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T. Tornyi

Publications and source records attributed to T. Tornyi.

15 recordsLinked to original sources

Shape evolution in even-mass $^{98-104}$Zr isotopes via lifetime measurements using the $\gamma\gamma$-coincidence technique

The Zirconium (Z = 40) isotopic chain has attracted interest for more than four decades. The abrupt lowering of the energy of the first $2^+$ state and the increase in the transition strength B(E2; $2_1^\rightarrow 0_1^+$ going from $^{98}$Zr to $^{100}$Zr has been the first example of "quantum phase transition" in nuclear shapes, which has few equivalents in the nuclear chart. Although a multitude of experiments have been performed to measure nuclear properties related to nuclear shapes and collectivity in the region, none of the measured lifetimes were obtained using the Recoil Distance Doppler Shift method in the $\gamma\gamma$-coincidence mode where a gate on the direct feeding transition of the state of interest allows a strict control of systematical errors. This work reports the results of lifetime measurements for the first yrast excited states in $^{98-104}$Zr carried out to extract reduced transition probabilities. The new lifetime values in $\gamma\gamma$-coincidence and $\gamma$-single mode are compared with the results of former experiments. Recent predictions of the Interacting Boson Model with Configuration Mixing, the Symmetry Conserving Configuration Mixing model based on the Hartree-Fock-Bogoliubov approach and the Monte Carlo Shell Model are presented and compared with the experimental data.

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Direct measurement of hexacontatetrapole, $\textbf{E6}$ γ decay from $^{\textbf{53m}}$Fe

The only proposed observation of a discrete, hexacontatetrapole ($E6$) transition in nature occurs from the T$_{1/2}$ = 2.54(2)-minute decay of $^{53m}$Fe. However, there are conflicting claims concerning its $γ$-decay branching ratio, and a rigorous interrogation of $γ$-ray sum contributions is lacking. Experiments performed at the Australian Heavy Ion Accelerator Facility were used to study the decay of $^{53m}$Fe. For the first time, sum-coincidence contributions to the weak $E6$ and $M5$ decay branches have been firmly quantified using complementary experimental and computational methods. Agreement across the different approaches confirms the existence of the real $E6$ transition; the $M5$ branching ratio and transition rate have also been revised. Shell model calculations performed in the full $pf$ model space suggest that the effective proton charge for high-multipole, $E4$ and $E6$, transitions is quenched to approximately two-thirds of the collective $E2$ value. Correlations between nucleons may offer an explanation of this unexpected phenomenon, which is in stark contrast to the collective nature of lower-multipole, electric transitions observed in atomic nuclei.

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$E0$ transition strength in stable Ni isotopes

Excited states in $^{58,60,62}$Ni were populated via inelastic proton scattering at the Australian National University as well as via inelastic neutron scattering at the University of Kentucky Accelerator Laboratory. The Super-e electron spectrometer and the CAESAR Compton-suppressed HPGe array were used in complementary experiments to measure conversion coefficients and $δ(E2/M1)$ mixing ratios, respectively, for a number of $2^+ \rightarrow 2^+$ transitions. The data obtained were combined with lifetimes and branching ratios to determine $E0$, $M1$, and $E2$ transition strengths between $2^+$ states. The $E0$ transition strengths between $0^+$ states were measured using internal conversion electron spectroscopy and compare well to previous results from internal pair formation spectroscopy. The $E0$ transition strengths between the lowest-lying $2^+$ states were found to be consistently large for the isotopes studied.

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First-excited state $g$ factors in the stable, even Ge and Se isotopes

Transient-field $g$-factor measurements in inverse kinematics were performed for the first-excited states of the stable, even isotopes of Ge and Se. The $g$ factors of $^{74}$Ge and $^{74}$Se were measured simultaneously using a cocktail beam, which eliminates most possible sources of systematic error in a relative $g$-factor measurement. The results are $g(^{74}{\rm Se})/g(^{74}{\rm Ge})=1.34(7)$, $g(^{70}{\rm Ge})/g(^{74}{\rm Ge}) = 1.16(15)$, $g(^{72}{\rm Ge})/g(^{74}{\rm Ge})=0.92(13)$, $g(^{76}{\rm Ge})/g(^{74}{\rm Ge})=0.88(5)$, $g(^{76}{\rm Se})/g(^{74}{\rm Se})=0.96(7)$, $g(^{78}{\rm Se})/g(^{74}{\rm Se})=0.82(5)$, $g(^{80}{\rm Se})/g(^{74}{\rm Se})=0.99(7)$ and $g(^{82}{\rm Se})/g(^{74}{\rm Se})=1.19(6)$. The measured $g$-factor ratios are in agreement with ratios from previous measurements, despite considerable variation in previous reported absolute values. The absolute values of the $g$ factors remain uncertain, however the Rutgers parametrization was used to set the transient-field strength and then compare the experimental $g$ factors with shell-model calculations based on the JUN45 and jj44b interactions. Modest agreement was found between experiment and theory for both interactions. The shell model calculations indicate that the $g(2^+_1)$ values and trends are determined largely by the balance of the spin carried by orbital motion of the protons.

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Restricted spin-range correction in the Oslo Method: The example of nuclear level density and $γ$-ray strength function from $^{239}\mathrm{Pu}(\mathrm{d,p}γ)^{240}\mathrm{Pu}$

The Oslo Method has been applied to particle-$γ$ coincidences following the $^{239}\mathrm{Pu}$(d,p) reaction to obtain the nuclear level density (NLD) and $γ$-ray strength function ($γ$SF) of $^{240}\mathrm{Pu}$. The experiment was conducted with a 12 MeV deuteron beam at the Oslo Cyclotron Laboratory. The low spin transfer of this reaction leads to a spin-parity mismatch between populated and intrinsic levels. This is a challenge for the Oslo Method as it can have a significant impact on the extracted NLD and $γ$SF. We have developed an iterative approach to ensure consistent results even for cases with a large spin-parity mismatch, in which we couple Green's Function Transfer calculations of the spin-parity dependent population cross-section to the nuclear decay code RAINIER. The resulting $γ$SF shows a pronounced enhancement between 2-4 MeV that is consistent with the location of the low-energy orbital $M1$ scissors mode.

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Impact of restricted spin-ranges in the Oslo Method: The example of (d,p)$^{240}\mathrm{Pu}$

In this paper we present the first systematic analysis of the impact of the populated vs. intrinsic spin distribution on the nuclear level density and $γ$-ray strength function retrieved through the Oslo Method. We illustrate the effect of the spin distribution on the recently performed $^{239}\mathrm{Pu}$(d,p$γ$)$^{240}\mathrm{Pu}$ experiment using a 12 MeV deuteron beam performed at the Oslo Cyclotron Lab. In the analysis we couple state-of-the-art calculations for the populated spin-distributions with the Monte-Carlo nuclear decay code RAINIER to compare Oslo Method results to the known input. We find that good knowledge of the populated spin distribution is crucial and show that the populated distribution has a significant impact on the extracted nuclear level density and $γ$-ray strength function for the $^{239}\mathrm{Pu}$(d,p$γ$)$^{240}\mathrm{Pu}$ case.

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Measurement of the intensity ratio of Auger and conversion electrons for the electron capture decay of $^{125}$I

Auger electrons emitted after nuclear decay have potential application in targeted cancer therapy. For this purpose it is important to know the Auger electron yield per nuclear decay. In this work we describe a measurement of the ratio of the number of conversion electrons (emitted as part of the nuclear decay process) to the number of Auger electrons (emitted as part of the atomic relaxation process after the nuclear decay) for the case of $^{125}$I. Results are compared with Monte-Carlo type simulations of the relaxation cascade using the BrIccEmis code. Our results indicate that for $^{125}$I the calculations based on rates from the Evaluated Atomic Data Library (EADL) underestimate the K Auger yields by 20\%.

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Identification of significant $E0$ strength in the $2^+_2 \rightarrow 2^+_1$ transitions of $^{58, 60, 62}$Ni

The $E0$ transition strength in the $2^+_2 \rightarrow 2^+_1$ transitions of $^{58,60,62}$Ni have been determined for the first time following a series of measurements at the Australian National University (ANU) and the University of Kentucky (UK). The CAESAR Compton-suppressed HPGe array and the Super-e solenoid at ANU were used to measure the $δ(E2/M1)$ mixing ratio and internal conversion coefficient of each transition following inelastic proton scattering. Level half-lives, $δ(E2/M1)$ mixing ratios and $γ$-ray branching ratios were measured at UK following inelastic neutron scattering. The new spectroscopic information was used to determine the $E0$ strengths. These are the first $2^+ \rightarrow 2^+$ $E0$ transition strengths measured in nuclei with spherical ground states and the $E0$ component is found to be unexpectedly large; in fact, these are amongst the largest $E0$ transition strengths in medium and heavy nuclei reported to date.

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Perturbed angular distributions with LaBr$_3$ detectors: the $g$ factor of the first ${10^+}$ state in $^{110}$Cd revisited

The Time Differential Perturbed Angular Distribution technique with LaBr$_3$ detectors has been applied to the $I^π= \frac{11}{2}^-$ isomeric state ($E_x = 846$ keV, $τ=107$~ns) in $^{107}$Cd, which was populated and recoil-implanted into a gadolinium host following the $^{98}$Mo($^{12}$C, $3n$)$^{107}$Cd reaction. The static hyperfine field strength of Cd recoil implanted into gadolinium was thus measured, together with the fraction of nuclei implanted into field-free sites, under similar conditions as pertained for a previous implantation perturbed angular distribution $g$-factor measurement on the $I^π= 10^+$ state in $^{110}$Cd. The $^{110}$Cd $g(10^+)$ value was thereby re-evaluated, bringing it into agreement with the value expected for a seniority-two $νh_{\frac{11}{2}}$ configuration.

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Study of the 238U(d,p) surrogate reaction via the simultaneous measurement of gamma-decay and fission probabilities

We investigated the 238U(d,p) reaction as a surrogate for the n + 238U reaction. For this purpose we measured for the first time the gamma-decay and fission probabilities of 239U* simultaneously and compared them to the corresponding neutron-induced data. We present the details of the procedure to infer the decay probabilities, as well as a thorough uncertainty analysis, including parameter correlations. Calculations based on the continuum-discretized coupled-channels and distorted-wave Born approximations were used to correct our data from detected protons originating from elastic and inelastic deuteron breakup. In the region where the fission and gamma-decay probabilities compete, the corrected fission probability is in agreement with neutron-induced data, whereas the gamma-decay probability is much higher than the neutron-induced data. The performed statistical-model calculations are not able to explain these results.

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Level densities and thermodynamical properties of Pt and Au isotopes

The nuclear level densities of $^{194-196}$Pt and $^{197,198}$Au below the neutron separation energy have been measured using transfer and scattering reactions. All the level density distributions follow the constant-temperature description. Each group of isotopes is characterized by the same temperature above the energy threshold corresponding to the breaking of the first Cooper pair. A constant entropy excess $ΔS=1.9$ and $1.1$ $k_B$ is observed in $^{195}$Pt and $^{198}$Au with respect to $^{196}$Pt and $^{197}$Au, respectively, giving information on the available single-particle level space for the last unpaired valence neutron. The breaking of nucleon Cooper pairs is revealed by sequential peaks in the microcanonical caloric curve.

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Shell-gap reduced level densities in $^{89,90}$Y

Particle-$γ$ coincidences from the $^{89}$Y($p,p' γ$)$^{89}$Y and $^{89}$Y($d,p γ$)$^{90}$Y reactions were utilized to obtain $γ$-ray spectra as function of excitation energy. The Oslo method was used to extract the level density from the particle-$γ$ coincidence matrices. The impact of the $N=50$ shell closure on the level densities is discussed within the framework of a combinatorial quasi-particle model.

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Evidence for dipole nature of the low-energy $γ$ enhancement in $^{56}$Fe

The $γ$-ray strength function of $^{56}$Fe has been measured from proton-$γ$ coincidences for excitation energies up to $\approx 11$ MeV. The low-energy enhancement in the $γ$-ray strength function, which was first discovered in the ($^3$He,$αγ$)$^{56}$Fe reaction, is confirmed with the ($p,p^\primeγ$)$^{56}$Fe experiment reported here. Angular distributions of the $γ$ rays give for the first time evidence that the enhancement is dominated by dipole transitions.

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Neutron-skin thickness of $^{208}$Pb, and symmetry-energy constraints from the study of the anti-analog giant dipole resonance

The $^{208}$Pb($p$,$nγ\bar p$) $^{207}$Pb reaction at a beam energy of 30 MeV has been used to excite the anti-analog of the giant dipole resonance (AGDR) and to measure its $γ$-decay to the isobaric analog state in coincidence with proton decay of IAS. The energy of the transition has also been calculated with the self-consistent relativistic random-phase approximation (RRPA), and found to be linearly correlated to the predicted value of the neutron-skin thickness ($ΔR_{pn}$). By comparing the theoretical results with the measured transition energy, the value of 0.190 $\pm$ 0.028 fm has been determined for $ΔR_{pn}$ of $^{208}$Pb, in agreement with previous experimental results. The AGDR excitation energy has also been used to calculate the symmetry energy at saturation ($J=32.7 \pm 0.6$ MeV) and the slope of the symmetry energy ($L=49.7 \pm 4.4$ MeV), resulting in more stringent constraints than most of the previous studies.

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Constant-temperature level densities in the quasi-continuum of Th and U isotopes

Particle-gamma coincidences have been measured to obtain gamma-ray spectra as a function of excitation energy for 231-233Th and 237-239U. The level densities, which were extracted using the Oslo method, show a constant temperature behavior. The isotopes display very similar temperatures in the quasi-continuum, however, the even-odd isotopes reveal a constant entropy increase Delta S compared to their even-even neighbors. The entropy excess depends on available orbitals for the last unpaired valence neutron of the heated nuclear system. Also, experimental microcanonical temperature and heat capacity have been extracted. Several poles in the heat capacity curve support the idea that an almost continuous melting of Cooper pairs is responsible for the constant-temperature behavior.

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