arXiv subjects

T. Shibauchi

Publications and source records attributed to T. Shibauchi.

At least 91 records · Page 5Linked to original sources

arXiv2015

Thermal conductivity of quantum magnetic monopoles in the frustrated pyrochlore Yb2Ti2O7

We report low-temperature thermal conductivity $κ$ of pyrochlore Yb$_2$Ti$_2$O$_7$, which contains frustrated spin-ice correlations with significant quantum fluctuations. In the disordered spin-liquid regime, $κ(H)$ exhibits a nonmonotonic magnetic field dependence, which is well explained by the strong spin-phonon scattering and quantum monopole excitations. We show that the excitation energy of quantum monopoles is strongly suppressed from that of dispersionless classical monopoles. Moreover, in stark contrast to the diffusive classical monopoles, the quantum monopoles have a very long mean free path. We infer that the quantum monopole is a novel heavy particle, presumably boson, which is highly mobile in a three-dimensional spin liquid.

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arXiv2015

Evidence for time-reversal symmetry breaking of the superconducting state near twin-boundary interfaces in FeSe

Junctions and interfaces consisting of unconventional superconductors provide an excellent experimental playground to study exotic phenomena related to the phase of the order parameter. Not only the complex structure of unconventional order parameters have an impact on the Josephson effects, but also may profoundly alter the quasi-particle excitation spectrum near a junction. Here, by using spectroscopic-imaging scanning tunneling microscopy, we visualize the spatial evolution of the local density of states (LDOS) near twin boundaries (TBs) of the nodal superconductor FeSe. The $π/2$ rotation of the crystallographic orientation across the TB twists the structure of the unconventional order parameter, which may, in principle, bring about a zero-energy LDOS peak at the TB. The LDOS at the TB observed in our study, in contrast, does not exhibit any signature of a zero-energy peak and an apparent gap amplitude remains finite all the way across the TB. The low-energy quasiparticle excitations associated with the gap nodes are affected by the TB over a distance more than an order of magnitude larger than the coherence length $ξ_{ab}$. The modification of the low-energy states is even more prominent in the region between two neighboring TBs separated by a distance $\approx7ξ_{ab}$. In this region the spectral weight near the Fermi level ($\approx\pm$0.2~meV) due to the nodal quasiparticle spectrum is almost completely removed. These behaviors suggest that the TB induces a fully-gapped state, invoking a possible twist of the order parameter structure which breaks time-reversal symmetry.

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arXiv2015

Momentum-dependent sign-inversion of orbital polarization in superconducting FeSe

We investigate the electronic reconstruction across the tetragonal-orthorhombic structural transition in FeSe by employing polarization-dependent angle-resolved photoemission spectroscopy (ARPES) on detwinned single crystals. Across the structural transition, the electronic structures around the G and M points are modified from four-fold to two-fold symmetry due to the lifting of degeneracy in dxz/dyz orbitals. The dxz band shifts upward at the G point while it moves downward at the M point, suggesting that the electronic structure of orthorhombic FeSe is characterized by a momentum-dependent sign-changing orbital polarization. The elongated directions of the elliptical Fermi surfaces (FSs) at the G and M points are rotated by 90 degrees with respect to each other, which may be related to the absence of the antiferromagnetic order in FeSe.

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arXiv2015

Dichotomy between the hole and electrons behavior in the multiband FeSe probed by ultra high magnetic fields

Magnetoresistivity \r{ho}xx and Hall resistivity \r{ho}xy in ultra high magnetic fields up to 88T are measured down to 0.15K to clarify the multiband electronic structure in high-quality single crystals of superconducting FeSe. At low temperatures and high fields we observe quantum oscillations in both resistivity and Hall effect, confirming the multiband Fermi surface with small volumes. We propose a novel and independent approach to identify the sign of corresponding cyclotron orbit in a compensated metal from magnetotransport measurements. The observed significant differences in the relative amplitudes of the quantum oscillations between the \r{ho}xx and \r{ho}xy components, together with the positive sign of the high-field \r{ho}xy , reveal that the largest pocket should correspond to the hole band. The low-field magnetotransport data in the normal state suggest that, in addition to one hole and one almost compensated electron bands, the orthorhombic phase of FeSe exhibits an additional tiny electron pocket with a high mobility.

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arXiv2014

Anomalous critical fields in quantum critical superconductors

Fluctuations around an antiferromagnetic quantum critical point (QCP) are believed to lead to unconventional superconductivity and in some cases to high-temperature superconductivity. However, the exact mechanism by which this occurs remains poorly understood. The iron-pnictide superconductor BaFe$_2$(As$_{1-x}$P$_x$)$_2$ is perhaps the clearest example to date of a high temperature quantum critical superconductor, and so it is a particularly suitable system in which to study how the quantum critical fluctuations affect the superconducting state. Here we show that the proximity of the QCP yields unexpected anomalies in the superconducting critical fields. We find that both the lower and upper critical fields strongly violate the expectations from the conventional theory taking into account the observed mass enhancement near the QCP. These anomalous behaviours of the critical fields imply that the energy of superconducting vortices is enhanced, possibly due to a microscopic mixing of antiferromagnetism and superconductivity, suggesting that a highly unusual vortex state is realised in quantum critical superconductors.

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arXiv2014

Fermi surface of IrTe2 in the valence-bond state as determined by quantum oscillations

We report the observation of the de Haas-van Alphen effect in IrTe2 measured using torque magnetometry at low temperatures down to 0.4 K and in high magnetic fields up to 33T. IrTe2 undergoes a major structural transition around 283 K due to the formation of planes of Ir and Te dimers that cut diagonally through the lattice planes, with its electronic structure predicted to change significantly from a layered system with predominantly three-dimensional character to a tilted quasi-two dimensional Fermi surface. Quantum oscillations provide direct confirmation of this unusual tilted Fermi surface and also reveal very light quasiparticle masses (less than 1 me), with no significant enhancement due to electronic correlations. We find good agreement between the angular dependence of the observed and calculated de Haas-van Alphen frequencies, taking into account the contribution of different structural domains that form while cooling IrTe2.

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arXiv2014

Colossal thermomagnetic response in the exotic superconductor URu2Si2

When a superconductor is heated above its critical temperature $T_c$, macroscopic coherence vanishes, leaving behind droplets of thermally fluctuating Cooper pair. This superconducting fluctuation effect above $T_c$ has been investigated for many decades and its influence on the transport, thermoelectric and thermodynamic quantities in most superconductors is well understood by the standard Gaussian fluctuation theories. The transverse thermoelectric (Nernst) effect is particularly sensitive to the fluctuations, and the large Nernst signal found in the pseudogap regime of the underdoped high-$T_c$ cuprates has raised much debate on its connection to the origin of superconductivity. Here we report on the observation of a colossal Nernst signal due to the superconducting fluctuations in the heavy-fermion superconductor URu$_2$Si$_2$. The Nernst coefficient is enhanced by as large as one million times over the theoretically expected value within the standard framework of superconducting fluctuations. This, for the first time in any known material, results in a sizeable thermomagnetic figure of merit approaching unity. Moreover, contrary to the conventional wisdom, the enhancement in the Nernst signal is more significant with the reduction of the impurity scattering rate. This anomalous Nernst effect intimately reflects the highly unusual superconducting state embedded in the so-called hidden-order phase of URu$_2$Si$_2$. The results invoke possible chiral or Berry-phase fluctuations originated from the topological aspect of this superconductor, which are associated with the effective magnetic field intrinsically induced by broken time-reversal symmetry of the superconducting order parameter.

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arXiv2014

Field-induced superconducting phase of FeSe in the BCS-BEC cross-over

Fermi systems in the crossover regime between weakly coupled Bardeen-Cooper-Schrieffer (BCS) and strongly coupled Bose-Einstein-condensate (BEC) limits are among the most fascinating objects to study the behavior of an assembly of strongly interacting particles. The physics of this crossover has been of considerable interest both in the fields of condensed matter and ultracold atoms. One of the most challenging issue in this regime is the effect of large spin imbalance on a Fermi system under magnetic fields. Although several exotic physical properties have been predicted theoretically, the experimental realization of such an unusual superconducting state has not been achieved so far. Here we show that pure single crystals of superconducting FeSe offer the possibility to enter the previously unexplored realm where the three energies, Fermi energy $\varepsilon_{\rm F}$, superconducting gap $Δ$ and Zeeman energy, become comparable. Through the superfluid response, transport, thermoelectric response, and spectroscopic-imaging scanning tunneling microscopy, we demonstrate that $\varepsilon_{\rm F}$ of FeSe is extremely small, with the ratio $Δ/\varepsilon_{\rm F}\sim1 (\sim0.3)$ in the electron (hole) band. Moreover, thermal-conductivity measurements give evidence of a distinct phase line below the upper critical field, where the Zeeman energy becomes comparable to $\varepsilon_{\rm F}$ and $Δ$. The observation of this field-induced phase provides insights into previously poorly understood aspects of the highly spin-polarized Fermi liquid in the BCS-BEC crossover regime.

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arXiv2014

Superconducting gap structure of BaFe_2(As_{1-x}P_{x})_2

We present a study of the superconducting gap structure in the iron-pnictide series BaFe2(As1-xPx)2. By measuring the variation of the specific heat as a function of temperature and magnetic field we are able to determine the number and Fermi surface location of the nodes in the superconducting gap. In particular, from measurements of the variation of the specific heat as the magnetic field is rotated in the ab plane of the sample we conclude that the nodes are in the [110] directions. Then from a quantitative analysis of the temperature and field dependence of the specific heat we further conclude that nodes exists on all Fermi surface sheets.

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arXiv2014

Structural origin of the anomalous temperature dependence of the local magnetic moments in the CaFe$_{2}$As$_{2}$ family of materials

We report a combination of Fe K$β$ x-ray emission spectroscopy and $ab$-intio calculations to investigate the correlation between structural and magnetic degrees of freedom in CaFe$_{2}$(As$_{1-x}$P$_{x} $)$_{2}$. The puzzling temperature behavior of the local moment found in rare earth-doped CaFe$_{2}$As$_{2}$ [\textit{H. Gretarsson, et al., Phys. Rev. Lett. {\bf 110}, 047003 (2013)}] is also observed in CaFe$_{2}$(As$_{1-x}$P$_{x}$)$_{2}$. We explain this phenomenon based on first-principles calculations with scaled magnetic interaction. One scaling parameter is sufficient to describe quantitatively the magnetic moments in both CaFe$_{2}$(As$_{1-x}$P$_{x} $)$_{2}$ ($x=0.055$) and Ca$_{0.78}% $La$_{0.22}$Fe$_{2}$As$_{2}$ at all temperatures. The anomalous growth of the local moments with increasing temperature can be understood from the observed large thermal expansion of the $c$-axis lattice parameter combined with strong magnetoelastic coupling. These effects originate from the strong tendency to form As-As dimers across the Ca layer in the CaFe$_{2}$As$_{2}$ family of materials. Our results emphasize the dual local-itinerant character of magnetism in Fe pnictides.

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arXiv2014

Direct observation of lattice symmetry breaking at the hidden-order transition in URu2Si2

Since the 1985 discovery of the phase transition at $T_{\rm HO}=17.5$ K in the heavy-fermion metal URu$_2$Si$_2$, neither symmetry change in the crystal structure nor magnetic ordering have been observed, which makes this "hidden order" enigmatic. Some high-field experiments have suggested electronic nematicity which breaks fourfold rotational symmetry, but direct evidence has been lacking for its ground state at zero magnetic field. Here we report on the observation of lattice symmetry breaking from the fourfold tetragonal to twofold orthorhombic structure by high-resolution synchrotron X-ray diffraction measurements at zero field, which pins down the space symmetry of the order. Small orthorhombic symmetry-breaking distortion sets in at $T_{\rm HO}$ with a jump, uncovering the weakly first-order nature of the hidden-order transition. This distortion is observed only in ultrapure sample, implying a highly unusual coupling nature between the electronic nematicity and underlying lattice.

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arXiv2014

Broken symmetries in URu2Si2

To resolve the nature of the hidden order below 17.5\,K in the heavy fermion compound URu$_2$Si$_2$, identifying which symmetries are broken below the hidden order transition is one of the most important steps. Several recent experiments on the electronic structure have shown that the Fermi surface in the hidden order phase is quite close to the result of band-structure calculations within the framework of itinerant electron picture assuming the antiferromagnetism. This provides strong evidence for the band folding along the c-axis with the ordering vector of $(0\,0\,1)$, corresponding to broken translational symmetry. In addition to this, there is growing evidence for fourfold rotational symmetry breaking in the hidden-order phase from measurements of the in-plane magnetic anisotropy and the effective mass anisotropy in the electronic structure, as well as the orthorhombic lattice distortion. This broken fourfold symmetry gives a stringent constraint that the symmetry of the hidden order parameter should belong to the degenerate $E$-type irreducible representation. We also discuss a possibility that time reversal symmetry is also broken, which further narrows down the order parameter that characterizes the hidden order.

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arXiv2014

Disorder-induced topological change of the superconducting gap structure in iron pnictides

In superconductors with unconventional pairing mechanisms, the energy gap in the excitation spectrum often has nodes, which allow quasiparticle excitations at low energies. In many cases, e.g. $d$-wave cuprate superconductors, the position and topology of nodes are imposed by the symmetry, and thus the presence of gapless excitations is protected against disorder. Here we report on the observation of distinct changes in the gap structure of iron-pnictide superconductors with increasing impurity scattering. By the successive introduction of nonmagnetic point defects into BaFe$_2$(As$_{1-x}$P$_x$)$_2$ crystals via electron irradiation, we find from the low-temperature penetration depth measurements that the nodal state changes to a nodeless state with fully gapped excitations. Moreover, under further irradiation the gapped state evolves into another gapless state, providing bulk evidence of unconventional sign-changing $s$-wave superconductivity. This demonstrates that the topology of the superconducting gap can be controlled by disorder, which is a strikingly unique feature of iron pnictides.

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arXiv2014

On infrared pseudogap in cuprate and pnictide high-temperature superconductors

We investigate infrared manifestations of the pseudogap in the prototypical cuprate and pnictide superconductors: YBa2Cu3Oy and BaFe2As2 (Ba122) systems. We find remarkable similarities between the spectroscopic features attributable to the pseudogap in these two classes of superconductors. The hallmarks of the pseudogap state in both systems include a weak absorption feature at about 500 cm-1 followed by a featureless continuum between 500 and 1500 cm-1 in the conductivity data and a significant suppression in the scattering rate below 700 - 900 cm-1. The latter result allows us to identify the energy scale associated with the pseudogap $Δ_{PG}$. We find that in the Ba122-based materials the superconductivity-induced changes of the infrared spectra occur in the frequency region below 100 - 200 cm-1, which is much lower than the energy scale of the pseudogap. We performed theoretical analysis of the scattering rate data of the two compounds using the same model which accounts for the effects of the pseudogap and electron-boson coupling. We find that the scattering rate suppression in Ba122-based compounds below $Δ_{PG}$ is solely due to the pseudogap formation whereas the impact of the electron-boson coupling effects is limited to lower frequencies. The magnetic resonance modes used as inputs in our modeling are found to evolve with the development of the pseudogap, suggesting an intimate correlation between the pseudogap and magnetism.

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arXiv2014

Controllable Rashba spin-orbit interaction in artificially engineered superlattices involving the heavy-fermion superconductor CeCoIn5

By using a molecular beam epitaxy technique, we fabricate a new type of superconducting superlattices with controlled atomic layer thicknesses of alternating blocks between heavy fermion superconductor CeCoIn_5, which exhibits a strong Pauli pair-breaking effect, and nonmagnetic metal YbCoIn_5. The introduction of the thickness modulation of YbCoIn_5 block layers breaks the inversion symmetry centered at the superconducting block of CeCoIn_5. This configuration leads to dramatic changes in the temperature and angular dependence of the upper critical field, which can be understood by considering the effect of the Rashba spin-orbit interaction arising from the inversion symmetry breaking and the associated weakening of the Pauli pair-breaking effect. Since the degree of thickness modulation is a design feature of this type of superlattices, the Rashba interaction and the nature of pair-breaking are largely tunable in these modulated superlattices with strong spin-orbit coupling.

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arXiv2013

Cyclotron resonance study of quasiparticle mass and scattering rate in the hidden-order and superconducting phases of URu2Si2

The observation of cyclotron resonance in ultra-clean crystals of URu2Si2 [S. Tonegawa et al., PRL 109, 036401 (2012)] provides another route besides quantum oscillations to the determination of the bulk electronic structure in the hidden order phase. We report detailed analyses of the resonance lines, which fully resolve the cyclotron mass structure of the main Fermi surface sheets. A particular focus is given to the anomalous splitting of the sharpest resonance line near the [110] direction under in-plane magnetic-field rotation, which implies peculiar electronic structure in the hidden order phase. The results under the field rotation from [110] toward [001] direction reveal that the splitting is a robust feature against field tilting from the basal plane. This is in sharp contrast to the reported frequency branch alpha in the quantum oscillation experiments showing a three-fold splitting that disappears by a small field tilt, which can be explained by the magnetic breakdown between the large hole sphere and small electron pockets. Our analysis of the cyclotron resonance profiles reveals that the heavier branch of the split line has a larger scattering rate, providing evidence for the existence of hot-spot regions along the [110] direction. These results are consistent with the broken fourfold rotational symmetry in the hidden-order phase, which can modify the interband scattering in an asymmetric manner. We also extend our measurements down to 0.7 K, which results in the observation of cyclotron resonance in the superconducting state, where novel effects of vortex dynamics may enter. We find that the cyclotron mass undergoes no change in the superconducting state. In contrast, the quasiparticle scattering rate shows a rapid decrease below the vortex-lattice melting transition temperature, which supports the formation of quasiparticle Bloch state in the vortex lattice phase.

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arXiv2013

Pseudogap formation above the superconducting dome in iron-pnictides

The nature of the pseudogap in high transition temperature (high-Tc) superconducting cuprates has been a major issue in condensed matter physics. It is still unclear whether the high-Tc superconductivity can be universally associated with the pseudogap formation. Here we provide direct evidence of the existence of the pseudogap phase via angle-resolved photoemission spectroscopy in another family of high-Tc superconductor, iron-pnictides. Our results reveal a composition dependent pseudogap formation in the multi-band electronic structure of BaFe2(As1-xPx)2. The pseudogap develops well above the magnetostructural transition for low x, persists above the nonmagnetic superconducting dome for optimal x and is destroyed for x ~ 0.6, thus showing a notable similarity with cuprates. In addition, the pseudogap formation is accompanied by inequivalent energy shifts in xz/yz orbitals of iron atoms, indicative of a peculiar iron orbital ordering which breaks the four-fold rotational symmetry.

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arXiv2013

Superconducting gap with sign reversal between hole pockets in heavily hole-doped Ba1-xKxFe2As2

To gain insight into the unconventional superconductivity of Fe-pnictides with no electron pockets, we measure the thermal conductivity $κ$ and penetration depth $λ$ in the heavily hole-doped regime of Ba$_{1-x}$K$_x$Fe$_2$As$_2$. The residual thermal conductivity $(κ/T)_{T \rightarrow 0\,{\rm K}}$ and $T$-dependence of $λ$ consistently indicate the fully gapped superconductivity at $x=0.76$ and the (line) nodal superconductivity at higher hole concentrations. The magnitudes of $\fracκ{T}\cdot T_c|_{T \rightarrow 0\,{\rm K}}$ and $\frac{dλ}{d(T/T_c)}$ at low temperatures, both of which are determined by the properties of the low-energy excitations, exhibit a highly unusual non-monotonic x-dependence. These results indicate a dramatic change of the nodal characteristics in a narrow doping range, suggesting a doping crossover of the gap function between the s-wave states with and without sign reversal between $Γ$-centered hole pockets.

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