arXiv subjects

T. Sasaki

Publications and source records attributed to T. Sasaki.

At least 55 records · Page 3Linked to original sources

arXiv2014

Mott metal-insulator transition induced by utilizing a glass-like structural ordering in low-dimensional molecular conductors

We utilize a glass-like structural transition in order to induce a Mott metal-insulator transition in the quasi-two-dimensional organic charge-transfer salt $κ$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Br. In this material, the terminal ethylene groups of the BEDT-TTF molecules can adopt two different structural orientations within the crystal structure, namely eclipsed (E) and staggered (S) with the relative orientation of the outer C$-$C bonds being parallel and canted, respectively. These two conformations are thermally disordered at room temperature and undergo a glass-like ordering transition at $T_g \sim 75\,$K. When cooling through $T_g$, a small fraction that depends on the cooling rate remains frozen in the S configuration, which is of slightly higher energy, corresponding to a controllable degree of structural disorder. We demonstrate that, when thermally coupled to a low-temperature heat bath, a pulsed heating current through the sample causes a very fast relaxation with cooling rates at $T_g$ of the order of several 1000$\,$K/min. The freezing of the structural degrees of freedom causes a decrease of the electronic bandwidth $W$ with increasing cooling rate, and hence a Mott metal-insulator transition as the system crosses the critical ratio $(W/U)_{c}$ of bandwidth to on-site Coulomb repulsion $U$. Due to the glassy character of the transition, the effect is persistent below $T_g$ and can be reversibly repeated by melting the frozen configuration upon warming above $T_g$. Both by exploiting the characteristics of slowly-changing relaxation times close to this temperature and by controlling the heating power, the materials can be fine-tuned across the Mott transition. A simple model allows for an estimate of the energy difference between the E and S state as well as the accompanying degree of frozen disorder in the population of the two orientations.

cond-mat.str-el↗

arXiv2014

Universal Profiles of the Intracluster Medium from Suzaku X-Ray and Subaru Weak Lensing Obesrvations

We conduct a joint X-ray and weak-lensing study of four relaxed galaxy clusters (Hydra A, A478, A1689 and A1835) observed by both Suzaku and Subaru out to virial radii, with an aim to understand recently-discovered unexpected feature of the ICM in cluster outskirts. We show that the average hydrostatic-to-lensing total mass ratio for the four clusters decreases from \sim 70% to \sim 40% as the overdensity contrast decreases from 500 to the virial value.The average gas mass fraction from lensing total mass estimates increases with cluster radius and agrees with the cosmic mean baryon fraction within the virial radius, whereas the X-ray-based gas fraction considerably exceeds the cosmic values due to underestimation of the hydrostatic mass. We also develop a new advanced method for determining normalized cluster radial profiles for multiple X-ray observables by simultaneously taking into account both their radial dependence and multivariate scaling relations with weak-lensing masses. Although the four clusters span a range of halo mass, concentration, X-ray luminosity and redshift, we find that the gas entropy, pressure, temperature and density profiles are all remarkably self-similar when scaled with the lensing M_200 mass and r_200 radius.The entropy monotonically increases out to \sim 0.5r_200 following the accretion shock heating model K(r)\propto r^1.1, and flattens at \simgt 0.5r_200.The universality of the scaled entropy profiles indicates that the thermalization mechanism over the entire cluster region (>0.1r_200) is controlled by gravitation in a common to all clusters, although the heating efficiency in the outskirts needs to be modified from the standard law.The bivariate scaling functions of the gas density and temperature reveal that the flattening of the outskirts entropy profile is caused by the steepening of the temperature, rather than the flattening of the gas density.

astro-ph.CO↗

arXiv2014

Interface-dependent magnetotransport properties for thin Pt films on ferrimagnetic Y3Fe5O12

We have studied magnetoresistance and Hall effects for 1.8-nm-thick Pt films grown on a ferrimagnetic insulator Y3Fe5O12 in a wide temperature (0.46-300 K) and magnetic-field (-15-15 T) region. In the low-temperature regime where quantum corrections to conductivity are observed, weak antilocalization behavior observed in Pt films is critically suppressed when the film is attached to Y3Fe5O12. Hall resistance in the Pt film is also affected by Y3Fe5O12, and it exhibits logarithmic temperature dependence in a broad temperature range. The magnetotransport properties in the high-field range are significantly influenced by the interface between Pt and Y3Fe5O12.

cond-mat.mes-hall↗

arXiv2014

High-energy spin and charge excitations in electron-doped copper oxide superconductors

The evolution of electronic (spin and charge) excitations upon carrier doping is an extremely important issue in superconducting layered cuprates and the knowledge of its asymmetry between electron- and hole-dopings is still fragmentary. Here we combine x-ray and neutron inelastic scattering measurements to track the doping dependence of both spin and charge excitations in electron-doped materials. Copper L3 resonant inelastic x-ray scattering spectra show that magnetic excitations shift to higher energy upon doping. Their dispersion becomes steeper near the magnetic zone center and deeply mix with charge excitations, indicating that electrons acquire a highly itinerant character in the doped metallic state. Moreover, above the magnetic excitations, an additional dispersing feature is observed near the Γ-point, and we ascribe it to particle-hole charge excitations. These properties are in stark contrast with the more localized spin-excitations (paramagnons) recently observed in hole-doped compounds even at high doping-levels.

cond-mat.supr-con↗

arXiv2014

Collective excitation of a short-range charge ordering in $θ$-$\mbox{(BEDT-TTF)}_2\mbox{CsZn(SCN)}_4$

We find a characteristic low-energy peak structure located in the range of 100-300 cm$^{-1}$ in the optical conductivity spectra of a quasi-two-dimensional organic compound with a triangular lattice, $θ$-$\mbox{(BEDT-TTF)}_2\mbox{CsZn(SCN)}_4$, in which two different types of short-range charge orderings (COs) coexist. Upon lowering the temperature, the low-energy peak becomes significant and shifts to much lower frequencies only for the polarization of ${E \parallel a}$, in contrast to the other broad electronic bands in the mid-infrared region. On introducing disorder, the low-energy peak is strongly suppressed in comparison with the broad electronic bands. This result indicates that the low-energy peak is attributed to a collective excitation that originates from the short-range CO with a relatively long-period $3\times3$ pattern. The present results shed light on the understanding of the low-energy excitation in the glassy electronic state, where the charge degrees of freedom remain at low temperatures.

cond-mat.str-el↗

arXiv2013

Phonon-Spectrum Narrowing Induced by Ultrafast Charge Fluctuation in an Organic Dimer Mott Insulator

We have observed the characteristic temperature dependence of the intermolecular phonon spectrum in the organic dimer Mott insulator kappa-(ET)2Cu2(CN)3 exhibiting a dielectric anomaly at 30 K. The anomalous spectral narrowing of the 55 cm-1 phonon peak at 30 K was analyzed in terms of motional narrowing within the framework of a stationary Gaussian process, i. e., the phonon frequency is modulated by the ultrafast charge fluctuation. The spectral narrowing occurs because the time constant of the correlation time tau_c and the amplitude of the frequency modulation delta satisfy the relation tau_c<delta at 30 K. At temperatures below 30 K, the motional narrowing is disturbed by the increasing of tau_c, near the charge-glass or the short-range order at 6 K. On the other hand, for temperatures above 30 K, the motional narrowing is disturbed by the increase of delta with increasing temperature.

cond-mat.str-el↗

arXiv2013

Structure of Surface-H2O Layers of Ice-covered Planets with High-pressure Ice

Many extrasolar (bound) terrestrial planets and free-floating (unbound) planets have been discovered. The existence of bound and unbound terrestrial planets with liquid water is an important question, and of particular importance is the question of their habitability. Even for a globally ice-covered planet, geothermal heat from the planetary interior may melt the interior ice, creating an internal ocean covered by an ice shell. In this paper, we discuss the conditions that terrestrial planets must satisfy for such an internal ocean to exist on the timescale of planetary evolution. The question is addressed in terms of planetary mass, distance from a central star, water abundance, and abundance of radiogenic heat sources. In addition, we investigate the structures of the surface-H2O layers of ice-covered planets by considering the effects of ice under high pressure (high-pressure ice). As a fiducial case, 1M$\oplus$ planet at 1 AU from its central star and with 0.6 to 25 times the H2O mass of Earth could have an internal ocean. We find that high-pressure ice layers may appear between the internal ocean and the rock portion on a planet with an H2O mass over 25 times that of Earth. The planetary mass and abundance of surface water strongly restrict the conditions under which an extrasolar terrestrial planet may have an internal ocean with no high-pressure ice under the ocean. Such high-pressure-ice layers underlying the internal ocean are likely to affect the habitability of the planet.

astro-ph.EP↗

arXiv2013

Thermodynamics of the Coma Cluster Outskirts

We present results from a large mosaic of Suzaku observations of the Coma Cluster, the nearest and X-ray brightest hot, dynamically active, non-cool core system, focusing on the thermodynamic properties of the ICM on large scales. For azimuths not aligned with an infalling subcluster towards the southwest, our measured temperature and X-ray brightness profiles exhibit broadly consistent radial trends, with the temperature decreasing from about 8.5 keV at the cluster center to about 2 keV at a radius of 2 Mpc, which is the edge of our detection limit. The SW merger significantly boosts the surface brightness, allowing us to detect X-ray emission out to ~2.2 Mpc along this direction. Apart from the southwestern infalling subcluster, the surface brightness profiles show multiple edges around radii of 30-40 arcmin. The azimuthally averaged temperature profile, as well as the deprojected density and pressure profiles, all show a sharp drop consistent with an outward propagating shock front located at 40 arcmin, corresponding to the outermost edge of the giant radio halo observed at 352 MHz with the WSRT. The shock front may be powering this radio emission. A clear entropy excess inside of r_500 reflects the violent merging events linked with these morphological features. Beyond r_500, the entropy profiles of the Coma Cluster along the relatively relaxed directions are consistent with the power-law behavior expected from simple models of gravitational large-scale structure formation. The pressure is also in agreement at these radii with the expected values measured from SZ data from the Planck satellite. However, due to the large uncertainties associated with the Coma Cluster measurements, we cannot yet exclude an entropy flattening in this system consistent with that seen in more relaxed cool core clusters.

astro-ph.CO↗

arXiv2013

Evolution of the electronic state through the reduction annealing in electron-doped Pr_1.3-x_La_0.7_Ce_x_CuO_4+delta_ (x=0.10) single crystals: Antiferromagnetism, Kondo effect and superconductivity

The evolution of the electronic state through the reduction annealing has been investigated in electron-doped Pr_1.3-x_La_0.7_Ce_x_CuO_4+delta_ (x=0.10) single crystals with the so-called T' structure. From the ab plane and c axis electrical resistivity measurements in magnetic fields, it has been found that, through the reduction annealing, the strongly localized state of carriers accompanied by the antiferromagnetic (AF) pseudogap in the as-grown crystal changes to a metallic state bringing about the Kondo effect without AF pseudogap and to a superconducting state. These results are able to be understood in terms of a model based on the strong electron correlation. The complete removal of excess oxygen in the T'-cuprates is expected to result in the appearance of superconductivity in a wide range of the Ce concentration including the parent compound of x=0.

cond-mat.supr-con↗

arXiv2013

Relaxor ferroelectricity induced by electron correlations in a molecular dimer Mott insulator

We have investigated the dielectric response in an antiferromagnetic dimer-Mott insulator beta'-(BEDT-TTF)2ICl2 with square lattice, compared to a spin liquid candidate kappa-(BEDT-TTF)2Cu2(CN)3. Temperature dependence of the dielectric constant shows a peak structure obeying Curie-Weiss law with strong frequency dependence. We found an anisotropic ferroelectricity by pyrocurrent measurements, which suggests the charge disproportionation in a dimer. The ferroelectric actual charge freezing temperature is related to the antiferromagnetic interaction, which is expected to the charge-spin coupled degrees of freedom in the system.

cond-mat.str-el↗

arXiv2013

Collective excitation of electric dipole on molecular dimer in organic dimer-Mott insulator

The terahertz (THz) response in 10-100 cm^-1 was investigated in an organic dimer-Mott (DM) insulator kappa-(ET)_2Cu_2(CN)_3 that exhibits a relaxor-like dielectric anomaly. 30 cm^-1 band in the optical conductivity was attributable to collective excitation of the intra-dimer electric dipoles which are formed by an electron correlation. We succeeded in observing photoinduced enhancement of this 30 cm^-1 band, reflecting the growth of the electric dipole cluster in the DM phase. Such optical responses in kappa-(ET)_2Cu_2(CN)_3 reflect instability near the boundary between the DM-ferroelectric charge ordered phases.

cond-mat.str-el↗

arXiv2013

Metal-mass-to-light ratios of the Perseus cluster out to the virial radius

We analyzed XMM-Newton data of the Perseus cluster out to $\sim$1 Mpc, or approximately half the virial radius. Using the flux ratios of Lyalpha lines of H-like Si and S to Kalpha line of He-like Fe, the abundance ratios of Si/Fe and S/Fe of the intracluster medium (ICM) were derived using the APEC plasma code v2.0.1. The temperature dependence of the line ratio limits the systematic uncertainty in the derived abundance ratio. The Si/Fe and S/Fe in the ICM of the Perseus cluster show no radial gradient. The emission-weighted averages of the Si/Fe and S/Fe ratios outside the cool core are 0.91 +- 0.08 and 0.93 +- 0.10, respectively, in solar units according to the solar abundance table of Lodders (2003). These ratios indicate that most Fe was synthesized by supernovae Ia. We collected K-band luminosities of galaxies and calculated the ratio of Fe and Si mass in the ICM to K-band luminosity, iron-mass-to-light ratio (IMLR) and silicon-mass-to-light ratio (SMLR). Within $\sim$1 Mpc, the cumulative IMLR and SMLR increase with radius. Using Suzaku data for the northwest and east directions, we also calculated the IMLR out to $\sim$ 1.8 Mpc, or about the virial radius. We constrained the SMLR out to this radius and discussed the slope of the initial mass function of stars in the cluster. Using the cumulative IMLR profile, we discuss the past supernova Ia rate.

astro-ph.CO↗

arXiv2012

Two-band superconductivity featuring different anisotropies in the ternary iron silicide Lu$_{2}$Fe$_{3}$Si$_{5}$

We report detailed studies of the upper critical field and low-temperature specific heat in the two-gap superconductor Lu$_{2}$Fe$_{3}$Si$_{5}$. The anisotropy of the upper critical field suggests that the active band is quasi-one-dimensional. Low-temperature specific heat in magnetic fields reveals that the virtual $H_{c2}$ in the passive band is almost isotropic. These results strongly indicate that the two bands have two different anisotropies, similar to the typical two-gap superconductor MgB$_{2}$, and their interplay may be essential to the two-gap superconductivity in Lu$_{2}$Fe$_{3}$Si$_{5}$.

cond-mat.supr-con↗

arXiv2011

Observation of weak temperature dependence of spin diffusion length in highly-doped Si by using a non-local 3-terminal method

We conduct an experimental investigation of temperature dependence of spin diffusion length in highly-doped n-type silicon by using a non-local 3-terminal method. Whereas an effect of spin drift is not ignorable to bias- and temperature-dependence of spin signals in non-metallic systems except for the case of a non-local 4-terminal method, it is not fully conclusive how the spin drift affects spin transport properties in highly-doped Si in a non-local 3-terminal method that is often used in Si spintronics. Here, we report on temperature dependence of spin diffusion length in the Si, and it is clarified that the spin transport is less affected by an external electric field.

cond-mat.mtrl-sci↗

arXiv2011

Study of the K0(L) --> pi0 pi0 nu nu-bar decay

The rare decay K0(L) --> pi0 pi0 nu nu-bar was studied with the E391a detector at the KEK 12-GeV proton synchrotron. Based on 9.4 x 10^9 K0L decays, an upper limit of 8.1 x 10^{-7} was obtained for the branching fraction at 90% confidence level. We also set a limit on the K0(L) --> pi0 pi0 X (X --> invisible particles) process; the limit on the branching fraction varied from 7.0 x 10^{-7} to 4.0 x 10^{-5} for the mass of X ranging from 50 MeV/c^2 to 200 MeV/c^2.

hep-ex↗

arXiv2011

Suppression of superconductivity by non-magnetic disorder in organic superconductor $κ$-(BEDT-TTF)$_{2}$Cu(NCS)$_{2}$

The suppression of superconductivity by nonmagnetic disorder is investigated systematically in the organic superconductor $κ$-(BEDT-TTF)$_2$Cu(NCS)$_2$. We introduce a nonmagnetic disorder arising from molecule substitution in part with deuterated BEDT-TTF or BMDT-TTF for BEDT-TTF molecules and molecular defects introduced by X-ray irradiation. A quantitative evaluation of the scattering time $τ_{\rm dHvA}$ is carried out by de Haas-van Alphen (dHvA) effect measurement. A large reduction in $T_{\rm c}$ with a linear dependence on $1/τ_{\rm dHvA}$ is found in the small-disorder region below $1/τ_{\rm dHvA} \simeq$ 1 $\times$ 10$^{12}$ s$^{-1}$ in both the BMDT-TTF molecule-substituted and X-ray-irradiated samples. The observed linear relation between $T_{\rm c}$ and $1/τ_{\rm dHvA}$ is in agreement with the Abrikosov-Gorkov (AG) formula, at least in the small-disorder region. This observation is reasonably consistent with the unconventional superconductivity proposed thus far for the present organic superconductor. A deviation from the AG formula, however, is observed in the large-disorder region above $1/τ_{\rm dHvA} \simeq$ 1 $\times$ 10$^{12}$ s$^{-1}$, which reproduces the previous transport study (J. G. Analytis {\it et al.}: Phys. Rev. Lett. {\bf 96} (2006) 177002). We present some interpretations of this deviation from the viewpoints of superconductivity and the inherent difficulties in the evaluation of scattering time.

cond-mat.supr-con↗

arXiv2011

Two pseudogaps with different energy scales at the antinode of the high-temperature Bi$_2$Sr$_2$CuO$_6$ superconductor using angle-resolved photoemission spectroscopy

We have performed high-resolution angle-resolved photoemission spectroscopy on single-layered cuprate Bi$_2$Sr$_2$CuO$_6$ to clarify the origin of the pseudogap. By using various photon energies, we have succeeded in directly observing two different pseudogaps with two different energy scales which coexist in the antinodal region: one reflects the $d_{x^2-y^2}$-wave pairing strength while the other has a larger energy scale suggesting an origin distinct from superconductivity. The observed two-pseudogap behavior provides a key to fully understand the pseudogap phenomena in cuprates.

cond-mat.supr-con↗

arXiv2010

Search for the decay $K_L^0 \rightarrow 3γ$

We performed a search for the decay $K_L^0 \rightarrow 3γ$ with the E391a detector at KEK. In the data accumulated in 2005, no event was observed in the signal region. Based on the assumption of $K_L^0 \rightarrow 3γ$ proceeding via parity-violation, we obtained the single event sensitivity to be $(3.23\pm0.14)\times10^{-8}$, and set an upper limit on the branching ratio to be $7.4\times10^{-8}$ at the 90% confidence level. This is a factor of 3.2 improvement compared to the previous results. The results of $K_L^0 \rightarrow 3γ$ proceeding via parity-conservation were also presented in this paper.

hep-ex↗