arXiv subjects

T. Ziman

Publications and source records attributed to T. Ziman.

At least 19 recordsLinked to original sources

arXiv2025

Longitudinal magnons in large-$S$ easy-axis magnets

Longitudinal magnons are a distinct type of multipolar excitations in magnetic materials with large spins $S\ge 1$ and strong easy-axis anisotropy. These excitations have angular momentum $S^z = \pm 2S$ and can be viewed as a propagating full spin reversal. We study longitudinal magnons for the nearest-neighbor Heisenberg ferromagnet and antiferromagnet on a square lattice with large single-ion anisotropy. In the strong-coupling limit, we derive an effective spin-1/2 model including two leading contributions in $J/D$. The effective model provides a simple description of the longitudinal magnon dynamics. For $S=1$, we compare results from several theoretical approaches that include the effective spin-1/2 model, the linked-cluster expansion, the multiboson spin-wave theory, and, for a ferromagnet, an exact two-particle solution. Among these approaches, the multiboson spin-wave theory provides the decay rate of longitudinal magnons and describes evolution of the excitation spectra from strong to weak anisotropy.

cond-mat.str-el↗

arXiv2025

Fully-frustrated octahedral antiferromagnets: emergent complexity in external field

Octahedral antiferromagnets are distinguished by crystal lattices composed of octahedra of magnetic ions. In the fully frustrated case, the Heisenberg Hamiltonian can be represented as a sum of squares of total spins for each octahedral block. We study the fully frustrated spin model for a lattice of edge-shared octahedra, which corresponds to the J1-J2 fcc antiferromagnet with J2/J1 = 1/2. The magnetization process at this strongly frustrated point features a remarkably rich sequence of different magnetic phases that include fractional plateaus at m = 1/3 and 2/3 values of the total magnetization. By performing extensive Monte Carlo simulations we construct the H-T phase diagram of the classical model with eight field-induced states, which acquire stability via the order by disorder mechanism. These antiferromagnetic states have distinct spin configurations of their octahedral blocks. The same spin configurations are also relevant for the fully frustrated corner-shared model bringing an apparent similarity to their field-induced states.

cond-mat.str-el↗

arXiv2022

Ground state selection by magnon interactions in the fcc antiferromagnet

We study the nearest-neighbor Heisenberg antiferromagnet on a face-centered cubic lattice with arbitrary spin S. The model exhibits degenerate classical ground states including two collinear structures AF1 and AF3 described by different propagation vectors that are prime candidates for the quantum ground state. We compute the energy for each of the two states as a function of S using the spin-wave theory that includes magnon-magnon interaction in a self-consistent way and the numerical coupled cluster method. Our results unambiguously demonstrate that quantum fluctuations stabilize the AF1 state for realistic values of spin. Transition to the harmonic spin-wave result, which predicts the AF3 state, takes place only for S > 10. We also study quantum renormalization of the magnon spectra for both states as a function of spin.

cond-mat.str-el↗

arXiv2022

Noncoplanar multi-k states in frustrated spinel and kagome magnets

We investigate analytically and numerically the classical ground states of frustrated Heisenberg models on pyrochlore and kagome lattices in zero and finite magnetic fields. Each model has a wide region in the microscopic parameter space, where the propagation vector is turned to a commensurate position equal to a half of the reciprocal lattice vector with a nontrivial star. Within these regions the zero-field ground states for both models correspond to noncoplanar triple-k spin configurations. A universal appearance of the 3-k states can be related to the spin-space dimensionality. A strong magnetic field freezes the longitudinal spin component reducing the spin-space dimensionality. Accordingly, we find transitions into the double-k magnetic structures induced by applied field for both spin models. The predicted transition between 3-k and 2-k states may explain the hitherto unexplained transitions observed experimentally in cubic spinels GeNi2O4 and GeCo2O4 under magnetic field.

cond-mat.str-el↗

arXiv2021

Superconducting spin valves based on a single spiral magnetic layer

A detailed investigation of a superconducting spin-triplet valve is presented. This spin-valve consists of a superconducting film covering a metal with an intrinsic spiral magnetic order, which could result from competing isotropic exchanges or, if the crystal lattice breaks central symmetry, from asymmetric Dzyaloshinskii-Moriya exchange. Depending on the anisotropy, such a metal may change its magnetization either from a spiral to uniform order, as seen in Ho and Er, or in the direction of the spiral itself, as in crystals of the B20-type structure (such as MnSi, (Fe,Co)Si, FeGe, etc.). The nonuniform magnetic order controls the appearance of long-range triplet superconducting correlations at strong exchange fields, affecting the detailed character of the proximity effect. We show that the magnetic control of the spin-valve behavior can also be obtained from moderately low exchange fields (typically associated to negligible long-range triplet correlations), thanks to an orientation-dependent averaging mechanism of the magnetic inhomogeneity on the scale of the Cooper pairs. Our numerical calculations reveal that the spin-valve effect is in fact magnified at moderately low exchange fields, when the exchange splitting in the spiral magnet is comparable to the superconducting gap, and the spiral period is less than or equal to the superconducting coherence length in the magnet multiplied by $2\pi$.

cond-mat.supr-con↗

arXiv2020

Quantum versus thermal fluctuations in the fcc antiferromagnet: alternative routes to order by disorder

In frustrated magnetic systems with competing interactions fluctuations can lift the residual accidental degeneracy. We argue that the state selection may have different outcomes for quantum and thermal order by disorder. As an example, we consider the semiclassical Heisenberg fcc antiferromagnet with only the nearest-neighbor interactions. Zero-point oscillations select the type 3 collinear antiferromagnetic state at T=0. Thermal fluctuations favor instead the type 1 antiferromagnetic structure. The opposite tendencies result in a finite-temperature transition between the two collinear states. Competition between effects of quantum and thermal order by disorder is a general phenomenon and is also realized in the J1-J2 square-lattice antiferromagnet at the critical point J2 = 0.5 J1.

cond-mat.str-el↗

arXiv2020

Evidence for biquadratic exchange in the quasi-two-dimensional antiferromagnet FePS$_3$

FePS$_3$ is a van der Waals compound with a honeycomb lattice that is a good example of a two-dimensional antiferromagnet with Ising-like anisotropy. Neutron spectroscopy data from FePS3 were previously analysed using a straight-forward Heisenberg Hamiltonian with a single-ion anisotropy. The analysis captured most of the elements of the data, however some significant discrepancies remained. The discrepancies were most obvious at the Brillouin zone boundaries. The data are subsequently reanalysed allowing for unequal exchange between nominally equivalent nearest-neighbours, which resolves the discrepancies. The source of the unequal exchange is attributed to a biquadratic exchange term in the Hamiltonian which most probably arises from a strong magnetolattice coupling. The new parameters show that there are features consistent with Dirac magnon nodal lines along certain Brillouin zone boundaries.

cond-mat.mtrl-sci↗

arXiv2019

Observation of the Magnon Polarization

We measure the mode-resolved direction of the precessional motion of the magnetic order, i.e., magnon polarization, via the chiral term of inelastic polarized neutron scattering spectra. The magnon polarisation is important in spintronics, affecting thermodynamic properties such as the magnitude and sign of the spin Seebeck effect. The observation of both signs of magnon polarization in Y3Fe5O12 also gives direct proof of its ferrimagnetic nature. The experiments agree very well with atomistic simulations of the scattering cross section.

cond-mat.mtrl-sci↗

arXiv2019

Magnetic order and single-ion anisotropy in Tb$_3$Ga$_5$O$_{12}$

Terbium gallium garnet (TGG), Tb$_3$Ga$_5$O$_{12}$, is well known for its applications in laser optics, but also exhibits complex low-temperature magnetism that is not yet fully understood. Its low-temperature magnetic order is determined by means of time-of-flight neutron powder diffraction. It is found to be a multiaxial antiferromagnet with magnetic Tb$^{3+}$ ions forming six sublattices of magnetic moments aligned parallel and anti-parallel to the $\langle100\rangle$ crystallographic directions of the cubic unit cell. The structure displays strong easy-axis anisotropy with respect to a two-fold axis of symmetry in the local orthorhombic environment of the Tb$^{3+}$ sites. The crystal-field splitting within the single-ion ground-state manifold is investigated by inelastic neutron scattering on powder samples. A strong temperature dependence of the quasidoublet ground-state is observed and revised parameters of the crystal-field Hamiltonian are given. The results of bulk magnetic susceptibility and magnetisation measurements are in good agreement with values based on the crystal-field model down to 20~K, where the onset of magnetic correlations is observed.

cond-mat.str-el↗

arXiv2016

Helicity, anisotropies and their competition in a multiferroic magnet: insight from the phase diagram

Motivated by the complex phase diagram of MnWO4, we investigate competition between anisotropy, magnetic field, and helicity for the anisotropic next-nearest-neighbor Heisenberg model. Apart from two competing exchanges, which favor a spiral magnetic structure, the model features the bi-axial single-ion anisotropy. The model is treated in the real-space mean-field approximation and the phase diagram containing various incommensurate and commensurate states is obtained for different field orientations. We discuss similarities and differences of the theoretical phase diagram and the experimental diagram of MnWO4.

cond-mat.str-el↗

arXiv2015

Strong Suppression of the Spin Hall Effect in the Spin Glass State

We have measured spin Hall effects in spin glass metals, CuMnBi alloys, with the spin absorption method in the lateral spin valve structure. Far above the spin glass temperature Tg where the magnetic moments of Mn impurities are randomly frozen, the spin Hall angle of CuMnBi ternary alloy is as large as that of CuBi binary alloy. Surprisingly, however, it starts to decrease at about 4Tg and becomes as little as 7 times smaller at 0.5Tg. A similar tendency was also observed in anomalous Hall effects in the ternary alloys. We propose an explanation in terms of a simple model considering the relative dynamics between the localized moment and the conduction electron spin.

cond-mat.mes-hall↗

arXiv2015

Neutrons on a surface of liquid helium

We investigate the possibility of ultracold neutron (UCN) storage in quantum states defined by the combined potentials of the Earth's gravity and the neutron optical repulsion by a horizontal surface of liquid helium. We analyse the stability of the lowest quantum state, which is most susceptible to perturbations due to surface excitations, against scattering by helium atoms in the vapor and by excitations of the liquid, comprised of ripplons, phonons and surfons. This is an unusual scattering problem since the kinetic energy of the neutron parallel to the surface may be much greater than the binding energies perpendicular. The total scattering time constant of these UCNs at 0.7 K is found to exceed one hour, and rapidly increasing with decreasing temperature. Such low scattering rates should enable high-precision measurements of the scheme of discrete energy levels, thus providing improved access to short-range gravity. The system might also be useful for neutron beta-decay experiments. We also sketch new experimental concepts for level population and trapping of UCNs above a flat horizontal mirror.

nucl-ex↗

arXiv2012

Theory of the spin Hall effect, and its inverse, in a ferromagnetic metal near the Curie temperature

We give a theory of the inverse spin Hall effect (ISHE) in ferromagnetic metals based on skew scattering via collective spin fluctuations. This extends Kondo's theory of the anomalous Hall effect (AHE) to include short-range spin-spin correlations. We find a relation between the ISHE and the four-spin correlations near the Curie temperature TC. Such four-spin correlations do not contribute to the AHE, which relates to the three-spin correlations. Thus our theory shows an essential difference between the AHE and ISHE, providing an essential complement to Kondo's classic theory of the AHE in metals. We note the relation to skew-scattering mechanisms based on impurity scattering. Our theory can be compared to recent experimental results byWei et al. [Nat. Commun. 3, 1058 (2012)] for the ISHE in ferromagnetic alloys.

cond-mat.mes-hall↗

arXiv2012

The spin Hall effect as a probe of nonlinear spin fluctuations

The spin Hall effect and its inverse play key roles in spintronic devices since they allow conversion of charge currents to and from spin currents. The conversion efficiency strongly depends on material details, such as the electronic band structure and the nature of impurities. Here we show an anomaly in the inverse spin Hall effect in weak ferromagnetic NiPd alloys near their Curie temperatures with a shape independent of material details, such as Ni concentrations. By extending Kondo's model for the anomalous Hall effect, we explain the observed anomaly as originating from the second-order nonlinear spin fluctuation of Ni moments. This brings to light an essential symmetry difference between the spin Hall effect and the anomalous Hall effect which reflects the first order nonlinear fluctuations of local moments. Our finding opens up a new application of the spin Hall effect, by which a minuscule magnetic moment can be detected.

cond-mat.mes-hall↗

arXiv2011

Competing Hyperfine and Spin-Orbit Couplings: Spin Relaxation in a Quantum Hall Ferromagnet

Spin relaxation in a quantum Hall ferromagnet, where filling is $ν=1, 1/3, 1/5,...$, can be considered in terms of spin wave annihilation/creation processes. Hyperfine coupling with the nuclei of the GaAs matrix provides spin non-conservation in the two-dimensional electron gas and determines spin relaxation in the quantum Hall system. This mechanism competes with spin-orbit coupling channels of spin-wave decay and can even dominate in a low-temperature regime where $T$ is much smaller than the Zeeman gap. In this case the spin-wave relaxation process occurs non-exponentially with time and does not depend on the temperature. The competition of different relaxation channels results in crossovers in the dominant mechanism, leading to non-monotonic behavior of the characteristic relaxation time with the magnetic field. We predict that the relaxation times should reach maxima at $B\simeq 18\,$T in the $ν=1$ Quantum Hall system and at $B\simeq 12\,$T for that of $ν=1/3\,$. We estimate these times as $\sim10\,-\,30\,μ$s and $\sim2\,-\,5\,μ$s, respectively.

cond-mat.str-el↗

arXiv2010

Surface-assisted Spin Hall Effect in Au Films with Pt Impurities

We show, both experimentally and theoretically, a novel route to obtain giant room temperature spin Hall effect due to surface-assisted skew scattering. In the experiment, we report the spin Hall effect in Pt-doped Au films with different thicknesses $t_N$. The giant spin Hall angle $\gamma_S$ = $0.12 \pm 0.04$ is obtained for $t_N$ = 10 nm at room temperature, while it is much smaller for $t_N$ = 20 nm sample. Combined ab initio and quantum Monte Carlo calculations for the skew scattering due to a Pt impurity show $\gamma_S$ $\cong$ 0.1 on the Au (111) surface, while it is small in bulk Au. The quantum Monte Carlo results show that the spin-orbit interaction of the Pt impurity on the Au (111) surface is enhanced, because the Pt 5d levels are lifted to the Fermi level due to the valence fluctuation. In addition, there are two spin-orbit interaction channels on the Au (111) surface, while only one in bulk Au.

cond-mat.mtrl-sci↗

arXiv2009

Glassy Spin Freezing and Gapless Spin Dynamics in a Spatially Anisotropic Triangular Antiferromagnet Ag2MnO2

Using elastic and inelastic neutron scattering techniques, we show that upon cooling a spatially anisotropic triangular antiferromagnet Ag$_2$MnO$_2$ freezes below $T_f ~\sim 50$ K into short range collinear state. The static spin correlations are extremely two-dimensional, and the spin fluctuations are gapless with two characteristic relaxation rates that behave linearly with temperature.

cond-mat.str-el↗

arXiv2006

Magnon Dispersion and Anisotropies in SrCu$_2$(BO$_3$)$_2$

We study the dispersion of the magnons (triplet states) in SrCu$_2$(BO$_3$)$_2$ including all symmetry-allowed Dzyaloshinskii-Moriya interactions. We can reduce the complexity of the general Hamiltonian to a new simpler form by appropriate rotations of the spin operators. The resulting Hamiltonian is studied by both perturbation theory and exact numerical diagonalization on a 32-site cluster. We argue that the dispersion is dominated by Dzyaloshinskii-Moriya interactions. We point out which combinations of these anisotropies affect the dispersion to linear-order, and extract their magnitudes.

cond-mat.mtrl-sci↗