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T. V. Raziman

Publications and source records attributed to T. V. Raziman.

15 recordsLinked to original sources

Graph-theoretic design of lasing networks for physical vision

Physical neural networks perform learning through the intrinsic nonlinear dynamics of matter. Optimising their design presents a considerable challenge: complex many-body physics can provide powerful computation, but are expensive to simulate and large experimental optimisation runs are impractical to fabricate. Hence, the high-dimensional space of possible network topologies cannot be effectively directly searched. Here, we show that this search can be efficiently performed in an abstract graph space that is vastly cheaper to explore. Using random lasing networks -- composed of interconnected nanoscale waveguides and hosting strongly coupled lasing modes -- as an exemplar physical vision system, we establish a quantitative three-layer link: simple graph-theoretic metrics predict the nonlinear lasing physics, which in turn predicts vision performance. After validating this relationship using physical simulations, we exploit it to drive an evolutionary algorithm using graph metrics, producing network topologies that outperform random designs at a fraction of the computational cost (3000$\times$ speed-up compared to physical simulation). On simulated image-classification tasks, graph-optimised networks substantially improve classification accuracy. As our framework operates on network topology rather than substrate-specific physics, we anticipate it can transfer to other network-based physical learning systems, providing an efficient route for the directed design and optimisation of complex, strongly-interacting physical neural networks.

cond-mat.dis-nn

Programmable Synthetic Motion at a Time-Varying Interface

Space-time metamaterials that exhibit synthetic motion promise arbitrary control over the momentum, frequency and energy of scattered light, but realising the required space-time modulation in a programmable way remains a challenge. Here we program synthetic motion using a single spatial light modulator in a 4f geometry which imprints a continuously tunable pulse-front tilt onto a high-intensity pump pulse, inducing reflectivity modulations at a sub-wavelength indium tin oxide thin film with synthetic velocities spanning the sub- and superluminal regimes. The angle-resolved spectrum of a scattered probe pulse reveals space-time diffraction patterns whose gradient and bandwidth vary continuously with synthetic velocity, in excellent agreement with theory. Splitting the shaped pump into two independently controlled pulses yields space-time double-slit diffraction with tunable fringe separation and frequency-momentum gradient. This programmable platform opens a path towards non-linear and periodic space-time trajectories for tabletop analogue studies of relativistic phenomena and space-time metasurfaces.

physics.optics

Surface Plasmon Polariton Excitation in Time-modulated Media

Surface plasmon polaritons (SPPs) are central to application areas such as sensing, energy harvesting, and nanoscale optics, and are typically excited via spatial structuring -- an approach lacking dynamic control. We demonstrate that step-like time modulation allows the excitation and out-coupling of SPPs through modulating a dispersive Drude-like metal thereby modelling realistic transparent conducting oxides; this establishes a pathway for the active control and extraction of plasmons in experimentally viable time-varying systems. Using finite-difference time-domain simulations we show that time modulation facilitates both the launching and radiation of surface plasmons with frequencies governed by the dispersion of the bounding media. Our results also reveal the generation of time-reflected waves and the emergence of a magnetostatic mode required for matching boundary conditions at the temporal interface.

physics.optics

Space-Time Optical Diffraction from Synthetic Motion

The interaction of light with objects and media moving at relativistic and superluminal speeds enables unconventional phenomena such as Fresnel drag, Hawking radiation, and light amplification. Synthetic motion, facilitated by modulated internal degrees of freedom, enables the study of relativistic phenomena unrestricted by the speed of light. In this study, we investigate synthetically moving apertures created by high-contrast reflectivity modulations, which are generated by ultrafast laser pulses on a subwavelength thin film of indium tin oxide. The space-time diffraction of a weaker probe beam reveals a complex, non-separable spatio-temporal transformation, where changes in the frequency of the wave are correlated to changes in its momentum. By using schemes of continuous or discrete modulation we demonstrate tunable frequency-momentum diffraction patterns with gradients that depend upon the relative velocity between the modulation and the probe wave. The diffraction patterns are matched by operator-based theory and the gradients are analytically predicted using a super-relativistic Doppler model, where the modulation is described as a superluminally moving scattering particle. Our experiments open a path towards mimicking relativistic mechanics and developing complex and programmable spatio-temporal transformations of light.

physics.optics

Single-mode emission by phase-delayed coupling between nano-lasers

Near-field coupling between nanolasers enables collective high-power lasing but leads to complex spectral reshaping and multimode operation, limiting the emission brightness, spatial coherence and temporal stability. Many lasing architectures have been proposed to circumvent this limitation, based on symmetries, topology, or interference. We show that a much simpler and robust method exploiting phase-delayed coupling, where light exchanged by the lasers carries a phase, can enable stable single-mode operation. Phase-delayed coupling changes the modal amplification: for pump powers close to the anyonic parity-time (PT) symmetric exceptional point, a high phase delay completely separates the mode thresholds, leading to single mode operation. This is shown by stability analysis with nonlinear coupled mode theory and stochastic differential equations for two coupled nanolasers and confirmed by realistic semi-analytical treatment of a dimer of lasing nanospheres. Finally, we extend the mode control to large arrays of nanolasers, featuring lowered thresholds and higher power. Our work promises a novel solution to engineer bright and stable single-mode lasing from nanolaser arrays with important applications in photonic chips for communication and lidars.

physics.optics

Mode visualisation and control of complex lasers using neural networks

Understanding the behaviour of complex laser systems is an outstanding challenge, especially in the presence of nonlinear interactions between modes. Hidden features, such as the gain distributions and spatial localisation of lasing modes, often cannot be revealed experimentally, yet they are crucial to determining the laser action. Here, we introduce a lasing spectroscopy method that can visualise the gain profiles of the modes in complex lasers using an artificial neural network. The spatial gain distributions of different lasing modes in a disorderly coupled microring array are reconstructed without prior knowledge of the laser topology. We further extend the neural network to a tandem neural network that can control the laser emission by matching the modal gain/loss profile to selectively enhance the targeted modes. This mode visualisation method offers a new approach to extracting hidden spatial mode features from photonic structures, which could improve our understanding and control of complex photonic systems.

physics.optics

Surface lattice resonance lasers with epitaxial InP gain medium

Surface lattice resonance (SLR) lasers, where gain is supplied by a thin film active material and the feedback comes from multiple scattering by plasmonic nanoparticles, have shown both low threshold lasing and tunability of the angular and spectral emission. However, typically used materials such as organic dyes and QD films suffer from photo-degradation which hampers practical applications. Here, we demonstrate photo-stable single-mode lasing of SLR modes sustained in an epitaxial solid-state InP slab waveguide. The nanoparticle array is weakly coupled to the optical modes, which decreases the scattering losses and hence the experimental lasing threshold is as low as 90 $μ$J/cm$^{2}$. The nanoparticle periodicity defines the lasing wavelength and enables tuneable emission wavelengths over a 70 nm spectral range. Combining plasmonic nanoparticles with an epitaxial solid-state gain medium paves the way for large-area on-chip integrated SLR lasers for applications including optical communication, optical computing, sensing, and LiDAR.

physics.optics

Guiding light with surface exciton-polaritons in atomically thin superlattices

Two-dimensional materials give access to the ultimate physical limits of Photonics with appealing properties for ultracompact optical components such as waveguides and modulators. Specifically, in monolayer semiconductors, a strong excitonic resonance leads to a sharp oscillation in permittivity; at energies close to an exciton, the real part of the permittivity can reach high positive values or even become negative. This extreme optical response enables surface exciton-polaritons to guide visible light bound to an atomically thin layer. However, such ultrathin waveguides support a transverse electric (TE) mode with low confinement and a transverse magnetic (TM) mode with short propagation. Here, we propose that realistic semiconductor-insulator-semiconductor superlattices consisting of monolayer WS$_2$ and hexagonal boron nitride (hBN) can improve the properties of both TE and TM modes. Compared to a single monolayer, a heterostructure with a 1-nm hBN spacer improves the confinement of the TE mode from 1.2 to around 0.5 $μ$m, whereas the out-of-plane extension of the TM mode increases from 25 to 50 nm. We propose two simple additivity rules for mode confinement valid in the ultrathin film approximation for heterostructures with increasing spacer thickness. Stacking additional WS2 monolayers into superlattices further enhances the waveguiding properties. Our results underscore the potential of monolayer superlattices as a platform for visible nanophotonics with promising optical, electrical, and magnetic tunability

physics.optics

Fluorescence enhancement in topologically optimized gallium phosphide all-dielectric nanoantennas

Nanoantennas capable of large fluorescence enhancement with minimal absorption are crucial for future optical technologies from single-photon sources to biosensing. Efficient dielectric nanoantennas have been designed, however, evaluating their performance at the individual emitter level is challenging due to the complexity of combining high-resolution nanofabrication, spectroscopy and nanoscale positioning of the emitter. Here, we study the fluorescence enhancement in infinity-shaped gallium phosphide (GaP) nanoantennas based on a topologically optimized design. Using fluorescence correlation spectroscopy (FCS), we probe the nanoantennas enhancement factor and observed an average of 63-fold fluorescence brightness enhancement with a maximum of 93-fold for dye molecules in nanogaps between 20 nm and 50 nm. The experimentally determined fluorescence enhancement of the nanoantennas was confirmed by numerical simulations of the local density of optical states (LDOS). Furthermore, we show that beyond design optimisation of dielectric nanoantennas, increased performances can be achieved via tailoring of nanoantenna fabrication.

physics.optics

Second harmonic generation at a time-varying interface

Time-varying metamaterials rely on large and fast changes of the linear permittivity. Beyond the linear terms, however, the effect of a non-perturbative modulation of the medium on harmonic generation and the associated nonlinear susceptibilities remains largely unexplored. In this work, we study second harmonic generation at an optically pumped time-varying interface between air and a 310 nm Indium Tin Oxide film. We observe an enhancement of the modulation contrast at the second harmonic wavelength, up to 93% for a pump intensity of 100 GW/cm$^2$, leading to large frequency broadening and shift. We demonstrate that, in addition to the quadratic dependence on the fundamental field, a significant contribution to the enhancement comes from the temporal modulation of the second order nonlinear susceptibility, whose relative change is double that of the linear term. Moreover, the spectra resulting from single and double-slit time diffraction show significantly enhanced frequency shift, broadening and modulation depth, when compared to the infrared fundamental beam, and could be exploited for optical computing and sensing. Enhanced time-varying effects on the harmonic signal extends the application of materials to the visible range and calls for further theoretical exploration of non-perturbative nonlinear optics.

physics.optics

Controlling lasing around Exceptional Points in Coupled Nanolasers

Coupled nanolasers are of growing interest for on-chip optical computation and data transmission, which requires an understanding of how lasers interact to form complex systems. The non-Hermitian interaction between two coupled resonators, when excited selectively, can lead to parity-time symmetry, the formation of exceptional points, and subsequently spectral control and increased sensitivity. These investigations have been limited to pump energies close to the lasing threshold, and large or narrow-line lasers. Here, by programmable optical excitation we study two coupled nanolasers significantly above threshold, where mode instability plays an important role. We map the mode evolution around two exceptional points, and observe lasing gaps due to reversed pump dependence which compare well with nonlinear theory. Finally, the coupling can be exploited to control the lasing threshold and wavelength, and for frequency switching around the lasing gap. Controlled and integrated nanolasers constitutes a promising platform for future highly sensitive and programmable on-chip laser sources.

physics.optics

Impact of indirect transitions on valley polarization in WS$_2$ and WSe$_2$

Controlling the momentum of carriers in semiconductors, known as valley polarization, is a new resource for optoelectronics and information technologies. Materials exhibiting high polarization are needed for valley-based devices. Few-layer WS$_2$ shows a remarkable spin-valley polarization above 90%, even at room temperature. In stark contrast, polarization is absent for few-layer WSe$_2$ despite the expected material similarities. Here, we explain the origin of valley polarization in both materials based on the interplay between two indirect optical transitions. We show that the relative energy minima at the $Λ$- and K-valleys in the conduction band determine the spin-valley polarization of the direct K-K transition. Polarization appears as the energy of the K-valley rises above the $Λ$-valley as a function of temperature and number of layers. Our results advance the understanding of the high spin-valley polarization in WS$_2$. This insight will impact the design of both passive and tunable valleytronic devices operating at room temperature.

cond-mat.mes-hall

Exciton diffusion and annihilation in nanophotonic Purcell landscapes

Excitons spread through diffusion and interact through exciton-exciton annihilation. Nanophotonics can counteract the resulting decrease in light emission. However, conventional enhancement treats emitters as immobile and noninteracting. Here, we go beyond the localized Purcell effect to exploit exciton dynamics. As interacting excitons diffuse through optical hotspots, the balance of excitonic and nanophotonic properties leads to either enhanced or suppressed photoluminescence. We identify the dominant enhancement mechanisms in the limits of high and low diffusion and annihilation to turn their detrimental impact into additional emission. Our guidelines are relevant for efficient and high-power light-emitting diodes and lasers based on monolayer semiconductors, perovskites, or organic crystals.

physics.optics

Collective Mie Exciton-Polaritons in an Atomically Thin Semiconductor

Optically induced Mie resonances in dielectric nanoantennas feature low dissipative losses and large resonant enhancement of both electric and magnetic fields. They offer an alternative platform to plasmonic resonances to study light-matter interactions from the weak to the strong coupling regimes. Here, we experimentally demonstrate the strong coupling of bright excitons in monolayer WS$_2$ with Mie surface lattice resonances (Mie-SLRs). We resolve both electric and magnetic Mie-SLRs of a Si nanoparticle array in angular dispersion measurements. At the zero detuning condition, the dispersion of electric Mie-SLRs (e-SLRs) exhibits a clear anti-crossing and a Rabi-splitting of 32 meV between the upper and lower polariton bands. The magnetic Mie-SLRs (m-SLRs) nearly cross the energy band of excitons. These results suggest that the field of m-SLRs is dominated by out-of-plane components that do not efficiently couple with the in-plane excitonic dipoles of the monolayer WS$_2$. In contrast, e-SLRs in dielectric nanoparticle arrays with relatively high quality factors (Q $\sim$ 120) facilitate the formation of collective Mie exciton-polaritons, and may allow the development of novel polaritonic devices which can tailor the optoelectronic properties of atomically thin two-dimensional semiconductors.

physics.optics

Enhanced light emission by magnetic and electric resonances in dielectric metasurfaces

We demonstrate an enhanced emission of high quantum yield molecules coupled to dielectric metasurfaces formed by periodic arrays of polycrystalline silicon nanoparticles. Radiative coupling of the nanoparticles, mediated by in-plane diffraction, leads to the formation of collective Mie scattering resonances or Mie surface lattice resonances (M-SLRs), with remarkable narrow line widths. These narrow line widths and the intrinsic electric and magnetic dipole moments of the individual Si nanoparticles allow to resolve electric and magnetic M-SLRs. Incidence angle- and polarization-dependent extinction measurements and high-accuracy surface integral simulations show unambiguously that magnetic M-SLRs arise from in- and out-of-plane magnetic dipoles, while electric M-SLRs are due to in-plane electric dipoles. Pronounced changes in the emission spectrum of the molecules are observed, with almost a 20-fold enhancement of the emission in defined directions of molecules coupled to electric M-SLRs, and a 5-fold enhancement of the emission of molecules coupled to magnetic M-SLRs. These measurements demonstrate the potential of dielectric metasurfaces for emission control and enhancement, and open new opportunities to induce asymmetric scattering and emission using collective electric and magnetic resonances.

physics.optics