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Takahiro Urata

Publications and source records attributed to Takahiro Urata.

7 recordsLinked to original sources

Altermagnetic spin-split Fermi surfaces in CrSb revealed by quantum oscillation measurements

We report a comprehensive quantum oscillation study of the prototypical altermagnet CrSb, combining high-field magnetotransport and torque measurements with DFT + $U$ calculations including spin-orbit coupling. Multiple quantum oscillation frequencies were observed and tracked over wide angular ranges. The measured frequency branches are consistently explained by the spin-split Fermi surfaces arising from the altermagnetic electronic structure. Our determined Fermi surface reveals that bands 1 and 2 form closed pockets centered at the A point, rather than the tubular $c$-axis-open sheets or $Γ$-centered closed pockets proposed in previous studies. Our findings establish the Fermi-surface topology of CrSb and provide a firm basis for exploring emergent phenomena in altermagnetic materials.

cond-mat.mtrl-sci

High mobility charge transport in a multicarrier altermagnet CrSb

A newly identified magnetic phase called altermagnet is being actively studied because of its unprecedented spin-dependent phenomena. Among the candidate materials, CrSb has a particularly high ordering temperature and a large spin-splitting energy, but its transport properties have remained unexplored. In this study, we report the magnetotransport properties of CrSb measured on single crystals. We found that the Hall resistivity shows a nonlinear dependence on the magnetic field at low temperatures. From symmetry-based considerations, however, this behavior can not be attributed to an anomalous Hall effect, but to a multicarrier effect. A multicarrier fitting to the in-plane conductivity tensor revealed the presence of carriers with high mobility in CrSb, which is an advantage for efficient spin current generation.

cond-mat.mtrl-sci

Single Crystal Growth and Transport Properties of van der Waals Materials $AB$Te$_\mathbf{4}$ ($A/B$ = Ti, Zr, Hf)

Monolayers of $AB$Te$_4$ ($A$/$B$ = Ti, Zr, Hf) were theoretically predicted to be two-dimensional topological insulators, but little has been known about the physical properties of these compounds. Here, we report on the single crystal growth, bulk transport properties, and band structure calculations of these compounds. The magnetotransport properties indicate that all three compounds are multi-carrier systems. The experimental results of ZrTiTe$_4$ and HfTiTe$_4$ can be well fitted by the multi-carrier formula assuming two types of carriers, while three carrier components were necessary for HfZrTe$_4$. Interestingly, one of the carrier mobilities of HfZrTe$_4$ exceeded 1000 cm$^2$V$^{-1}$s$^{-1}$, which was nearly one order in magnitude larger than the carrier mobilities of ZrTiTe$_4$ and HfTiTe$_4$. Our band structure calculations showed that all three compounds are semimetals consistent with the magnetotransport properties. The band structure around the $Γ$-point of HfZrTe$_4$ exhibits features that are distinct from the other two compounds, which is likely the reason of the different carrier properties.

cond-mat.mtrl-sci

Electronic States and Energy Dissipations of Vortex Core in Pure FeSe Single Crystals Investigated by Microwave Surface Impedance Measurements

In order to clarify electronic states and energy dissipations due to a motion of a vortex core in pure FeSe, which is a candidate superconductor possessing a super-clean core, we measured the microwave surface impedance of pure FeSe single crystals under finite magnetic fields. From the magnetic-field dependence of the flux-flow resistivity, we found that a barometer of electronic states inside the vortex core $ω_{0}τ_{\rm core}$ is $1\pm0.5$, suggesting that the vortex core of pure FeSe is in the moderately clean regime contrary to the expectation of the super-clean core. We also found that the mean-free path inside the vortex core is suppressed at the distance of the order of the core radius. Based on observed results and previous reports, we discussed possible origins of rather small $ω_{0}τ_{\rm core}$ value in terms of the multiple-bands nature of FeSe and additional mechanisms producing extra energy dissipations specific to the vortex core in motion.

cond-mat.supr-con

Separate tuning of nematicity and spin fluctuations to unravel the origin of superconductivity in FeSe

The interplay of orbital and spin degrees of freedom is the fundamental characteristic in numerous condensed matter phenomena, including high temperature superconductivity, quantum spin liquids, and topological semimetals. In iron-based superconductors (FeSCs), this causes superconductivity to emerge in the vicinity of two other instabilities: nematic and magnetic. Unveiling the mutual relationship among nematic order, spin fluctuations, and superconductivity has been a major challenge for research in FeSCs, but it is still controversial. Here, by carrying out 77Se nuclear magnetic resonance (NMR) measurements on FeSe single crystals, doped by cobalt and sulfur that serve as control parameters, we demonstrate that the superconducting transition temperature Tc increases in proportion to the strength of spin fluctuations, while it is independent of the nematic transition temperature Tnem. Our observation therefore directly implies that superconductivity in FeSe is essentially driven by spin fluctuations in the intermediate coupling regime, while nematic fluctuations have a marginal impact on Tc.

cond-mat.str-el

Novel method to study strain effect of thin films using a piezoelectric-based device and a flexible metallic substrate

For applying tensile or compressive uniaxial strain to functional thin films, we propose a novel approach in combining a piezoelectric-based device and a technical metallic substrate used widely in the 2nd generation coated conductors (i.e. superconducting tapes). A strain-induced shift of the superconducting transition temperature of 0.1 K for Co-doped BaFe2As2 was observed along [100] direction, corresponding to a uniaxial pressure derivative dTc/dp100=-4 K/GPa. For Mn3CuN, a uniaxial strain derivative along [100] direction of the Curie temperature dTC/de100=13 K/% was observed. The current approach is applicable to various functional thin films in a wide range of temperatures.

cond-mat.supr-con

Non-Fermi liquid behavior of electrical resistivity close to the nematic critical point in Fe$_{1-x}$Co$_x$Se and FeSe$_{1-y}$S$_y$

Temperature dependence of resistivity of single crystals of Fe$_{1-x}$Co$_x$Se and FeSe$_{1-y}$S$_y$ is studied in detail under zero and high magnetic field (magnetoresistance), the latter of which enables to monitor the temperature ($T$) evolution of resistivity below the onset of superconducting transition temperature ($T_{\rm c}$). In FeSe$_{1-y}$S$_y$, $T$-linear dependence of resistivity is prominent in $y$ = 0.160 below 40 K, whereas it changes to a Fermi-liquid(FL)-like $T^2$ one below 10 K in $y$ = 0.212. These suggest that the quantum critical point (QCP) originating from the electronic nematicity resides around $y$ = 0.160 and the fluctuation in QCP gives rise anomalous $T$-linear dependence in resistivity in a wide $T$ range. In Fe$_{1-x}$Co$_x$Se, resistivity gradually changes from linear- to quadratic- $T$-dependent one at low temperatures in the range between $x$ = 0.036 and 0.075. These could be interpreted by scenarios of both the nematic QCP and the crossover in the ground states between the orthorhombic nematic phase and the tetragonal phase. The anomalies found as $T$-linear resistivity are discussed in terms of orbital and spin fluctuation arising from the nematic QCP.

cond-mat.supr-con