arXiv subjects

T. S. Monteiro

Publications and source records attributed to T. S. Monteiro.

At least 19 recordsLinked to original sources

arXiv2026

Nanoparticle arrays levitated in a cavity for quantum sensing

Levitated nanoparticles are being investigated as ultrasensitive quantum sensors of forces and accelerations, with applications ranging from fundamental physics phenomena such as dark matter or quantum gravity to real world applications. Attention is now turning to multiparticle regimes, and an important question is whether collective effects offer advantages for sensing. We investigate here the spectral characteristics of collective motion of $N $ trapped nanoparticles interacting via the optical mode of a cavity. We find the collective motion typically exhibit two generic spectral features: a broad spectral feature, the collective bright mode (CBM) which has been previously studied; but we find also a new structure of sharp peaks , the mechanical mode comb (MMC). We can describe all the detailed spectral features of the system, with a simple closed-form expression, by reducing the motion to a 1D generic collective mode which is non-Hermitian. We show that the MMC is more advantageous than the usual CBM for increased sensitivity in force sensing. We find that the mechanical comb can autonomously repair loss of `teeth' due to particle loss, a feature that may offer robustness in sensing.

physics.optics↗

arXiv2025

Feedback cooling scheme for an optically levitated oscillator with controlled cross-talk

Levitated optical mechanical systems have demonstrated excellent force and impulse sensitivity and are currently being developed for the creation of non-classical states of motion in these new quantum systems. An important requirement in the design of these systems is the ability to independently control and cool all three translational degrees of freedom. Here we describe the design and implementation of a stable and robust 3D velocity feedback cooling scheme with particular emphasis on creating minimal cross-talk between the independent oscillatory modes when cooling.

physics.optics↗

arXiv2024

Hyperpolarisation Dynamics: Asymptotic Polarisation

For applications of solid state quantum computing and quantum simulations, high fidelity initialisation of thermally mixed electronic and nuclear spin qubits is essential. Whereas electronic spins can readily be initialised optically to high fidelity, initialisation of the nuclear spins requires alternative approaches, such as dynamic nuclear polarisation (DNP) via the electronic spin. Pulse-based DNP methods, such as PulsePol, are already widely utilised. By means of repeated application of PulsePol sequences, interspersed with re-initialisation of the electronic spin, high levels of nuclear polarisation -- termed hyperpolarisation -- have been achieved. From theoretical analysis of these protocols perfect nuclear initialisation is expected; however, in practice, saturation below $\sim$ 95$\%$ is seen in experiment. We develop an analytical model to describe hyperpolarisation dynamics, predicting non-maximal nuclear polarisation saturation in the asymptotic limit for realistic nuclear spin clusters. We argue that perfect initialisation of a typical nuclear cluster using this method may not, in general, be possible even with an arbitrarily large number of repetitions.

quant-ph↗

arXiv2023

Sensing microscopic directional noise baths with an optically cooled and levitated nanoparticle

Optomechanical devices are being harnessed as sensors of ultraweak forces for applications ranging from inertial sensing to the search for the elusive dark matter. For the latter, there is a focus on detection of either higher energy single recoils or ultralight, narrowband sources; a directional signal is expected. However, the possibility of searching for a stochastic stream of weak impulses, or more generally a directional broadband signal, need not be excluded; with this and other applications in mind, we investigate the experimental signature of Gaussian white noise impulses with a well defined direction $Ψ$ on a levitated nanosphere, trapped and 3D cooled in an optical tweezer. We find that cross-correlation power spectra offer a calibration-free distinctive signature of the presence of a directional but stochastic microscopic force and its orientation quadrant, unlike normal power spectral densities (PSDs). We obtain excellent agreement between theoretical and experimental results. With calibration we are able to measure the angle $Ψ$, akin to a force compass in a plane. We discuss prospects for extending this technique into quantum regime and compare the expected behaviour of quantum baths and classical baths.

physics.optics↗

arXiv2023

Hyperpolarisation of nuclear spins: polarisation blockade

Efficient hyperpolarisation of nuclear spins via optically active defect centers, such as the nitrogen vacancy (NV) center in diamond, has great potential for enhancing NMR based quantum information processing and nanoscale magnetic resonance imaging. Recently, pulse-based protocols have been shown to efficiently transfer optically induced polarisation of the electron defect spin to surrounding nuclear spins -- at particular resonant pulse intervals. In this work, we investigate the performance of these protocols, both analytically and experimentally, with the electronic spin of a single NV defect. We find that whenever polarisation resonances of nuclear spins are near-degenerate with a `blocking' spin, which is single spin with stronger off-diagonal coupling to the electronic central spin, they are displaced out of the central resonant region -- without, in general, significant weakening of the resonance. We analyse the underlying physical mechanism and obtain a closed form expression for the displacement. We propose that spin blocking represents a common but overlooked effect in hyperpolarisation of nuclear spins and suggest solutions for improved protocol performance in the presence of (naturally occurring) blocking nuclear spins.

quant-ph↗

arXiv2022

Towards directional force sensing in levitated optomechanics

Levitated nanoparticles are being intensively investigated from two different perspectives: as a potential realisation of macroscopic quantum coherence; and as ultra-sensitive sensors of force, down to the zeptoNewton level, with a range of various applications, including the search for Dark Matter. A future aim is to merge these two strands, enabling the development of quantum-limited sensors. Here we propose that mechanical cross-correlation spectra $S_{xy}(ω)$ offer new possibilities: once detector misalignment errors are minimised, the spectral shape of $S_{xy}(ω)$ directly points out the orientation of an external stochastic force, offering something akin to a compass in the $x-y$ plane. We analyse this for detection of microscopic gas currents, but any broad spectrum directed force will suffice, enabling straightforward investigation with laboratory test forces with or without cavities. For a cavity set-up, we analyse misalignment imprecisions between detectors and motional modes due to for example optical back-actions that mask the signature of the directed forces, and show how to suppress them. Near quantum regimes, we quantify the imprecision due to the $x-y$ correlating effect of quantum shot noise imprecision.

quant-ph↗

arXiv2022

Controlling mode orientations and frequencies in levitated cavity optomechanics

Cavity optomechanics offers quantum cooling, quantum control and measurement of small mechanical oscillators. However the optical backactions that underpin quantum control can significantly disturb the oscillator modes: mechanical frequencies are shifted by the optical spring effect and light-matter hybridisation in strong coupling regimes; mechanical modes hybridise with each other via the cavity mode. This is even more pertinent in the field of levitated optomechanics, where optical trapping fully determines the mechanical modes and their frequencies. Here, using the coherent-scattering (CS) set-up that allowed quantum ground state cooling of a levitated nanoparticle, we show that -- when trapping away from a node of the cavity standing wave -- the CS field opposes optical spring shifts and mechanical mode hybridisation. At an optimal cancellation point, independent of most experimental parameters, we demonstrate experimentally that it is possible to strongly cavity cool and control the {\em unperturbed} modes. Suppression of the cavity-induced mode hybridisation in the $x-y$ plane is quantified by measuring the $S_{xy}(ω)$ correlation spectra which are seen to always be anti-correlated except at the cancellation point where they become uncorrelated. The findings have implications for directional force sensing using CS set-ups.

quant-ph↗

arXiv2021

Adiabatic Dynamical-Decoupling Based Control of Nuclear Spin Registers

The use of the nuclear spins surrounding electron spin qubits as quantum registers and long-lived memories opens the way to new applications in quantum information and biological sensing. Hence, there is a need for generic and robust forms of control of the nuclear registers. Although adiabatic gates are widely used in quantum information, they can become too slow to outpace decoherence. Here, we introduce a technique whereby adiabatic gates arise from the dynamical decoupling protocols that simultaneously extend coherence. We illustrate this pulse-based adiabatic control for nuclear spins around NV centers in diamond. We obtain a closed-form expression from Landau-Zener theory and show that it reliably describes the dynamics. By identifying robust Floquet states, we show that the technique enables polarisation, one-shot flips and state storage for nuclear spins. These results introduce a new control paradigm that combines dynamical decoupling with adiabatic evolution.

quant-ph↗

arXiv2019

Quantum displacement sensing and cooling in 3D levitated cavity optomechanics

Ultra-high sensitivity detection of quantum-scale displacements in cavity optomechanics optimises the combined errors from measurement back-action and imprecisions from incoming quantum noises. This sets the well-known Standard Quantum Limit (SQL). Normal quantum cavity optomechanics allows cooling and detection of a single degree of freedom, along the cavity axis. However, a recent breakthrough that allows quantum ground-state cooling of levitated nanoparticles [Delic et al, arxiv:1911.04406], is uniquely 3D in character, with coupling along the $x$, $y$ and $z$ axes. We investigate current experiments and show that the underlying behaviour is far from the addition of independent 1D components and that ground-state cooling and sensing analysis must consider- to date neglected- 3D hybridisation effects. We characterise the additional 3D spectral contributions and find direct and indirect hybridising pathways can destructively interfere suppressing of 3D effects at certain parameters in order to approach, and possibly surpass, the SQL. We identify a sympathetic cooling mechanism that can enhance cooling of weaker coupled modes, arising from optomechanically induced correlations.

quant-ph↗

arXiv2019

Quantum bath control with nuclear spin state selectivity via pulse-adjusted dynamical decoupling

Dynamical decoupling (DD) is a powerful method for controlling arbitrary open quantum systems. In quantum spin control, DD generally involves a sequence of timed spin flips ($π$ rotations) arranged to average out or selectively enhance coupling to the environment. Experimentally, errors in the spin flips are inevitably introduced, motivating efforts to optimise error-robust DD. Here we invert this paradigm: by introducing particular control "errors" in standard DD, namely a small constant deviation from perfect $π$ rotations (pulse adjustments), we show we obtain protocols that retain the advantages of DD while introducing the capabilities of quantum state readout and polarisation transfer. We exploit this nuclear quantum state selectivity on an ensemble of nitrogen-vacancy centres in diamond to efficiently polarise the $^{13}$C quantum bath. The underlying physical mechanism is generic and paves the way to systematic engineering of pulse-adjusted protocols with nuclear state selectivity for quantum control applications.

quant-ph↗

arXiv2019

The non-vanishing effect of detuning errors in dynamical decoupling based quantum sensing experiments

Characteristic dips appear in the coherence traces of a probe qubit when dynamical decoupling (DD) is applied in synchrony with the precession of target nuclear spins, forming the basis for nanoscale nuclear magnetic resonance (NMR). The frequency of the microwave control pulses is chosen to match the qubit transition but this can be detuned from resonance by experimental errors, hyperfine coupling intrinsic to the qubit, or inhomogeneous broadening. The detuning acts as an additional static field which is generally assumed to be completely removed in Hahn echo and DD experiments. Here we demonstrate that this is not the case in the presence of finite pulse-durations, where a detuning can drastically alter the coherence response of the probe qubit, with important implications for sensing applications. Using the electronic spin associated with a nitrogen-vacancy centre in diamond as a test qubit system, we analytically and experimentally study the qubit coherence response under CPMG and XY8 dynamical decoupling control schemes in the presence of finite pulse-durations and static detunings. Most striking is the splitting of the NMR resonance under CPMG, whereas under XY8 the amplitude of the NMR signal is modulated. Our work shows that the detuning error must not be neglected when extracting data from quantum sensor coherence traces.

quant-ph↗

arXiv2018

Dynamical decoupling protocols with nuclear spin state selectivity

The ability to initialise nuclear spins, which are typically in a mixed state even at low temperature, is a key requirement of many protocols used in quantum computing and simulations as well as in magnetic resonance spectroscopy and imaging. Yet, it remains a challenging task that typically involves complex and inefficient protocols, limiting the fidelity of ensuing operations or the measurement sensitivity. We introduce here a class of dynamical nuclear spin state selective (DNSS) protocols which, when applied to a polarised electron spin such as the nitrogen-vacancy (NV) centre in diamond, permit the addressing of selected nuclear states of the mixture. It works by splitting the underlying eigenstates into two distinct symmetries dependent on the nuclear spin state, and independent of the electron-nuclear coupling strength. As a particular example, we show that DNSS is achievable by simply introducing a detuning in the common Carr-Purcell-Meiboom-Gill (CPMG) protocol, where the state selection is then controlled by the inter-pulse spacing. This approach offers advantages in ultra-high fidelity initialisation of nuclear registers, ensemble polarisation and single-gate manipulation of nuclei.

quant-ph↗

arXiv2018

Stochastic Langevin propagation for classical and quantum optomechanics

Interesting experimental signatures of quantum cavity optomechanics arise because the quantum back-action induces correlations between incident quantum shot noise and the cavity field. While the quantum linear theory of optomechanics (QLT) has provided vital understanding across many experimental platforms, in certain new set-ups it may be insufficient: analysis in the time domain may be needed, but QLT obtains only spectra in frequency space; and nonlinear behavior may be present. Direct solution of the stochastic equations of motion in time is an alternative, but unfortunately standard methods do not preserve the important optomechanical correlations. We introduce two-timescale stochastic Langevin (T2SL) propagation as an efficient and straightforward method to obtain time traces with the correct correlations. We show that T2SL, in contrast to standard stochastic simulations, can efficiently simulate correlation phenomena such as ponderomotive squeezing and reproduces accurately cavity sideband structures on the scale of the applied quantum noise and even complicated features entirely submerged below the quantum shot noise imprecision floor. We investigate nonlinear regimes and find where comparison is possible, that the method agrees with analytical results obtained with master equations at low temperatures and in perturbative regimes.

quant-ph↗

arXiv2017

Imaging correlations in heterodyne-detected spectra for quantum sensing

The extraordinary sensitivity of the output field of an optical cavity to small quantum-scale displacements has led to breakthroughs such as the first detection of gravitational waves \cite{LIGO,LIGODC} and of the motions of quantum ground-state cooled mechanical oscillators \cite{Teufel2011,Chan2011}. While heterodyne detection of the cavity field preserves asymmetries which provide a key signature that mechanical oscillators has attained the quantum regime, detection of a rotating quadrature of the light averages out important quantum correlations, yielding a weaker signal and lower sensitivity than homodyne detection. In turn, homodyning, detects a single optical quadrature, but loses the important quantum sideband asymmetries. In the present work we present and experimentally demonstrate a technique, involving judicious construction of the autocorrelators of the output current using filter functions, which can restore the lost correlations (whether classical or quantum), drastically augmenting the useful information extracted: the filtering adjusts for moderate errors in the locking phase of the local oscillator, allowing efficient single-shot measurement of hundreds of different field quadratures and rapid mapping of detailed features from a simple heterodyne trace. One may also control whether the correlations are recovered in isolation or interfere with the usual stationary heterodyne sidebands. In the latter case we obtain a spectrum of hybrid homodyne-heterodyne character, with motional sidebands of combined amplitudes comparable to homodyne. We term such recovery of lost heterodyne correlations with filter functions r-heterodyning: although investigated here in a thermal regime, its robustness and generality represents a promising new approach to sensing of quantum-scale displacements.

quant-ph↗

arXiv2017

Quantum noise spectra for periodically-driven cavity optomechanics

A growing number of experimental set-ups in cavity optomechanics exploit periodically driven fields. However, such set-ups are not amenable to analysis using simple, yet powerful, closed-form expressions of linearized optomechanics, which have provided so much of our present understanding of experimental optomechanics. In the present paper, we formulate a new method to calculate quantum noise spectra in modulated optomechanical systems, which we analyze, compare, and discuss with two other recently proposed solutions: we term these (i) frequency-shifted operators (ii) Floquet and (iii) iterative analysis. We prove that (i) and (ii) yield equivalent noise spectra, and find that (iii) is an analytical approximation to (i) for weak modulations. We calculate the noise spectra of a doubly-modulated system describing experiments of levitated particles in hybrid electro-optical traps. We show excellent agreement with Langevin stochastic simulations in the thermal regime and predict squeezing in the quantum regime. Finally, we reveal how experimentally inaccessible spectral components of a modulated system can be measured in heterodyne detection through an appropriate choice of modulation frequencies.

quant-ph↗

arXiv2017

Proposal for enhanced resolution in nanoscale NMR: quantum sensing with pulses of finite duration

The nitrogen vacancy (NV) color center in diamond is an enormously important platform for the development of quantum sensors, including for single spin and single molecule NMR. Detection of weak single-spin signals is greatly enhanced by repeated sequences of microwave pulses; in these dynamical decoupling (DD) techniques, the key control parameters swept in the experiment are the time intervals, $τ$, between pulses. Here we show that, in fact, the pulse duration offers a powerful additional control parameter. While previously, a non-negligible pulse-width has been considered simply a source of experimental error, here we elucidate the underlying quantum dynamics: we identify a landscape of quantum-state crossings which are usually closed (inactive) but may be controllably activated (opened) by adjusting the pulse-width from zero. We identify these crossings with recently observed but unexpected dips (so called spurious dips) seen in the quantum coherence of the NV spin. With this new understanding, both the position and strength of these sharp features may be accurately controlled; they co-exist with the usual broader coherence dips of short-duration microwave pulses, but their sharpness allows for higher resolution spectroscopy with quantum diamond sensors, or their analogues.

quant-ph↗

arXiv2017

Recovering correlations in optomechanical heterodyne spectra for high-precision quantum displacement sensing

Homodyne and heterodyne detection represent "twin-pillars" of quantum displacement sensing using optical cavities, having permitted major breakthroughs including detection of gravitational waves and of the motion of quantum ground-state cooled mechanical oscillators. Both can suffer disadvantages as diagnostics in quantum optomechanics, either through symmetrisation (homodyne), or loss of correlations (heterodyne). We show that, for modest heterodyne beat frequencies ($Ω\sim ω_M/10 \gg Γ$), judicious construction of the autocorrelation of the measured current can either recover (i) a spectrum with strong sidebands but without an imprecision noise floor (ii) a spectrum which is a hybrid, combining both homodyne and heterodyne sideband features. We simulate an experimental realisation with stochastic numerics and find excellent agreement with analytical quantum noise spectra. We term such retrospective recovery of lost heterodyne correlations "r-heterodyning": as the method simply involves post-processing of a normal heterodyne time signal, there is no additional experimental constraint other than on the magnitude of $Ω$.

quant-ph↗

arXiv2016

Split-sideband spectroscopy in slowly modulated optomechanics

Optomechanical coupling between the motion of a mechanical oscillator and a cavity represents a new arena for experimental investigation of quantum effects on the mesoscopic and macroscopic scale.The motional sidebands of the output of a cavity offer ultra-sensitive probes of the dynamics. We introduce a scheme whereby these sidebands split asymmetrically and show how they may be used as experimental diagnostics and signatures of quantum noise limited dynamics. We show split-sidebands with controllable asymmetry occur by simultaneously modulating the light-mechanical coupling $g$ and $ω_M$ - slowly and out of-phase. Such modulations are generic but already occur in optically trapped set-ups where the equilibrium point of the oscillator is varied cyclically. We analyse recently observed, but overlooked, experimental split-sideband asymmetries; although not yet in the quantum regime, the data suggests that split sideband structures are easily accessible to future experiments.

quant-ph↗