arXiv subjects

Tai Hyun Yoon

Publications and source records attributed to Tai Hyun Yoon.

17 recordsLinked to original sources

arXiv2026

Quantum Optical Simulator for Unruh-DeWitt Detector Dynamics

We present a quantum-optical platform for simulating relativistic detector-field interactions using entangled nonlinear biphoton sources (ENBSs), realized through phase-controlled single-photon frequency-comb (SPFC) sources. By mapping the dynamical evolution of this system onto the Unruh-DeWitt (UDW) detector model, we show that signal-mode excitations emulate detector transitions driven by vacuum fluctuations, while coherently seeded idler modes act as an effective quantum field. This correspondence enables tabletop exploration of Unruh-like excitation, coherence harvesting, and field-induced entanglement. We derive the effective interaction Hamiltonian and Lindblad master equation for two coherently seeded ENBS units and obtain analytical solutions for the signal photon number $N_{\rm sig}(t)$ and second-order correlation function $g^{(2)}(0;t)$. Numerical simulations confirm that phase-dependent biphoton dynamics reproduce UDW-type behavior, including tunable excitation and quantum correlations. The output signal state exhibits controllable fidelity, interference visibility, and entanglement entropy as functions of the seeding phase and amplitude. These results establish ENBSs as experimentally accessible quantum simulators of relativistic field phenomena, providing a photonic testbed for analog gravitational effects, vacuum fluctuations, and spacetime-induced coherence-all within reach of current nonlinear-optics technology.

quant-ph↗

arXiv2026

Measurement-defined control of single-particle interference

Interference is conventionally attributed to path-accumulated phase differences, with measurement treated as a passive readout. Here we demonstrate that single-particle interference is governed by the relative phase between the prepared quantum state and the detector-defined measurement basis -- a joint quantity that is operationally inaccessible in any conventional interferometer. Using coherently seeded entangled nonlinear biphoton sources, we show that independently scanning the pump phase difference, the seed phase difference, or the signal interferometric phase each produces identical sinusoidal fringes ($V\approx0.99$) -- a three-scan equivalence impossible in any two-mode interferometer. The fringe visibility is continuously controlled through the idler-state overlap, directly encoding quantum distinguishability without idler detection. The same measurement-defined interference law persists from the single-photon to the high-flux regime. The bright-dark collective-state structure demonstrated here unifies coherent population trapping and electromagnetically induced transparency in atomic $Λ$-systems, discrete photonic interference, and single-slit diffraction within a common framework differing only in dark-subspace dimensionality, establishing measurement-defined photonic modes as a fundamental resource for quantum photonics.

quant-ph↗

arXiv2026

A hardware-native time-frequency GKP logical qubit toward fault-tolerant photonic operation

We realize a hardware-native time--frequency Gottesman--Kitaev--Preskill (GKP) logical qubit encoded in the continuous phase space of single photons, establishing a propagating photonic implementation of bosonic grid encoding. Finite-energy grid states are generated deterministically using coherently driven entangled nonlinear biphoton sources that produce single-photon frequency-comb supermodes. An optical-frequency-comb reference anchors the time--frequency phase space and enforces commuting displacement stabilizers directly at the hardware level, continuously defining the logical subspace. Timing jitter, spectral drift, and phase noise map naturally onto Gaussian displacement errors within this lattice, yielding intrinsic correctability inside a stabilizer cell. Logical operations correspond to experimentally accessible phase and delay controls, enabling deterministic state preparation and manipulation. Building on the modal time--frequency GKP framework, we identify a concrete pathway toward active syndrome extraction and deterministic displacement recovery using ancillary grid states and interferometric time--frequency measurements. These primitives establish a hardware-compatible route for integrating the time--frequency GKP logical layer into erasure-aware and fusion-based fault-tolerant photonic architectures.

quant-ph↗

arXiv2025

MAQCY: Modular Atom-Array Quantum Computing with Space-Time Hybrid Multiplexing

We present a modular atom-array quantum computing architecture with space-time hybrid multiplexing (MAQCY), a dynamic optical tweezer-based protocol for fully connected and scalable universal quantum computation. By extending the concept of globally controlled static dual-species Rydberg atom wires [1], we develop an entirely new approach using Q-Pairs, which consist of globally controlled and temporally multiplexed dual-species Rydberg blockaded atom and superatom pairs. Space-time hybrid multiplexing of Q-Pairs achieves O(N) linear scaling in the number of required physical qubits, while preserving coherence and mitigating circuit-depth limitations through in-situ atom replacement. To demonstrate MAQCY's versatility, we implement a three-qubit quantum Fourier transform using only global operations and atom transport. We also propose a concrete implementation using ytterbium isotopes, paving the way toward large-scale, fault-tolerant quantum computing.

quant-ph↗

arXiv2025

In situ and real-time ultrafast spectroscopy of photoinduced reactions in perovskite nanomaterials

Employing two synchronized mode-locked femtosecond lasers and interferometric detection of the pump-probe spectra -- referred to as asynchronous and interferometric transient absorption (AI-TA) -- we have developed a method for broad dynamic range and rapid data acquisition. Using AI-TA, we examined photochemical changes during femtosecond pump-probe experiments on all-inorganic cesium lead halide nanomaterials, including perovskite nanocrystals (PeNCs) and nanoplatelets (PeNPLs). The laser pulse train facilitates photoreactions while allowing real-time observation of charge carrier dynamics. In PeNCs undergoing halide anion photo-substitution, transient absorption spectra showed increasing bandgap energy and faster relaxation dynamics as the Cl/Br ratio increased. For colloidal PeNPLs, continuous observation revealed both spectral and kinetic changes during the light-induced coalescence of nanoplatelets, by analyzing temporal segments. This integrated technique not only deepens understanding of exciton dynamics and environmental influences in perovskite nanomaterials but also establishes AI-TA as a transformative tool for real-time observation of photochemical dynamics.

cond-mat.mes-hall↗

arXiv2023

Multi-ensemble metrology by programming local rotations with atom movements

Current optical atomic clocks do not utilize their resources optimally. In particular, an exponential gain in sensitivity could be achieved if multiple atomic ensembles were to be controlled or read-out individually, even without entanglement. However, controlling optical transitions locally remains an outstanding challenge for neutral atom based clocks and quantum computing platforms. Here we show arbitrary, single-site addressing for an optical transition via sub-wavelength controlled moves of tweezer-trapped atoms, which we perform with $99.84(5)\%$ fidelity and with $0.1(2)\%$ crosstalk to non-addressed atoms. The scheme is highly robust as it relies only on relative position changes of tweezers and requires no additional addressing beams. Using this technique, we implement single-shot, dual-quadrature readout of Ramsey interferometry using two atomic ensembles simultaneously, and show an enhancement of the usable interrogation time at a given phase-slip error probability. Finally, we program a sequence which performs local dynamical decoupling during Ramsey evolution to evolve three ensembles with variable phase sensitivities, a key ingredient of optimal clock interrogation. Our results demonstrate the potential of fully programmable quantum optical clocks even without entanglement and could be combined with metrologically useful entangled states in the future.

quant-ph↗

arXiv2022

Continuous collective strong coupling between atoms and a high finesse optical cavity

We demonstrate continuous loading of strontium atoms into a high finesse ring cavity and observe continuous strong collective coupling in the form of a vacuum Rabi splitting between the atoms and the cavity on the 7.5 kHz transition $^1{\rm S}_0$ to $^3{\rm P}_1$. The atoms are loaded into the cavity from a 3D narrow linewidth molasses, thus avoiding large magnetic field gradients and associated broadening of transition frequencies. The ring cavity allows us to realize a deterministic conveyor belt to transport atoms away from the loading region where the laser cooling beams lead to broadening of the strontium clock transition. We trap up to $10^6$ atoms in an intracavity 813 nm lattice in the Lamb-Dicke regime, and transport the atoms along the cavity axis. This work opens the path to the creation of a continuous wave superradiant laser with millihertz linewidth enabling searches for new physics and the use of high-precision optical frequency references outside of low vibration laboratory environments.

physics.atom-ph↗

arXiv2022

Underdamped harmonic oscillator driven by a train of short pulses: Analytical analysis

A theoretical model of an underdamped harmonic oscillator (UHO) driven by periodic short pulses may find plenty of applications in classical, semiclassical, and quantum physics. We present here two different forms of analytical solutions: {\it time-periodic solutions} and {\it harmonic solutions} for one-dimensional classical UHO driven by three different trains of short pulses. They are a Dirac comb, a train of square pulses, and a train of Gaussian pulses with the same pulse-to-pulse time interval $T$ and pulse width $2τ$. Two solutions for square and Gaussian pulses approach to that of the Dirac comb when the pulse width $2τ\rightarrow 0$ as expected. In particular, the harmonic solutions for Dirac comb and Gaussian pulses could be expressed approximately with harmonic terms of the repetition frequency $ω_{\rm R} = 2π/T$ up to the second order. The presented analytical solutions would provide a practical way to determine experimentally the system parameters such as the underdamped oscillation frequency $ω= \sqrt{ω_0^2-γ^2}$, the natural frequency $ω_0$, and the damping rate $γ$, by nonlinear curve fitting procedures for different driving force parameters of $T$ and $2τ$.

quant-ph↗

arXiv2021

Quantitative Complementarity of Wave-Particle Duality

To test the principle of complementarity and wave-particle duality quantitatively, we need a quantum composite system that can be controlled by experimental parameters. Here, we demonstrate that a double-path interferometer consisting of two parametric downconversion crystals seeded by coherent idler fields, where the generated coherent signal photons are used for quantum interference and the conjugate idler fields are used for which-path detectors with controllable fidelity, is useful for elucidating the quantitative complementarity. We show that the source purity $μ_s$ is tightly bounded by the entanglement measure $E$ by the relation $μ_s=\sqrt{1-E^2 }$ and the visibility $V$ and detector fidelity $F$ determine the coherence of the quantons, i.e., $C = V|F|$. The quantitative complementarity of the double-path interferometer we developed recently is explained in terms of the quanton-detector entanglement or quanton source purity that are expressed as functions of injected seed photon numbers. We further suggest that the experimental scheme utilizing two stimulated parametric downconversion processes is an ideal tool for investigating and understanding wave-particle duality and complementarity quantitatively.

quant-ph↗

arXiv2020

Two-dimensional electronic spectroscopy of bacteriochlorophyll a with synchronized dual mode-locked lasers

How atoms and electrons in a molecule move during a chemical reaction and how rapidly energy is transferred to or from the surroundings can be studied with flashes of laser light. However, despite prolonged efforts to develop various coherent spectroscopic techniques, the lack of an all-encompassing method capable of both femtosecond time resolution and nanosecond relaxation measurement has hampered various applications of studying correlated electron dynamics and vibrational coherences in functional materials and biological systems. Here, we demonstrate that two broadband (>300 nm) synchronized mode-locked lasers enable two-dimensional electronic spectroscopy (2DES) study of chromophores such as bacteriochlorophyll a in condensed phases to measure both high-resolution coherent vibrational spectrum and nanosecond electronic relaxation. We thus anticipate that the dual mode-locked laser-based 2DES developed and demonstrated here would be of use for unveiling the correlation between the quantum coherence and exciton dynamics in light-harvesting protein complexes and semiconducting materials.

physics.chem-ph↗

arXiv2020

Broadband infrared spectroscopy of condensed phases with two intra-pulse difference-frequency-generation frequency combs

Mid-infrared (mid-IR) spectroscopy provides a way to study structures and dynamics of complicated molecules in condensed phases. Therefore, developing compact and broadband mid-IR spectrometer has been a long-standing challenge. Here, we show that a highly coherent and broadband mid-IR frequency comb can be generated by using an intra-pulse difference-frequency-generation with a train of pulses from a few-cycle Ti:Sapphire oscillator. By tightly focusing the oscillator output beam into a single-pass fan-out-type periodically-poled lithium niobate crystal and tilting the orientation of the crystal with respect to incident beam, it is shown that mid-IR frequency comb with more than an octave spectral bandwidth from 1550 cm-1 (46 THz) to 3650 cm-1 (110 THz) and vanishing carrier-envelop offset phase can be generated. Then, using two coherent mid-IR frequency combs, we demonstrate that ultrabroad mid-IR dual frequency comb spectroscopy of both aromatic compounds and amino acids in solutions is experimentally feasible. We thus anticipate that our mid-IR frequency combs could be used to further develop ultrafast and broadband IR spectroscopy of chemically reactive and biological molecules in condensed phases.

physics.optics↗

arXiv2019

An atomic array optical clock with single-atom readout

Currently, the most accurate and stable clocks use optical interrogation of either a single ion or an ensemble of neutral atoms confined in an optical lattice. Here, we demonstrate a new optical clock system based on an array of individually trapped neutral atoms with single-atom readout, merging many of the benefits of ion and lattice clocks as well as creating a bridge to recently developed techniques in quantum simulation and computing with neutral atoms. We evaluate single-site resolved frequency shifts and short-term stability via self-comparison. Atom-by-atom feedback control enables direct experimental estimation of laser noise contributions. Results agree well with an ab initio Monte Carlo simulation that incorporates finite temperature, projective read-out, laser noise, and feedback dynamics. Our approach, based on a tweezer array, also suppresses interaction shifts while retaining a short dead time, all in a comparatively simple experimental setup suited for transportable operation. These results establish the foundations for a third optical clock platform and provide a novel starting point for entanglement-enhanced metrology, quantum clock networks, and applications in quantum computing and communication with individual neutral atoms that require optical clock state control.

physics.atom-ph↗

arXiv2019

Theory of three-pulse photon echo spectroscopy with dual frequency combs

A theoretical analysis is carried out for the recently developed three-pulse photon echo spectroscopy employing dual frequency combs (DFC) as the light sources. In this method, the molecular sample interacts with three pulse trains derived from the DFC and the generated third-order signal is displayed as a two-dimensional (2D) spectrum that depends on the waiting time introduced by employing asynchronous optical sampling method. Through the analysis of the heterodyne-detected signal interferogram using a local oscillator derived from one of the optical frequency combs, we show that the 2D spectrum closely matches the spectrum expected from a conventional approach with four pulses derived from a single femtosecond laser pulse and the waiting time between the second and third field-matter interactions is given by the down-converted detection time of the interferogram. The theoretical result is applied to a two-level model system with solvation effect described by solvatochromic spectral density. The model 2D spectrum reproduces spectral features such as the loss of frequency correlation, dephasing, and spectral shift as a function of the population time. We anticipate that the present theory will be the general framework for quantitative descriptions of DFC-based nonlinear optical spectroscopy.

physics.chem-ph↗

arXiv2019

Enhancing entanglement detection of quantum optical frequency combs via stimulated emission

We investigate the performance of a certain nonclassicality identifier, expressed via integrated second-order intensity moments of optical fields, in revealing bipartite entanglement of quantum-optical frequency combs (QOFCs), which are generated in both spontaneous and stimulated parametric down-conversion processes. We show that, by utilizing that nonclassicality identifier, one can well identify the entanglement of the QOFC directly from the experimentally measured intensity moments without invoking any state reconstruction techniques or homodyne detection. Moreover, we demonstrate that the stimulated generation of the QOFC improves the entanglement detection of these fields with the nonclassicality identifier. Additionally, we show that the nonclassicality identifier can be expressed in a factorized form of detectors quantum efficiencies and the number of modes, if the QOFC consists of many copies of the same two-mode twin beam. As an example, we apply the nonclassicality identifier to two specific types of QOFC, where: (i) the QOFC consists of many independent two-mode twin beams with non-overlapped spatial frequency modes, and (ii) the QOFC contains entangled spatial frequency modes which are completely overlapped, i.e., each mode is entangled with all the remaining modes in the system. We show that, in both cases, the nonclassicality identifier can reveal bipartite entanglement of the QOFC including noise, and that it becomes even more sensitive for the stimulated processes.

quant-ph↗

arXiv2013

Absolute frequency measurement of 1S0 (F = 1/2) - 3P0 (F = 1/2) transition of 171Yb atoms in a one-dimensional optical lattice at KRISS

We measured the absolute frequency of the optical clock transition 1S0 (F = 1/2) - 3P0 (F = 1/2) of 171Yb atoms confined in a one-dimensional optical lattice and it was determined to be 518 295 836 590 863.5(8.1) Hz. The frequency was measured against Terrestrial Time (TT; the SI second on the geoid) by using an optical frequency comb of which the frequency was phase-locked to an H-maser as a flywheel oscillator traceable to TT. The magic wavelength was also measured as 394 798.48(79) GHz. The results are in good agreement with two previous measurements of other institutes within the specified uncertainty of this work.

physics.atom-ph↗

arXiv2004

Laser induced birefringence in a wavelength-mismatched cascade system of inhomogeneously broadened Yb atoms

We report the observation of laser induced birefringence (LIB) in a wavelength-mismatched cascade system (J=0 \leftrightarrow J=1 \leftrightarrow J=0 transitions) of inhomogeneously broadened ytterbium atoms with strong pump and probe fields. We investigate the transmission spectrum of two circular polarization (σ_p^+ and σ_p^-) components of strong probe field at fixed frequency, depending on the detuning of circularly polarized (σ_c^-) coupling field from two-photon resonance. We find that σ_p^+ (σ_p^-) polarized component exhibits a narrow electromagnetically induced absorption (transparency) spectrum. Numerical solutions of density matrix equations show qualitative agreement with experimental results. A Doppler-free dispersive LIB signal is obtained by detecting the Stokes parameter of the probe field, enabling us to stabilize the frequency of coupling laser without frequency modulation.

physics.atom-ph↗

arXiv2003

Efficient magneto-optical trapping of Yb atoms with a violet laser diode

We report the first efficient trapping of rare-earth Yb atoms with a high-power violet laser diode (LD). An injection-locked violet LD with a 25 mW frequency-stabilized output was used for the magneto-optical trapping (MOT) of fermionic as well as bosonic Yb isotopes. A typical number of $4\times 10^6$ atoms for $^{174}$Yb with a trap density of $\sim 1\times10^8/$cm$^3$ was obtained. A 10 mW violet external-cavity LD (ECLD) was used for the one-dimensional (1D) slowing of an effusive Yb atomic beam without a Zeeman slower resulting in a 35-fold increase in the number of trapped atoms. The overall characteristics of our compact violet MOT, e.g., the loss time of 1 s, the loading time of 400 ms, and the cloud temperature of 0.7 mK, are comparable to those in previously reported violet Yb MOTs, yet with a greatly reduced cost and complexity of the experiment.

physics.atom-ph↗