron cross sections using mono-energetic photon beams and advanced neutron detection systems have been performed allowing for the validation of the evaluations and assessments of the experimental data. Furthermore, technological advances have led to the construction of new and more powerful gamma-beam facilities, therefore new data needs are emerging. We report our coordinated efforts to address these data needs and present the results of the new evaluations of more than 200 nuclides included in the new updated IAEA Photonuclear Data Library, where the photon energy goes up to 200 MeV. We discuss the new assessment method and make recommendations to the user community in cases where the experimental data are discrepant and the assessments disagree. In addition, in the absence of experimental data, we present model predictions for photo-induced reaction cross section on nuclides of potential interest to medical radioisotope production.

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Impact of restricted spin-ranges in the Oslo Method: The example of (d,p)$^{240}\mathrm{Pu}$

In this paper we present the first systematic analysis of the impact of the populated vs. intrinsic spin distribution on the nuclear level density and $γ$-ray strength function retrieved through the Oslo Method. We illustrate the effect of the spin distribution on the recently performed $^{239}\mathrm{Pu}$(d,p$γ$)$^{240}\mathrm{Pu}$ experiment using a 12 MeV deuteron beam performed at the Oslo Cyclotron Lab. In the analysis we couple state-of-the-art calculations for the populated spin-distributions with the Monte-Carlo nuclear decay code RAINIER to compare Oslo Method results to the known input. We find that good knowledge of the populated spin distribution is crucial and show that the populated distribution has a significant impact on the extracted nuclear level density and $γ$-ray strength function for the $^{239}\mathrm{Pu}$(d,p$γ$)$^{240}\mathrm{Pu}$ case.

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Consolidating the concept of low-energy magnetic dipole decay radiation

We have made a thorough study of the low-energy behaviour of the $γ$-ray strength function within the framework of the shell model. We have performed large-scale calculations spanning isotopic and isotonic chains over several mass regions, with the purpose of studying the systematic behavior of the low-energy enhancement (LEE) for $M1$ transitions. There are clear trends in the calculations: From being all but absent in the lowest mass region, the LEE becomes steeper and more pronounced as the mass number increases, and for a given mass region it further increases towards shell closures. Moreover, the LEE is found to be steeper in regions near doubly-magic nuclei where proton particles couple to neutron holes. These trends enable us to consolidate several previous works on the LEE into a single, consistent concept. We compare the inferred trends to the available experimental data from the Oslo method, and find suppport for the systematic behaviour. Lastly we have compared the calculations to strength functions compiled from discrete, experimental lifetimes, and find excellent agreement; the discrete data are consistent with a LEE, and indicate that the slope varies as function of mass number.

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The $γ$-ray strength function for Thallium isotopes relevant to the $^{205}$Pb - $^{205}$Tl chronometry

Photoneutron cross sections were measured for $^{203}$Tl and $^{205}$Tl at energies between the one- and two-neutron thresholds using quasi-monochromatic $γ$-ray beams produced in laser Compton-scattering at the NewSUBARU synchrotron radiation facility. Our new measurement results in cross sections significantly different from the previously reported bremsstrahlung experiment, leading to rather different GDR parameters, in particular to lower GDR peak energies and higher peak cross sections. The photoneutron data are used to constrain the $γ$-ray strength function on the basis of the Hartree-Fock-Bogolyubov plus quasi-particle random phase approximation using the Gogny D1M interaction. Supplementing the experimentally constrained $γ$-ray strength function with the zero-limit E1 and M1 contributions for the de-excitation mode, we estimate the Maxwellian-averaged cross section for the s-process branching-point nucleus $^{204}$Tl in the context of the $^{205}$Pb - $^{205}$Tl chronometry.

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Photoneutron cross sections for Ni isotopes: Toward understanding $(n,γ)$ cross sections relevant to the weak s-process nucleosynthesis

Photoneutron cross sections were measured for $^{58}$Ni, $^{60}$Ni, $^{61}$Ni, and $^{64}$Ni at energies between the one-neutron and two-neutron thresholds using quasi-monochromatic $γ$-ray beams produced in laser Compton-scattering at the NewSUBARU synchrotron radiation facility. The new photoneutron data are used to extract the $γ$-ray strength function above the neutron threshold complementing the information obtained by the Oslo method below the threshold. We discuss radiative neutron capture cross sections and the Maxwellian-averaged cross sections for Ni isotopes including $^{63}$Ni, a branching point nucleus along the weak s-process path. The cross sections are calculated with the experimentally constrained $γ$-ray strength functions from the Hartree-Fock-Bogolyubov plus quasi-particle-random phase approximation based on the Gogny D1M interaction for both $E1$ and $M1$ components and supplemented with the $M1$ upbend.

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Enhanced low-energy $γ$-decay strength of $^{70}$Ni and its robustness within the shell model

Neutron-capture reactions on very neutron-rich nuclei are essential for heavy-element nucleosynthesis through the rapid neutron-capture process, now shown to take place in neutron-star merger events. For these exotic nuclei, radiative neutron capture is extremely sensitive to their $γ$-emission probability at very low $γ$ energies. In this work, we present measurements of the $γ$-decay strength of $^{70}$Ni over the wide range $1.3 \leq E_γ \leq 8 $ MeV. A significant enhancement is found in the $γ$-decay strength for transitions with $E_γ< 3$ MeV. At present, this is the most neutron-rich nucleus displaying this feature, proving that this phenomenon is not restricted to stable nuclei. We have performed $E1$-strength calculations within the quasiparticle time-blocking approximation, which describe our data above $E_γ\simeq 5$ MeV very well. Moreover, large-scale shell-model calculations indicate an $M1$ nature of the low-energy $γ$ strength. This turns out to be remarkably robust with respect to the choice of interaction, truncation and model space, and we predict its presence in the whole isotopic chain, in particular the neutron-rich $^{72,74,76}\mathrm{Ni}$.

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