arXiv subjects

Takahiro Tomita

Publications and source records attributed to Takahiro Tomita.

15 recordsLinked to original sources

arXiv2022

Chiral-anomaly-driven magnetotransport in the correlated Weyl magnet Mn$_3$Sn

The quest for topological states in strongly correlated materials is challenging but essential from fundamental research and application perspectives. The magnetic Weyl semimetal (WSM) state in the chiral antiferromagnet Mn$_3$Sn emerges with strong electronic correlations, offering an intriguing arena for exploring the interplay between Weyl fermions and correlation physics. One prominent characteristic of the WSM state is the chiral anomaly, yet the potential effects of electronic correlations on the chiral anomaly remain unexplored. Here, we report a comprehensive study of the in-plane magnetotransport properties of single-crystal Mn$_{3+x}$Sn$_{1-x}$ with three different Mn doping levels ($x=0.053$, 0.070, and 0.090). The excess Mn leads to glassy ferromagnetic behavior and the Kondo effect, aside from shifting the chemical potential relative to the Weyl nodes. Thus, systematic tuning of the Mn doping level enables us to study the interplay between the spin-fluctuation scatterings, the correlation effect, and the chiral anomaly. We identify negative longitudinal magnetoresistance and planar Hall effect specific to the chiral anomaly for all three doping levels, indicating that the chiral anomaly persists in the presence of strong correlations.

cond-mat.str-el↗

arXiv2022

Structural Phase Transition and Possible Valence Instability of Ce$-4f$ Electron Induced by Pressure in CeCoSi

X-ray powder diffraction and electrical resistivity measurements were performed on the tetragonal compound CeCoSi under pressure to elucidate the phase boundary of the pressure-induced structural transition and the change in the 4$f$ electronic state. The temperature-pressure phase diagram has been determined from the shift of the Bragg peaks and from the anomaly in the resistivity. The critical pressure, $P_{\rm s}$ $\sim$ 4.9 GPa at 300 K, decreases to $P_{\rm s}$ $\sim$ 3.6 GPa at 10 K. The decrease of $P_{\rm s}$ is due not only to the decrease in volume of the unit cell but also to an anisotropic shrinkage by cooling. When crossing the boundary to the high-pressure phase, the resistivity shows a significant drop to exhibit a metallic temperature dependence. The results of this study strongly suggest that the structural phase transition can be ascribed to valence instability of Ce-$4f$ electron.

cond-mat.str-el↗

arXiv2021

Giant effective damping of octupole oscillation in an antiferromagnetic Weyl semimetal

A magnetic Weyl semimetal is a recent focus of extensive research as it may exhibit large and robust transport phenomena associated with topologically protected Weyl points in momentum space. Since a magnetic texture provides a handle for the configuration of the Weyl points and its transport response, understanding of magnetic dynamics should form a basis of future control of a topological magnet. Mn3Sn is an example of an antiferromagnetic Weyl semimetal that exhibits a large response comparable to the one observed in ferromagnets despite a vanishingly small magnetization. The non-collinear spin order in Mn3Sn can be viewed as a ferroic order of cluster magnetic octupole and breaks the time-reversal symmetry, stabilizing Weyl points and the significantly enhanced Berry curvature near the Fermi energy. Here we report our first observation of time-resolved octupole oscillation in Mn3Sn. In particular, we find the giant effective damping of the octupole dynamics, and it is feasible to conduct an ultrafast switching at < 10 ps, a hundred times faster than the case of spin-magnetization in a ferromagnet. Moreover, high domain wall velocity over 10 km/s is theoretically predicted. Our work paves the path towards realizing ultrafast electronic devices using the topological antiferromagnet.

cond-mat.mtrl-sci↗

arXiv2021

Logarithmic Criticality in Transverse Thermoelectric Conductivity of the Ferromagnetic Topological Semimetal CoMnSb

We report the results of our experimental studies on the magnetic, transport and thermoelectric properties of the ferromagnetic metal CoMnSb. Sizable anomalous Hall conductivity $σ_{yx}$ and transverse thermoelectric conductivity $α_{yx}$ are found experimentally and comparable in size to the values estimated from density-functional theory. Our experiment further reveals that CoMnSb exhibits $-T\ln T$ critical behavior in $α_{yx}(T)$, deviating from Fermi liquid behavior $α_{yx}\sim T$ over a decade of temperature between 10 K to 400 K, similar to ferromagnetic Weyl and nodal-line semimetals. Our theoretical calculation for CoMnSb also predicts the $-T\ln T$ behavior when the Fermi energy locates near the Weyl nodes in momentum space.

cond-mat.mtrl-sci↗

arXiv2021

High temperature antiferromagnetism in Yb based heavy fermion systems proximate to a Kondo insulator

Given the parallelism between the physical properties of Ce and Yb based magnets and heavy fermions due to the electron-hole symmetry, it has been rather odd that the transition temperature of the Yb based compounds is normally very small, as low as $\sim$ 1 K or even lower, whereas Ce counterparts may often have the transition temperature well exceeding 10 K. Here, we report our experimental discovery of the transition temperature reaching 20 K for the first time in a Yb based compound at ambient pressure. The Mn substitution at the Al site in an intermediate valence state of $α$-YbAlB$_{4}$ not only induces antiferromagnetic transition at a record high temperature of 20 K but also transforms the heavy fermion liquid state in $α$-YbAlB$_{4}$ into a highly resistive metallic state proximate to a Kondo insulator.

cond-mat.str-el↗

arXiv2020

Anomalous transport due to Weyl fermions in the chiral antiferromagnets Mn$_3$$X$, $X$ = Sn, Ge

The recent discoveries of strikingly large zero-field Hall and Nernst effects in antiferromagnets Mn$_3$$X$, ($X$ = Sn, Ge) have brought the study of magnetic topological states to the forefront of condensed matter research and technological innovation. These effects are considered fingerprints of Weyl nodes residing near the Fermi energy, promoting Mn$_3$$X$, ($X$ = Sn, Ge) as a fascinating platform to explore the elusive magnetic Weyl fermions. In this review, we provide recent updates on the insights drawn from experimental and theoretical studies of Mn$_3$$X$, ($X$ = Sn, Ge) by combining previous reports with our new, comprehensive set of transport measurements of high-quality Mn$_3$Sn and Mn$_3$Ge single crystals. In particular, we report magnetotransport signatures specific to chiral anomalies in Mn$_3$Ge and planar Hall effect in Mn$_3$Sn, which have not yet been found in earlier studies. The results summarized here indicate the essential role of magnetic Weyl fermions in producing the large transverse responses in the absence of magnetization.

cond-mat.mtrl-sci↗

arXiv2019

Anomalous thermal Hall effect in the topological antiferromagnetic state

The anomalous Hall effect (AHE), a Hall signal occurring without an external magnetic field, is one of the most significant phenomena. However, understanding the AHE mechanism has been challenging and largely restricted to ferromagnetic metals. Here, we investigate the recently discovered AHE in the chiral antiferromagnet Mn3Sn by measuring a thermal analog of the AHE, known as an anomalous thermal Hall effect (ATHE). The amplitude of the ATHE scales with the anomalous Hall conductivity of Mn3Sn over a wide temperature range, demonstrating that the AHE of Mn3Sn arises from a dissipationless intrinsic mechanism associated with the Berry curvature. Moreover, we find that the dissipationless AHE is significantly stabilized by shifting the Fermi level toward the magnetic Weyl points. Thus, in Mn3Sn, the Berry curvature emerging from the proposed magnetic Weyl fermion state is a key factor for the observed AHE and ATHE.

cond-mat.str-el↗

arXiv2017

Large anomalous Nernst effect at room temperature in a chiral antiferromagnet

Temperature gradient in a ferromagnetic conductor may generate a spontaneous transverse voltage drop in the direction perpendicular to both magnetization and heat current. This anomalous Nernst effect (ANE) has been considered to be proportional to the magnetization, and thus observed only in ferromagnets, while recent theories indicate that ANE provides a measure of the Berry curvature at the Fermi energy $E_{\rm F}$. Here we report the observation of a large ANE at zero field in the chiral antiferromagnet Mn$_3$Sn. Despite a very small magnetization $\sim 0.002$ $μ_{\rm B}/$Mn, the transverse Seebeck coefficient at zero field is $\sim 0.35~μ$V/K at room temperature and reaches $\sim 0.6~μ$V/K at 200 K, comparable with the maximum value known for a ferromagnetic metal. Our first-principles calculation reveals that the large ANE comes from a significantly enhanced Berry curvature associated with the Weyl points nearby $E_{\rm F}$. The ANE is geometrically convenient for the thermoelectric power generation, as it enables a lateral configuration of the modules to efficiently cover the heat source. Our observation of the large ANE in an antiferromagnet paves a way to develop a new class of thermoelectric material using topological magnets to fabricate an efficient, densely integrated thermopile.

cond-mat.mes-hall↗

arXiv2016

Pressure-induced magnetic transition exceeding 30 K in the Yb-based heavy fermion superconductor $β$-YbAlB$_4$

Measurements of the electric resistivity $ρ(T)$ under pressure up to 8 GPa were performed on high-quality single-crystals of the Yb-based heavy fermion system $β$-YbAlB$_4$ in the temperature range $2<T<$ 300 K. In the resistivity data, we observed pressure-induced magnetic ordering above the critical pressure $P_{\rm c} \sim$ 2 GPa. Clear difference in the phase diagram under pressure using two types of pressure mediums indicates that the transition temperature may be further enhanced under application of uniaxial pressure. With pressure, this phase transition temperature $T_{\rm M}$ is enhanced reaching 32 K at 8 GPa, which is the highest transition temperature so far recorded for the Yb-based heavy fermion compounds. The power-law exponent $α$ in $ρ=ρ_0+ AT^α$ below $T_{\rm M}$ gradually changes from 3/2 to 5/2 with increasing pressure from 2 to 8 GPa. In contrast, the resistivity exhibits a $T$-linear behavior in the temperature range 2 $\le T \le$ 20 K and is insensitive to pressure below $P_{\rm c}$. In this pressure regime, the magnetization is also nearly independent of pressure and shows no anomaly above 2 K. Our results indicate that a quantum critical point for $β$-YbAlB$_4$ is also located near $P_{\rm c}$ in addition to the strange metal region near the ambient pressure.

cond-mat.str-el↗

arXiv2016

Giant Anomalous Hall Effect in the Chiral Antiferromagnet Mn3Ge

The external field control of antiferromagnetism is a significant subject both for basic science and technological applications. As a useful macroscopic response to detect magnetic states, the anomalous Hall effect (AHE) is known for ferromagnets, but it has never been observed in antiferromagnets until the recent discovery in Mn3Sn. Here we report another example of the AHE in a related antiferromagnet, namely, in the hexagonal chiral antiferromagnet Mn3Ge. Our single-crystal study reveals that Mn3Ge exhibits a giant anomalous Hall conductivity $|σ_{xz}|$ ~ 60 per ohm per cm at room temperature and approximately 380 per ohm per cm at 5 K in zero field, reaching nearly half of the value expected for the quantum Hall effect per atomic layer with Chern number of unity. Our detailed analyses on the anisotropic Hall conductivity indicate that in comparison with the in-plane-field components $|σ_{xz}|$ and $|σ_{zy}|$, which are very large and nearly comparable in size, we find $|σ_{yx}|$ obtained in the field along the c axis is found to be much smaller. The anomalous Hall effect shows a sign reversal with the rotation of a small magnetic field less than 0.1 T. The soft response of the AHE to magnetic field should be useful for applications, for example, to develop switching and memory devices based on antiferromagnets.

cond-mat.str-el↗

arXiv2015

Strange metal without magnetic criticality

A fundamental challenge to our current understanding of metals is the frequent observation of qualitative departures from Fermi liquid behavior. The standard view attributes such non-Fermi liquid phenomena to the scattering of electrons off quantum critical fluctuations of an underlying order parameter. While the possibility of non-Fermi liquid behavior isolated from the border of magnetism has long been speculated, no experimental confirmation has been made. Here we report on the observation of a strange metal region in the absence of a magnetic instability in an ultrapure single crystal. In particular, we show that the heavy fermion superconductor $β$-YbAlB$_4$ forms a possible phase with strange metallic behavior across an extensive pressure regime, distinctly separated from a high-pressure magnetic quantum phase transition by a Fermi liquid phase.

cond-mat.str-el↗

arXiv2015

High Pressure Measurements of the Resistivity of $β$-YbAlB$_4$

The electric resistivity $ρ(T)$ under hydrostatic pressure up to 8 GPa was measured above 2 K using a high-quality single crystal of the Yb-based heavy fermion system $β$-YbAlB$_4$. We found pressure-induced magnetic ordering above the critical pressure $P_{\rm c} \approx $ 2.4 GPa. This phase transition temperature $T_M$ is enhanced with pressure and reaches 30 K at a pressure of 8 GPa, which is the highest transition temperature for the Yb-based heavy fermion compounds. In contrast, the resistivity is insensitive to pressure below $P_c$ and exhibits the $T$-linear behavior in the temperature range between 2 and 20 K. Our results indicate that quantum criticality for $β$-YbAlB$_4$ is also located near $P_{\rm c}$ in addition to the ambient pressure.

cond-mat.str-el↗

arXiv2014

Heavy Fermion Superconductivity in the Quadrupole Ordered State of PrV2Al20

PrV$_2$Al$_{20}$ is a rare example of a heavy fermion system based on strong hybridization between conduction electrons and nonmagnetic quadrupolar moments of the cubic $Γ_3$ ground doublet. Here, we report that a high-quality single crystal of PrV$_2$Al$_{20}$ exhibits superconductivity at $T_{\rm c}=$ 50 mK in the antiferroquadrupole-ordered state under ambient pressure. The heavy fermion character of the superconductivity is evident from the specific heat jump of $ΔC/T \sim 0.3$ J/mol K$^2$ and the effective mass $m^*/m_0 \sim 140$ estimated from the temperature dependence of the upper critical field. Furthermore, the high-quality single crystals exhibit double transitions at $T_{\rm Q}$ = 0.75 K and $T^{*}$ = 0.65 K associated with quadrupole and octapole degrees of freedom of the $Γ_3$ doublet. In the ordered state, the specific heat $C/T$ shows a $T^3$ dependence, indicating the gapless mode associated with the quadrupole and/or octapole order. The strong sensitivity to impurity of the superconductivity suggests unconventional character due to significant quadrupolar fluctuations.

cond-mat.str-el↗

arXiv2013

Pressure-induced Enhancement of Superconductivity in BiS$_2$-layered LaO$_{1-x}$F$_x$BiS$_2$

The newly discovered BiS$_2$-based LaO$_{1-x}$F$_{x}$BiS$_2$ ($x$=0.5) becomes superconductive at $T_c$=2.5 K. Electrical resistivity and magnetization measurements are performed under pressure to determine the pressure dependence of the superconducting transition temperature $T_c$. We observe that $T_c$ abruptly increases from 2.5 K to 10.7 K at a pressure of 0.7 GPa. According to high-pressure X-ray diffraction measurements, a structural phase transition from a tetragonal phase ($P$4/$nmm$) to a monoclinic phase ($P$2$_1/m$) also occurs at around $\sim$ 1 GPa. We consider that a pressure-induced enhancement of superconductivity is caused by the structural phase transition.

cond-mat.supr-con↗

arXiv2010

Anomalous Spin Dynamics observed by High Frequency ESR in Honeycomb Lattice Antiferromagnet InCu2/3V1/3O3

High-frequency ESR results on the S=1/2 Heisenberg hexagonal antiferromagnet InCu2/3V1/3O3 are reported. This compound appears to be a rare model substance for the honeycomb lattice antiferromagnet with very weak interlayer couplings. The high-temperature magnetic susceptibility can be interpreted by the S=1/2 honeycomb lattice antiferromagnet, and it shows a magnetic-order-like anomaly at TN=38 K. Although, the resonance field of our high-frequency ESR shows the typical behavior of the antiferromagnetic resonance, the linewidth of our high-frequency ESR continues to increase below TN, while it tends to decrease as the temperature in a conventional three-dimensional antiferromagnet decreases. In general, a honeycomb lattice antiferromagnet is expected to show a simple antiferromagnetic order similar to that of a square lattice antiferromagnet theoretically because both antiferromagnets are bipartite lattices. However, we suggest that the observed anomalous spin dynamics below TN is the peculiar feature of the honeycomb lattice antiferromagnet that is not observed in the square lattice antiferromagnet.

cond-mat.str-el↗