arXiv subjects

T. Takeda

Publications and source records attributed to T. Takeda.

12 recordsLinked to original sources

arXiv2026

Realization of a parity-violating antiferromagnetic state in LaMnSi

Spontaneous symmetry breaking underlies functional electronic phenomena in quantum materials. Breaking space-inversion ($\mathcal{P}$) or time-reversal ($\mathcal{T}$) symmetry can generate spin-split electronic bands central to modern spintronics. By contrast, parity-violating antiferromagnetic (AFM) order breaks both $\mathcal{P}$ and $\mathcal{T}$ while preserving the combined $\mathcal{PT}$ symmetry, enabling spin-degenerate yet momentum-asymmetric electronic bands. This momentum asymmetry has been proposed as a microscopic origin of unconventional nonreciprocal and nonlinear responses but its experimental verification has remained challenging because it requires establishing both the symmetry-breaking magnetic order and the associated electronic structure. Here we combine soft x-ray angle-resolved photoemission spectroscopy (ARPES) and polarization-resolved optical second-harmonic generation (SHG) microscopy to study LaMnSi, a candidate parity-violating AFM metal. Soft x-ray ARPES resolves the three-dimensional bulk band structures in agreement with density functional theory calculations for the AFM phase, whereas SHG microscopy detects sign-reversing nonlinear optical responses from opposite AFM domains that carry $\mathcal{T}$-odd parity-violating order. Together, these results provide direct evidence for parity-violating AFM state in LaMnSi, establish LaMnSi as a parity-violating AFM metal, and identify this class of AFMs as a promising platform for symmetry-controlled nonreciprocal and nonlinear electronic responses.

cond-mat.mtrl-sci↗

arXiv2023

Gas selection for Xe-based LCP-GEM detectors onboard the CubeSat X-ray observatory NinjaSat

We present a gas selection for Xe-based gas electron multiplier (GEM) detectors, Gas Multiplier Counters (GMCs) onboard the CubeSat X-ray observatory NinjaSat. To achieve an energy bandpass of 2-50 keV, we decided to use a Xe-based gas mixture at a pressure of 1.2 atm that is sensitive to high-energy X-rays. In addition, an effective gain of over 300 is required for a single GEM so that the 2 keV X-ray signal can be sufficiently larger than the electrical noise. At first, we measured the effective gains of GEM in nine Xe-based gas mixtures (combinations of Xe, Ar, CO2, CH4, and dimethyl ether; DME) at 1.0 atm. The highest gains were obtained with Xe/Ar/DME mixtures, while relatively lower gains were obtained with Xe/Ar/CO2, Xe/Ar/CH4, and Xe+quencher mixtures. Based on these results, we selected the Xe/Ar/DME (75%/24%/1%) mixture at 1.2 atm as the sealed gas for GMC. Then we investigated the dependence of an effective gain on the electric fields in the drift and induction gaps ranging from 100-650 V cm$^{-1}$ and 500-5000 V cm$^{-1}$, respectively, in the selected gas mixture. The effective gain weakly depended on the drift field while it was almost linearly proportional to the induction field: 2.4 times higher at 5000 V cm$^{-1}$ than at 1000 V cm$^{-1}$. With the optimal induction and drift fields, the flight model GMC achieves an effective gain of 460 with an applied GEM voltage of 590 V.

astro-ph.IM↗

arXiv2022

Rhombic Fermi surfaces in a ferromagnetic MnGa thin film with perpendicular magnetic anisotropy

Mn$_{1-x}$Ga$_x$ (MnGa) with the $L1_0$ structure is a ferromagnetic material with strong perpendicular magneto-crystalline anisotropy. Although MnGa thin films have been successfully grown epitaxially and studied for various spintronics devices, fundamental understandings of its electronic structure are still lacking. To address this issue, we have investigated $L1_0$-MnGa thin films using angle-resolved photoemission spectroscopy (ARPES). We have observed a large Fermi surface with a rhombic shape in the $k_x$-$k_y$ plane overlapping neighboring Fermi surfaces. The $k_z$ dependence of the band structure suggests that the band dispersion observed by ARPES comes from the three-dimensional band structure of MnGa folded by a $\sqrt{2} \times \sqrt{2}$ reconstruction. The band dispersion across the corner of the rhombic Fermi surface forms an electron pocket with a weak $k_z$ dependence. The effective mass and the mobility of the bands crossing the Fermi level near the corner are estimated from the ARPES images. Based on the experimental findings, the relationship between the observed band structure and the spin-dependent properties in MnGa-based heterostructures is discussed.

cond-mat.mtrl-sci↗

arXiv2021

Magnetic anisotropy of the van der Waals ferromagnet Cr$_2$Ge$_2$Te$_6$ studied by angular-dependent XMCD

The van der Waals ferromagnet Cr$_2$Ge$_2$Te$_6$ (CGT) has a two-dimensional crystal structure where each layer is stacked through van der Waals force. We have investigated the nature of the ferromagnetism and the weak perpendicular magnetic anisotropy (PMA) of CGT by means of X-ray absorption spectroscopy and X-ray magnetic circular dichroism (XMCD) studies of CGT single crystals. The XMCD spectra at the Cr $L_{2,3}$ edge for different magnetic field directions were analyzed on the basis of the cluster-model multiplet calculation. The Cr valence is confirmed to be 3+ and the orbital magnetic moment is found to be nearly quenched, as expected for the high-spin $t_{2g}$$^3$ configuration of the Cr$^{3+}$ ion. A large ($\sim 0.2$ eV) trigonal crystal-field splitting of the $t_{2g}$ level caused by the distortion of the CrTe$_6$ octahedron has been revealed, while the single-ion anisotropy (SIA) of the Cr atom is found to have a sign {\it opposite} to the observed PMA and too weak compared to the reported anisotropy energy. The present result suggests that anisotropic exchange coupling between the Cr atoms through the ligand Te $5p$ orbitals having strong spin-orbit coupling has to be invoked to explain the weak PMA of CGT, as in the case of the strong PMA of CrI$_3$.

cond-mat.mtrl-sci↗

arXiv2021

Observation of Coulomb-assisted nuclear bound state of $Ξ^-$-$^{14}$N system

In an emulsion-counter hybrid experiment performed at J-PARC, a $Ξ^-$ absorption event was observed which decayed into twin single-$Λ$ hypernuclei. Kinematic calculations enabled a unique identification of the reaction process as $Ξ^{-} + ^{14}$N$\ \rightarrow\ ^{10}_Λ$Be + $^5_Λ$He. For the binding energy of the $Ξ^{-}$ hyperon in the $Ξ^-$-$^{14}$N system a value of $1.27 \pm 0.21$ MeV was deduced. The energy level of $Ξ^-$ is likely a nuclear $1p$ state which indicates a weak $ΞN$-$ΛΛ$ coupling.

nucl-ex↗

arXiv2021

Itinerant ferromagnetism mediated by giant spin polarization of metallic ligand band in van der Waals magnet Fe5GeTe2

We investigate near-Fermi-energy (EF) element-specific electronic and spin states of ferromagnetic van der Waals (vdW) metal Fe5GeTe2. The soft x-ray angle-resolved photoemission spectroscopy (SX-ARPES) measurement provides spectroscopic evidence of localized Fe 3d band. We also find prominent hybridization between the localized Fe 3d band and the delocalized Ge/Te p bands. This picture is strongly supported from direct observation of the remarkable spin polarization of the ligand p bands near EF, using x-ray magnetic circular dichroism (XMCD) measurements. The strength of XMCD signal from ligand element Te shows the highest value, as far as we recognize, among literature reporting finite XMCD signal for none-magnetic element in any systems. Combining SX-ARPES and elemental selective XMCD measurements, we collectively point an important role of giant spin polarization of the delocalized ligand Te states for realizing itinerant long-range ferromagnetism in Fe5GeTe2. Our finding provides a fundamental elemental selective view-point for understanding mechanism of itinerant ferromagnetism in low dimensional compounds, which also leads insight for designing exotic magnetic states by interfacial band engineering in heterostructures.

cond-mat.str-el↗

arXiv2020

Tailoring Magnetism in Self-intercalated Cr1+δTe2 Epitaxial Films

Magnetic transition metal dichalcogenide (TMD) films have recently emerged as promising candidates to host novel magnetic phases relevant to next-generation spintronic devices. However, systematic control of the magnetization orientation, or anisotropy, and its thermal stability, characterized by Curie temperature (Tc) remains to be achieved in such films. Here we present self-intercalated epitaxial Cr1+δTe2 films as a platform for achieving systematic/smooth magnetic tailoring in TMD films. Using a molecular beam epitaxy (MBE) based technique, we have realized epitaxial Cr1+δTe2 films with smoothly tunable over a wide range (0.33-0.82), while maintaining NiAs-type crystal structure. With increasing δ, we found monotonic enhancement of Tc from 160 to 350 K, and the rotation of magnetic anisotropy from out-of-plane to in-plane easy axis configuration for fixed film thickness. Contributions from conventional dipolar and orbital moment terms are insufficient to explain the observed evolution of magnetic behavior with δ. Instead, ab initio calculations suggest that the emergence of antiferromagnetic interactions with δ, and its interplay with conventional ferromagnetism, may play a key role in the observed trends. To our knowledge, this constitutes the first demonstration of tunable Tc and magnetic anisotropy across room temperature in TMD films, and paves the way for engineering novel magnetic phases for spintronic applications.

cond-mat.mtrl-sci↗

arXiv2019

Neutron quadrupole transition strength in $^{10}$C deduced from the $^{10}$C$(α,α')$ measurement with the MAIKo active target

Elastic and inelastic alpha scatterings on $^{10}$C were measured using a 68-MeV/u radioactive $^{10}$C beam incident on the recently developed MAIKo active target system. The phenomenological effective $α$-$N$ interaction and the point-nucleon density distribution in the ground state were determined from the elastic scattering data. The cross sections of the inelastic alpha scattering were calculated using this interaction and density distribution and were compared with the experiment to determine the neutron quadrupole transition matrix element $M_{n}$ between the ground state and the $2_{1}^{+}$ state at $E_{x} = 3.35$ MeV in $^{10}$C. The deduced neutron transition matrix element is $M_{n} = 6.9\, \pm0.7\, \mathrm{(fit)}\, \pm1.2\, \mathrm{(sys)}$ fm$^{2}$. The ratio of the neutron transition strength to proton transition strength was determined as $M_{n}/M_{p} = 1.05\, \pm0.11\, \mathrm{(fit)}\, \pm0.17\, \mathrm{(sys)}$, which indicates that the quadrupole transition between the ground state and the $2_{1}^{+}$ state in $^{10}$C is less neutron dominant compared to that in $^{16}$C.

nucl-ex↗

arXiv2019

Observation of a Be double-Lambda hypernucleus in the J-PARC E07 experiment

A double-$Λ$ hypernucleus, ${}_{ΛΛ}\mathrm{Be}$, was observed by the J-PARC E07 collaboration in nuclear emulsions tagged by the $(K^{-},K^{+})$ reaction. This event was interpreted as a production and decay of $ {}_{ΛΛ}^{\;10}\mathrm{Be}$, ${}_{ΛΛ}^{\;11}\mathrm{Be}$, or ${}_{ΛΛ}^{\;12}\mathrm{Be}^{*}$ via $Ξ^{-}$ capture in ${}^{16}\mathrm{O}$. By assuming the capture in the atomic 3D state, the binding energy of two $Λ$ hyperons$\,$($B_{ΛΛ}$) of these double-$Λ$ hypernuclei are obtained to be $15.05 \pm 0.11\,\mathrm{MeV}$, $19.07 \pm 0.11\,\mathrm{MeV}$, and $13.68 \pm 0.11\,\mathrm{MeV}$, respectively. Based on the kinematic fitting, ${}_{ΛΛ}^{\;11}\mathrm{Be}$ is the most likely explanation for the observed event.

nucl-ex↗

arXiv2006

A swollen phase observed between the liquid-crystalline phase and the interdigitated phase induced by pressure and/or adding ethanol in DPPC aqueous solution

A swollen phase, in which the mean repeat distance of lipid bilayers is larger than the other phases, is found between the liquid-crystalline phase and the interdigitated gel phase in DPPC aqueous solution. Temperature, pressure and ethanol concentration dependences of the structure were investigated by small-angle neutron scattering, and a bending rigidity of lipid bilayers was by neutron spin echo. The nature of the swollen phase is similar to the anomalous swelling reported previously. However, the temperature dependence of the mean repeat distance and the bending rigidity of lipid bilayers are different. This phase could be a precursor to the interdigitated gel phase induced by pressure and/or adding ethanol.

cond-mat.soft↗

arXiv2005

Optical investigations on $Y_{2-x} Bi_x Ru_2 O_7$: Electronic structure evolutions related to the metal-insulator transition

Optical conductivity spectra of cubic pyrochlore $Y_{2-x} Bi_x Ru_2 O_7$ (0.0$\leq ${\it x}$\leq $2.0) compounds are investigated. As a metal-insulator transition (MIT) occurs around {\it x}$=$0.8, large spectral changes are observed. With increase of {\it x}, the correlation-induced peak between the lower and the upper Hubbard bands seems to be suppressed, and a strong mid-infrared feature is observed. In addition, the $p-d$ charge transfer peak shifts to the lower energies. The spectral changes cannot be explained by electronic structural evolutions in the simple bandwidth-controlled MIT picture, but are consistent with those in the filling-controlled MIT picture. In addition, they are also similar to the spectral changes of Y$_{2-x}$Ca$_{x}$Ru$_{2}$O$_{7}$ compounds, which is a typical filling-controlled system. This work suggests that, near the MIT, the Ru bands could be doped with the easily polarizable Bi cations.

cond-mat.str-el↗

arXiv2001

Optical investigation on the electronic structures of Y_{2}Ru_{2}O_{7}, CaRuO_{3}, SrRuO_{3}, and Bi_{2}Ru_{2}O_{7}

We investigated the electronic structures of the bandwidth-controlled ruthenates, Y$_{2}$Ru$_{2}$O$_{7}$, CaRuO$_{3}$, SrRuO$_{3}$, and Bi$_{2}$Ru$% _{2}$O$_{7}$, by optical conductivity analysis in a wide energy region of 5 meV $\sim $ 12 eV. We could assign optical transitions from the systematic changes of the spectra and by comparison with the O 1$s$ x-ray absorption data. We estimated some physical parameters, such as the on-site Coulomb repulsion energy and the crystal-field splitting energy. These parameters show that the 4$d$ orbitals should be more extended than 3$d$ ones. These results are also discussed in terms of the Mott-Hubbard model.

cond-mat.str-el↗