arXiv subjects

T. Stauber

Publications and source records attributed to T. Stauber.

At least 19 recordsLinked to original sources

arXiv2025

Roadmap for Photonics with 2D Materials

Triggered by the development of exfoliation and the identification of a wide range of extraordinary physical properties in self-standing films consisting of one or few atomic layers, two-dimensional (2D) materials such as graphene, transition metal dichalcogenides (TMDs), and other van der Waals (vdW) crystals currently constitute a wide research field protruding in multiple directions in combination with layer stacking and twisting, nanofabrication, surface-science methods, and integration into nanostructured environments. Photonics encompasses a multidisciplinary collection of those directions, where 2D materials contribute with polaritons of unique characteristics such as strong spatial confinement, large optical-field enhancement, long lifetimes, high sensitivity to external stimuli (e.g., electric and magnetic fields, heating, and strain), a broad spectral range from the far infrared to the ultraviolet, and hybridization with spin and momentum textures of electronic band structures. The explosion of photonics with 2D materials as a vibrant research area is producing breakthroughs, including the discovery and design of new materials and metasurfaces with unprecedented properties as well as applications in integrated photonics, light emission, optical sensing, and exciting prospects for applications in quantum information, and nanoscale thermal transport. This Roadmap summarizes the state of the art in the field, identifies challenges and opportunities, and discusses future goals and how to meet them through a wide collection of topical sections prepared by leading practitioners.

cond-mat.mtrl-sci↗

arXiv2023

Zigzag materials: selective interchain couplings control the coexistence of one-dimensional physics and deviations from it

The coexistence in the low-temperature spin-conducting phases of the zigzag materials BaCo2V2O8 and SrCo2V2O8 of one-dimensional (1D) physics with important deviations from it is not well understood. The studies of this paper account for an important selection rule that follows from interchain spin states being coupled more strongly within the spin dynamical structure factor of such zigzag materials whenever they are connected by a specific symmetry operation of the underlying lattice. In the case of excited states, this symmetry operation is only a symmetry in spin-space ifno electronic spin flip is performed within the generation of such states. Our results on both the role of selective interchain couplings in protecting the 1D physics and being behind deviations from it and on the dynamical properties being controlled by scattering of singlet pairs of physical spins 1/2 open the door to a key advance in the understanding of the physics of the spin chains in BaCo2V2O8 and SrCo2V2O8.

cond-mat.str-el↗

arXiv2023

Ising superconductivity induced from spin-selective valley symmetry breaking in twisted trilayer graphene

We show that the $e$-$e$ interaction induces a strong breakdown of valley symmetry for each spin channel in twisted trilayer graphene, leading to a ground state where the two spin projections have opposite sign of the valley symmetry breaking order parameter. This leads to a spin-valley locking in which the electrons of a Cooper pair are forced to live on different Fermi lines attached to opposite valleys. Furthermore, we find an effective intrinsic spin-orbit coupling explaining the protection of the superconductivity against in-plane magnetic fields. The effect of spin-selective valley symmetry breaking is validated as it reproduces the experimental observation of the reset of the Hall density at 2-hole doping. It also implies a breakdown of the symmetry of the bands from $C_6$ to $C_3$, with an enhancement of the anisotropy of the Fermi lines which is at the origin of a Kohn-Luttinger (pairing) instability. The isotropy of the bands is gradually recovered, however, when the Fermi level approaches the bottom of the second valence band, explaining why the superconductivity fades away in the doping range beyond 3 holes per moiré unit cell in twisted trilayer graphene.

cond-mat.supr-con↗

arXiv2023

Neutral magic-angle bilayer graphene: Condon instability and chiral resonances

We discuss the full optical response of twisted bilayer graphene at the neutrality point close to the magic angle within the continuum model (CM). Firstly, we identify three different channels consistent with the underlying $D_3$ symmetry, yielding the total, magnetic, and chiral response. Secondly, we numerically calculate the full optical response in the immediate vicinity of the magic angle $θ_m$ which provides a direct mapping of the CM onto an effective two-band model. We, further, show that the ground-state of the CM in the immediate vicinity of $θ_m$ is unstable towards transverse current fluctuations, a so-called Condon instability. Thirdly, due to the large counterflow, the acoustic plasmonic excitations with typical wave numbers have larger energies than the optical ones and their energy density may be largely enhanced at certain frequencies which we denominate as {\it chiral resonances}. Finally, we discuss symmetry relations for the optical response and their consequences for the chiral response.

cond-mat.mes-hall↗

arXiv2023

Universal mechanism of Ising superconductivity in twisted bilayer, trilayer and quadrilayer graphene

We show that the superconducivity in twisted graphene multilayers originates from a common feature, which is the strong valley symmetry breaking characteristic of these moiré systems at the magic angle. This leads to a breakdown of the rotational symmetry of the flat moiré bands down to $C_3$, and to ground states in which the time-reversal symmetry is broken for a given spin projection. However, this symmetry can be recovered upon exchange of spin-up and spin-down electrons, as we illustrate by means of a self-consistent microscopic Hartree-Fock resolution where the states for the two spin projections acquire opposite sign of the valley polarization. There is then a spin-valley locking by which the Fermi lines for the two spin projections are different and related by inversion symmetry. This effect represents a large renormalization of the bare spin-orbit coupling of the graphene multilayers, lending protection to the superconductivity against in-plane magnetic fields. In the twisted bilayer as well as in trilayer and quadrilayer graphene, the pairing glue is shown to be given by the nesting between parallel segments of the Fermi lines which arise from the breakdown of symmetry down to $C_3$. This leads to a strong Kohn-Luttinger pairing instability, which is relevant until the Fermi line recovers gradually a more isotropic shape towards the bottom of the second valence band, explaining why the superconductivity fades away beyond three-hole doping of the moiré unit cell.

cond-mat.mes-hall↗

arXiv2021

Collective magnetic excitations in AA- and AB-stacked graphene bilayers

We discuss novel transverse plasmon-polaritons that are hosted by AA- and AB-stacked bilayer graphene due to perfect nesting. They are composed of oscillating counterflow currents in between the layers, giving a clear interpretation for these collective modes as magnetic excitations carrying magnetic moment parallel to the planes. For AA-stacked bilayer graphene, these modes can reach zero frequency at the neutrality point and we thus predict a symmetry broken ground-state leading to in-plane orbital ferromagnetism. Even though it could be hard to detect them in real solid-state devices, these novel magnetic plasmons should be observable in artificial set-ups such as optical lattices. Also, our results might be relevant for magic angle twisted bilayer graphene samples as their electronic properties are mostly determined by confined AA-stacked regions.

cond-mat.mes-hall↗

arXiv2021

Magnetic phases from competing Hubbard and extended Coulomb interactions in twisted bilayer graphene

We implement a self-consistent Hartree-Fock approximation based on a microscopic model in real space, which allows us to consider the interplay between the Hubbard and the extended Coulomb interaction in twisted bilayer graphene at the magic angle. These two interactions tend to favor different symmetry breaking patterns, having therefore complementary roles in the regimes where one or the other dominates. We show that, for sufficiently large values of the on-site Hubbard repulsion, magic angle graphene has an antiferromagnetic ground state at the charge neutrality point, while at half-filling of the lowest valence band the state becomes fully spin-polarized. In general, a suitable screening of the extended Coulomb interaction is required to observe the magnetic state in either case, as otherwise the instabilities take place in the charge sector, preferentially in the form of time-reversal, chiral or valley symmetry breaking.

cond-mat.mes-hall↗

arXiv2020

Flat-band ferromagnetism in twisted bilayer graphene

We discuss twisted bilayer graphene (TBG) based on a theorem of flat band ferromagnetism put forward by Mielke and Tasaki. According to this theorem, ferromagnetism occurs if the single particle density matrix of the flat band states is irreducible and we argue that this result can be applied to the quasi-flat bands of TBG that emerge around the charge-neutrality point for twist angles around the magic angle $θ\sim1.05^\circ$. We show that the density matrix is irreducible in this case, thus predicting a ferromagnetic ground state for neutral TBG ($n=0$). We then show that the theorem can also be applied only to the flat conduction or valence bands, if the substrate induces a single-particle gap at charge neutrality. Also in this case, the corresponding density matrix turns out to be irreducible, leading to ferromagnetism at half filling ($n=\pm2$).

cond-mat.str-el↗

arXiv2020

Plasmon-enhanced near-field chirality in twisted van der Waals heterostructures

It is shown that chiral plasmons, characterized by a longitudinal magnetic moment accompanying the longitudinal charge plasmon, lead to electromagnetic near-fields that are also chiral. For twisted bilayer graphene, we estimate that the near field chirality of screened plasmons can be several orders of magnitude larger than that of the related circularly polarized light. The chirality also manifests itself in a deflection angle that is formed between the direction of the plasmon propagation and its Poynting vector. Twisted van der Waals heterostructures might thus provide a novel platform to promote enantiomer-selective physio-chemical processes in chiral molecules without the application of a magnetic field or external nano-patterning that break time-reversal, mirror plane or inversion symmetry, respectively.

cond-mat.mes-hall↗

arXiv2020

Change of chirality at magic angles of twisted bilayer graphene

We derive a simple formula for the real-space chirality of twisted bilayer graphene that can be related to the cross-product of its sheet currents. This quantity shows well-defined plateaus for the first remote band as function of the gate voltage which are approximately quantized for commensurate twist angles. The zeroth plateau corresponds to the first magic angle where a sign change occurs due to an emergent $C_6$-symmetry. Our observation offers a new definition of the magic angle based on a macroscopic observable which is accessible in typical transport experiments.

cond-mat.mes-hall↗

arXiv2020

Emergent magnetic texture in driven twisted bilayer graphene

The transport properties of a twisted bilayer graphene barrier are investigated for various twist angles. Remarkably, for small twist angles around the magic angle $θ_m \sim 1.05^{\circ}$, the local currents around the AA-stacked regions are strongly enhanced compared to the injected electron rate. Furthermore, the total and counterflow (magnetic) current patterns show high correlations in these regions, given rise to well-defined magnetic moments that form a magnetic Moiré superlattice. The orientation and magnitude of these magnetic moments changes as function of the gate voltage and possible implications for emergent spin-liquid behaviour are discussed.

cond-mat.mes-hall↗

arXiv2020

Non-local quantum effects in plasmons of graphene superlattices

By using a non-local, quantum mechanical response function we study graphene plasmons in a one-dimensional superlattice (SL) potential $V_0 \cos G_0x$. The SL introduces a quantum energy scale $E_G \sim \hbar v_F G_0$ associated to electronic sub-band transitions. At energies lower than $E_G$, the plasmon dispersion is highly anisotropic; plasmons propagate perpendicularly to the SL axis, but become damped by electronic transitions along the SL direction. These results question the validity of semiclassical approximations for describing low energy plasmons in periodic structures. At higher energies, the dispersion becomes isotropic and Drude-like with effective Drude weights related to the average of the absolute value of the local chemical potential. Full quantum mechanical treatment of the kinetic energy thus introduces non-local effects that delocalize the plasmons in the SL, making the system behave as a meta-material even near singular points where the charge density vanishes.

cond-mat.mes-hall↗

arXiv2020

Plasmonic Dirac Cone in Twisted Bilayer Graphene

We discuss plasmons of biased twisted bilayer graphene when the Fermi level lies inside the gap. The collective excitations are a network of chiral edge plasmons (CEP) entirely composed of excitations in the topological electronic edge states (EES) that appear at the AB-BA interfaces. The CEP form an hexagonal network with an unique energy scale $ε_p=\frac{e^2}{ε_0εt_0}$ with $t_0$ the moiré lattice constant and $ε$ the dielectric constant. From the dielectric matrix we obtain the plasmon spectra that has two main characteristics: (i) a diverging density of states at zero energy, and (ii) the presence of a plasmonic Dirac cone at $\hbarω\simε_p/2$ with sound velocity $v_D=0.0075c$, which is formed by zigzag and armchair current oscillations. A network model reveals that the antisymmetry of the plasmon bands implies that CEP scatter at the hexagon vertices maximally in the deflected chiral outgoing directions, with a current ratio of 4/9 into each of the deflected directions and 1/9 into the forward one. We show that scanning near-field microscopy should be able to observe the predicted plasmonic Dirac cone and its broken symmetry phases.

cond-mat.mes-hall↗

arXiv2020

Time-reversal versus chiral symmetry breaking in twisted bilayer graphene

By applying a self-consistent Hartree-Fock approximation, we show that the mechanism of dynamical symmetry breaking can account for the insulating phase that develops about the charge neutrality point of twisted bilayer graphene around the magic angle. ($i$) If the Coulomb interaction is screened by metallic gates, the opening of a gap between the lowest-energy valence and conduction bands proceeds through the breakdown of chiral symmetry at strong coupling. Increasing the dielectric screening, however, we find a critical coupling at which chiral symmetry breaking is suppressed, triggering a very strong signal for time-reversal symmetry breaking with Haldane mass. ($ii$) If the long-range tail of the Coulomb interaction is not screened, we see the appearance of yet a different dominant pattern at strong coupling, which is characterized by breaking the time-reversal invariance but with opposite flux in the two sublattices of each carbon layer, with the consequent valley symmetry breaking. In this case a gap is also opened in the Dirac cones, but superposed to the splitting of the degeneracy of the low-energy bands at the $K$ points of the moiré Brillouin zone.

cond-mat.mes-hall↗

arXiv2020

Marginal Fermi liquid in twisted bilayer graphene

Linear resistivity at low temperatures is a prominent feature of high-T$_c$ superconductors which has also been found recently in twisted bilayer graphene. We show that due to an extended van Hove singularity (vHS), the $T$-linear resistivity can be obtained from a microscopic tight-binding model for filling factors close to the vHS. The linear behavior is shown to be related to the linear energy dependence of the electron quasiparticle decay rate which implies the low-energy logarithmic attenuation of the quasiparticle weight. These are distinctive features of a marginal Fermi liquid, which we also see reflected in the respective low-temperature logarithmic corrections of the heat capacity and the thermal conductivity, leading to the consequent violation of the Wiedemann-Franz law. We also show that there is a crossover at $T \sim 6$ K from the marginal Fermi liquid regime to a regime dominated by excitations on the Dirac cone right above the vHS that also yields a linear resistivity albeit with smaller slope, in agreement with experimental observations.

cond-mat.mes-hall↗

arXiv2019

Unidirectional plasmonic edge modes on general two-dimensional materials

We investigate the field and spin-momentum coupling of edge plasmons hosted by general two-dimensional materials and identify sweet spots depending on the polarisation plane, ellipticity and the position of an electric dipole relative to the plane and edge. Exciting the dipole at these sweet spots by propagating light leads to uni-directional propagating edge plasmons or edge modes are totally suppressed. We also extent previous approximate treatments [A. Fetter Phys. Rev. B 32, 7676 (1985)] to include anisotropy and hyperbolic systems, elucidating its predictions for the existence of edge modes. A thorough assessment of the approximate description is carried out, comparing its spin-momentum coupling features in the near field with exact results from Wiener-Hopf techniques. Simulations are also performed confirming the overall picture. Our results shed new light on the quest of chiral plasmonics in 2D materials and should be relevant for future experiments.

cond-mat.mes-hall↗

arXiv2019

Photonic crystals for nano-light in moiré graphene superlattices

Graphene is an atomically thin plasmonic medium that supports highly confined plasmon polaritons, or nano-light, with very low loss. Electronic properties of graphene can be drastically altered when it is laid upon another graphene layer, resulting in a moiré superlattice. The relative twist angle between the two layers is a key tuning parameter of the interlayer coupling in thus obtained twisted bilayer graphene (TBG). We studied propagation of plasmon polaritons in TBG by infrared nano-imaging. We discovered that the atomic reconstruction occurring at small twist angles transforms the TBG into a natural plasmon photonic crystal for propagating nano-light. This discovery points to a pathway towards controlling nano-light by exploiting quantum properties of graphene and other atomically layered van der Waals materials eliminating need for arduous top-down nanofabrication.

cond-mat.mes-hall↗

arXiv2019

Kohn-Luttinger Superconductivity in Twisted Bilayer Graphene

We show that the recently observed superconductivity in twisted bilayer graphene (TBG) can be explained as a consequence of the Kohn-Luttinger (KL) instability which leads to an effective attraction between electrons with originally repulsive interaction. Usually, the KL instability takes place at extremely low energy scales, but in TBG, a doubling and subsequent strong coupling of the van Hove singularities (vHS) in the electronic spectrum occurs as the magic angle is approached, leading to extended saddle points in the highest valence band (VB) with almost perfect nesting between states belonging to different valleys. The highly anisotropic screening induces an effective attraction in a $p$-wave channel with odd parity under the exchange of the two disjoined patches of the Fermi line. We also predict the appearance of a spin-density wave (SDW) instability, adjacent to the superconducting phase, and the opening of a gap in the electronic spectrum from the condensation of spins with wave vector corresponding to the nesting vector close to the vHS.

cond-mat.mes-hall↗