arXiv subjects

Takatoshi Ichikawa

Publications and source records attributed to Takatoshi Ichikawa.

14 recordsLinked to original sources

arXiv2022

Optimization of basis functions for the multi-configuration mixing using the Replica Exchange Monte-Carlo method and its application to $^{12}$C

To calculate excited states in quantum many-body systems, multi-configuration mixing has often been employed. However, it has been still unclear how to choose important Slater determinants from a huge model space. We propose a novel efficient method as the Replica Exchange Monte-Carlo (RXMC) method to sample important Slater determinants and optimize and analyze the obtained results. As an application, we apply it to the ground and excited states of $^{12}$C based on the Bloch-Brink $α$ cluster model and show the detailed structure of the obtained states. The RXMC method enables us to efficiently sample Slater determinants following the Boltzmann distribution on the multi-dimensional potential energy surface (PES) under a given model space. To analyze the obtained excited states, we embed sampled basis functions onto the PES calculated with the $β$-$γ$ constraint method and discuss the main component in the state. The RXMC method can efficiently perform the samplings with a temperature parameter of $T_L=2.5$ MeV in $^{12}$C. We obtain the gas-like state with a wide density distribution in the tail part in the second $0^+$ state. We also obtain the linear-chain-like states with the bending and stretching vibrational modes in the third and fourth $0^+$ states, respectively. In the fifth $0^+$ state, the main component of the basis functions contains expanded equilateral triangle configurations. The second $0^+$ gas-like state emerges at the local minimum in the PES, which is the beginning of the valley structure connected to the linear-chain breakup channel. The third and fourth linear-chain-like states emerge in this valley structure. We conclude that the RXMC method is a powerful method to calculate the excited states of nuclei, which would be applied to much complicated nuclear fission dynamics in heavier nuclei.

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arXiv2018

Nascent fragment shell effects on the nuclear fission processes in semiclassical periodic orbit theory

Making use of the semiclassical periodic orbit theory (POT), we propose, for the first time, a method to exclusively evaluate the shell effects associated with each of the nascent fragments (prefragments) generated by the neck formation in nuclear fission processes. In spite of the strong indication of such shell effects in asymmetric fragment mass distributions, they could not have been accessed by any previous theoretical approach since most of the single-particle wave functions are delocalized. In the POT, we have found that the prefragment shell effects can be naturally and unambiguously identified as the ontributions of the classical periodic orbits localized in each of the prefragments. For a numerical test, simple cavity potential models are employed with the shape described by the three-quadratic-surface shape parametrization. Deformed shell energies are studied with the trace formula for degenerate orbits in a runcated spherical cavity which was recently derived [K. Arita, Phys. Rev. C 98, 064310 (2018)]. In this simple model, it is shown that the prefragment shell effect dominates the total shell energy shortly after the neck formation, and the magicity of the heavier prefragment plays a significant role in establishing the fission saddle with asymmetric shape which leads to an asymmetric scission.

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arXiv2015

Systematic investigations of deep sub-barrier fusion reactions using an adiabatic approach

To describe fusion hindrance observed in fusion reactions at extremely low incident energies, I propose a novel extension of the standard CC model by introducing a damping factor that describes a smooth transition from sudden to adiabatic processes. I demonstrate the performance of this model by systematically investigating various deep sub-barrier fusion reactions. I extend the standard CC model by introducing a damping factor into the coupling matrix elements in the standard CC model. I adopt the Yukawa-plus-exponential (YPE) model as a basic heavy ion-ion potential, which is advantageous for a unified description of the one- and two-body potentials. For the purpose of these systematic investigations, I approximate the one-body potential with a third-order polynomial function based on the YPE model. Calculated fusion cross sections for the medium-heavy mass systems of $^{64}$Ni + $^{64}$Ni, $^{58}$Ni + $^{58}$Ni, and $^{58}$Ni + $^{54}$Fe, the medium-light mass systems of $^{40}$Ca + $^{40}$Ca, $^{48}$Ca + $^{48}$Ca, and $^{24}$Mg + $^{30}$Si, and the mass-asymmetric systems of $^{48}$Ca + $^{96}$Zr and $^{16}$O + $^{208}$Pb are consistent with the experimental data. The astrophysical S factor and logarithmic derivative representations of these are also in good agreement with the experimental data. Since the results calculated with the damping factor are in excellent agreement with the experimental data in all systems, I conclude that the smooth transition from the sudden to adiabatic processes occurs and that a coordinate-dependent coupling strength is responsible for the fusion hindrance. In all systems, the potential energies at the touching point $V_{\rm Touch}$ strongly correlate with the incident threshold energies for which the fusion hindrance starts to emerge, except for the medium-light mass systems.

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arXiv2015

Examination of the stability of a rod-shaped structure in $^{24}$Mg

The stable existence of a six-$α$ linear structure in highly excited states of $^{24}$Mg is studied based on a systematic Cranked Hartree-Fock calculation with various Skyrme-type interactions. Its stability is examined by allowing the transition of the cluster structure to the shell-model like structure. Especially, the six-$α$ linear state is exposed to two major instabilities: the bending motion, which is the main path for the transition to low-lying states, and the spin-orbit interaction, which is the driving force to break the $α$ clusters and enhance the independent motion of the nucleons. The linear structure with large angular momentum is obtained as a meta-stable stationary state.

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arXiv2015

A Universal Damping Mechanism of Quantum Vibrations in Deep Sub-Barrier Fusion Reactions

We demonstrate the damping of quantum octupole vibrations near the touching point when two colliding nuclei approach each other in the mass-asymmetric $^{208}$Pb + $^{16}$O system, for which the strong fusion hindrance was clearly observed. We, for the first time, apply the random-phase approximation method to the heavy-mass asymmetric di-nuclear system to calculate the transition strength $B$(E3) as a function of the center-of-mass distance. The obtained $B$(E3) strengths are substantially damped near the touching point, because the single-particle wave functions of the two nuclei strongly mix with each other and a neck is formed. The energy-weighted sums of $B$(E3) are also strongly correlated with the damping factor which is phenomenologically introduced in the standard coupled-channel calculations to reproduce the fusion hindrance. This strongly indicates that the damping of the quantum vibrations universally occurs in the deep sub-barrier fusion reactions.

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arXiv2013

Damping of Quantum Vibrations Revealed in Deep Sub-barrier Fusion

We demonstrate that when two colliding nuclei approach each other, their quantum vibrations are damped near the touching point. We show that this damping is responsible for the fusion hindrance phenomena measured in the deep sub-barrier fusion reactions. To show those, we for the first time apply the random-phase-approximation (RPA) method to the two-body $^{16}$O + $^{16}$O and $^{40}$Ca + $^{40}$Ca systems. We calculate the octupole transition strengths for the two nuclei adiabatically approaching each other. The calculated transition strength drastically decreases near the touching point, strongly suggesting the vanishing of the quantum couplings between the relative motion and the vibrational intrinsic degrees of freedom of each nucleus. Based on this picture, we also calculate the fusion cross section for the $^{40}$Ca + $^{40}$Ca system using the coupled-channel method with the damping factor simulating the vanishing of the couplings. The calculated results reproduce well the experimental data, indicating that the smooth transition from the sudden to adiabatic processes indeed occurs in the deep sub-barrier fusion reactions.

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arXiv2013

The character and prevalence of third minima in actinide fission barriers

The double-humped structure of many actinide fission barriers is well established both experimentally and theoretically. There is also evidence, both experimental and theoretical, that some actinide nuclei have barriers with a third minimum, outside the second, fission-isomeric minimum. We perform a large-scale, systematic calculation of actinide fission barriers to identify which actinide nuclei exhibit third minima. We find that only a relatively few nuclei accessible to experiment exhibit third minima in their barriers, approximately nuclei with proton number $Z$ in the range $88 \leq Z \leq 94$ and nucleon number $A$ in the range $230 \leq A \leq 236 $. We find that the third minimum is less than 1 MeV deep for light Th and U isotopes. This is consistent with some previous experimental and theoretical results, but differs from some others. We discuss possible origins of these incompatible results and what are the most realistic predictions of where third minima are observable.

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arXiv2012

The contrasting fission potential-energy structure of actinides and mercury isotopes

Fission-fragment mass distributions are asymmetric in fission of typical actinide nuclei for nucleon number $A$ in the range $228 \lnsim A \lnsim 258$ and proton number $Z$ in the range $90\lnsim Z \lnsim 100$. For somewhat lighter systems it has been observed that fission mass distributions are usually symmetric. However, a recent experiment showed that fission of $^{180}$Hg following electron capture on $^{180}$Tl is asymmetric. We calculate potential-energy surfaces for a typical actinide nucleus and for 12 even isotopes in the range $^{178}$Hg--$^{200}$Hg, to investigate the similarities and differences of actinide compared to mercury potential surfaces and to what extent fission-fragment properties, in particular shell structure, relate to the structure of the static potential-energy surfaces. Potential-energy surfaces are calculated in the macroscopic-microscopic approach as functions of fiveshape coordinates for more than five million shapes. The structure of the surfaces are investigated by use of an immersion technique. We determine properties of minima, saddle points, valleys, and ridges between valleys in the 5D shape-coordinate space. Along the mercury isotope chain the barrier heights and the ridge heights and persistence with elongation vary significantly and show no obvious connection to possible fragment shell structure, in contrast to the actinide region, where there is a deep asymmetric valley extending from the saddle point to scission. The mechanism of asymmetric fission must be very different in the lighter proton-rich mercury isotopes compared to the actinide region and is apparently unrelated to fragment shell structure. Isotopes lighter than $^{192}$Hg have the saddle point blocked from a deep symmetric valley by a significant ridge. The ridge vanishes for the heavier Hg isotopes, for which we would expect a qualitatively different asymmetry of the fragments.

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arXiv2011

Cluster formations in deformed states for $^{28}$Si and $^{32}$S

We study cluster formation in strongly deformed states for $^{28}$Si and $^{32}$S using a macroscopic-microscopic model. The study is based on calculated total-energy surfaces, which are the sums of deformation-dependent macroscopic-microscopic potential-energy surfaces and rotational-energy contributions. We analyze the angular-momentum-dependent total-energy surfaces and identify the normal- and super-deformed states in $^{28}$Si and $^{32}$S, respectively. We show that at sufficiently high angular momenta strongly deformed minima appear. The corresponding microscopic density distributions show cluster structure that closely resemble the $^{16}$O+$^{12}$C and $^{16}$O+$^{16}$O configurations. At still higher deformations, beyond the minima, valleys develop in the calculated surfaces. These valleys lead to mass divisions that correspond to the target-projectile configurations for which molecular resonance states have been observed. We discuss the relation between the one-body deformed minima and the two-body molecular-resonance states.

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arXiv2010

Calculations of Branching Ratios for Radiative-Capture, One-Proton, and Two-Neutron Channels in the Fusion Reaction $^{209}$Bi+$^{70}$Zn

We discuss the possibility of the non-one-neutron emission channels in the cold fusion reaction $^{70}$Zn + $^{209}$Bi to produce the element Z=113. For this purpose, we calculate the evaporation-residue cross sections of one-proton, radiative-capture, and two-neutron emissions relative to the one-neutron emission in the reaction $^{70}$Zn + $^{209}$Bi. To estimate the upper bounds of those quantities, we vary model parameters in the calculations, such as the level-density parameter and the height of the fission barrier. We conclude that the highest possibility is for the 2n reaction channel, and its upper bounds are 2.4$%$ and at most less than 7.9% with unrealistic parameter values, under the actual experimental conditions of [J. Phys. Soc. Jpn. {\bf 73} (2004) 2593].

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arXiv2009

Signature of smooth transition from diabatic to adiabatic states in heavy-ion fusion reactions at deep subbarrier energies

We propose a novel extension of the standard coupled-channels framework for heavy-ion reactions in order to analyze fusion reactions at deep subbarrier incident energies. This extension simulates a smooth transition between the diabatic two-body and the adiabatic one-body states. To this end, we damp gradually the off-diagonal part of the coupling potential, for which the position of the onset of the damping varies for each eigen channel. We show that this model accounts well for the steep falloff of the fusion cross sections for the $^{16}$O+$^{208}$Pb, $^{64}$Ni+$^{64}$Ni, and $^{58}$Ni+$^{58}$Ni reactions.

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arXiv2008

Origin of the narrow, single peak in the fission-fragment mass distribution for $^{258}$Fm

We discuss the origin of the narrowness of the single peak at mass-symmetric division in the fragment mass-yield curve for spontaneous fission of $^{258}$Fm. For this purpose, we employ the macroscopic-microscopic model, and calculate a potential-energy curve at the mass-symmetric compact scission configuration, as a function of the fragment mass number, which is obtained from the single-particle wave-function densities. In the calculations, we minimize total energies by varying the deformations of the two fragments, with constraints on the mass quadrupole moment and keeping the neck radius zero, as a function of mass asymmetry. Using the obtained potential, we solve the one-dimensional Schrödinger equation with a microscopic coordinate-dependent inertial mass to calculate the fragment mass-yield curve. The calculated mass yield, expressed in terms of the microscopic mass density, is consistent with the extremely narrow experimental mass distribution.

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arXiv2007

Existence of One-Body Barrier Revealed in Deep Sub-Barrier Fusion

Based on the adiabatic picture for heavy-ion reactions, in which the neck formation in the one-body system is taken into account, we propose a two-step model for fusion cross sections at deep subbarrier energies. This model consists of the capture process in the two-body potential pocket, which is followed by the penetration of the adiabatic one-body potential to reach a compound state after the touching configuration. We describe the former process with the coupled-channels framework, while the latter with the WKB approximation by taking into account the coordinate dependent inertia mass. The effect of the one-body barrier is important at incident energies below the potential energy at the touching configuration. We show that this model well accounts for the steep fall-off phenomenon of fusion cross sections at deep subbarrier energies for the $^{64}$Ni+$^{64}$Ni and $^{58}$Ni+$^{58}$Ni reactions.

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arXiv2007

Systematics of threshold incident energy for deep sub-barrier fusion hindrance

We systematically evaluate the potential energy at the touching configuration for heavy-ion reactions using various potential models. We point out that the energy at the touching point, especially that estimated with the Krappe-Nix-Sierk (KNS) potential, strongly correlates with the threshold incident energy for steep fall-off of fusion cross sections observed recently for several systems at extremely low energies. This clearly indicates that the steep fall-off phenomenon can be attributed to the dynamics after the target and projectile touch with each other, e.g., the tunneling process and the nuclear saturation property in the overlap region.

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