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Takashi Uchino

Publications and source records attributed to Takashi Uchino.

14 recordsLinked to original sources

Imaging and characterization of spontaneous vortices in a proximity-induced superconductor

Observation of spontaneous symmetry breaking is crucial for understanding continuous second-order phase transitions from disordered to ordered states, which often leads to the formation of topological defects. In superconductors, such topological defects manifest as quantized vortices. However, the formation and observation of spontaneous vortices in a uniform superconductor are challenging because extremely rapid cooling (>108 K/s) is generally required for that purpose. Here we conducted scanning superconducting quantum interference device microscope (SSM) measurements on an MgB2-based proximity-induced superconductor, an intrinsically inhomogeneous system. In this system, individual superconducting domains will reach internal equilibrium independently during cooling and choose their own phase before the global phase coherence is established via the long-range proximity coupling. The SSM measurements demonstrate that vortices are nucleated spontaneously even at a relatively slow cooling rate (~0.2 K/s). We also find that the vortices with different polarities, sizes, and shapes appear stochastically under near-zero-field conditions. The geometry of the spontaneous vortices is more extended than that of the field-induced Abrikosov vortices. Magnetic field profile analysis based on the London model elucidates that penetration depths of the extended vortices are anomalously large, exceeding several micrometers. This unusual morphology of the spontaneous vortices most likely imprints the information that is frozen at the moment of vortex formation. Our findings not only provide insights into the local phase differences present in the early stage of the phase transition in this proximity-induced superconducting system, but they also shed insights into the structure, formation, and stabilization of topological defects in highly disordered and inhomogeneous superconducting systems.

cond-mat.supr-con↗

Establishment of global phase coherence in a highly disordered fractal MgO/MgB2 nanocomposite: Roles of interface, morphology and defect

Recently, we have reported that a highly disordered fractal MgO/MgB2 nanocomposite exhibits bulk-like superconducting properties with isotropic pinning, showing an excellent phase-coherent capability irrespective of the low volume fraction (~30 vol. %) of MgB2 [Uchino et al., Phys. Rev. B 101, 035146 (2020); Teramachi et al,, Phys. Rev. B 108, 155146 (2023)]. Hence, this nanocomposite provides a useful experimental system to investigate the relationship between the structural disorder and the establishment of the superconducting phase coherence. In this work, we show from 3D focused ion beam scanning electron microscopy (FIB-SEM) data that in the nanocomposite, a complex MgO/MgB2 microstructure spreads isotropically throughout the sample with a constant fractal dimension of ~1.67. Atomic-resolution scanning transmission electron microscopy (STEM) has revealed that the MgO/MgB2 interfaces are atomically clean and free from amorphous grain boundaries, even leading to atomically coherent interfaces. Detailed ac susceptibility measurements have demonstrated a smooth crossover from an intragranular to an intergranular superconducting regime, giving evidence of the establishment of the critical state due to strong intergranular coupling just below the superconducting transition temperature. Also, spatially-resolved cathodoluminescence measurements have demonstrated that oxygen vacancies in the MgO-rich phase tend to aggregate near the MgO/MgB2 boundary regions, forming long channels of oxygen vacancies through the nanocomposite. These channels of oxygen vacancies will contribute to the long-range carrier transfer and the related Andreev reflection via coherent tunneling of charge carriers among the oxygen vacancy sites.

cond-mat.supr-con↗

Atomic-Scale Observation of Moire potential in Twisted Hexagonal Boron Nitride Layers by Electron Microscopy

Moire superlattices (MSLs) are an emerging class of two-dimensional functional materials whose electronic states can be tuned by the twist angle between two van der Waals layers and/or the relative placement of the layers. The intriguing properties of MSLs are closely correlated to the moiré potential, which is the electrostatic potential induced by interlayer coupling. Intensive efforts have been made to understand the nature and distribution of the moire potential by using various experimental and theoretical techniques. However, the experimental observation of the moiré potential is still challenging because of the possible presence of the surface and/or interlayer contaminants. In this work, we develop a method to obtain hexagonal boron nitride (hBN) nanolayers (with or without twist) using a specially designed chemical exfoliation technique. The resulting hBN nanolayers are atomically clean and strain free, hence providing ideal MSLs for the investigation of their moiré potential. Aberration-corrected high resolution transmission electron microscopy measurements on the twisted hBN nanolayers allow us to observe moiré diffraction spots in Fourier space. Then, the moire potential is reconstructed by the inverse fast Fourier transform of the moire diffraction spots. It has been revealed that the local interlayer atomic overlap plays a decisive role in determining the periodicity and distribution of the moiré potential, as supported by density functional theory calculations. This work not only provides a general strategy to observe the moire potential in MSLs, but it also expands the application of electron microscopy to the further study of MSLs with atomic resolution.

cond-mat.mtrl-sci↗

Strong phase coherence and vortex matter in a fractal system with proximity-induced superconductivity

The proximity effect in normal/superconductor heterostructures is an intriguing phenomenon in that the normal side takes on the properties of a superconductor with an induced gap. However, the structural and pinning properties of vortices inside the normal regions remain poorly understood. Here, we report structure and superconducting properties of a proximity-coupled Mg/MgO/MgB2 system with ~30 vol. % of superconducting MgB2, in which MgB2 nanograins are distributed in a fractal manner to form a proximity network with clean interfaces. Conductivity and magnetic measurements demonstrate that this proximity-coupled system acts as a fully phase coherent superconductor with isotropic pinning. Magneto-optical imaging also reveals a rather homogeneous flux density distribution with no apparent granularity. Furthermore, we observe quantized proximity vortices and their clustering behavior by scanning superconducting quantum interface device microscopy. These results show that in contrast to the case of conventional granular superconductors, the grain boundaries in the present sample carry high critical currents and have high vortex pinning efficiency, resulting in a robust phase coherent state irrespective of the low volume fraction of the MgB2 nanograins. This finding not only reveals the features of proximity-induced vortices, but also demonstrates an excellent phase-locked capability of the proximity-coupled fractal system.

cond-mat.supr-con↗

Enhancement of the superconducting transition temperature of MgB2 by proximity effect of d0 ferromagnet

Heterostructures of superconducting and ferromagnetic materials are of fundamental interest because of the mutual interaction of antagonistic kinds of ordering at the S-F interface. Normally, the superconducting transition temperature Tc should be strongly suppressed at the S-F interface owing to the penetration of Cooper pairs into the ferromagnetic side. Nevertheless, constructive interactions between S and F orders have been suggested to occur via the modification of ferromagnetic order by the superconducting state. This may induce an inhomogeneous magnetic state, often called a cryptoferromagnetic state, and the relevant domain wall effect, which will lead to a local decrease of the pair-breaking parameter. However, the domain wall effect, even if it exists, is quite subtle from the experimental view point and is normally difficult to observe. Here we show that the defect-related d0 ferromagnetism in MgO and the superconductivity in MgB2 do not antagonize, but rather enhance the superconducting transition temperature Tc to any significant degree. We found in superconducting MgB2-d0 ferromagnetic MgO composites that the superconducting transition proceeds in two steps. The first at the S-F interface, between 110-120 K, then in the rest of the bulk at 39 K, which is the Tc of single phase MgB2 superconductor. Moreover, the additional transition emerges at 60 K at the S-F interface especially in the ferromagnetic side, showing a spin-glass-like magnetic state. Our findings reveal that the proximity effect in the superconductor-d0 ferromagnet heterostructures will provide the knowledge and basis to enhance the Tc value of the existing superconductors.

cond-mat.supr-con↗

Spontaneous vortex state in a superconductor/ferromagnet nanocomposite

The mechanism of the interplay between superconductivity and magnetism is one of the intriguing and challenging problems in physics. Theory has predicted that the ferromagnetic order can coexist with the superconducting order in the form of a spontaneous vortex phase in which magnetic vortices nucleate in the absence of an external field. However, there has been no rigorous demonstration of spontaneous vortices by bulk magnetic measurements. Here we show the results of experimental observations of spontaneous vortices using a superconductor/ferromagnet fractal nanocomposite, in which superconducting MgB2 and ferromagnetic nanograins are dispersedly embedded in the normal matrix to realize the remote electromagnetic interaction and also to induce a long-range Josephson coupling. We found from bulk magnetization measurements that the sample with nonzero remanent magnetization exhibits the magnetic behaviors which are fully consistent with a spontaneous vortex scenario predicted theoretically for magnetic inclusions in a superconducting material. The resulting spontaneous vortex state is in equilibrium and coexists surprisingly with a Meissner state (complete shielding of an external magnetic field). The present observation not only reveals the evolution process of the spontaneous vortices in superconductor/ferromagnet hybrids, but it also sheds light on the role of the fractal disorder and structural heterogeneity on the vortex nucleation under the influence of Josephson superconducting currents.

cond-mat.supr-con↗

Macroscale three-dimensional proximity effect in disordered normal/superconductor nanocomposites

Recently, interest in Superconductor (S)-Normal (N) interfaces was renewed by the observation of exotic proximity effects in various systems, including S/semiconductor, S/ferromagnet, and S/topological insulator. In general, the proximity effect is enhanced in transparent weak links where coherent Andreev reflection is possible. Also, it is a common knowledge that the proximity effect is, by definition, is a localized phenomenon that can only be active in each S/N interface region. However, here we show that a three-dimensional (3D) macroscale proximity effect is realized in few-micrometer-thick MgO/Mg2Si/MgB2 nanocomposite layers with atomically smooth and clean heterointerfaces. We found from scanning superconducting quantum interference device (SQUID) microscopy measurements that a normal region of more than 100x100 square micrometers totally undergoes transition into a bulk-like superconducting state although the normal host originally contains less than ~10 vol % of superconducting MgB2 nanograins in a dispersed manner. In the proximity-induced superconducting region, vortex formation and annihilation processes as well as vortex-free Meissner regions were observed with respect to applied fields in a similar manner as Abrikosov vortices in type-II superconductors. Furthermore, we found that the induced superconducting layers exhibit an anisotropic magnetization behavior, in consistent with the formation of the large-scale superconducting coherence. This unusually extended proximity effect suggests that disorder-induced interaction and coupling of Andreev bound states, which are coherent superposition of time reversed electron hole pairs, is realized in the nanocomposite. Thus, the present results not only expand the limit of the proximity effect to bulk scales, but also provides a new route to obtain a proximity-induced superconducting state from disordered systems.

cond-mat.supr-con↗

Experimental realization of purely excitonic lasing in ZnO microcrystals at room temperature: transition from exciton-exciton to exciton-electron scattering

Since the seminal observation of room-temperature laser emission from ZnO thin films and nanowires, numerous attempts have been carried out for detailed understanding of the lasing mechanism in ZnO. In spite of the extensive efforts performed over the last decades, the origin of optical gain at room temperature is still a matter of considerable discussion,. We show that ZnO microcrystals with a size of a few micrometers exhibit purely excitonic lasing at room temperature without showing any symptoms of electron-hole plasma emission. We then present the distinct experimental evidence that the room-temperature excitonic lasing is achieved not by exciton-exciton scattering, as has been generally believed, but by exciton-electron scattering. As the temperature is lowered below ~150 K, the lasing mechanism is shifted from the exciton-electron scattering to the exciton-exciton scattering. We also argue that the ease of carrier diffusion plays a significant role in showing room-temperature excitonic lasing.

cond-mat.mtrl-sci↗

Hole-doping driven antiparallel magnetic order underlying the superconducting and pseudogap states in high-temperature cuprate superconductor

Unveiling the nature of the pseudogap and its relation to both superconductivity and antiferromagnetic Mott insulators, the pairing mechanism, and a non-Fermi liquid phase is a key issue for understanding high temperature superconductivity in cuprates.We here show that antiparallel magnetic order can be reasonably and naturally predicted in hole-doped CuO2 planes by starting from the ground state of a weakly doped antiferromagnetic insulator, where a Skyrmion-type three-dimensional spin texture is created around the doped hole. The superconducting transition temperature Tc can be understood in terms of the temperature at which long-range antiparallel magnetic ordering is established, resulting in the magnetically mediated superconducting state with phase-coherent Cooper pairs. Upon heating above Tc, long-range phase coherence in the pair state is lost, but the pair condensate still survives on the medium-range length scale, transforming to the pseudogap state with charge and magnetic orders. We believe the present model provides a key initial point to unravel a wide variety of the apparently complex phenomena related to high temperature cuprate superconductors.

cond-mat.supr-con↗

Towards a complete understanding of pseudogap and pairing mechanisms in high-temperature superconducting cuprates

Unveiling the nature of the pseudogap and its relation to both superconductivity and antiferromagnetic Mott insulators, the pairing mechanism, and a non-Fermi liquid phase is a key issue for understanding high temperature superconductivity in cuprates. A number of experimental results gathered especially in recently years have revealed an unexpected inhomogeneous nature of cuprates at the nanoscale, indicating the fundamental inapplicability of the conventional theories based on homogeneous systems. Here we show a microscopic model of pseudogap and pairing mechanisms on the basis of the consideration of the spin state around a bound hole in a CuO2 plane and the resulting magnetic orders, leading eventually to the spin-Peierls distortion responsible for the Cooper pair formation. The present model fits and accounts for the accumulated experimental findings reported previously for cuprates, including stripe-like electronic order, breaking of the rotational symmetry, and the so-called 1/8 anomaly. We believe that the present model can help to develop a complete theoretical framework applicable to a large family of high-temperature superconductors, including ferropnictides and ferrochalcogenides.

cond-mat.supr-con↗

Spin-Polarized Ground States and Ferromagnetic Order Induced by Low-Coordinated Surface Atoms and Defects in Nanoscale Magnesium Oxide

We investigate the effect of low-coordinated surface atoms on the defect-induced magnetism in MgO nanocrystallites using hybrid density functional theory calculations. It has been demonstrated that when Mg vacancies are introduced at the corners of cube-like MgO clusters, a magnetic state becomes lower in total energy than the nonmagnetic singlet state by 1-2 eV, resulting in the spin-polarized ground state. The spin density is not only located at the surrounding O atoms neighbor to the corner Mg vacancy site but is also extended to the distant (1 nm or longer) low-coordinated surface O atoms along the <110> directions. This directional spin delocalization allows a remote Mg vacancy-Mg vacancyinteraction, eventually leading to a spontaneous long-range ferromagnetic interaction.

cond-mat.mes-hall↗

Symmetry and Nonstoichiometry as Possible Origin of Ferromagnetism in Nanoscale oxides

We show through density functional theory calculations that extended magnetic states can inherently occur in oxides as the size of the crystals is reduced down to the nanometer scale even when they do not explicitly include intrinsic defects. This is because in nanoscale systems crystallographically perfect crystallites paradoxically result in nonstoichiometric compositions owing to the finite number of constituting atoms. In these structurally perfect but stoichiometrically imperfect nanocrystallites, the spin-triplet state is found to be more stable than the spin-singlet state, giving rise to an extended spin distribution that expands over the entire crystal. According to this picture, long-range magnetic order arises from the combined effect of crystal symmetry and nonstoichiometry that can coexist exclusively in nanoscale systems. The idea can also give reasonable explanations for the unprecedented ferromagnetic features observed commonly in nanoscale oxides, including ubiquity, anisotropy, and diluteness.

cond-mat.mes-hall↗

Supersymmetric Quantum Mechanics under Point Singularities

We provide a systematic study on the possibility of supersymmetry (SUSY) for one dimensional quantum mechanical systems consisting of a pair of lines $\R$ or intervals [-l, l] each having a point singularity. We consider the most general singularities and walls (boundaries) at $x = \pm l$ admitted quantum mechanically, using a U(2) family of parameters to specify one singularity and similarly a U(1) family of parameters to specify one wall. With these parameter freedoms, we find that for a certain subfamily the line systems acquire an N = 1 SUSY which can be enhanced to N = 4 if the parameters are further tuned, and that these SUSY are generically broken except for a special case. The interval systems, on the other hand, can accommodate N = 2 or N = 4 SUSY, broken or unbroken, and exhibit a rich variety of (degenerate) spectra. Our SUSY systems include the familiar SUSY systems with the Dirac $δ(x)$-potential, and hence are extensions of the known SUSY quantum mechanics to those with general point singularities and walls. The self-adjointness of the supercharge in relation to the self-adjointness of the Hamiltonian is also discussed.

hep-th↗

Supersymmetric Quantum Mechanics with a Point Singularity

We study the possibility of supersymmetry (SUSY) in quantum mechanics in one dimension under the presence of a point singularity. The system considered is the free particle on a line R or on the interval [-l, l] where the point singularity lies at x = 0. In one dimension, the singularity is known to admit a U(2) family of different connection conditions which include as a special case the familiar one that arises under the Dirac delta-potential. Similarly, each of the walls at x = l and x = -l admits a U(1) family of boundary conditions including the Dirichlet and the Neumann boundary conditions. Under these general connection/boundary conditions, the system is shown to possess an N = 1 or N = 2 SUSY for various choices of the singularity and the walls, and the SUSY is found to be `good' or `broken' depending on the choices made. We use the supercharge which allows for a constant shift in the energy, and argue that if the system is supersymmetric then the supercharge is self-adjoint on states that respect the connection/boundary conditions specified by the singularity.

quant-ph↗