arXiv subjects

Taka-hisa Arima

Publications and source records attributed to Taka-hisa Arima.

At least 55 records · Page 3Linked to original sources

arXiv2025

Perfectly harmonic spin cycloid and multi-$Q$ textures in the Weyl semimetal GdAlSi

A fundamental question concerns how topological electronic states are influenced by many-body correlations, and magnetic Weyl semimetals represent an important material platform to address this problem. However, the magnetic structures realized in these materials are limited, and in particular, no clear example of an undistorted helimagnetic state has been definitively identified. Here, we report clear evidence of a harmonic helimagnetic cycloid with an incommensurate magnetic propagation vector in the Weyl semimetal GdAlSi via resonant elastic X-ray scattering, including rigorous polarization analysis. This cycloidal structure is consistent with the Dzyaloshinskii-Moriya (DM) interaction prescribed by the polar crystal structure of GdAlSi. Upon applying a magnetic field, the cycloid undergoes a transition to a novel multi-$Q$ state. This field-induced, noncoplanar texture is consistent with our numerical spin model, which incorporates the DM interaction and, crucially, anisotropic exchange. The perfectly harmonic Weyl helimagnet GdAlSi serves as a prototypical platform to study electronic correlation effects in periodically modulated Weyl semimetals.

cond-mat.str-el↗

arXiv2025

Canted antiferromagnetism in a spin-orbit coupled $S_{\text{eff}} = 3/2$ triangular-lattice magnet DyAuGe

Exploration of nontrivial magnetic states induced by strong spin-orbit interaction is a central topic of frustrated magnetism. Extensive studies are concentrated on rare-earth-based magnets and 4d/5d transition metal compounds, which are mostly described by an effective spin $S_{\text{eff}} = 1/2$ for the Kramers doublet of the lowest crystal-electric-field levels. Variety of magnetic orderings may be greatly enhanced when magnetic dipolar moments intertwined with multipolar degrees of freedom which are described by higher-rank tensors and often require the magnetic ions with $S_{\text{eff}} > 1/2$. Here, our synchrotron x-ray diffraction near the Dy $L_3$ edge has unveiled a canted antiferromagnetic ground state arising from a quasi-quartet ($S_{\text{eff}} = 3/2$) of 4f electrons in a triangular-lattice (TL) rare-earth intermetallics DyAuGe. Magnetic moment and electric-quadrupole moment are closely interlocked and noncollinear magnetic-dipole alignment is induced by antiferroic electric-quadrupole (AFQ) ordering in the TL layers. The correlation between the AFQ and canted magnetic structures is further confirmed by phase transitions in an in-plane magnetic field. These findings offer insights into the emergence of nontrivial magnetic states in frustrated TL systems described beyond the $S_{\text{eff}} = 1/2$.

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arXiv2025

Incommensurate broken helix induced by nonstoichiometry in the axion insulator candidate EuIn$_{2}$As$_{2}$

Zintl phase EuIn$_{2}$As$_{2}$ has garnered growing attention as an axion insulator candidate, triggered by the identification of a commensurate double-${\mathbf Q}$ broken-helix state in previous studies, however, its periodicity and symmetry remain subjects of debate. Here, we perform resonant x-ray scattering experiments on EuIn$_{2}$As$_{2}$, revealing an incommensurate nature of the broken-helix state, where both the wave number and the amplitude of the helical modulation exhibit systematic sample dependence. Furthermore, the application of an in-plane magnetic field brings about a fanlike state that appears to preserve the double-${\mathbf Q}$ nature, which might be attributed to multiple-spin interactions in momentum space. We propose that the itinerant character of EuIn$_{2}$As$_{2}$, most likely induced by Eu deficiency, gives rise to the helical modulation and impedes the realization of a theoretically-predicted axion state with the collinear antiferromagnetic order.

cond-mat.str-el↗

arXiv2024

Magnetic structure of polar magnet GaV$_4$Se$_8$ with Néel-type skyrmion lattice probed by $^{51}$V NMR

We report the magnetization and the $^{51}$V NMR measurements in the polar magnet GaV$_4$Se$_8$ in which a magnetic skyrmion lattice appears in the structural domain with the polar axis parallel to the magnetic field. Although we successfully separate the $^{51}$V NMR signals in the domain from those in the other structural domains, only the high-frequency region of NMR spectrum is observed due to a significant increase of the spin-echo decay rate in the low-frequency region. In $B_{\rm{ext}}\parallel[111]$, we find the NMR signals from the supermagnetized cycloidal state in the parallel domains as well as from the conical state in domains where the polar axis is tilted from the magnetic field. No NMR signal from the skyrmion lattice state is observed, suggesting a significant increase of the decay rate by additional low-energy excitations caused by dynamics of the skyrmions. In $B_{\rm{ext}}\parallel[001]$, where all the structural domains are magnetically equivalent, multiple NMR peaks converge into one peak at the saturation magnetic field. This field dependence is explained by the closing of magnetic cones as approaching the forced-ferromagnetic state.

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arXiv2024

Giant Hall effect in a highly conductive frustrated magnet GdCu$_2$

The Hall effect is one of the most fundamental but elusive phenomena in condensed matter physics due to the rich variety of underlying mechanisms. Here we report an exceptionally large Hall effect in a frustrated magnet GdCu$_2$ with high conductivity. The Hall conductivity at the base temperature is as high as 4 x 10$^4$ $Ω^{-1}$cm$^{-1}$ and shows abrupt sign changes under magnetic fields. Remarkably, the giant Hall effect is rapidly suppressed as the longitudinal conductivity is lowered upon increasing temperature or introducing tiny amount of quenched disorder. Our systematic transport measurements together with neutron scattering measurements and ab initio band calculations indicate that the unusual Hall effect can be understood in terms of spin-splitting induced emergence/disappearance of Fermi pockets as well as skew scattering from spin-chiral cluster fluctuations in a field-polarized state. The present study demonstrates complex interplay among magnetization, spin-dependent electronic structure, and spin fluctuations in producing the giant Hall effect in highly conductive frustrated magnets.

cond-mat.str-el↗

arXiv2024

Reconsidering the nonlinear emergent inductance: time-varying Joule heating and its impact on the AC electrical response

A nonlinearly enhanced electrical reactance, $\Im Z$, under a large AC current has been measured to explore emergent inductors, which constitute a new class of inductors based on the spin-transfer torque effect. A nonlinear $\Im Z$ has been observed in conducting magnets that contain noncollinear spin textures and interpreted as the realization of an inductance due to current-induced spin dynamics. However, curious behavior has concomitantly been observed. For instance, the nonlinear $\Im Z$ always has a cutoff frequency of $10^0$--$10^4$ Hz, which is much lower than the resonance frequency of a ferromagnetic domain wall, $\sim$10$^7$ Hz; furthermore, the temperature and magnetic field variations in $\Im Z$ appear to be considerably correlated with those in the temperature derivative of resistance. This behavior appears to be difficult to understand in terms of the current-induced spin dynamics, and therefore, the earlier interpretation of the nonlinear $\Im Z$ should be further verified. Here, we theoretically and experimentally show that time-varying Joule heating and its impact on the AC electrical response can naturally explain these observations. In the experimental approach, we study the nonlinear AC electrical response of two conducting materials that exhibit no magnetic order, CuIr$_2$S$_4$ and 1$T$'-MoTe$_2$. Under time-varying Joule heating, a nonlinearly enhanced $\Im Z$ with the curious behavior mentioned above is observed in both systems. Our study implies that the nonlinear $\Im Z$ previously observed in noncollinear magnets includes a considerable contribution of the Joule-heating-induced apparent AC impedance.

cond-mat.mtrl-sci↗

arXiv2024

Contrasting magnetothermal conductivity in sibling Co-based honeycomb-lattice antiferromagnets

Honeycomb-lattice antiferromagnets have attracted wide attention for exploration of exotic heat transport and their interplay with magnetic excitations. In this work, we have revealed a contrasting behavior in the magneto-thermal conductivity (MTC) between two Co-based honeycomb-lattice magnets Co4M2O9 (M = Nb, Ta), despite their identical lattice structures and quite similar magnetism. Co4Ta2O9 exhibits enhanced MTC of about 550% at 9 T of an in-plane magnetic field, comparable to other honeycomb-magnets, while MTC for Co4Nb2O9 reaches only ~30%. This marked difference is ascribed to distinct features in the field-induced evolution of magnetic excitations that resonantly scatter phonons. This finding sheds light on implicit impacts of non-magnetic ions on thermal transport, and hints at the potential for broad heat-transport tunability while preserving magnetism and lattice structures.

cond-mat.str-el↗

arXiv2024

Metamagnetism and anomalous magnetotransport properties in rare-earth-based polar semimetals $R$AuGe ($R =$ Dy, Ho, and Gd)

We report the magnetic, magnetoelastic, and magnetotransport properties of single crystals of polar magnets $R$AuGe ($R=$ Dy, Ho, and Gd), grown by Au-Ge self-flux. Magnetization and magnetostriction measurements reveal multi-step metamagnetic transitions for the $c$-axis magnetic field ($H\parallel c$) for DyAuGe and HoAuGe, suggesting magnetic frustration in the triangular lattice of $R$ ions. The magnetic phase diagrams have clarified a close connection between the magnetoelastic property and the emergence of the intermediate metamagentic phase. The magnetic-field dependence of the resistivity and Hall resistivity reveal the semimetallic transport dominated by hole-type carriers, consistent with the behavior in a nonmagnetic analogue YAuGe. We also identify a signature of an anomalous Hall effect (AHE) proportional to the field-induced magnetization in $R=$ Dy, Ho, and Gd. GdAuGe shows magnetic and transport behavior as reported in a previous study using Bi-flux grown single crystals, while the self-flux grown crystal shows larger magnetoresistance ($\sim$ 345\%, at 1.8 K and 9 T) due to higher hole-type carrier mobility ($\sim$ 6400 cm$^2$/Vs). Using the two-band model analysis considering the mobility change during the magnetization process, we extract the anomalous Hall conductivity: $\sim 1200$ S/cm and $\sim 530$ S/cm for $R=$ Dy and Ho, respectively, at 1.8 K with 9 T for $H\parallel c$. The magnitude of conductivity suggests a contribution of intrinsic origin, possibly related to the Berry curvature in the electron bands induced by the time-reversal symmetry breaking and the polar lattice.

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arXiv2024

Spin-lattice-coupled helical magnetic order in breathing pyrochlore magnets, CuAlCr$_{4}$S$_{8}$ and CuGaCr$_{4}$S$_{8}$

We report low-temperature powder X-ray and neutron diffraction studies on breathing pyrochlore magnets Cu$M$Cr$_{4}$S$_{8}$ ($M$ = Al, Ga), which undergo a magnetic transition at $T_{\rm N} \approx$ 21 and 31 K for {$M$ = Al and Ga, respectively. X-ray diffraction reveals that the magnetic transition accompanies a structural transition from cubic $F{\overline 4}3m$ to polar orthorhombic $Imm2$ symmetry for both the compounds, with larger distortion observed for $M$ = Ga at low temperatures. Neutron diffraction reveals incommensurate magnetic modulation ${\mathbf Q} = (q_{\rm IC}, 0.5, 0)$ in the orthorhombic setting, where $q_{\rm IC} \approx$ 0.39 and 0.31 for $M$ = Al and Ga, respectively. Our magnetic-structure analysis suggests cycloid-type magnetic order but not proper-screw type for both the compounds. We find strong correlation between the local spin configuration and Cr-Cr bond lengths, indicating that the spin-lattice coupling as well as the magnetic frustration play an important role in determining the ground state. Cu$M$Cr$_{4}$S$_{8}$ potentially offers a platform to explore magnetoelectric effects arising from the helimagnet driven electric polarity.

cond-mat.mtrl-sci↗

arXiv2024

Cluster rearrangement by chiral charge order in lacunar spinel GaNb$_4$Se$_8$

Transition-metal atoms with d electrons sometimes form clusters in crystals, which significantly affects the physical properties. Such a cluster formation frequently accompanies a change in the crystal system, leading to the presence of domains with different crystal orientations. In particular, the cubic symmetry is rarely retained after the cluster formation. Here, we identify a cubic-to-cubic phase transition in lacunar spinel GaNb$_4$Se$_8$, where the change in the lattice parameter is less than 0.0001%. Each Nb$^{3.25+}$ tetramer with seven 4d electrons is distorted into a Nb$^{3+}$ trimer and a Nb$^{4+}$ monomer induced by charge disproportionation among Nb ions. While the Nb$^{3+}$ trimer with six 4d electrons forms spin-singlets in the sigma-bonding orbitals for three Nb-Nb bonds, a localized S=1/2 spin remains on the Nb$^{4+}$ ion. Furthermore, a local electric dipole moment is induced along the three-fold rotation axis of each distorted tetramer by the cluster rearrangement. The electric dipole moments are regularly arranged to maintain the cubic symmetry, giving rise to chiral order.

cond-mat.str-el↗

arXiv2024

Molecular orbital formation and metastable short-range ordered structure in VO$_2$

The metal-insulator transition (MIT) in vanadium dioxide VO$_2$ due to V-V dimerization has been extensively discussed for decades. While it is widely acknowledged that electron correlations, Peierls instabilities, and molecular orbital formations are crucial for understanding the MIT of VO$_2$, the primary origin of the MIT remains controversial. In this study, we delve into the crystal structure and orbital state of VO$_2$ through synchrotron x-ray diffraction experiments. The molecular orbital formation corresponding to the V-V dimerization is directly observed in the low-temperature insulating monoclinic phase, called the M1 phase, as indicated by the valence electron density distribution. Moreover, diffuse scattering observed in the high-temperature metal phase of rutile structure suggests the presence of short-range correlation of V displacements, which is not directly attributed to the structural fluctuation of the M1 phase. The short-range order in the rutile phase will be the key to understanding the MIT in this system.

cond-mat.str-el↗

arXiv2024

Lattice-commensurate skyrmion texture in a centrosymmetric breathing kagome magnet

Skyrmion lattices (SkL) in centrosymmetric materials typically have a magnetic period on the nanometer-scale, so that the coupling between magnetic superstructures and the underlying crystal lattice cannot be neglected. Here, we reveal the commensurate locking of a SkL to the atomic lattice in Gd$_3$Ru$_4$Al$_{12}$ via high-resolution resonant elastic x-ray scattering (REXS). Weak easy-plane magnetic anisotropy, demonstrated here by a combination of ferromagnetic resonance and REXS, penalizes placing a skyrmion core on a site of the atomic lattice. Under these conditions, a commensurate SkL, locked to the crystal lattice, is stable at finite temperatures -- but gives way to a competing incommensurate ground state upon cooling. We discuss the role of Umklapp-terms in the Hamiltonian for the formation of this lattice-locked state, its magnetic space group, the role of slight discommensurations, or (line) defects in the magnetic texture, and contrast our findings with the case of SkLs in noncentrosymmetric material platforms.

cond-mat.str-el↗

arXiv2024

Non-coplanar helimagnetism in the layered van-der-Waals metal DyTe$_3$

Magnetic materials with highly anisotropic chemical bonding can be exfoliated to realize ultrathin sheets or interfaces with highly controllable optical or spintronics responses, while also promising novel cross-correlation phenomena between electric polarization and the magnetic texture. The vast majority of these van-der-Waals magnets are collinear ferro-, ferri-, or antiferromagnets, with a particular scarcity of lattice-incommensurate helimagnets of defined left- or right-handed rotation sense, or helicity. Here we use polarized neutron scattering to reveal cycloidal, or conical, magnetic structures in DyTe$_3$, with coupled commensurate and incommensurate order parameters, where covalently bonded double-slabs of dysprosium square nets are separated by highly metallic tellurium layers. Based on this ground state and its evolution in a magnetic field as probed by small-angle neutron scattering (SANS), we establish a one-dimensional spin model with off-diagonal on-site terms, spatially modulated by the unconventional charge order in DyTe$_3$. The CDW-driven term couples to antiferromagnetism, or to the net magnetization in applied magnetic field, and creates a complex magnetic phase diagram indicative of competing interactions in an easily cleavable helimagnet. Our work paves the way for twistronics research, where helimagnetic layers can be combined to form complex spin textures on-demand, using the vast family of rare earth chalcogenides and beyond.

cond-mat.mtrl-sci↗

arXiv2024

Electric-field-enhanced second-harmonic domain contrast and nonreciprocity in a van der Waals antiferromagnet

Imaging antiferromagnetic 180° domains with actively controlled visibility is vital for both fundamental science and sophisticated applications. While optical second-harmonic generation (SHG) is a well-known technique for distinguishing such domains in non-centrosymmetric antiferromagnets, a general material-based strategy to control domain contrast remains elusive. Using van der Waals antiferromagnet MnPS$_3$ as a proof of concept, we demonstrate the tuning of nonreciprocity-induced domain contrast in SHG through applying an in-plane electric field that transforms the magnetic point group to its unitary subgroup. The interference among intrinsic electric-dipole, magnetic-dipole, and field-induced electric-dipole transitions, each carrying distinct characters under space-inversion ($\mathcal{P}$) and time-reversal ($\mathcal{T}$) operations, enables large tuning of domain contrast and nonreciprocity in a broad spectral range. This strategy, generically applicable to systems characterized by $\mathcal{PT}$-symmetric magnetic groups with a polar unitary subgroup, offers a path to fast electrical modulation of nonlinear nonreciprocal photonic behaviors using antiferromagnets.

cond-mat.str-el↗

arXiv2023

Real-Space Observation of Ligand Hole State in Cubic Perovskite SrFeO$_3$

An anomalously high valence state sometimes shows up in transition-metal oxide compounds. In such systems, holes tend to occupy mainly the ligand $p$ orbitals, giving rise to interesting physical properties such as superconductivity in cuprates and rich magnetic phases in ferrates. However, no one has ever observed the distribution of ligand holes in real space. Here, we report a successful observation of the spatial distribution of valence electrons in cubic perovskite SrFeO$_3$ by high-energy X-ray diffraction experiments and precise electron density analysis using a core differential Fourier synthesis method. A real-space picture of ligand holes formed by the orbital hybridization of Fe 3$d$ and O 2$p$ is revealed. The anomalous valence state in Fe is attributed to the considerable contribution of the ligand hole, which is related to the metallic nature and the absence of Jahn-Teller distortions in this system.

cond-mat.str-el↗

arXiv2023

Exciton-magnon splitting in van der Waals antiferromagnet MnPS$_3$ unveiled by second-harmonic generation

Ultrafast and coherent generation of magnons is of great significance for high-speed antiferromagnetic spintronics. One possible route is by exciton-magnon pairwise optical excitation. To date, such exciton-magnon transitions have been studied mostly by linear optical means in a limited number of conventional three-dimensional antiferromagnets. Here we investigate this correlated transition in van der Waals antiferromagnet MnPS$_3$ by using resonant second-harmonic generation spectroscopy, a nonlinear optical probe sensitive to the symmetry of electronic and magnetic excitations. Two exciton-magnon peaks are observed, in line with the exciton-induced splitting of magnon density of states predicted by a Koster-Slater type theory, indicating significant exciton-magnon interactions. In addition, a large linear magnetoelectric effect of excitons is observed. These findings provide renewed understandings on the correlation effects in two-dimensional magnets with enhanced quasiparticle scattering cross-sections, and point to potential coherent control among charge, spin and orbital degrees of freedom in two-dimensional magnets by optical means.

cond-mat.str-el↗

arXiv2023

Direct observations of spin fluctuations in spin-hedgehog-anti-hedgehog lattice states in MnSi$_{1-x}$Ge$_x$ ($x=0.6$ and $0.8$) at zero magnetic field

The helimagnetic compounds MnSi$_{1-x}$Ge$_{x}$ show the three-dimensional multiple-$q$ order as referred to as spin-hedgehog-anti-hedgehog (SHAH) lattice. Two representative forms of SHAH are cubic-3$q$ lattice with $q \| \langle100\rangle$ and tetrahedral-4$q$ lattice with $q \| \langle111\rangle$, which show up typically for $x=1.0-~0.8$ and for $x=0.6$, respectively. Here, we have investigated the spin fluctuations in the MnSi$_{1-x}$Ge$_{x}$ polycrystalline samples with $x=0.6$ and $0.8$ by using the time-of-flight (TOF) neutron inelastic scattering and MIEZE-type neutron spin echo techniques to elucidate the microscopic origin of the unconventional Hall effect in the SHAH lattice states. This research is motivated by the observation of a sign change in the unconventional Hall resistivity as a function of temperature [Y. Fujishiro et al., Nat. Comm. $\textbf{10}$, 1059 (2019)]. The present results reveal the correspondences between the temperature ranges where the positive Hall resistivity and spin fluctuations are observed. These results agree well with the theoretical model of the conduction electrons scattered by the fluctuating spin clusters with a non-zero average of sign-biased scalar spin chirality as a mechanism of the positive Hall resistivity [H. Ishizuka and N. Nagaosa, Sci. Adv. $\textbf{4}$, eaap9962 (2018)].

cond-mat.str-el↗

arXiv2023

Magnetoelectrocaloric effect of multiferroic GdFeO3

We report an experimental demonstration of the magnetoelectrocaloric effect (MECE) in multiferroic $\mathrm{GdFeO_3}$. The temperature of the magnetic material changes when an external electric field is suddenly changed. MECE is the largest below the ordering temperature of Gd moments and modifiable by a magnetic field, suggesting that the ferroelectric transition affects MECE. The observed MECE shows a higher energy efficiency than typical magnetocaloric effects and adiabatic nuclear demagnetization. The present findings provide a proof of concept of MECE in multiferroics.

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