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T. S. Mahesh

Publications and source records attributed to T. S. Mahesh.

At least 55 records · Page 3Linked to original sources

Freezing a Quantum Magnet by Repeated Quantum Interference: An Experimental Realization

We experimentally demonstrate the phenomenon of dynamical many-body freezing in a periodically driven Ising chain. Theoretically [Phys. Rev. B 82, 172402 (2010)], for certain values of the drive parameters all fundamental degrees of freedom contributing to the response dynamics freeze for all time and for arbitrary initial states. Also, since the condition of freezing involves only the drive parameters and not on the quantization of the momentum (i.e., the system-size), our simulation with a small (3-spin) chain captures all salient features of the freezing phenomenon predicted for the infinite chain. Using optimal control techniques, we realize high-fidelity cosine modulated drive, and observe non-monotonic freezing of magnetization at specific frequencies of modulation. Time-evolution of the excitations in momentum space has been tracked directly through magnetization measurements.

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Benford Analysis: A useful paradigm for spectroscopic analysis

Benford's law is a statistical inference to predict the frequency of significant digits in naturally occurring numerical databases. In such databases this law predicts a higher occurrence of the digit 1 in the most significant place and decreasing occurrences to other larger digits. Although counter-intuitive at first sight, Benford's law has seen applications in a wide variety of fields like physics, earth-science, biology, finance etc. In this work, we have explored the use of Benford's law for various spectroscopic applications. Although, we use NMR signals as our databases, the methods described here may also be extended to other spectroscopic techniques. In particular, with the help of Benford analysis, we demonstrate the detection of weak NMR signals and spectral corrections. We also explore a potential application of Benford analysis in the image-processing of MRI data.

physics.data-an↗

Benford distributions in NMR

Benford's Law is an empirical law which predicts the frequency of significant digits in databases corresponding to various phenomena, natural or artificial. Although counter intuitive at the first sight, it predicts a higher occurrence of digit 1, and decreasing occurrences to other larger digits. Here we report the Benford analysis of various NMR databases and draw several interesting inferences. We observe that, in general, NMR signals follow Benford distribution in time-domain as well as in frequency domain. Our survey included NMR signals of various nuclear species in a wide variety of molecules in different phases, namely liquid, liquid-crystalline, and solid. We also studied the dependence of Benford distribution on NMR parameters such as signal to noise ratio, number of scans, pulse angles, and apodization. In this process we also find that, under certain circumstances, the Benford analysis can distinguish a genuine spectrum from a visually identical simulated spectrum. Further we find that chemical-shift databases and amplitudes of certain radio frequency pulses generated using optimal control techniques also satisfy Benford's law to a good extent.

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Single-Shot Quantum Process Tomography

The standard procedure for quantum process tomography (QPT) involves applying the quantum process on a system initialized in each of a complete set of orthonormal states. The corresponding outputs are then characterized by quantum state tomography (QST), which itself requires the measurement of non-commuting observables realized by independent experiments on identically prepared system states. Thus QPT procedure demands a number of independent measurements, and moreover, this number increases rapidly with the size of the system. However, the total number of independent measurements can be greatly reduced with the availability of ancilla qubits. Ancilla assisted process tomography (AAPT) has earlier been shown to require a single QST of system-ancilla space. Ancilla assisted quantum state tomography (AAQST) has also been shown to perform QST in a single measurement. Here we combine AAPT with AAQST to realize a `single-shot QPT' (SSPT), a procedure to characterize a general quantum process in a single collective measurement of a set of commuting observables. We demonstrate experimental SSPT by characterizing several single-qubit processes using a three-qubit NMR quantum register. Furthermore, using the SSPT procedure we experimentally characterize the twirling process and compare the results with theory.

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Estimating Franck-Condon factors using an NMR quantum processor

Interaction of molecules with light may lead to electronic transitions and simultaneous vibrational excitations. Franck-Condon factors (FCFs) play an important role in quantifying the intensities of such vibronic transitions occurring during molecular photo-excitations. In this article, we describe a general method for estimating FCFs using a quantum information processor. The method involves the application of a translation operator followed by the measurement of certain projections. We also illustrate the method by experimentally estimating FCFs with the help of a three-qubit NMR quantum information processor. We describe two methods for the measurement of projections - (i) using diagonal tomography and (ii) using Moussa protocol. The experimental results agree fairly well with the theory.

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Engineered Decoherence: Characterization and Suppression

Due to omnipresent environmental interferences, quantum coherences inevitably undergo irreversible transformations over certain time-scales, thus leading to the loss of encoded information. This process, known as decoherence, has been a major obstacle in realizing efficient quantum information processors. Understanding the mechanism of decoherence is crucial in developing tools to inhibit it. Here we utilize a method proposed by Cory and co-workers [Phys. Rev. A 67, 062316 (2003)] to engineer artificial decoherence in the system qubits by randomly perturbing their surrounding ancilla qubits. Using a two qubit nuclear magnetic resonance quantum register, we characterize the artificial decoherence by noise spectroscopy and quantum process tomography. Further, we study the efficacy of dynamical decoupling sequences in suppressing the artificial decoherence. Here we describe the experimental results and their comparisons with theoretical simulations.

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Monogamy of quantum correlations reveals frustration in a quantum Ising spin system: Experimental demonstration

We report a nuclear magnetic resonance experiment, which simulates the quantum transverse Ising spin system in a triangular configuration and further show that the monogamy of quantum correlations can be used to distinguish between the frustrated and non-frustrated regimes in the ground state of this system. Adiabatic state preparation methods are used to prepare the ground states of the spin system. We employ two different multipartite quantum correlation measures to analyze the experimental ground state of the system in both the frustrated and non-frustrated regimes. In particular, we use multipartite quantum correlation measures generated by monogamy considerations of negativity, a bipartite entanglement measure, and that of quantum discord, an information-theoretic quantum correlation measure. As expected from theoretical predictions, the experimental data confirm that the non-frustrated regime shows higher multipartite quantum correlations compared to the frustrated one.

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Simulation of mirror inversion of quantum states in an XY spin chain using NMR

We report an experimental quantum simulation of unitary dynamics of an XY spin chain with pre-engineered couplings. Using this simulation, we demonstrate the mirror inversion of quantum states, proposed by Albanese et al. [Phys. Rev. Lett. 93, 230502 (2004)]. The experiment is performed with a 5-qubit dipolar coupled spin system using nuclear magnetic resonance techniques. To perform quantum simulation we make use of the recently proposed unitary operator decomposition algorithm of Ajoy et al. [Phys. Rev. A 85, 030303 (2012)] along with numerical pulse optimization techniques. Further, using mirror inversion, we demonstrate that entangled states can be transferred from one end of the chain to the other end. The simulations are implemented with high experimental fidelity, which implies that these kind of simulations may be possible in larger systems.

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Quantum simulations of a particle in one-dimensional potentials using NMR

A classical computer simulating Schrodinger dynamics of a quantum system requires resources which scale exponentially with the size of the system, and is regarded as inefficient for such purposes. However, a quantum computer made up of a controllable set of quantum particles has the potential to efficiently simulate other quantum systems of matching dimensions. In this work we studied quantum simulations of single particle Schrodinger equation for certain one-dimensional potentials. In particular, we report the following cases: (i) spreading of wave-function of a free-particle, (ii) evolution of a particle in a potential-well, and (iii) reflection of a particle from a potential-barrier. Using a five-qubit NMR system, we achieve space discretization with four qubits, and the other qubit is used for preparation of initial states as well as measurement of spatial probabilities. The experimental relative probabilities compare favorably with the theoretical values, thus effectively mimicking a small-scale quantum simulator.

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Inversion of moments to retrieve joint probabilities in quantum sequential measurements

A sequence of moments encode the corresponding probability distribution. Probing if quantum joint probability distribution can be retrieved from the associated set of moments -- realized in the sequential measurement of a dichotomic observable at different time intervals -- reveals a negative answer i.e., the joint probabilities of sequential measurements do not agree with the ones obtained by inverting the moments. This is indeed a reflection of the non-existence of a bonafide grand joint probability distribution, consistent with all the physical marginal probability distributions. Here we explicitly demonstrate that given the set of moments, it is not possible to retrieve the three-time quantum joint probability distribution resulting from quantum sequential measurement of a single qubit dichotomic observable at three different times. Experimental results using a nuclear magnetic resonance (NMR) system are reported here to corroborate these theoretical observations viz., the incompatibility of the three-time joint probabilties with those extracted from the moment sequence.

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Ancilla Assisted Quantum State Tomography in Many-Qubit Registers

The standard method of Quantum State Tomography (QST) relies on the measurement of a set of noncommuting observables, realized in a series of independent experiments. Ancilla Assisted QST (AAQST) proposed by Nieuwenhuizen and co-workers (Phys. Rev. Lett., 92, 120402 (2004)) greatly reduces the number of independent measurements by exploiting an ancilla register in a known initial state. In suitable conditions AAQST allows mapping out density matrix of an input register in a single experiment. Here we describe methods for explicit construction of AAQST experiments in multi-qubit registers. We also report nuclear magnetic resonance studies on AAQST of (i) a two- qubit input register using a one-qubit ancilla in an isotropic liquid-state system and (ii) a three-qubit input register using a two-qubit ancilla register in a partially oriented system. The experimental results confirm the effectiveness of AAQST in such many-qubit registers.

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Violation of Entropic Leggett-Garg Inequality in Nuclear Spins

We report an experimental study of recently formulated entropic Leggett-Garg inequality (ELGI) by Usha Devi et al. (arXiv: 1208.4491v2 (2012)). This inequality places a bound on the statistical measurement outcomes of dynamical observables describing a macrorealistic system. Such a bound is not necessarily obeyed by quantum systems, and therefore provides an important way to distinguish quantumness from classical behavior. Here we study ELGI using a two-qubit nuclear magnetic resonance system. To perform the noninvasive measurements required for the ELGI study, we prepare the system qubit in a maximally mixed state as well as use the `ideal negative result measurement' procedure with the help of an ancilla qubit. The experimental results show a clear violation of ELGI by over four standard deviations. These results agree with the predictions of quantum theory. The violation of ELGI is attributed to the fact that certain joint probabilities are not legitimate in the quantum scenario, in the sense they do not reproduce all the marginal probabilities. Using a three-qubit system, we experimentally demonstrate that three-time joint probabilities do not reproduce certain two-time marginal probabilities.

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Evolution of Quantum Discord and its Stability in Two-Qubit NMR Systems

We investigate evolution of quantum correlations in ensembles of two-qubit nuclear spin systems via nuclear magnetic resonance techniques. We use discord as a measure of quantum correlations and the Werner state as an explicit example. We first introduce different ways of measuring discord and geometric discord in two-qubit systems and then describe the following experimental studies: (a) We quantitatively measure discord for Werner-like states prepared using an entangling pulse sequence. An initial thermal state with zero discord is gradually and periodically transformed into a mixed state with maximum discord. The experimental and simulated behavior of rise and fall of discord agree fairly well. (b) We examine the efficiency of dynamical decoupling sequences in preserving quantum correlations. In our experimental setup, the dynamical decoupling sequences preserved the traceless parts of the density matrices at high fidelity. But they could not maintain the purity of the quantum states and so were unable to keep the discord from decaying. (c) We observe the evolution of discord for a singlet-triplet mixed state during a radio-frequency spin-lock. A simple relaxation model describes the evolution of discord, and the accompanying evolution of fidelity of the long-lived singlet state, reasonably well.

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Characterization of RF Inhomogeneity via NOON states

We describe a method for quantitative characterization of radio-frequency (RF) inhomogeneity using NOON states. NOON states are special multiple-quantum coherences which can be easily prepared in star-topology spin-systems. In this method we exploit the high sensitivity of the NOON states for z-rotations. As a result, Torrey oscillations with NOON states decay much faster than that of single quantum coherences. Therefore the present method requires shorter pulse durations, and enables the study of inhomogeneity at higher RF powers. To model such a inhomogeneity profile, we propose a two-parameter asymmetric Lorentzian function. The experiments are carried out in 1H channels of two different high-resolution NMR probes and the results are compared. Finally, we also extend the NOON state method to characterize the inhomogeneity correlations between two RF channels. We obtain the correlation profile between 1H and 31P channels of an NMR probe by constructing a five-parameter asymmetric-3D Lorentzian model.

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NMR implementation of Quantum Delayed-Choice Experiment

We report the first experimental demonstration of quantum delayed-choice experiment via nuclear magnetic resonance techniques. An ensemble of molecules each with two spin-1/2 nuclei are used as target and the ancilla qubits to perform the quantum circuit corresponding the delayed-choice setup. As expected in theory, our experiments clearly demonstrate the continuous morphing of the target qubit between particle-like and wave-like behaviors. The experimental visibility of the interference patterns shows good agreement with the theory.

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Dynamical Decoupling of Spin-Clusters using Solid State NMR

In this work we experimentally study the efficiency of various dynamical decoupling sequences for suppressing decoherence of single as well as multiple quantum coherences on large spin-clusters. The system involves crystallites of a powdered sample containing a large number of molecular protons interacting via long-range dipole-dipole interaction. The multiple quantum coherences are prepared by progressively creating correlations in the spin lattice using standard pulse sequences implementing two-quantum average Hamiltonian. The spin system is then subjected to various dynamical decoupling sequences, followed by conversion into observable single quantum coherence by using time-reversal sequence. The experiments reveal superior performance of the recently introduced RUDD sequences in suppressing the decoherence.

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Measurement of Translational Diffusion Constant using Noon State

A method for measuring translational diffusion constant in liquids via NOON state is described using a quantum circuit and is experimentally demonstrated using a model system. When compared with the standard single quantum method, the NOON state method requirs shorter diffusion delays and weaker gradients. These improvements depend on the on the size of the NOON state. Due to the high sensitivity of the NOON state for the changes in the local magnetic fields, this method enables studying slow diffusion and studying diffusion with limited strengths of pulsed-field-gradients.

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Storing entanglement of nuclear spins via Uhrig Dynamical Decoupling

Stroboscopic spin flips have already been shown to prolong the coherence times of quantum systems under noisy environments. Uhrig's dynamical decoupling scheme provides an optimal sequence for a quantum system interacting with a dephasing bath. Several experimental demonstrations have already verified the efficiency of such dynamical decoupling schemes in preserving single qubit coherences. In this work we describe the experimental study of Uhrig's dynamical decoupling in preserving two-qubit entangled states using an ensemble of spin-1/2 nuclear pairs in solution state. We find that the performance of odd-order Uhrig sequences in preserving entanglement is superior to both even-order Uhrig sequences and periodic spin-flip sequences. We also find that there exists an optimal length of the Uhrig sequence at which the decoherence time gets boosted from a few seconds to about 30 seconds.

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