arXiv subjects

T. Yu

Publications and source records attributed to T. Yu.

33 records · Page 2Linked to original sources

arXiv2014

Theory optical excitation spectra and depolarization dynamics in bilayer WS$_2$ from viewpoint of excimers

We investigate the optical excitation spectra and the photoluminescence depolarization dynamics in bilayer WS$_2$. A different understanding of the optical excitation spectra in the recent photoluminescence experimentby Zhu {\em et al.} [arXiv:1403.6224] in bilayer WS$_2$ is proposed. In the experiment, four excitations (1.68, 1.93, 1.99 and 2.37 eV) are observed and identified to be indirect exciton for the $Γ$ valley, trion, A exciton and B exciton excitations, respectively, with the redshift for the A exciton energy measured to be 30$\sim$50 meV when the sample synthesized from monolayer to bilayer. According to our study, by considering there exist both the intra-layer and charge-transfer excitons in the bilayer WS$_2$, with inter-layer hopping of the hole, there exists excimer state composed by the superposition of the intra-layer and charge-transfer exciton states. Accordingly, we show that the four optical excitations in the bilayer WS$_2$ are the A charge-transfer exciton, ${\rm A}'$ excimer, ${\rm B}'$ excimer and B intra-layer exciton states, respectively, with the calculated resonance energies showing good agreement with the experiment. In our picture, the speculated indirect exciton, which involves a high-order phonon absorption/emission process, is not necessary. Furthermore, the binding energy for the excimer state is calculated to be 40 meV, providing reasonable explanation for the experimentally observed energy redshift of the A exciton. Based on the excimer states, we further derive the exchange interaction Hamiltonian. Then the photoluminescence depolarization dynamics due to the electron-hole exchange interaction is studied in the pump-probe setup by the kinetic spin Bloch equations. We find that ......

cond-mat.mes-hall↗

arXiv2014

Structural Changes Related to the Magnetic Transitions in Hexagonal InMnO3

Two magnetic ordering transitions are found in InMnO3, the paramagnetic to antiferromagnetic transition near ~118 K and a lower possible spin rotation transition near ~42 K. Multiple length scale structural measurements reveal enhanced local distortion found to be connected with tilting of the MnO5 polyhedra as temperature is reduced. Strong coupling is observed between the lattice and the spin manifested as changes in the structure near both of the magnetic ordering temperatures (at ~42 K and ~ 118 K). External parameters such as pressure are expected to modify the coupling.

cond-mat.mtrl-sci↗

arXiv2014

Pressure Dependent Structural Changes and Predicted Electrical Polarization in Perovskite RMnO3

High pressure x-ray diffraction (XRD) measurements on RMnO3 (R=Dy, Ho and Lu) reveals that varying structural changes occurs for different R ions. Large lattice changes (orthorhombic strain) occur in DyMnO3 and HoMnO3 while the Jahn-Teller (JT) distortion remains stable. On the other hand, in LuMnO3, Mn-O bond distortions are observed in the region 4-8 GPa with the broad minimum in the JT distortion. High pressure IR measurements indicate that a phonon near 390 cm-1 corresponding to the complex motion of the Mn and O ions changes anomalously for LuMnO3. It softens in the 4-8 GPa region, which is consistent with the structural change in Mn-O bonds and then hardens at high pressures. By contrast, the phonons continuously harden with increasing pressure for DyMnO3 and HoMnO3. DFT calculations show that the E-phase LuMnO3 is the most stable phase up to the 10 GPa pressure examined. Simulations indicate that the distinct structural change under pressure in LuMnO3 can possibly be used to optimize the electric polarization by pressure/strain.

cond-mat.str-el↗

arXiv2014

Nature of Structural Changes Near the Magnetic Ordering Temperature in Small-Ion Rare Earth Perovskites RMnO3

Detailed structural measurements were conducted on a new perovskite, ScMnO3, and on orthorhombic LuMnO3. Complementary density functional theory (DFT) calculations were carried out, and predict that ScMnO3 possesses E-phase magnetic order at low temperature with displacements of the Mn sites (relative to the high temperature state) of ~0.07 Å, compared to ~ 0.04 Å predicted for LuMnO3. However, detailed local, intermediate and long-range structural measurements by x-ray pair distribution function analysis, single crystal x-ray diffraction and x-ray absorption spectroscopy, find no local or long- range distortions on crossing into the low temperature E-phase of the magnetically ordered state. The measurements place upper limits on any structural changes to be at most one order of magnitude lower than density functional theory predictions and suggest that this theoretical approach does not properly account for the spin-lattice coupling in these oxides and may possibly predict the incorrect magnetic order at low temperatures. The results suggest that the electronic contribution to the electrical polarization dominates and should be properly treated in theoretical models.

cond-mat.str-el↗

arXiv2014

Valley depolarization due to inter- and intra-valley electron-hole exchange interactions in monolayer MoS$_{2}$

We investigate the valley depolarization due to the electron-hole exchange interaction in monolayer MoS$_{2}$. Both the long- and short-range parts of the intra- and inter-valley electron-hole exchange interactions are calculated. We find that both the long- and short-range exchange interactions can cause the inter- and intra-valley bright exciton transitions. With the intra-valley bright exciton transition channel nearly forbidden due to the large splitting of the valence bands, the inter-valley channel due to the exchange interaction can cause the valley depolarization efficiently by the Maialle-Silva-Sham mechanism [Phys. Rev. B {\bf 47}, 15776 (1993)]. With only the long-range exchange interaction, the calculations show good agreement with the recent valley polarization experiments, including the time-resolved valley polarization measurement, the pump-probe experiment and the steady-state PL polarization measurement. We further show that for the A-exciton with large (small) center-of-mass momentum, the long-range exchange interaction can cause the {\em fast} ({\em slow}) inter-valley exciton transition.

cond-mat.mes-hall↗

arXiv2013

Anomalous D'yakonov-Perel' spin relaxation in InAs (110) quantum wells under strong magnetic field: role of Hartree-Fock self-energy

We investigate the influence of the Hartree-Fock self-energy, acting as an effective magnetic field, on the anomalous D'yakonov-Perel' spin relaxation in InAs (110) quantum wells when the magnetic field in the Voigt configuration is much stronger than the spin-orbit-coupled field. The transverse and longitudinal spin relaxations are discussed both analytically and numerically. For the transverse configuration, it is found that the spin relaxation is very sensitive to the Hartree-Fock effective magnetic field, which is very different from the conventional D'yakonov-Perel' spin relaxation. Even an extremely small spin polarization ($P=0.1\%$) can significantly influence the behavior of the spin relaxation. It is further revealed that this comes from the {\em unique} form of the effective inhomogeneous broadening, originated from the mutually perpendicular spin-orbit-coupled field and strong magnetic field. It is shown that this effective inhomogeneous broadening is very small and hence very sensitive to the Hartree-Fock field. Moreover, we further find that in the spin polarization dependence, the transverse spin relaxation time decreases with the increase of the spin polarization in the intermediate spin polarization regime, which is also very different from the conventional situation, where the spin relaxation is always suppressed by the Hartree-Fock field. It is revealed that this {\em opposite} trends come from the additional spin relaxation channel induced by the HF field. For the longitudinal configuration, we find that the spin relaxation can be either suppressed or enhanced by the Hartree-Fock field if the spin polarization is parallel or antiparallel to the magnetic field.

cond-mat.mes-hall↗

arXiv2013

Spin relaxation in ultracold spin-orbit coupled $^{40}$K gas

We report the anomalous Dyakonov-Perel' spin relaxation in ultracold spin-orbit coupled $^{40}$K gas when the coupling between $|9/2,9/2\ >$ and $|9/2,7/2\ >$ states (atcing as the effective Zeeman magnetic field) is much stronger than the spin-orbit coupled field. Both the transverse and longitudinal spin relaxations are investigated with small and large spin polarizations. It is found that with small spin polarization, the transverse (longitudinal) spin relaxation is divided into four (two) regimes: the normal weak scattering regime, the anomalous Dyakonov-Perel'-like regime, the anomalous Elliott-Yafet-like regime and the normal strong scattering regime (the anomalous Elliott-Yafet-like regime and the normal strong scattering regime), with only the normal weak scattering regime being in the weak scattering limit. This is very different from the conventional situation under the weak magnetic field, which is divided into the weak and strong scattering regimes according to the weak/strong scattering limit. With large spin polarization, we find that the Hartree-Fock self-energy, which acts as an effective magnetic field, can markedly suppress the transverse spin relaxation in both weak and strong scattering limits. Moreover, by noting that as both the momentum relaxation time and the Hartree-Fock effective magnetic field vary with the scattering length in cold atoms, the anomalous Dyakonov-Perel'-like regime is suppressed and the transverse spin relaxation is hence divided into three regimes in the scattering length dependence: the normal weak scattering regime, the anomalous Elliott-Yafet-like regime and the strong scattering regime. On the other hand, the longitudinal spin relaxation is again divided into the anomalous EY-like and normal strong scattering regimes. ...

cond-mat.quant-gas↗

arXiv2013

Anomalous D'yakonov-Perel' spin relaxation in semiconductor quantum wells under strong magnetic field in Voigt configuration

We report an anomalous scaling of the D'yakonov-Perel' spin relaxation with the momentum relaxation in semiconductor quantum wells under a strong magnetic field in the Voigt configuration. We focus on the case that the external magnetic field is perpendicular to the spin-orbit-coupling--induced effective magnetic field and its magnitude is much larger than the later one. It is found that the longitudinal spin relaxation time is proportional to the momentum relaxation time even in the strong scattering limit, indicating that the D'yakonov-Perel' spin relaxation shows the Elliott-Yafet-like behaviour. Moreover, the transverse spin relaxation time is inversely proportional (proportional) to the momentum relaxation time in the weak (strong) scattering limit, both in the opposite trends against the well-established conventional D'yakonov-Perel' spin relaxation behaviours. We further demonstrate that all the above anomalous scaling relations come from the unique form of the effective inhomogeneous broadening.

cond-mat.mes-hall↗

arXiv2013

Ferroelectricity in Single Crystal InMnO3

Single crystal synthesis, structure, electric polarization and heat capacity measurements on hexagonal InMnO3 show that this small R ion in the RMnO3 series is ferroelectric (space group P63cm). Structural analysis of this system reveals a high degree of order within the MnO5 polyhedra but significant distortions in the R-O bond distributions compared to the previously studied materials. Point-charge estimates of the electric polarization yield an electrical polarization of approximately 7.8 micro C/cm^2, 26% larger than the well-studied YMnO3 system. This system with enhanced room temperature polarization values may serve as a possible replacement for YMnO3 in device application.

cond-mat.mtrl-sci↗

arXiv2011

Local Structure of the Superconductor K0.8Fe1.6+xSe2: Evidence of Large Structural Disorder

The local structure of superconducting single crystals of K0.8Fe1.6+xSe2 with Tc = 32.6 K was studied by x-ray absorption spectroscopy. Near-edge spectra reveal that the average valence of Fe is 2+. The room temperature structure about the Fe, K and Se sites was examined by iron, selenium and potassium K-edge measurements. The structure about the Se and Fe sites shows a high degree of order in the nearest neighbor Fe-Se bonds. On the other hand, the combined Se and K local structure measurements reveal a very high level of structural disorder in the K layers. Temperature dependent measurements at the Fe sites show that the Fe-Se atomic correlation follows that of the Fe-As correlation in the superconductor LaFeAsO0.89F0.11 - having the same effective Einstein temperature (stiffness). In K0.8Fe1.6+xSe2, the nearest neighbor Fe-Fe bonds has a lower Einstein temperature and higher structural disorder than in LaFeAsO0.89F0.11. The moderate Fe site and high K site structural disorder is consistent with the high normal state resistivity seen in this class of materials. For higher shells, an enhancement of the second nearest neighbor Fe-Fe interaction is found just below Tc and suggests that correlations between Fe magnetic ion pairs beyond the first neighbor are important in models of magnetic order and superconductivity in these materials.

cond-mat.supr-con↗

arXiv2009

Fabrication of graphene nanogap with crystallographically matching edges and its electron emission properties

We demonstrate the fabrication of graphene nanogap with crystallographically matching edges on SiO2Si substrates by divulsion. The current-voltage measurement is then performed in a high-vacuum chamber for a graphene nanogap with few hundred nanometers separation. The parallel edges help to build uniform electrical field and allow us to perform electron emission study on individual graphene. It was found that current-voltage characteristics are governed by the space-charge-limited flow of current at low biases while the FN model fits the I-V curves in high voltage regime. We also examined electrostatic gating effect of the vacuum electronic device. Graphene nanogap with atomically parallel edges may open up opportunities for both fundamental and applied research of vacuum nanoelectronics.

cond-mat.mes-hall↗

arXiv2008

Fabrication of graphene nanodisk arrays using nanosphere lithography

Ordered graphene nanodisk arrays have been successfully fabricated by combining nanosphere lithography (NSL) and reactive ion etching (RIE) processes. The dimension of graphene nanodisks can be effectively tuned by varying the size of polystyrene spheres, which function as masks during RIE. Low voltage scanning electron microscopy shows that the graphene sheet could be readily patterned into periodic disk-like nanostructures by oxygen RIE. Raman mapping and spectroscopy further visualize such nanodisk arrays and reveal the nature of disks are crystalline single layer graphene. This work demonstrates an efficient and manageable way to pattern graphene. Considering the periodicity, nanometer dimension and large edge to body ratio, the graphene nanodisk arrays, such two dimensional assembly of carbon atoms offer intrisic advantages in various electronic and spintronic fabrications.

cond-mat.mtrl-sci↗

arXiv2008

Raman spectroscopy of epitaxial graphene on a SiC substrate

The fabrication of epitaxial graphene (EG) on SiC substrate by annealing has attracted a lot of interest as it may speed up the application of graphene for future electronic devices. The interaction of EG and the SiC substrate is critical to its electronic and physical properties. In this work, Raman spectroscopy was used to study the structure of EG and its interaction with SiC substrate. All the Raman bands of EG blue shift from that of bulk graphite and graphene made by micromechanical cleavage, which was attributed to the compressive strain induced by the substrate. A model containing 13 x 13 honeycomb lattice cells of graphene on carbon nanomesh was constructed to explain the origin of strain. The lattice mismatch between graphene layer and substrate causes the compressive stress of 2.27 GPa on graphene. We also demonstrate that the electronic structures of EG grown on Si and C terminated SiC substrates are quite different. Our experimental results shed light on the interaction between graphene and SiC substrate that are critical to the future applications of EG.

cond-mat.mtrl-sci↗

arXiv2002

Phonon decoherence of quantum entanglement: Robust and fragile states

We study the robustness and fragility of entanglement of open quantum systems in some exactly solvable models in which the decoherence is caused by a pure dephasing process. In particular, for the toy models presented in this paper, we identify two different time scales, one is responsible for local dephasing, while the other is for entanglement decay. For a class of fragile entangled states defined in this paper, we find that the entanglement of two qubits, as measured by concurrence, decays faster asymptotically than the quantum dephasing of an individual qubit.

quant-ph↗

arXiv1995

Alternative Derivation of the Hu-Paz-Zhang Master Equation for Quantum Brownian Motion

Hu, Paz and Zhang [ B.L. Hu, J.P. Paz and Y. Zhang, Phys. Rev. D {\bf 45} (1992) 2843] have derived an exact master equation for quantum Brownian motion in a general environment via path integral techniques. Their master equation provides a very useful tool to study the decoherence of a quantum system due to the interaction with its environment. In this paper, we give an alternative and elementary derivation of the Hu-Paz-Zhang master equation, which involves tracing the evolution equation for the Wigner function. We also discuss the master equation in some special cases.

quant-ph↗