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Takashi Oka

Publications and source records attributed to Takashi Oka.

At least 19 recordsLinked to original sources

Floquet Driving of Enzymatic Reactions: Counting Statistics and Long-Time Currents

Technologies for artificially controlling chemical reaction systems, such as optogenetics, are rapidly advancing, making it increasingly important to understand reaction dynamics under time-dependent control. When the modulation of reaction rates is periodic in time, the Floquet formalism provides a systematic framework. We develop a Floquet theory for classical stochastic processes that enables the calculation of the current and its counting statistics under such periodic modulation. In particular, we formulate the theory in terms of a counting field and derive general expressions for the first cumulant and the corresponding current. The current is expressed using the effective Floquet generator and the kicked state, and we further obtain general asymptotic expressions for the current in both the high- and low-frequency regimes. As a concrete example to test our analytical expressions, we then apply the results to discrete Floquet driving -- a non-perturbative, stepwise protocol. The setup is motivated by a biochemical system known as cyclic adenosine monophosphate (cAMP) production, which is an enzymatic reaction activated and inhibited by G-proteins. This is formulated as a discretely driven Michaelis--Menten-type reaction model, in which the catalytic activity is switched on and off abruptly in time, and we obtain analytical expressions and numerical results showing how periodic switching of reaction rates generates a long-time product current. In particular, in the high-frequency limit, we show that the effect of the periodic driving can be interpreted through an effective modification of the chemical reaction rates. These results provide a basis for Floquet analysis of periodically driven chemical reactions.

cond-mat.stat-mech

Geometric modulation of transition and survival intensities in non-Hermitian systems

The time evolution of non-Hermitian systems is generally nonunitary. Dynamics governed by time-dependent non-Hermitian Hamiltonians lead to a variety of novel phenomena, one of which is state amplification or suppression induced by the complex Berry phase. Here, we extend the framework of geometric modulation to multi-level systems and show that both transition and survival intensities can be modulated. We apply our theory to the non-Hermitian Landau-Zener (LZ) problem. First, we show that, in the half-LZ problem, both the transition and survival probabilities exhibit nonreciprocity due to the complex Berry phase. In the non-Hermitian standard LZ problem, only the survival intensity is known to exhibit nonreciprocity, whereas the transition intensity does not. However, the physical origin of this nonreciprocal behavior remains unclear. In this work, we show that the nonreciprocity originates from the complex Berry phase.

quant-ph

Magnetism and Topology from Circularly Polarized Phonon Floquet Engineering

We theoretically show that circularly polarized phonons induce electronic magnetization and drive a topological phase transition via phonon Floquet engineering. Considering the electronic states modulated by circularly polarized phonons on a honeycomb lattice, we show that such lattice dynamics generates an effective next-nearest-neighbor electron hopping, leading to a Haldane-type mass term. Circularly polarized phonon breaks time-reversal symmetry (TRS) and opens a gap at valley points, undergoing phase transition from a trivial insulator to a Chern insulator. Moreover, the orbital and spin magnetizations emerge due to the breaking of TRS. Our results show that circularly polarized phonons serve as an effective magnetic field to engineer magnetism and topology, offering new opportunities for phonon Floquet approaches.

cond-mat.mes-hall

Direct probing the quantum geometric tensor for bosonic collective excitations

The quantum geometric tensor (QGT), whose real and imaginary parts define the quantum metric and Berry curvature, encodes the intrinsic geometry of quantum states. While electronic QGT has recently become experimentally accessible and linked to diverse physical phenomena, its bosonic counterpart remains largely unexplored. Here we show that the dynamical structure factor encodes the momentum-space structure of bosonic wave functions and thereby provides direct access to the full bosonic QGT throughout the Brillouin zone. Applying this framework, we uncover clear geometric signatures in the twofold quadrupole-Weyl phonon of BaPtGe and the nodal-line magnon in Gd, and further generalize the formalism to multiband systems. Our results establish a general route to measuring (non-)Abelian quantum geometry in bosonic systems, a crucial step toward elucidating its impact on condensed matter phenomena.

cond-mat.mtrl-sci

Geometric Effects on Tunneling in Driven Quantum Systems

We review quantum tunneling provoked by external field driving, focusing on the role of geometric effects. The discussion begins with an overview of tunneling phenomena, including the Landau-Zener model and the Schwinger effect, both of which are essential frameworks to describe the generation of elementary excitation of the system. We also refer to the relation between the modern theory of polarization and the geometry of the system, and introduce the shift vector via adiabatic perturbation theory. Then we introduce the twisted Landau-Zener model and shown how the shift vector modulates tunneling probability, followed by several illustrative applications of this model. We also explain the Keldysh crossover, which is the crossover from a quantum tunneling regime to photon absorption regime in driven systems.

cond-mat.str-el

Chern-Simons type cross-correlations and geometric Born effective charge of phonons

The interplay between different degrees of freedom in condensed matter systems engenders a rich variety of emergent phenomena. In particular, fermions with non-trivial quantum geometry can generate Chern-Simons (CS)-like terms in effective field theories for different gauge fields. For phonons, such terms can result in chiral phonon splitting. Here, we propose that the local Berry curvature can influence the spectra and dynamics of optical phonons, even in materials with zero Chern number, which we demonstrate with a gapped Dirac model. We identify a previously overlooked CS like cross-correlation between electromagnetic and pseudo-gauge fields in 2+1 dimensions which depends on valley Chern number. It facilitates a direct coupling between phonons and photons by inducing a geometric Born effective charge. This opens up a new route for coherent Raman phonon excitation and quantum geometry probes.

cond-mat.mes-hall

Long-range electron coherence in Kagome metals

The wave-like nature of electrons lies at the core of quantum mechanics, distinguishing them from classical particles. Landmark experiments have revealed phase coherence of mobile electrons within solids, such as Aharonov-Bohm interference in mesoscopic rings. However, this coherence is typically limited by numerous environmental interactions. Controlling and ideally mitigating such decoherence remains a central challenge in condensed matter physics. Here, we report magnetoresistance oscillations in mesoscopic pillars of the Kagome metal CsV$_3$Sb$_5$ for fields applied parallel to the Kagome planes. Their periodicity is independent of materials parameters, simply given by the number of flux quanta $h/e$ threading between adjacent Kagome layers akin to an atomic-scale Aharonov-Bohm interferometer. Intriguingly they occur under conditions not favorable for typical interference in solids, at temperatures above 20 K and in micrometer-scale devices well exceeding the single-particle mean free path. Further, the oscillations exhibit non-analytic field-angle dependence and scale consistently with a broad range of key electronic responses in CsV$_3$Sb$_5$, pointing to a cooperative mechanism that establishes intrinsic coherence. Our findings provide new insights into the debated origin of correlated order in CsV$_3$Sb$_5$ and establish Kagome metals as a promising platform for interaction-stabilized long-range electron coherence - crucial for both fundamental studies and technological advancements in quantum interference in metallic systems.

cond-mat.str-el

Semi-Analytical Engineering of Strongly Driven Nonlinear Systems Beyond Floquet and Perturbation Theory

Strongly driven nonlinear systems are frequently encountered in physics, yet their accurate control is generally challenging due to the intricate dynamics. In this work, we present a non-perturbative, semi-analytical framework for tailoring such systems. The key idea is heuristically extending the Floquet theory to nonlinear differential equations using the Harmonic Balance method. Additionally, we establish a novel constrained optimization technique inspired by the Lagrange multiplier method. This approach enables accurate engineering of effective potentials across a broader parameter space, surpassing the limitations of perturbative methods. Our method offers practical implementations in diverse experimental platforms, facilitating nonclassical state generation, versatile bosonic quantum simulations, and solving complex optimization problems across quantum and classical applications.

quant-ph

Shockwave-Enhanced Floquet Engineering in Relativistic Quasiparticles

We investigate Floquet engineering of three-dimensional Dirac fermions driven by propagating waves, identifying distinct quantum states and phase transitions in the time-like, light-like, and space-like regimes. Notably, we uncover a novel regime where Floquet Weyl bands emerge and transition into Type-II Weyl states as the wave speed nears the Fermi velocity. Using Floquet-Bloch theory, we demonstrate that Lorentz contraction strongly amplifies Floquet band modulation effects, leading to a shockwave-like state synchronized with the wave motion. These findings extend beyond electrons to quasiparticles with relativistic dispersions, opening new avenues for dynamic band engineering in quantum materials.

cond-mat.mes-hall

Light-induced anomalous Hall conductivity in massive 3D Dirac semimetal Co$_3$Sn$_2$S$_2$

Weyl semimetals can emerge from Dirac semimetals when the time-reversal or spatial-inversion symmetries are broken. Recently, it has been proposed based on the Floquet theory that Dirac semimetals can be converted into Weyl semimetals even by shining circularly polarized light (CPL). Here we have investigated the possibility of such a Dirac-Weyl conversion by measuring the CPL-induced anomalous Hall conductivity (AHC) in a massive 3D Dirac semimetal Co$_3$Sn$_2$S$_2$ in the paramagnetic phase using ultrafast mid-infrared pump-terahertz Faraday rotation probe spectroscopy. We find that the field-strength and driving frequency dependence of the observed AHC is well accounted for by CPL-induced nonzero Berry curvature associated with the splitting of the Dirac bands as predicted by the Floquet theory. The estimated splitting of the Dirac bands reaches about 60 % of the mass gap and the calculated CPL-induced AHC quantitatively reproduces the experimental observation, demonstrating a promising route toward the realization of Floquet-Weyl states from massive Dirac semimetals.

cond-mat.mes-hall

Inverse Spin Hall Effect in Nonequilibrium Dirac Systems Induced by Anomalous Flow Imbalance

We study Dirac fermions in the presence of a space-dependent chiral gauge field and thermodynamic gradients, establishing a connection to the inverse spin Hall effect. The chiral gauge field induces a chiral magnetic field, resulting in a surface Fermi arc state and a chiral Landau level state which, although is delocalized in the bulk, we show to be more robust against impurities. By applying chemical potential and temperature gradients, we achieve nonzero charge currents, with each gradient leading to distinct Fermi level dependencies, both of which have been observed in a recent experiment. Unlike the conventional mixed axial-gravitational anomaly, our currents require a noncollinear chiral magnetic field and thermodynamic gradient. We further derive low-energy transport formulas and demonstrate the importance of carefully treating the ultraviolet cutoff for understanding our lattice calculations.

cond-mat.mes-hall

Many-body Keldysh Crossover in the DC-driven Haldane Spin Chain

We theoretically study nonlinear processes driven by a DC spin-electric field in the antiferromagnetic spin-1 Heisenberg model starting from the ground state in the Haldane phase. The DC spin-electric field generates finite spin current and accumulation since the symmetry protected topological order is destroyed by the field. We find two microscopic mechanisms responsible for the breakdown and a crossover between them: In weak fields, tripron-antitripron pair creation occurs through the tunneling mechanism, and in strong fields, the system is described by an effective Hamiltonian breaking the protecting symmetries. We analyze the numerically obtained results in terms of the Dykhne--Davis--Pechukas theory and Floquet theory, verifying the universal picture of the many-body Keldysh crossover in the DC-driven quantum spin systems.

cond-mat.str-el

Dirac Electrons in AC-Magnetic Fields: $\pi$-Landau Levels and Chiral Anomaly-Induced Homodyne Effect

Floquet engineering, which involves controlling systems through time-periodic driving, is a method for coherently manipulating quantum materials and realizing dynamical states with novel functionalities. Most research in solid-state systems has focused on the use of AC-\textit{electric} fields as the controlling drive. In this study, we investigate the effects of AC-\textit{magnetic} fields on two-dimensional (2D) Dirac electrons and report the emergence of new states and new transport phenomena. In a magnetic field that temporarily changes its direction, the 2D Dirac electrons form a new localized state with a flat band dispersion, dubbed as a $\pi$-Landau level. Its wave function is a superposition of the clockwise and counterclockwise cyclotron orbits with time-periodic amplitudes, resulting in a novel closed trajectory shaped like a figure eight. Then, what would be the counterpart of the Hall effect in AC-magnetic fields? We find that a DC-current in the transverse direction, \textit{i.e.} a homodyne Hall current, is generated when an additional AC-electric field is applied. In the case of Dirac electrons, several electronic states contribute to this phenomenon including the $\pi$-Landau level. However, when the chemical potential $\mu$ is near the Dirac point, the dominant contribution comes from the low-energy electrons and we numerically find the homodyne Hall current to behave as $I_y=-\frac{e}{h}\mu$ per valley and spin. We explain this phenomenon through the high-frequency effective Floquet Hamiltonian which resembles the chiral Landau level Hamiltonian of three-dimensional Weyl Hamiltonian exhibiting chiral anomaly. We discuss the experimental feasibility and conclude that it is possible to realize this new exotic state using techniques such as THz metamaterial enhancement of magnetic fields.

cond-mat.mes-hall

Anomalous Hall transport by optically injected isospin degree of freedom in Dirac semimetal thin film

Chirality of massless fermions emergent in condensed matter is a key to understand their characteristic behavior as well as to exploit their functionality. However, chiral nature of massless fermions in Dirac semimetals has remained elusive, due to equivalent occupation of carriers with the opposite chirality in thermal equilibrium. Here, we show that the isospin degree of freedom, which labels the chirality of massless carriers from a crystallographic point of view, can be injected by circularly polarized light. Terahertz Faraday rotation spectroscopy successfully detects the anomalous Hall conductivity by a light-induced isospin polarization in a three-dimensional Dirac semimetal, Cd$_3$As$_2$. Spectral analysis of the Hall conductivity reveals a long scattering time and a long decay time, which are characteristic of the isospin. The long-lived, robust, and reversible character of the isospin promises potential application of Dirac semimetals in future information technology.

cond-mat.mes-hall

Disentangling the Competing Mechanisms of Light-Induced Anomalous Hall Conductivity in Three-Dimensional Dirac Semimetal

We experimentally elucidate the origin of the anomalous Hall conductivity in a three-dimensional Dirac semimetal, Cd$_3$As$_2$, driven by circularly polarized light. Using time-resolved terahertz Faraday rotation spectroscopy, we determine the transient Hall conductivity spectrum with special attention to its sign. Our results clearly show the dominance of direct photocurrent generation assisted by the terahertz electric field. The contribution from the Floquet-Weyl nodes is found to be minor when the driving light is in resonance with interband transitions. We develop a generally applicable classification of microscopic mechanisms of light-induced anomalous Hall conductivity.

cond-mat.mtrl-sci

Demonstration of geometric diabatic control of quantum states

Geometric effects can play a pivotal role in streamlining quantum manipulation. We demonstrate a geometric diabatic control, that is, perfect tunneling between spin states in a diamond by a quadratic sweep of a driving field. The field sweep speed for the perfect tunneling is determined by the geometric amplitude factor and can be tuned arbitrarily. Our results are obtained by testing a quadratic version of Berry's twisted Landau-Zener model. This geometric tuning is robust over a wide parameter range. Our work provides a basis for quantum control in various systems, including condensed matter physics, quantum computation, and nuclear magnetic resonance.

quant-ph

Confinement Phase in Carbon-Nanotubes and the Extended Massive Schwinger Model

Carbon nanotube with electric fluxes confined in one dimension is studied. We show that a Coulomb interaction \propto |x| leads to a confinement phase with many properties similar to QCD in 4D. Low-energy physics is described by the massive Schwinger model with multi-species fermions labeled by the band and valley indices. We propose two means to detect this state. One is through an optical measurement of the exciton spectrum, which has been calculated via the 't Hooft-Berknoff equation with the light-front field theory. We show that the Gell-Mann-Oakes-Renner relation is satisfied by a dark exciton. The second is the nonlinear transport which is related to Coleman's "half-asymptotic" state.

cond-mat.str-el

Anomalous Hall effect of light-driven three-dimensional Dirac electrons in bismuth

Recent advancement in laser technology has opened the path toward the manipulation of functionalities in quantum materials by intense coherent light. Here, we study three-dimensional (3D) Dirac electrons driven by circularly polarized light (CPL), when the photon energy lies within the Dirac bands. As an experimental realization of this setup, we irradiate a thin film sample of elemental bismuth, which is a well-known semimetal hosting 3D Dirac electrons, with mid-infrared CPL. We successfully observe the emergence of the anomalous Hall effect (AHE) via terahertz Faraday rotation that is both pump-helicity-dependent and instantaneous. We compare our experimental findings with the results of Floquet theory, which is a powerful framework for analyzing the electronic band structure driven by coherent light. The contribution from the band structures near the one-photon resonant positions to the AHE shows a field-strength dependence consistent with our experimental results. The effective Hamiltonian on which we base our model calculations also implies that a pair of "double Weyl points" emerge due to the CPL-induced hybridization between the occupied and unoccupied 3D Dirac bands. Our findings shed light on ultrafast control of material properties in nonlinear topological optics.

cond-mat.mes-hall