arXiv subjects

Takeshi Kondo

Publications and source records attributed to Takeshi Kondo.

At least 37 records · Page 2Linked to original sources

arXiv2023

Spin-polarized saddle points in the topological surface states of the elemental Bismuth revealed by a pump-probe spin-resolved ARPES

We use a pump-probe, spin-, and angle-resolved photoemission spectroscopy (ARPES) with a 10.7 eV laser accessible up to the Brillouin zone edge, and reveal for the first time the entire band structure, including the unoccupied side, for the elemental bismuth (Bi) with the spin-polarized surface states. Our data identify Bi as in a strong topological insulator phase ($Z_2$=1) against the prediction of most band calculations. We unveil that the unoccupied topological surface states possess spin-polarized saddle points yielding the van Hove singularity, providing an excellent platform for the future development of opto-spintronics.

cond-mat.mtrl-sci↗

arXiv2023

Testing Electron-phonon Coupling for the Superconductivity in Kagome Metal $\rm{CsV_3Sb_5}$

In crystalline materials, electron-phonon coupling (EPC) is a ubiquitous many-body interaction that drives conventional Bardeen-Cooper-Schrieffer superconductivity. Recently, in a new kagome metal $\rm{CsV_3Sb_5}$, superconductivity that possibly intertwines with time-reversal and spatial symmetry-breaking orders is observed. Density functional theory calculations predicted weak EPC strength,$λ$, supporting an unconventional pairing mechanism in $\rm{CsV_3Sb_5}$. However, experimental determination of $λ$ is still missing, hindering a microscopic understanding of the intertwined ground state of $\rm{CsV_3Sb_5}$. Here, using 7-eV laser-based angle-resolved photoemission spectroscopy and Eliashberg function analysis, we determine an intermediate $λ$=0.45~0.6 at T=6 K for both Sb 5p and V 3d electronic bands, which can support a conventional superconducting transition temperature on the same magnitude of experimental value in $\rm{CsV_3Sb_5}$. Remarkably, the EPC on the V 3d-band enhances to $λ$~0.75 as the superconducting transition temperature elevated to 4.4 K in $\rm{Cs(V_{0.93}Nb_{0.07})_3Sb_5}$. Our results provide an important clue to understand the pairing mechanism in the Kagome superconductor $\rm{CsV_3Sb_5}$.

cond-mat.supr-con↗

arXiv2023

Frequency-multiplexed storage and distribution of narrowband telecom photon pairs over a 10-km fiber link with long-term system stability

The ability to transmit quantum states over long distances is a fundamental requirement of the quantum internet and is reliant upon quantum repeaters. Quantum repeaters involve entangled photon sources that emit and deliver photonic entangled states at high rates and quantum memories that can temporarily store quantum states. Improvement of the entanglement distribution rate is essential for quantum repeaters, and multiplexing is expected to be a breakthrough. However, limited studies exist on multiplexed photon sources and their coupling with a multiplexed quantum memory. Here, we demonstrate the storing of a frequency-multiplexed two-photon source at telecommunication wavelengths in a quantum memory accepting visible wavelengths via wavelength conversion after 10-km distribution. To achieve this, quantum systems are connected via wavelength conversion with a frequency stabilization system and a noise reduction system. The developed system was stably operated for more than 42 h. Therefore, it can be applied to quantum repeater systems comprising various physical systems requiring long-term system stability.

quant-ph↗

arXiv2023

Nodeless electron pairing in CsV$_3$Sb$_5$-derived kagome superconductors

The newly discovered kagome superconductors represent a promising platform for investigating the interplay between band topology, electronic order, and lattice geometry. Despite extensive research efforts on this system, the nature of the superconducting ground state remains elusive. In particular, consensus on the electron pairing symmetry has not been achieved so far, in part owing to the lack of a momentum-resolved measurement of the superconducting gap structure. Here we report the direct observation of a nodeless, nearly isotropic, and orbital-independent superconducting gap in the momentum space of two exemplary CsV$_3$Sb$_5$-derived kagome superconductors -- Cs(V$_{0.93}$Nb$_{0.07}$)$_3$Sb$_5$ and Cs(V$_{0.86}$Ta$_{0.14}$)$_3$Sb$_5$, using ultrahigh resolution and low-temperature angle-resolved photoemission spectroscopy (ARPES). Remarkably, such a gap structure is robust to the appearance or absence of charge order in the normal state, tuned by isovalent Nb/Ta substitutions of V. Moreover, we observe a signature of the time-reversal symmetry (TRS) breaking inside the superconducting state, which extends the previous observation of TRS-breaking CDW in the kagome lattice. Our comprehensive characterizations of the superconducting state provide indispensable information on the electron pairing of kagome superconductors, and advance our understanding of unconventional superconductivity and intertwined electronic orders.

cond-mat.supr-con↗

arXiv2023

A robust weak topological insulator in a bismuth halide Bi4Br2I2

We apply a topological material design concept for selecting a bulk topology of 3D crystals by different van-der-Waals stacking of 2D topological insulator layers, and find a bismuth halide Bi4Br2I2 to be an ideal weak topological insulator (WTI) with the largest band gap (~230 meV) among all the WTI candidates, by means of angle-resolved photoemission spectroscopy (ARPES), density functional theory (DFT) calculations, and resistivity measurements. Our results vastly expand future opportunities for fundamental research and device applications with a robust WTI.

cond-mat.mtrl-sci↗

arXiv2022

Direct observation of topological surface state in the topological superconductor 2M-WS2

The quantum spin Hall (QSH) effect has attracted extensive research interest because of the potential applications in spintronics and quantum computing, which is attributable to two conducting edge channels with opposite spin polarization and the quantized electronic conductance of 2e2/h. Recently, 2M-WS2, a new stable phase of transition metal dichalcogenides with a 2M structure showing an identical layer configuration to that of the monolayer 1T' TMDs, was suggested to be a QSH insulator as well as a superconductor with critical transition temperature around 8 K. Here, high-resolution angle-resolved photoemission spectroscopy (ARPES) and spin-resolved ARPES are applied to investigate the electronic and spin structure of the topological surface states (TSS) in the superconducting 2M-WS2. The TSS exhibits characteristic spin-momentum-locking behavior, suggesting the existence of long-sought nontrivial Z2 topological states therein. We expect that 2M-WS2 with co-existing superconductivity and TSS might host the promising Majorana bound states.

cond-mat.supr-con↗

arXiv2022

Tunable vortex Majorana modes controlled by strain in homogeneous LiFeAs

The iron-based superconductors (FeSCs) have recently emerged as a promising single-material Majorana platform by hosting isolated Majorana zero modes (MZMs) at relatively high temperatures. To further verify its Majorana nature and move forward to build topological quantum qubit, it is highly desirable to achieve tunability for MZMs on homogeneous FeSCs. Here, with an in-situ strain device, we can controllably create MZMs on the homogeneous surface of stoichiometric superconductor LiFeAs by inducing a topological phase transition. The evolution of discrete energy modes inside a strained vortex is found to mimics exactly as the predicted topological vortex case, proving the Majorana nature of emerging zero modes of vortex. Such tunability of MZMs in a homogeneous superconductor is an important step toward their application in topological quantum computation.

cond-mat.supr-con↗

arXiv2022

Single-shot high-resolution identification of discrete frequency modes of single-photon-level optical pulses

Frequency-multiplexed quantum communication usually requires a single-shot identification of the frequency mode of a single photon . In this paper, we propose a scheme that can identify the frequency mode with high-resolution even for spontaneously emitted photons whose generation time is unknown, by combining the time-to-space and frequency-to-time mode mapping. We also demonstrate the mapping of the frequency mode (100 MHz intervals) to the temporal mode (435 ns intervals) for weak coherent pulses using atomic frequency combs. This frequency interval is close to the minimum frequency mode interval of the atomic frequency comb quantum memory with Pr3+ ion-doped Y2SiO5 crystal, and the proposed scheme has the potential to maximize the frequency multiplexing of the quantum repeater scheme with the memory.

quant-ph↗

arXiv2022

Angle-resolved photoemission spectroscopy

For solid-state materials, the electronic structure, E(k), is critical in determining a crystal's physical properties. By experimentally detecting the electronic structure, the fundamental physics can be revealed. Angle-resolved photoemission spectroscopy (ARPES) is a powerful technique for directly observing the electronic structure with energy- and momentum-resolved information. Over the past decades, major improvements in the energy and momentum resolution, alongside the extension of ARPES observables to spin (SpinARPES), micrometer or nanometer lateral dimensions (MicroARPES/NanoARPES), and femtosecond timescales (TrARPES), have led to major scientific advances. These advantages have been achieved across a wide range of quantum materials, such as high-temperature superconductors, topological materials, two-dimensional materials and heterostructures. This primer introduces key aspects of ARPES principles, instrumentation, data analysis, and representative scientific cases to demonstrate the power of the method. Perspectives and challenges on future developments are also discussed.

cond-mat.mtrl-sci↗

arXiv2022

Puddle formation, persistent gaps, and non-mean-field breakdown of superconductivity in overdoped (Pb,Bi)2Sr2CuO6+δ

The cuprate high-temperature superconductors exhibit many unexplained electronic phases, but it was often thought that the superconductivity at sufficiently high doping is governed by conventional mean-field Bardeen-Cooper-Schrieffer (BCS) theory[1]. However, recent measurements show that the number of paired electrons (the superfluid density) vanishes when the transition temperature Tc goes to zero[2], in contradiction to expectation from BCS theory. The origin of this anomalous vanishing is unknown. Our scanning tunneling spectroscopy measurements in the overdoped regime of the (Pb,Bi)2Sr2CuO6+δ high-temperature superconductor show that it is due to the emergence of puddled superconductivity, featuring nanoscale superconducting islands in a metallic matrix[3,4]. Our measurements further reveal that this puddling is driven by gap filling, while the gap itself persists beyond the breakdown of superconductivity. The important implication is that it is not a diminishing pairing interaction that causes the breakdown of superconductivity. Unexpectedly, the measured gap-to-filling correlation also reveals that pair-breaking by disorder does not play a dominant role and that the mechanism of superconductivity in overdoped cuprate superconductors is qualitatively different from conventional mean-field theory.

cond-mat.supr-con↗

arXiv2022

Strange metal dynamics across the phase diagram of Bi$_{2}$Sr$_{2}$CuO$_{6+δ}$ cuprates

Unlocking the mystery of the strange metal state has become the focal point of high T$_{c}$ research, not because of its importance for superconductivity, but because it appears to represent a truly novel phase of matter dubbed `quantum supreme matter'. Detected originally through high magnetic field, transport experiments, signatures of this phase have now been uncovered with a variety of probes. Our high resolution optical data of the low T$_{c}$ cuprate superconductor, Bi$_{2-x}$Pb$_{x}$Sr$_{2-y}$La$_{y}$CuO$_{6+δ}$ allows us to probe this phase over a large energy and temperature window. We demonstrate that the optical signatures of the strange metal phase persist throughout the phase diagram. The strange metal signatures in the optical conductivity are two-fold, (i): a low energy Drude response with Drude width on the order of temperature and (ii): a high energy conformal tail with doping dependent power-law exponent. While the Drude weight evolves monotonously throughout the entire doping range studied, the spectral weight contained in the high energy conformal tail appears to be doping and temperature independent. Our analysis further shows that the temperature dependence of the optical conductivity is completely determined by the Drude parameters. Our results indicate that there is no critical doping level inside the superconducting dome where the carrier density starts to change drastically and that the previously observed 'return to normalcy' is a consequence of the increasing importance of the Drude component relative to the conformal tail with doping. Importantly, both the doping and temperature dependence of the resistivity are largely determined by the Drude width.

cond-mat.str-el↗

arXiv2022

Multipole polaron in the devil's staircase of CeSb

Rare-earth intermetallic compounds exhibit rich phenomena induced by the interplay between localized $f$ orbitals and conduction electrons. However, since the energy scale of the crystal-electric-field splitting is only a few millielectronvolts, the nature of the mobile electrons accompanied by collective crystal-electric-field excitations has not been unveiled. Here, we examine the low-energy electronic structures of CeSb through the anomalous magnetostructural transitions below the N$é$el temperature, $\sim$17 K, termed the 'devil's staircase', using laser angle-resolved photoemission, Raman and neutron scattering spectroscopies. We report another type of electron-boson coupling between mobile electrons and quadrupole crystal-electric-field excitations of the 4$f$ orbitals, which renormalizes the Sb 5$p$ band prominently, yielding a kink at a very low energy ($\sim$7 meV). This coupling strength is strong and exhibits anomalous step-like enhancement during the devil's staircase transition, unveiling a new type of quasiparticle, named the 'multipole polaron', comprising a mobile electron dressed with a cloud of the quadrupole crystal-electric-field polarization.

cond-mat.mtrl-sci↗

arXiv2022

Large anomalous Hall effect induced by weak ferromagnetism in the noncentrosymmetric antiferromagnet $\mathrm{Co}\mathrm{Nb}_3\mathrm{S}_6$

We study the mechanism of the exceptionally large anomalous Hall effect (AHE) in the noncentrosymmetric antiferromagnet $\mathrm{Co}\mathrm{Nb}_3\mathrm{S}_6$ by angle-resolved photoemission spectroscopy (ARPES) and magnetotransport measurements. From ARPES measurements of $\mathrm{Co}\mathrm{Nb}_3\mathrm{S}_6$ and its family compounds ($\mathrm{Fe}\mathrm{Nb}_3\mathrm{S}_6$ and $\mathrm{Ni}\mathrm{Nb}_3\mathrm{S}_6$), we find a band dispersion unique to the Co intercalation existing near the Fermi level. We further demonstrate that a slight deficiency of sulfur in $\mathrm{Co}\mathrm{Nb}_3\mathrm{S}_6$ eliminates the ferromagnetism and the AHE simultaneously while hardly changing the band structure, indicating that the weak ferromagnetism is responsible for the emergence of the large AHE. Based on our results, we propose Weyl points near the Fermi level to cause the large AHE.

cond-mat.mtrl-sci↗

arXiv2021

Coupling of a quantum memory and telecommunication wavelength photons for high-rate entanglement distribution in quantum repeaters

Quantum repeaters are indispensable tools for long-distance quantum communication. However, frequency matching between entangled photon sources and remote quantum memories (QMs) is difficult, which is an obstacle to the implementation of quantum repeaters. In this paper, we demonstrate a method to achieve the coupling of a Pr:YSO as a fixed-time QM with a single telecommunication-wavelength photon through frequency stabilization using an optical frequency comb over all applied laser wavelengths. The demonstrated method can lead to the implementation of a quantum repeater scheme enabling an improvement of the entanglement generation rate, paving the way for long-distance quantum communication.

quant-ph↗

arXiv2021

Selective observation of surface and bulk bands in polar WTe2 by laser-based spin- and angle-resolved photoemission spectroscopy

The electronic state of WTe2, a candidate of type-II Weyl semimetal, is investigated by using laser-based spin- and angle-resolved photoemission spectroscopy (SARPES). We prepare the pair of WTe2 samples, one with (001) surface and the other with (00-1) surface, by "sandwich method", and measure the band structures of each surface separately. The Fermi arcs are observed on both surfaces. We identify that the Fermi arcs on the two surfaces are both originating from surface states. We further find a surface resonance band, which connects with the Fermi-arc band, forming a Dirac-cone-like band dispersion. Our results indicate that the bulk electron and hole bands are much closer in momentum space than band calculations.

cond-mat.mtrl-sci↗

arXiv2021

Offset-locking-based frequency stabilization of external cavity diode lasers for long-distance quantum communication

Quantum repeaters are required for long-distance quantum communication. For efficient coupling of quantum entangled photon sources with narrow-linewidth quantum memories we performed the frequency stabilization of two lasers at 1514 and 1010 nm. The 1514 nm pump laser of the entangled photon source exhibited a frequency stability of 3.6 \times 10^{-12} (τ= 1 s). The 1010 nm pump laser of the wavelength conversion system exhibited a frequency stability of 3.4 \times 10^{-12} (τ= 1 s). The stabilities of both lasers were approximately two orders of magnitude smaller than the frequency width of 4 MHz of the Pr:YSO quantum memory. Such frequency-stabilized lasers can realize the remote coupling of a quantum memory and an entangled photon source in quantum repeaters.

quant-ph↗

arXiv2021

Visualization of the strain-induced topological phase transition in a quasi-one-dimensional superconductor TaSe3

Control of the phase transition from topological to normal insulators can allow for an on/off switching of spin current. While topological phase transitions have been realized by elemental substitution in semiconducting alloys, such an approach requires the preparation of materials with various compositions, thus it is quite far from a feasible device application, which demands a reversible operation. Here we use angle-resolved photoemission spectroscopy (ARPES) and spin-resolved ARPES to visualize the strain-driven band structure evolution of the quasi-1D superconductor TaSe3. We demonstrate that it undergoes reversible strain-induced topological phase transitions from a strong topological insulator phase with spin-polarized, quasi-1D topological surface states, to topologically trivial semimetal and band insulating phases. The quasi-1D superconductor TaSe3 provides a suitable platform for engineering the topological spintronics, for example as an on/off switch for spin current robust against impurity scattering.

cond-mat.mtrl-sci↗

arXiv2021

Visualization of optical polarization transfer to photoelectron spin vector emitted from the spin-orbit coupled surface state

Similar to light polarization that is selected by a superposition of optical basis, electron spin direction can be controlled through a superposition of spin basis. We investigate such a spin interference occurring in photoemission of the spin-orbit coupled surface state in Bi2Se3 by using spin- and angle-resolved photoemission spectroscopy combined with laser light source (laser-SARPES). Our laser-SARPES with three-dimensional spin detection and tunable laser polarization including elliptical and circular polarization enables us to directly visualize how the direction of the fully-polarized photoelectron spin changes according to the optical phase and orientation of the incident laser polarization. By this advantage of our laser-SARPES, we demonstrate that such optical information can be projected to the three-dimensional spin vector of the photoelectrons. Our results, therefore, present a novel spin-polarized electron source permitting us to optically control the pure spin state pointing to the arbitrary direction.

cond-mat.mtrl-sci↗