arXiv subjects
Publications and source records attributed to T. Yankova.
Dielectric spectroscopy is used to check for the onset of polar order in the quasi one-dimensional quantum spin system Sul-Cu2Cl4 when passing from the spin-liquid state into the ordered spiral phase in an external magnetic field. We find clear evidence for multiferroicity in this material and treat in detail its H-T phase diagram close to the quantum-critical regime.
Neutron diffraction and calorimetric measurements are used to study the field-induced quantum phase transition in piperazinium-Cu$_2$(Cl$_{1-x}$Br$_x$)$_6$ ($x=0$, x=3.5% and x=7.5%), a prototypical quantum antiferromagnet with random bonds. The critical indexes $ϕ$ and $β$ are determined. The findings contradict some original predictions for Bose Glass based on the assumption $z=d$, but are consistent with recent theoretical results implying $z<d$. Inelastic neutron experiments reveal that disorder has a profound effect on the lowest-energy magnetic gap excitation in the system.
The effect of disorder is studied on the field-induced quantum phase transition in the frustrated spin-ladder compound H8C4SO2Cu2(Cl[1-x]Brx)4 using bulk magnetic and thermodynamic measurements. The parent material (x=0) is a quantum spin liquid, which in applied fields is known to form a magnon condensate with long-range helimagnetic order. We show that bond randomness introduced by a chemical substitution on the non-magnetic halogene site destroys this phase transition at very low concentrations, already for x=0.01. The extreme fragility of the magnon condensate is attributed to random frustration in the incommensurate state.
We review a strategy for targeted synthesis of large single crystal samples of prototype quantum magnets for inelastic neutron scattering experiments. Four case studies of organic copper halogenide S=1/2 systems are presented. They are meant to illustrate that exciting experimental results pertaining to forefront many-body quantum physics can be obtained on samples grown using very simple techniques, standard laboratory equipment, and almost no experience in in advanced crystal growth techniques.
Inelastic neutron scattering is used to measure spin excitations in fully deuterated single crystal samples of the strong-leg antiferromagnetic S=1/2 spin ladder compound (C$_7$H$_{10}$N)$_2$CuBr$_4$. Sharp resolution-limited magnons are observed across the entire one-dimensional Brillouin zone. The results validate the previously proposed {\it symmetric} spin ladder model and provide a reliable estimate of the relevant exchange interactions.