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T. Sasagawa

Publications and source records attributed to T. Sasagawa.

84 records · Page 5Linked to original sources

Asymmetries in the electron-hole pair dynamics and strong Mott pseudogap effect in the phase diagram of cuprates

Electron behavior in doped Mott systems continues to be a major unsolved problem in quantum many-electron physics. A central issue in understanding the universal Mott behavior in a variety of complex systems is to understand the nature of their electron-hole pair excitation modes. Using high resolution resonant inelastic x-ray scattering (RIXS) we resolve the momentum dependence of electron-hole pair excitations in two major classes of doped copper oxides which reveals a Mott pseudogap over the full Brillouin zone and over the entire phase diagram. The pair bandwidth and zone-boundary pair velocity renormalize on either sides of the phase diagram at very different rates indicating strong particle-hole doping asymmetries observed for the first time.

cond-mat.str-el↗

The Dichotomy between Nodal and Antinodal Quasiparticles in Underdoped (La$_{2-x}$Sr$_x$)CuO$_4$ Superconductors

High resolution angle-resolved photoemission measurements on underdoped (La$_{2-x}$Sr$_x$)CuO$_4$ system show that, at energies below 70 meV, the quasiparticle peak is well defined around the ($π$/2,$π$/2) nodal region and disappears rather abruptly when the momentum is changed from the nodal point to the ($π$,0) antinodal point along the underlying ``Fermi surface''. It indicates that there is an extra low energy scattering mechanism acting upon the antinodal quasiparticles. We propose that this mechanism is the scattering of quasiparticles across the nearly parallel segments of the Fermi surface near the antinodes.

cond-mat.str-el↗

Nodal metallic behavior of lightly-doped La$_{2-x}$Sr$_x$CuO$_4$

Lightly-doped La$_{2-x}$Sr$_x$CuO$_4$ in the so-called "insulating" spin-glass/diagonal-stripe phase has been studied by angle-resolved photoemission spectroscopy. A quasi-particle (QP) peak crossing the Fermi level has been observed in the node direction of the d-wave superconducting gap, forming an "arc" of Fermi surface consistent with the recently observed metallic transport behavior at high temperatures of lightly-doped materials. The spectral weight of the nodal QP smoothly increases with hole doping, corresponding to the $n \sim x$ behavior of the carrier number in the underdoped and lightly-doped regions.

cond-mat.str-el↗

Gigantic anisotropic uniaxial pressure effect on superconductivity within the CuO2 plane of La1.64Eu0.2Sr0.16CuO4 - strain control of stripe criticality

The effect of uniaxial pressure on superconductivity was examined for a high-Tc cuprate La1.64Eu0.2Sr0.16CuO4, which is located at the boundary between the superconducting and stripe phases. We found remarkably large anisotropy of the uniaxial pressure effect not only between the in-plane and out-of-plane pressures but also within the CuO2-plane. When the pressure is applied along the tetragonal [110] direction, we found the largest pressure effect ever observed in cuprates, dTc/dP - 2.5 K/kbar, while the change of Tc was not appreciable when applied along [100]. This substantial in-plane anisotropy is attributed to an intimate link between the symmetry of the one-dimensional stripes and that of the strain produced within the CuO2 plane.

cond-mat.str-el↗

Magnetic Properties and Phase Diagram of Li-doped La(2)CuO(4): Common Magnetic Response of Hole-doped CuO2 Planes

Although La(2)Cu(1-x)Li(x)O(4) [Li-LCO] differs from La(2-x)Sr(x)CuO(4) [Sr-LCO] in many ways (e.g., the absence of metallic transport, high-Tc superconductivity, and incommensurate antiferromagnetic correlations), it has been known that certain magnetic properties are remarkably similar. The present work establishes the detailed bulk magnetic phase diagram of Li-LCO (0 <= x <= 0.07), which is found to be nearly identical to that of lightly-doped Sr-LCO, and therefore extends the universality of the phase diagram to hole-doped but nonsuperconducting cuprates.

cond-mat.str-el↗

Evolution of a Metal to Insulator Transition in Ca$_{2-x}$Na$_{x}$CuO$_{2}$Cl$_{2}$, as seen by ARPES

We present angle resolved photoemission (ARPES) data on Na-doped Ca$_2$CuO$_2$Cl$_2$. We demonstrate that the chemical potential shifts upon doping the system across the insulator to metal transition. The resulting low energy spectra reveal a gap structure which appears to deviate from the canonical $d_{x2-y2} ~ |cos(k_x a)-cos(k_y a)|$ form. To reconcile the measured gap structure with d-wave superconductivity one can understand the data in terms of two gaps, a very small one contributing to the nodal region and a very large one dominating the anti-nodal region. The latter is a result of the electronic structure observed in the undoped antiferromagnetic insulator. Furthermore, the low energy electronic structure of the metallic sample contains a two component structure in the nodal direction, and a change in velocity of the dispersion in the nodal direction at roughly 50 meV. We discuss these results in connection with photoemission data on other cuprate systems.

cond-mat.str-el↗

Angle-resolved photoemission spectroscopy of Na-doped Ca2CuO2Cl2 single crystals: Fingerprints of a magnetic insulator in a heavily underdoped superconductor

Electronic evolution from an antiferromagnet to a high-Tc superconductor is revealed by angle-resolved photoemission experiments on tetragonal Ca(1.9)Na(0.1)CuO(2)Cl(2) single crystals, which were successfully grown for the first time under high pressures. In this underdoped superconductor, we found clear fingerprints of the parent insulator: a shadow band and a large pseudo-gap. These observations are most likely described by a "chemical potential shift", which contrasts clearly with the prevailing wisdom of the "pinned chemical potential" learned from the prototype La(2-x)Sr(x)CuO(4), demonstrating that the route to a high-Tc superconductor is not unique.

cond-mat.supr-con↗

Antiferromagnetic vortex state in a high-temperature superconductor

There is strong evidence that magnetic interactions play a crucial role in the mechanism driving high-temperature superconductivity in cuprate superconductors. To investigate this further we have done neutron scattering experiments on the simplest high-temperature superconductor La(2-x)Sr(x)CuO(4) (LSCO) in an applied magnetic field. Below the superconducting transition temperature (Tc), the field penetrates the material via an array of normal state inclusions or vortices while phase coherent superconductivity characterized by zero resistance is suppressed to the lower field-dependent irreversibility temperature. The measurements described here were performed on underdoped LSCO (x=0.10), which develops static incommensurate order below Tc in zero field. Our results show that application of a magnetic field enhances this response without changing the onset temperature. For H=5T the field-induced signal saturates to three times the zero-field signal and phase coherent superconductivity is established within the antiferromagnetic phase.

cond-mat.supr-con↗

The Pseudogap in La(2-x)Sr(x)CuO(4): A Raman Viewpoint

We report the results of Raman scattering experiments on single crystals of La(2-x)Sr(x)CuO(4) [La214] as a function of temperature and doping. In underdoped compounds low-energy B1g spectral weight is depleted in association with the opening of a pseudogap on regions of the Fermi surface located near (pi, 0) and (0, pi). The magnitude of the depletion increases with decreasing doping, and in the most underdoped samples, with decreasing temperature. The spectral weight that is lost at low-energies (omega < 800 cm-1) is transferred to the higher energy region normally occupied by multi-magnon scattering. From the normal state B2g spectra we have determined the scattering rate Gamma(omega, T) of qausiparticles located near the diagonal directions in k-space, (pi/2, pi/2) regions. In underdoped compounds, Gamma(omega, T) is suppressed at low temperatures for energies less than Eg(x) ~ 800 cm-1. The observed doping dependence of the two-magnon scattering and the scattering rate suppression thus suggest that the pseudogap is characterized by an energy scale Eg ~ J, where J is the antiferromagnetic super-exchange energy. Comparison with the results from other techniques provides a consistent picture of the pseudogap in La214.

cond-mat.supr-con↗

Oxygen isotope effect on the in-plane penetration depth in underdoped La_{2-x}Sr_{x}CuO_{4} single crystals

We report measurements of the oxygen isotope effect (OIE) on the in-plane penetration depth λ_{ab}(0) in underdoped La_{2-x}Sr_{x}CuO_{4} single crystals. A highly sensitive magnetic torque sensor with a resolution of Δτ~ 10^{-12} Nm was used for the magnetic measurements on microcrystals with a mass of ~ 10 microg. The OIE on λ_{ab}^{-2}(0) is found to be -10(2)% for x = 0.080 and -8(1)% for x = 0.086. It arises mainly from the oxygen mass dependence of the in-plane effective mass m_{ab}*. The present results suggest that lattice vibrations are important for the occurrence of high temperature superconductivity.

cond-mat.supr-con↗

Torque magnetometry on single-crystal high temperature superconductors near the critical temperature: a scaling approach

Angular-dependent magnetic torque measurements performed near the critical temperature on single crystals of HgBa_{2}CuO_{4+y}, La_{2-x}Sr{x}CuO_{4}, and YBa_{2}Cu_{3}O_{6.93} are scaled, following the 3D XY model, in order to determine the scaling function dG^{\pm}(z)/dz which describes the universal critical properties near T_{c}. A systematic shift of the scaling function with increasing effective mass anisotropy γ= (m_{ab}*/m_{c}*)^{1/2} is observed, which may be understood in terms of a 3D-2D crossover. Further evidence for a 3D-2D crossover is found from temperature-dependent torque measurements carried out in different magnetic fields at different field orientations δ, which show a quasi 2D "crossing region'' (M*,T*). The occurrence of this "crossing phenomenon'' is explained in a phenomenological way from the weak z dependence of the scaling function around a value z = z*. The "crossing'' temperature T* is found to be angular-dependent. Torque measurements above T_{c} reveal that fluctuations are strongly enhanced in the underdoped regime where the anisotropy is large, whereas they are less important in the overdoped regime.

cond-mat.supr-con↗

Doping Dependent Density of States and Pseudogap Behavior in La2-xSrxCuO4

We have made a high-resolution photoemission study of La2-xSrxCuO4 in a wide hole concentration (x) range from a heavily overdoped metal to an undoped insulator. As x decreases, the spectral density of states at the chemical potential (μ) is suppressed with an x-dependence similar to the suppression of the electronic specific heat coefficient. In the underdoped region, the spectra show a pseudogap structure on the energy scale of 0.1 eV. The width of the pseudogap increases with decreasing x following the x-dependence of the characteristic temperatures of the magnetic susceptibility and the Hall coefficient.

cond-mat.supr-con↗