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Takahiro Morimoto

Publications and source records attributed to Takahiro Morimoto.

At least 19 recordsLinked to original sources

Reducing the Gate-Induced Drain-Leakage Current of Carbon-Nanotube Transistors by Subliming Dispersants with Back-End-of-Line Compatible Temperature

Carbon nanotube field-effect transistors (CNTFETs) are promising for monolithic 3D integration with silicon CMOS circuits in back-end-of-line (BEOL) processes. Further reduction in off-state leakage is essential for practical applications. In this study, we develop a low-temperature cleaning process for CNT-deposited wafers using a sublimable CNT dispersant. The process is carried out below 250 °C, making it BEOL-compatible, and does not deteriorate CNT morphology or lattice structure, as confirmed by atomic force microscopy and Raman spectroscopy. As a result, gate-induced drain leakage current originating from residual dispersants is reduced by approximately one order of magnitude. In addition, improvements in on-current, subthreshold slope, and threshold voltage variability are observed after the cleaning process. This study demonstrates a material-enabled approach to improve the transfer characteristics of CNTFETs and provides a practical route toward low-power CNT electronics.

cond-mat.mtrl-sci

Spinon shift current in a noncentrosymmetric quantum spin chain

We theoretically study direct current generation in a quantum spin chain induced by spinon excitations by light irradiation. We consider a $S=1/2$ one-dimensional (1D) antiferromagnetic XXZ model with magnetoelectric coupling that describes multiferroics with broken inversion symmetry. We perform the real-time simulation using infinite time-evolving block decimation, and demonstrate the direct current generation under light irradiation. By comparing the second order nonlinear conductivity and the two-spinon excitation spectra of a 1D XXZ model, we confirm that the spinon excitations are the origin for the direct current generation in the quantum spin chain. We find that the bulk photovoltaic effect is driven by electric polarization carried by the spinons through the shift current mechanism, and thus is regarded as ``the spinon shift current.''

cond-mat.str-el

Axion dark matter detection via shift current

We propose a novel method to detect axion dark matter based on a topological phenomenon known as the shift current. We make use of the second-order nonlinearity of the shift current by applying a strong oscillating electric field. This field enhances the axion-induced shift current signal and downconverts its frequency to a more accessible range. The nondissipative nature of the shift current allows us to achieve broadband detection via difference frequency generation. We demonstrate the possibility of probing QCD axions and axion-like particles using the properties of the type-I Weyl semimetal TaAs, targeting an axion mass of $O(10)\,\mathrm{meV}$, corresponding to a photon coupling of $g_{aγγ} \simeq \mathcal{O}(10^{-11})\,\mathrm{GeV}^{-1}$.

hep-ph

Emergent induction in magnetic Weyl semimetals

We theoretically study emergent electromagnetic responses in Weyl semimetals. Focusing on magnetic Weyl semimetals, we develop a general theory of emergent induction driven by magnetic dynamics. We show that magnetoelectric (ME) responses in Weyl semimetals give rise to emergent induction mediated by magnetization dynamics. Using effective two-band models for magnetic Weyl semimetals, we derive a formula for the ME response that includes both intraband and interband contributions. The resulting formula shows that the intraband contribution is proportional to the relaxation time $τ$, whereas the interband contribution is associated with the separation of the Weyl nodes. Applying the general formula to a model of polar Weyl ferromagnets, we demonstrate that the dynamics of the toroidal moment is closely related to the emergent inductive response in polar Weyl ferromagnets, as recently discovered by Suzuki et al. [Y. Suzuki et al. arXiv:2607.12322]. The chemical-potential dependence of the inductance indicates that the emergent electromagnetic response is enhanced in the energy range of the Weyl dispersion, reflecting the topological nature of Weyl semimetals.

cond-mat.mes-hall

Emergent toroidal induction in a polar Weyl ferromagnet

Spin-orbit coupling (SOC) underpins modern spintronics by enabling the electrical generation of spin torques. Its reciprocal counterpart, in which magnetization dynamics produce electromotive forces through a spin-dependent Berry phase, is known as emergent electromagnetic induction (EEMI). However, this effect has previously been observed only in magnetic textures with spatial gradients, such as domain walls, helices, and skyrmions. Here, we demonstrate that even a spatially uniform ferromagnet can host EEMI through a previously unrecognized Berry-phase mechanism inherent to noncentrosymmetric conductors. In the polar Weyl ferromagnet PrAlGe, an applied alternating current generates spin-orbit torques that drive collective magnetization dynamics. The resulting emergent toroidal moment (T = P \times M), where (P) is the crystal's polar axis and (M) is the net magnetization, acts as a gauge potential whose time derivative (dT/dt) induces a Hall voltage. This contribution appears specifically in the out-of-phase component of the AC Hall response and scales linearly with frequency, providing direct evidence for EEMI. First-principles calculations further reveal that this toroidal vector encodes the collective motion of Weyl nodes in momentum space. These findings establish "emergent toroidal induction" as a new manifestation of spin-orbit entanglement, unifying Berry phase, topology, and spin dynamics while opening a pathway toward intrinsic and energy-efficient spin-charge interconversion.

cond-mat.mtrl-sci

Electronic manipulation of polar order in electron crystal

When interaction among atoms or ions is strong enough, they often arrange periodically, forming a crystal. The arrangement patterns of atoms or ions can encode information, a concept that has enabled devices such as ferroelectric memories. It has been found that not only atoms or ions but also electrons in condensed matter can crystallize when Coulomb interaction is strong enough. Typical examples are charge-ordered states in solids, where different valences, or different electron numbers, of an ion spontaneously form a spatial pattern on the lattice. In such electron crystals, information is expected to be encoded into the electron-ordering patterns. Here, we demonstrate electronic manipulation and readout of charge-ordering directions in a paramagnetic semiconductor LuFe$_2$O$_4$. By applying current pulses at room temperature, we observed that the non-reciprocal resistivity of LuFe$_2$O$_4$ is modulated along with a sign reversal, which disappears above the charge-ordering temperature. A numerical calculation incorporating inter-band Berry curvature affected by the charge ordering is consistent with the experimental results. By applying the observed phenomenon, we also demonstrate a non-reciprocal resistance memory operation in the charge-ordered LuFe$_2$O$_4$. This result opens the door to realizing charge-ordering electronics.

cond-mat.mtrl-sci

Quantum-geometric shift of quasiequilibrium: Origin of nonreciprocal current driven by quantum-metric dipole

We study nonlinear DC electric transport of quantum-metric origin by combining adiabatic perturbation theory with the nonequilibrium Green function approach. The adiabatic ansatz provides a basis for directly treating a DC electric field in the velocity gauge, rather than introducing it as the zero-frequency limit of an AC field. The resulting adiabatic-basis Hamiltonian takes the same form as in the length gauge, enabling a systematic comparison across different formulations. Applying this fully quantum formulation, we find a longitudinal nonreciprocal current governed by the quantum-metric dipole. The essential ingredient is a quantum correction to the distribution function that is absent in semiclassical treatments. We trace this correction to the finite spread of an electron wave packet during relaxation under a bias field, thereby identifying shifted quasiequilibrium as the physical origin of quantum-metric nonreciprocal transport.

cond-mat.mes-hall

Nonreciprocal current induced by dissipation in time-reversal symmetric systems

We study nonreciprocal current response in noncentrosymmetric crystals under time-reversal symmetry. We reveal that the nonreciprocal current appears in a dissipative system through interband processes. We derive a formula for the nonreciprocal current using the Green's function technique. The nonreciprocal current of the present mechanism turns out to be of $O(1/τ)$ ($τ$: the lifetime of Bloch electrons) and arises from the shift of the electron wave packet during the interband processes which has a geometric origin. We present a numerical simulation of the nonreciprocal current in the one-dimensional Rice-Mele model and give its order estimation for nonmagnetic polar semiconductors.

cond-mat.mes-hall

Surface-switchable nonreciprocity protected by Fermi arcs in Weyl semimetal TaAs

Weyl semimetals host topologically protected surface states, known as Fermi arcs, which connect bulk Weyl nodes in momentum space. Both bulk Weyl nodes and Fermi arcs are anticipated to be chiral. The chirality of bulk bands has been confirmed through observations of the chiral anomaly and Weyl orbits. In contrast, despite their discovery more than a decade ago, the chiral nature of Fermi arcs has remained unresolved. Here we report Fermi-arc-induced nonlinear transport in the archetypal Weyl semimetal TaAs. Using focused ion beam techniques, we fabricated micro-scale devices that enable simultaneous transport measurements on opposing topological surfaces. While linear transport remains dominated by bulk conduction, nonlinear transport uncovers surface-specific contributions, including an exceptionally large third-order nonreciprocal response that exceeds conventional expectations and highlights the crucial role of the singular arc endpoints. Our findings unambiguously demonstrate the chiral nature of Fermi arcs and establish nonlinear transport as a direct probe of these topological surface states. By revealing a surface-switchable, room-temperature nonlinear response that is topologically protected, this work introduces a new functionality in Weyl semimetals. Given the abundance of natural materials predicted to host topological semimetal states, these results open opportunities for exploring nonlinear transport phenomena and device concepts across a broad class of systems.

cond-mat.mes-hall

Quantum Fisher information in many-photon states from shift current shot noise

Quantum Fisher information (QFI) sets the ultimate precision of optical phase measurements and reveals multiphoton entanglement, but it is not accessible with conventional photodetection. We theoretically predict that a photodetector utilizing the shot noise of the quantum-geometric shift current of exciton polaritons can directly measure the QFI of nonclassical light. By solving the Lindblad equation, we obtain the time-dependent nonlinear photocurrent for an arbitrary initial photon state. It turns out that, regardless of the quantum state of the incident light, the integrated current depends only on the mean photon number. In stark contrast, the shot noise retains the quantum information: its Fano factor is proportional to the photon number variance and therefore encodes the QFI. Numerical calculations confirm these relations for illumination with optical Schrödinger cat and squeezed vacuum states. Quantum correlations in nonclassical light, usually hidden from direct detection, become observable in the form of shift current shot noise

cond-mat.mes-hall

Raman response of collective modes in multicomponent superconductors

We formulate a microscopic theory of the Raman response of superconducting collective modes in multicomponent superconductors. Starting from a general Bogoliubov--de Gennes (BdG) Hamiltonian with a separable pairing interaction, we derive a gauge-invariant expression for the Raman susceptibility, including a long-range Coulomb interaction. The resulting Raman susceptibility is directly computable for an arbitrary BdG Hamiltonian, which contains single- and multiband systems, spin-singlet and triplet order parameters, and time-reversal-symmetric and time-reversal-symmetry-breaking superconducting states. Based on the microscopic coupling between a Raman source field and collective modes, we derive a symmetry selection rule for Raman-active collective modes and show a group-theoretical classification for all crystalline point groups. This classification provides a unified framework based on the ``higher-order Lifshitz-invariant'' to identify Raman-active collective modes such as Leggett mode, Bardasis-Schrieffer (BS) mode, and clapping mode. As an application, we focus on an effective model of the heavy-fermion superconductor UTe$_2$ with a fully gapped multicomponent odd-parity pairing state. We find sharp in-gap Raman resonances below the quasiparticle continuum, which do not correspond to a conventional Leggett mode but arise from the {\it intraband} relative modes between different pairing components.

cond-mat.supr-con

Interaction induced topological magnon in electron-magnon coupled systems

We theoretically study the emergence of topological magnons in electron-magnon coupled systems. The magnon dispersion in a ferromagnet usually possesses an effective time reversal symmetry in the absence of Dzyaloshinskii-Moriya (DM) interaction, preventing the appearance of topological magnons. When a spin system is coupled to itinerant electrons, we find that the magnon band structure of the spin system experiences time-reversal symmetry breaking with the electron-magnon interaction via the exchange coupling, where topological magnons arise without requiring strong DM. Specifically, we consider a heterostructure consisting of a ferromagnetic insulator and a transition metal dichalcogenide (TMD) monolayer and investigate topological gap opening in magnon bands. Our findings reveal that even trivial ferromagnets can host topological magnons via coupling to itinerant electronic systems.

cond-mat.str-el

Microwave Kerr/Faraday Resonance in Two-dimensional Chiral Superconductors

We investigate the polar Kerr and Faraday effects in two-dimensional multiband chiral superconductors. We show that the clapping modes--the relative phase and amplitude oscillations between two chiral components of the superconducting order parameter--lie well within the quasiparticle excitation gap in multiband systems and dominate these magneto-optical responses in the microwave regime. The Kerr and Faraday rotation angles exhibit the resonant enhancement with sign reversals in the microwave regime as a function of the light frequency, reaching peak values on the order of 100 nrad--10 $μ$rad in thin films of candidate chiral superconductors. These resonances are accessible in superconducting atomic layer materials and provide a generic probe of chiral superconductivity in two-dimensional systems.

cond-mat.supr-con

Role of Ward-Takahashi identity in an electron-phonon coupled system -- Revisiting phonon shift current

We study bulk photovoltaic effects in electron-phonon coupled systems. The conservation of current or gauge invariance, manifested as the Ward-Takahashi identity, plays an essential role in the analysis of the Feynman diagrams, and the leading order contribution to the phonon shift current is identified accordingly. The leading order contribution essentially arises from the electric polarization carried by optically excited phonons, where the shift current is generated due to a change of electric polarization in the steady state under the optical excitation of phonons.

cond-mat.str-el

Topological phases of electrons induced by electron-magnon interactions

Topological phases of electrons such as topological insulators and quantum Hall states typically require strong spin-orbit coupling or magnetic fields. In this study, we consider an electron system coupled to a spin system, where electrons interact with magnons, quasiparticles of spin waves. We show that the interaction between electrons and magnons transfers the effect of symmetry breaking in the spin system to the electron system, whereby a non-trivial topological phase can be induced in the electron system that is otherwise topologically trivial. Through this ``topology transfer'' mechanism, we demonstrate the realization of various topological phases, including quantum Hall and quantum spin Hall insulators, in simple ferromagnetic spin systems, without requiring strong spin-orbit coupling or external magnetic field for electron systems.

cond-mat.str-el

Formulation of the orbital magnetic moment in multiorbital tight-binding models: Application to the inverse Faraday effect

We establish a theoretical formulation of the orbital magnetic moment in multiorbital tight-binding models, focusing on the role of the electric dipole. We demonstrate that the total magnetic moment can be decomposed into several contributions in multiorbital tight-binding models generally. In particular, we reveal that the electric dipole moment of Wannier orbitals also contributes to the orbital magnetic moment, which is not included in the conventional expression for the orbital magnetic moment in lattice systems. The derived formulation for the magnetic moment is applied to the inverse Faraday effect (IFE), a phenomenon where circularly-polarized light induces a magnetic moment. To account for all possible contributions, we adopt an $s$-$p$ tight-binding system as a minimal model for studying the IFE. Using an analytical approach based on the Schrieffer-Wolff transformation, we clarify the physical origins of these contributions. Additionally, we quantitatively evaluate each contribution on an equal footing through a numerical approach based on the Floquet formalism. Our results reveal that the orbital magnetic moment exhibits a significantly larger response compared to the spin magnetic moment, with all contributions to the orbital magnetic moment being comparable in magnitude. These findings highlight the essential role of orbital degrees of freedom in the IFE.

cond-mat.mes-hall

Kapitza-Dirac interference of Higgs waves in superconductors

We present a novel framework for controlling Higgs mode and vortex dynamics in superconductors using structured light. We propose a phenomenon analog of the Kapitza-Dirac effect in superconductors, where Higgs waves scatter off light-induced vortex lattices, generating interference patterns akin to matter wave diffraction. We also find that the vortices enable the linear coupling of Higgs mode to the electromagnetic field. This interplay between light-engineered Higgs excitations and emergent vortex textures opens a pathway to probe nonequilibrium superconductivity with unprecedented spatial and temporal resolution. Our results bridge quantum optics and condensed matter physics, offering new examples of quantum printing where one uses structured light to manipulate the collective modes in correlated quantum fluids.

cond-mat.str-el

Quantum Optical Spanner: Twisting Superconductors with Vortex Beam via Higgs Mode

Light carrying orbital angular momentum (OAM)--known as vortex beams--has broadened the scope of understanding and applications of light's angular momentum. Optical tweezers using OAM, often referred to as optical spanners, have significantly expanded the tunability of optical manipulation. A key frontier now lies in understanding how vortex beams interact with quantum states of matter. In this work, we numerically investigate the dynamics of a superconductor under vortex beam illumination and demonstrate the transfer of angular momentum from light to the superconducting collective mode, resulting in mechanical rotation. Our findings open a pathway for optical manipulation in the quantum regime, which we term the quantum optical spanner.

cond-mat.str-el