arXiv subjects

T. Zou

Publications and source records attributed to T. Zou.

10 recordsLinked to original sources

arXiv2026

Magnetotransport Spectroscopy of Strongly Rashba-Split Hole Subbands Reveals Many-Body Interactions

We report the results of magnetotransport experiments carried out on low-disorder 2D hole gases (2DHG) in the strongly correlated liquid regime, hosted in dopant-free (100) GaAs/AlGaAs single heterojunctions. Over a wide range of 2DHG densities (from 0.7 $\times$ 10$^{15}$/m$^2$ to $2 \times 10^{15}$/m$^2$), Fourier analysis of low-field (B < 1 T) Shubnikov-de Haas oscillations reveals two spin-orbit-split heavy-hole (HH) subbands with distinct effective masses contributing to transport. Surprisingly, the lighter-mass HH subband exhibits a parabolic dispersion with Fermi wavevector below the anticrossing between the heavy-hole and light-hole subbands, while the heavier HH subband is non-parabolic throughout. Quantitative comparison with numerical calculations based on the Luttinger model reveals that both effective masses are enhanced by a common factor ($\approx$ 2.3), which we attribute to many-body interactions. This common scaling factor has a very weak dependence on the 2DHG density, likely due to band hybridization. Our measured hole masses are compared with published cyclotron resonance and magnetotransport values. We propose a cohesive framework reconciling the long-standing three-way discrepancy between Luttinger theory, magnetotransport, and cyclotron resonance measurements of density-dependent effective masses in partially spin-orbit-polarized heavy-hole systems in GaAs.

cond-mat.mes-hall↗

arXiv2026

Enhanced effective masses, spin-orbit polarization, and dispersion relations in 2D hole gases under strongly asymmetric confinement

The dispersion of Rashba-split heavy-hole subbands in GaAs two-dimensional hole gases (2DHGs) is difficult to access experimentally because strong heavy-hole-light-hole mixing produces non-parabolicity and breaks the usual correspondence between carrier density and Fermi wave vector. Here we use low-field magnetotransport (B < 1 T) to reconstruct the dispersions of the two spin-orbit-split heavy-hole branches (HH-, HH+) in undoped (100) GaAs/AlGaAs single heterojunction 2DHGs operated in an accumulation-mode field-effect geometry. The dopant-free devices sustain out-of-plane electric fields up to 26 kV/cm while maintaining mobilities up to 84 m$^2$/Vs and exhibiting a spin-orbit polarization as large as 36%. Fourier analysis of Shubnikov-de Haas (SdH) oscillations resolves the individual HH-/HH+ subband densities; fitting the temperature dependence of the corresponding Fourier amplitudes yields both branch-resolved SdH effective masses over the same magnetic field window. SdH regimes in which reliable subband parameters can be extracted are delineated. Over 2DHG densities (0.76-1.9) $\times$ 10$^{15}$ /m$^2$, the HH- mass is nearly density independent ($\approx 0.34m_e$), implying a near-parabolic HH- dispersion below the first LH+/HH- anticrossing, whereas HH+ exhibits strong non-parabolicity with an effective mass that increases with density. Combining the extracted dispersions yields a transport-based determination of the spin-orbit splitting energy $\Delta_\text{HH}$ between HH and HH+ as a function of in-plane wave vector. Parameter-free Luttinger-model calculations reproduce the qualitative trends but underestimate both masses by a common factor $\approx$ 2, suggesting a many-body renormalization of the heavy-hole mass in this strongly asymmetric regime.

cond-mat.mes-hall↗

arXiv2024

Magnetic structure and magnetoelectric coupling in antiferromagnet Co5(TeO3)4Cl2

The van der Waals (vdW) layered multiferroics, which host simultaneous ferroelectric and magnetic orders, have attracted attention not only for their potentials to be utilized in nanoelectric devices and spintronics, but also offer alternative opportunities for emergent physical phenomena. To date, the vdW layered multiferroic materials are still very rare. In this work, we have investigated the magnetic structure and magnetoelectric effects in Co5(TeO3)4Cl2, a promising new multiferroic compound with antiferromagnetic (AFM) Neel point TN = 18 K. The neutron powder diffraction reveals the non-coplanar AFM state with preferred Neel vector along the c-axis, while a spin re-orientation occurring between 8 K and 15 K is identified, which results from the distinct temperature dependence of the non-equivalent Co sites moment in Co5(TeO3)4Cl2. What is more, it is found that Co5(TeO3)4Cl2 is one of the best vdW multiferroics studied so far in terms of the multiferroic performance. The measured linear ME coefficient exhibits the emergent oscillation dependence of the angle between magnetic field and electric field, and the maximal value is as big as 45 ps/m. It is suggested that Co5(TeO3)4Cl2 is an appreciated platform for exploring the emergent multiferroicity in vdW layered compounds.

cond-mat.mtrl-sci↗

arXiv2023

Cokrig-and-Regress for Spatially Misaligned Environmental Data

Spatially misaligned data, where the response and covariates are observed at different spatial locations, commonly arise in many environmental studies. Much of the statistical literature on handling spatially misaligned data has been devoted to the case of a single covariate and a linear relationship between the response and this covariate. Motivated by spatially misaligned data collected on air pollution and weather in China, we propose a cokrig-and-regress (CNR) method to estimate spatial regression models involving multiple covariates and potentially non-linear associations. The CNR estimator is constructed by replacing the unobserved covariates (at the response locations) by their cokriging predictor derived from the observed but misaligned covariates under a multivariate Gaussian assumption, where a generalized Kronecker product covariance is used to account for spatial correlations within and between covariates. A parametric bootstrap approach is employed to bias-correct the CNR estimates of the spatial covariance parameters and for uncertainty quantification. Simulation studies demonstrate that CNR outperforms several existing methods for handling spatially misaligned data, such as nearest-neighbor interpolation. Applying CNR to the spatially misaligned air pollution and weather data in China reveals a number of non-linear relationships between PM$_{2.5}$ concentration and several meteorological covariates.

stat.ME↗

arXiv2020

Magnetic Field Induced Phase Transition in Spinel GeNi2O4

Cubic spinel GeNi2O4 exhibits intriguing magnetic properties with two successive antiferromagnetic phase transitions (TN1 12.1 and TN2 11.4 K) with the absence of any structural transition. We have performed detailed heat capacity and magnetic measurements in different crystallographic orientations. A new magnetic phase in presence of magnetic field (H > 4 T) along the [111] direction is revealed, which is not observed when the magnetic field is applied along the [100] and [110] directions. High field neutron powder diffraction measurements confirm such a change in magnetic phase, which could be ascribed to a spin reorientation in the presence of magnetic field. A strong magnetic anisotropy and competing magnetic interactions play a crucial role on the complex magnetic behavior in this cubic system.

cond-mat.str-el↗

arXiv2018

Colossal magnetoresistance in a Mott insulator via magnetic field-driven insulator-metal transition

We present a new type of colossal magnetoresistance (CMR) arising from an anomalous collapse of the Mott insulating state via a modest magnetic field in a bilayer ruthenate, Ti-doped Ca$_3$Ru$_2$O$_7$. Such an insulator-metal transition is accompanied by changes in both lattice and magnetic structures. Our findings have important implications because a magnetic field usually stabilizes the insulating ground state in a Mott-Hubbard system, thus calling for a deeper theoretical study to reexamine the magnetic field tuning of Mott systems with magnetic and electronic instabilities and spin-lattice-charge coupling. This study further provides a model approach to search for CMR systems other than manganites, such as Mott insulators in the vicinity of the boundary between competing phases.

cond-mat.str-el↗

arXiv2018

Non-Fermi surface nesting driven commensurate magnetic ordering in Fe-doped Sr$_2$RuO$_4$

Sr$_2$RuO$_4$, an unconventional superconductor, is known to possess an incommensurate spin density wave instability driven by Fermi surface nesting. Here we report a static spin density wave ordering with a commensurate propagation vector $q_c$ = (0.25 0.25 0) in Fe-doped Sr$_2$RuO$_4$, despite the magnetic fluctuations persisting at the incommensurate wave vectors $q_{ic}$ = (0.3 0.3 L) as in the parent compound. The latter feature is corroborated by the first principles calculations, which show that Fe substitution barely changes the nesting vector of the Fermi surface. These results suggest that in addition to the known incommensurate magnetic instability, Sr$_2$RuO$_4$ is also in proximity to a commensurate magnetic tendency that can be stabilized via Fe doping.

cond-mat.str-el↗

arXiv2016

Unusual UUDD magnetic chain structure of the spin-1/2 tetragonally distorted spinel GeCu2O4

GeCu2O4 exhibits a tetragonal spinel structure due to the strong Jahn-Teller distortion associated with Cu2+ ions. We show that its magnetic structure can be described as slabs composed of a pair of layers with orthogonally oriented spin 1/2 Cu chains in the basal ab plane. The spins between the two layers within a slab are collinearly aligned while the spin directions of neighboring slabs are perpendicular to each other. Interestingly, we find that spins along each chain form an unusual up-up-down-down (UUDD) pattern, suggesting a non-negligible nearest-neighbor biquadratic exchange interaction in the effective classical spin Hamiltonian. We hypothesize that spin-orbit coupling and orbital mixing of Cu2+ ions in this system is non-negligible, which calls for future calculations using perturbation theory with extended Hilbert (spin and orbital) space and calculations based on density functional theory including spin-orbit coupling and looking at the global stability of the UUDD state.

cond-mat.mtrl-sci↗

arXiv2016

Unusual interlayer quantum transport behavior caused by the zeroth Landau level in YbMnBi2

Relativistic fermions in topological quantum materials are characterized by linear energy-momentum dispersion near band crossing points. Under magnetic field, relativistic fermions acquire Berry phase of π in cyclotron motion, leading to a zeroth Landau level (LL) at the crossing point. Such field-independent zeroth LL, which distinguishes relativistic fermions from conventional electron systems, is hardly probed in transport measurements since the Fermi energy (EF) is usually not right at the band crossing points in most topological materials. Here we report the observation of exotic quantum transport behavior resulting from the zeroth LL in a multiband topological semimetal YbMnBi2 which possesses linear band crossings both at and away from the Fermi level (FL). We show that the Dirac bands with the crossing points being above or below the FL leads to Shubnikov de-Haas oscillations in the in-plane magnetoresistance, whereas the Dirac bands with the crossing points being at the FL results in unusual angular dependences of the out-of-plane magnetoresistance and in-plane Hall resistivity due to the dependence of the zeroth LL's degeneracy on field orientation. Our results shed light on the transport mechanism of the zeroth LL's relativistic fermions in layered materials.

cond-mat.mtrl-sci↗

arXiv2013

Magnetoelectric coupling in the paramagnetic state of a metal-organic framework

Although the magnetoelectric effects - the mutual control of electric polarization by magnetic fields and magnetism by electric fields, have been intensively studied in a large number of inorganic compounds and heterostructures, they have been rarely observed in organic materials. Here we demonstrate magnetoelectric coupling in a metal-organic framework [(CH3)2NH2]Mn(HCOO)3 which exhibits an order-disorder type of ferroelectricity below 185 K. The magnetic susceptibility starts to deviate from the Curie-Weiss law at the paraelectric-ferroelectric transition temperature, suggesting an enhancement of short-range magnetic correlation in the ferroelectric state. Electron spin resonance study further confirms that the magnetic state indeed changes following the ferroelectric phase transition. Inversely, the ferroelectric polarization can be improved by applying high magnetic fields. We interpret the magnetoelectric coupling in the paramagnetic state in the metal-organic framework as a consequence of the magnetoelastic effect that modifies both the superexchange interaction and the hydrogen bonding.

cond-mat.mtrl-sci↗