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Taichi Terashima

Publications and source records attributed to Taichi Terashima.

At least 19 recordsLinked to original sources

Altermagnetic spin-split Fermi surfaces in CrSb revealed by quantum oscillation measurements

We report a comprehensive quantum oscillation study of the prototypical altermagnet CrSb, combining high-field magnetotransport and torque measurements with DFT + $U$ calculations including spin-orbit coupling. Multiple quantum oscillation frequencies were observed and tracked over wide angular ranges. The measured frequency branches are consistently explained by the spin-split Fermi surfaces arising from the altermagnetic electronic structure. Our determined Fermi surface reveals that bands 1 and 2 form closed pockets centered at the A point, rather than the tubular $c$-axis-open sheets or $\Gamma$-centered closed pockets proposed in previous studies. Our findings establish the Fermi-surface topology of CrSb and provide a firm basis for exploring emergent phenomena in altermagnetic materials.

cond-mat.mtrl-sci

Fermi-surface-sheet dependent electron-phonon coupling in a borocarbide superconductor YNi$_2$B$_2$C

We performed de Haas-van Alphen (dHvA) oscillation measurements and band-structure calculations for YNi$_2$B$_2$C. Our improved band structure successfully explained the origins of the large dHvA frequencies $\beta$ and $\zeta$, which were inexplicable in previous works. By comparing experimental effective masses with band masses, we determined the electron-phonon coupling for each orbit. The results showed a clear Fermi-surface-sheet dependence of the electron-phonon coupling strength, especially highlighting that the coupling for the band-28 sheet is very weak, almost absent for the orbit with $B \parallel c$. This finding is consistent with previous observations of dHvA oscillations from this orbit in the mixed state down to very low fields. Amidst growing interest in high-temperature superconductivity driven by electron-phonon coupling in hydrides under high pressure, this study provides foundational data pivotal to precisely understanding electron-phonon coupling.

cond-mat.supr-con

In-plane and interlayer magnetoresistance in FeSe

We report measurements of the in-plane and interlayer magnetoresistances of FeSe. The in-plane magnetoresistance $\Delta \rho_{ab}/\rho_{ab}(0)$ for $B \parallel c$ is positive below $T_s$ and increases with decreasing temperature, exceeding 2.5 at $T$ = 10 K and $B$ = 14 T. The field-direction dependence indicates that the in-plane magnetoresistance is basically determined by the $c$-axis component of the magnetic field. The interlayer magnetoresistance $\Delta \rho_{c}/\rho_{c}(0)$ is negative below $T_s$ but turns positive below $\sim$18 K, which is probably due to the contamination by the large in-plane magnetoresistance. The field-direction dependence of the interlayer magnetoresistance can approximately be described by a standard formula for quasi-two-dimensional electron systems except near $B \parallel ab$. The experimental magnetoresistance near $B \parallel ab$ is larger than the formula, which can be attributed to the so-called interlayer coherence peak. The large width of the peak indicates the correspondingly large interlayer transfer energy.

cond-mat.supr-con

Multipolar Phase Transition in the 4$f^2$ fcc lattice compound PrCdNi$_{4}$

Transport and magnetic properties of a 4$f^{2}$ fcc lattice compound, PrCdNi$_4$, were studied. The magnetic susceptibility, $\chi(T)$, follows the Curie--Weiss law from 300 K to 20 K, as expected for a free Pr$^{3+}$ ion. As the temperature decreases below 5 K, $\chi(T)$ approaches a constant, indicating van-Vleck paramagnetic behavior. The specific heat, $C(T)$, displays a broad shoulder at around 4 K, which can be reproduced by a doublet triplet two-level model with an energy gap of 12 K. These results suggest a non-magnetic $\Gamma_3$ doublet ground state of the Pr$^{3+}$ ion in the cubic crystalline electric field. $C(T)$ exhibits a peak at $T_{\rm O}$ = 1.0 K and this peak remains robust against magnetic fields up to 5 T. In powder neutron diffraction measurements, no magnetic reflection was observed at 0.32 K $<$ $T_{\rm O}$. Two anomalies at $B$ = 2.1 and 5.3 T in magnetoresistance $\rho(B)$ at 0.05 K likely originate from switching in the order parameter. These results suggest that the phase transition at $T_{\rm O}$ is ascribed to an antiferro-type order of the electric quadrupole or magnetic octupole of the $\Gamma_3$ doublet in the 4$f^2$ fcc lattice.

cond-mat.str-el

Topological delocalization against Anderson localization observed in Bi-doped PbSb2Te4 disordered topological insulator

We experimentally investigate the tendency of localization in the bulk and the topological surface states in topological insulators Pb(Bi1-xSbx)2Te4 (x=0.793-0.818) through detailed transport measurements. The bulk electronic states in the range 0.793<=x<0.818 are situated on the insulator side of the Anderson transition, as indicated by k_Fl values (where k_F is the Fermi wavenumber and l is the mean free path) falling below the Ioffe-Regel criterion (i.e., k_F l<1). In contrast, the topological surface states retain high mobility and even exhibit quantum oscillations, demonstrating their resilient nature against strong disorder. These findings highlight the delocalized nature of the topological surface states despite Anderson localization of the bulk electronic states.

cond-mat.mtrl-sci

Apparent nonreciprocal transport in FeSe bulk crystals

We performed low-frequency ac first- and second-harmonic resistance measurements and dc $I-V$ measurements on bulk FeSe crystals in a temperature range between 1.8 and 150 K and in magnetic field up to 14 T. We observed considerable second-harmonic resistance, indicative of nonreciprocal charge transport, in some samples. By examining correlation between contact resistances and second-harmonic signals, we concluded that the second-harmonic resistance was not due to the genuine nonreciprocal transport effect but was caused by joule heating at a current contact through the thermoelectric effect. Our conclusion is consistent with a recent preprint (Nagata \textit{et al.}, arXiv:2409.01715), in which the authors reported a zero-field superconducting diode effect in devices fabricated with FeSe flakes and attributed it to the thermoelectric effect.

cond-mat.supr-con

Transport evidence for twin-boundary pinning of superconducting vortices in FeSe

We provide bulk transport evidence for twin-boundary pinning of vortices in FeSe. We measure interlayer resistance in FeSe in magnetic fields and find that, as the field is rotated in the $ab$ plane, the flux-flow resistivity is suppressed when the field direction is parallel to twinning planes. The width of the associated dip in the resistance vs in-plane field direction curve varies as $T^{1/2}B^{-3/4}$, consistent with the creation of kinked vortices near the parallel field geometry.

cond-mat.supr-con

Anomalous Hall effect with plateaus observed in a magnetic Weyl semimetal NdAlGe at low temperatures

In the $R$Al(Si,Ge) ($R$: lanthanides) family, both spatial inversion and time-reversal symmetries are broken. This may offer opportunities to study Weyl-fermion physics in nontrivial spin structures emerging from a noncentrosymmetric crystal structure. In this study, we investigated the anomalous Hall effect (AHE) in NdAlGe via magnetotransport, magnetization, and magnetic torque measurements down to 40 mK (0.4 K for magnetization). The single crystals grown by a laser-heated floating-zone method exhibit a single magnetic phase transition at $T_{\rm M}$ = 13.5 K, where the $T_{\rm M}$ is the transition temperature. With the magnetic field parallel to the easy $\lbrack$001$\rbrack$ axis, the AHE gradually evolves as the temperature decreases below $T_{\rm M}$. The anomalous Hall conductivity (AHC) reaches $\sim$320 $Ω^{-1}$cm$^{-1}$ at 40 mK in the magnetically saturated state. Except in low-temperature low-field plateau phases, the AHC and magnetization are proportional, and their ratio agrees with the ratios for conventional ferromagnets, suggesting that the intrinsic AHE occurs by the Karplus-Luttinger mechanism. Below $\sim$0.6 K, the curves of Hall resistivity against the field exhibit plateaus at low fields below $\sim$0.5 T, correlating with the plateaus in the magnetization curve. For the first plateau, the magnetization is one order of magnitude smaller than the magnetically saturated state, whereas the AHE is more than half that in the saturated state. This finding under well below $T_{\rm M}$ suggests that the AHE at the first plateau is not governed by the magnetization and may be interpreted based on a multipole or spin chirality.

cond-mat.str-el

Anomalous upper critical field in the quasicrystal superconductor Ta$_{1.6}$Te

Superconductivity in quasicrystals poses a new challenge in condensed matter physics. We measured the resistance and ac magnetic susceptibility of a Ta$_{1.6}$Te dodecagonal quasicrystal, which is superconducting below $T_c \sim$ 1 K. We show that the upper critical field increases linearly with a large slope of $-$4.4 T/K with decreasing temperature down to 0.04 K, with no tendency to level off. The extrapolated zero-temperature critical field exceeds the Pauli limit by a factor of 2.3. We also observed flux-flow resistance with thermally activated behavior and an irreversibility field that is distinct from the upper critical field. We discuss these peculiarities in terms of the nonuniform superconducting gap and spin--orbit interaction in quasicrystal structures.

cond-mat.supr-con

Experimental verification of band convergence in Sr and Na codoped PbTe

Scanning tunneling microscopy and transport measurements have been performed to investigate the electronic structure and its temperature dependence in heavily Sr and Na codoped PbTe, which is recognized as one of the most promising thermoelectric materials. Our main findings are as follows: (i) Below T=4.5 K, all carriers are distributed in the first valence band at the L point (L band), which forms tube-shaped Fermi surfaces with concave curvature. With Sr and Na doping, the dispersion of the L band changes, and the band gap increases from 200 meV to 300 meV. (ii) At T=4.5 K, the Fermi energy is located ~100 meV below the edge of the L band for the Sr/Na codoped PbTe. The second valence band at the Sigma point (Sigma band) is lower than the L band by 150 meV, which is significantly smaller than that of pristine PbTe (200 meV). The decrease in the band offset, leading to band convergence, provides a desirable condition for thermoelectric materials.(iii) With increasing temperature, the carrier distribution to the Sigma band starts at T=100 K and we estimate that about 50 percent of the total carriers are redistributed in the Sigma band at T=300 K.Our work demonstrates that scanning tunneling microscopy and angular dependent magnetoresistance measurements are particularly powerful tools to determine the electronic structure and carrier distribution. We believe that they will provide a bird's eye view of the doping strategy towards realizing high-efficiency thermoelectric materials.

cond-mat.mtrl-sci

Fermi surface and light quasi particles in hourglass nodal chain metal \b{eta}-ReO2

Quantum oscillations in magnetic torque and electrical resistivity were measured to investigate the electronic structure of \b{eta}-ReO2, a candidate hourglass nodal chain metal (Dirac loop chain metal). All the de Haas-van Alphen oscillation branches measured at 30 mK in magnetic fields of up to 17.5 T were consistent with first-principles calculations predicting four Fermi surfaces (FSs). The small-electron FS of the four FSs exhibited a very small cyclotron mass, 0.059 times that of the free electrons, which is likely to be related to the linear dispersion of the energy band. The consistency between the quantum oscillation results and band calculations indicates the presence of the hourglass nodal chain predicted for \b{eta}-ReO2 in the vicinity of the Fermi energy.

cond-mat.str-el

CeFe$_2$Al$_{10}$: a Correlated Metal with a Fermi Surface Exhibiting Nonmetallic Conduction

Metals can be defined as materials with a Fermi surface or as materials exhibiting metallic conduction (i.e., $\mathrm{d} ρ/ \mathrm{d}T > 0$). Usually, these definitions both hold at low temperatures, such as liquid-helium temperatures, as the Fermi energy is sufficiently larger than the thermal energy. However, they may not both hold in correlated electron systems where the Fermi energy is reduced by renormalization. In this paper, we demonstrate that although the resistivity of CeFe$_2$Al$_{10}$ increases with decreasing temperature below $\sim20$ K, CeFe$_2$Al$_{10}$ is a metal with a Fermi surface. This assertion is based on the observation of Shubnikov--de Haas oscillations and a Hall resistivity that changes sign with the magnetic field, which requires the coexistence of electron and hole carriers. Our analysis of Shubnikov--de Haas and magnetotransport data indicates that the Fermi energies are as small as $\sim$30 K and that, despite the increasing carrier mobility with decreasing temperature as in conventional metals, the loss of thermally excited carriers leads to nonmetallic conduction ($\mathrm{d} ρ/ \mathrm{d}T < 0$) below $\sim20$ K. Furthermore, we investigate how this anomalous metal transforms to a more conventional metal with metallic conduction by the application of high pressure and a high magnetic field. This study illustrates the subtle distinction between semimetals and semiconductors in correlated electron systems. This distinction is relevant to investigations of correlated topological insulators and semimetals.

cond-mat.str-el

In-plane electronic anisotropy revealed by interlayer resistivity measurements on the iron-based superconductor parent compound CaFeAsF

Both cuprates and iron-based superconductors demonstrate nematicity, defined as the spontaneous breaking of rotational symmetry in electron systems. The nematic state can play a role in the high-transition-temperature superconductivity of these compounds. However, the microscopic mechanism responsible for the transport anisotropy in iron-based compounds remains debatable. Here, we investigate the electronic anisotropy of CaFeAsF by measuring its interlayer resistivity under magnetic fields with varying field directions. Counterintuitively, the interlayer resistivity was larger in the longitudinal configuration ($B \parallel I \parallel c$) than in the transverse one ($B \perp I \parallel c$). The interlayer resistivity exhibited a so-called coherence peak under in-plane fields and was highly anisotropic with respect to the in-plane field direction. At $T$ = 4 K and $B$ = 14 T, the magnetoresistance $Δρ/ρ_0$ was seven times larger in the $B \parallel b_o$ than in the $B \parallel a_o$ configuration. Our theoretical calculations of the conductivity based on the first-principles electronic band structure qualitatively reproduced the above observations but underestimated the magnitudes of the observed features. The proposed methodology can be a powerful tool for probing the nematic electronic state in various materials.

cond-mat.supr-con

Anomalous High-Field Magnetotransport in CaFeAsF due to the Quantum Hall Effect

CaFeAsF is an iron-based superconductor parent compound whose Fermi surface is quasi-two dimensional, composed of Dirac-electron and Schrödinger-hole cylinders elongated along the $c$ axis. We measured the longitudinal and Hall resistivities in CaFeAsF with the electrical current in the $ab$ plane in magnetic fields up to 45 T applied along the $c$ axis and obtained the corresponding conductivities via tensor inversion. We found that both the longitudinal and Hall conductivities approached zero above $\sim$40 T as the temperature was lowered to 0.4 K. Our analysis indicates that the Landau-level filling factor is $ν$ = 2 for both electrons and holes at these high field strengths, resulting in a total filling factor $ν$ = $ν_{hole} - ν_{electron}$ = 0. We therefore argue that the $ν$ = 0 quantum Hall state emerges under these conditions.

cond-mat.supr-con

Topological frequency shift of quantum oscillation in CaFeAsF

Guo, Alexandradinata, \textit{et al.} have recently proposed that quantum-oscillation frequencies from Dirac/Weyl fermions exhibit a negative shift proportional to $T^2$ because of the energy dependence of the effective mass peculiar to a linear band-dispersion. We have measured Shubnikov--de Haas oscillation in CaFeAsF up to $T$ = 9 K. The frequency of the $α$ Dirac electron exhibits a negative shift with increasing $T$, while that of the $β$ Schrödinger hole does not. For $T \geqslant 5$ K where $β$ is negligible, the $α$-frequency shift is proportional to $T^2$ and its rate agrees with the theoretical prediction within experimental accuracy. At lower temperatures, the shifts of $α$ and $β$ deviate from theoretical expectations, which we ascribe to the inaccuracy in the frequency determination due to unfavorable interference between frequencies. Our results confirm that the topological frequency shift can be utilized to identify Dirac/Weyl fermions when quantum-oscillation frequencies can be determined accurately.

cond-mat.str-el

Antiperovskite superconductor LaPd$_{3}$P with noncentrosymmetric cubic structure

Antiperovskites are a promising candidate structure for the exploration of new materials. We discovered an antiperovskite phosphide, LaPd$_{3}$P, following our recent synthesis of $A$Pd$_{3}$P ($A$ = Ca, Sr, Ba). While $A$Pd$_{3}$P and (Ca,Sr)Pd$_{3}$P were found to be tetragonal or orthorhombic systems, LaPd$_{3}$P is a new prototype cubic system ($a$ = 9.0317(1) A) with a noncentrosymmetric space group ($I-43m$). LaPd$_{3}$P exhibited superconductivity with a transition temperature ($T_\mathrm{c}$) of 0.28 K. The upper critical field, Debye temperature, and Sommerfeld constant ($γ$) were determined as 0.305(8) kOe, 267(1) K, 6.06(4) mJ mol-1 K-2 f.u.-1, respectively. We performed first-principles electronic band structure calculations for LaPd$_{3}$P and compared the theoretical and experimental results. The calculated Sommerfeld constant (2.24 mJ mol-1 K-2 f.u.-1) was much smaller than the experimental value of $γ$ because the Fermi energy ($E_\mathrm{F}$) was located slightly below the density of states (DOS) pseudogap. This difference was explained by the increase in the DOS at $E_\mathrm{F}$ due to the approximately 5 at.% La deficiency (hole doping) in the sample. The observed Tc value was much lower than that estimated using the Bardeen-Cooper-Schrieffer equation. To explain the discrepancy, we examined the possibility of an unconventional superconductivity in LaPd$_{3}$P arising from the lack of space inversion symmetry.

cond-mat.supr-con

Ferromagnetism out of charge fluctuation of strongly correlated electrons in $κ$-(BEDT-TTF)$_2$Hg(SCN)$_2$Br

We perform magnetic susceptibility and magnetic torque measurements on the organic $κ$-(BEDT-TTF)$_2$Hg(SCN)$_2$Br, which is recently suggested to host an exotic quantum dipole-liquid in its low-temperature insulating phase. Below the metal-insulator transition temperature, the magnetic susceptibility follows a Curie-Weiss law with a positive Curie-Weiss temperature, and a particular $M\propto \sqrt{H}$ curve is observed. The emergent ferromagnetically interacting spins amount to about 1/6 of the full spin moment of localized charges. Taking account of the possible inhomogeneous quasi-charge-order that forms a dipole-liquid, we construct a model of antiferromagnetically interacting spin chains in two adjacent charge-ordered domains, which are coupled via fluctuating charges on a Mott-dimer at the boundary. We find that the charge fluctuations can draw a weak ferromagnetic moment out of the spin singlet domains.

cond-mat.str-el

Extraordinary $π$-Electron Superconductivity Emerging from a Quantum Spin Liquid

Quantum spin liquids (QSLs), in which spins are highly entangled, have been considered a groundwork for generating exotic superconductivity.Despite numerous efforts, superconductivity emerging from QSLs has been unrealized in actual materials due to the difficulties in stabilizing QSL states with metallic conductivity.Recently, an organic compound, $κ$-(BEDT-TTF)$_4$Hg$_{2.89}$Br$_8$, with a nearly regular triangular lattice of molecular dimers was recognized as a candidate for doped QSLs. In this study, we report an unusual superconducting phase of $κ$-(BEDT-TTF)$_4$Hg$_{2.89}$Br$_8$: unexpectedly large ratios of the upper critical field to the critical temperature $H_{\rm c2}$/$T_{\rm c}$ in fields not only parallel but also perpendicular to the two-dimensional conducting layers and a very wide region of fluctuating superconductivity above $T_{\rm c}$.Our results reveal that these peculiarities arise from strong electron correlations and possible quantum criticality unique to the doped QSL state, leading to a heavy mass of itinerant carriers and a large superconducting energy gap.

cond-mat.supr-con