arXiv subjects

Takuya Isogawa

Publications and source records attributed to Takuya Isogawa.

9 recordsLinked to original sources

arXiv2026

Agentic AI for Scientific Reasoning in Autonomous Quantum Sensing Experiments

We implement an agentic AI workflow built around a large language model (LLM) agent for autonomous experiments with nitrogen-vacancy (NV) centers in diamond. NV centers are a widely used platform for quantum sensing, and the ability to control many measurements from a computer makes NV experiments a natural setting for autonomous workflows. We make two main contributions. First, we demonstrate an autonomous NV experiment workflow that combines persistent project records, quantitative calculation and data analysis tools, and deterministic experiment control. In one autonomous experiment, the agent selected a single NV center, calibrated its resonant frequency, measured \(T_2^\ast\) with Ramsey measurements, and added a Carr--Purcell--Meiboom--Gill (CPMG) measurement to check a weak feature that could be related to nearby \(^{13}\mathrm{C}\). Second, we introduce two offline benchmarks that evaluate the agent's reasoning separately from laboratory execution. We evaluated both benchmarks with GPT-5.4, GPT-5.5, and GPT-5.6 Sol. In the Ramsey checkpoint benchmark, greater reasoning effort generally improved recognition of a residual resonance calibration offset. By contrast, in the pulsed optically detected magnetic resonance (pODMR) data evaluation benchmark, pulse sequence information alone produced more false positive resonance judgments at higher reasoning effort. Requiring an expected signal calculation kept false positive rates low across all three models and reasoning settings. The results suggest a clear division of labor for autonomous experiments. The agent forms scientific hypotheses and uses quantitative tools to evaluate data, while deterministic code controls the hardware and enforces safety constraints.

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arXiv2026

Approaching the Limit in Multiparameter AC Magnetometry with Quantum Control

Simultaneously estimating multiple parameters at the ultimate limit is a central challenge in quantum metrology, often hindered by inherent incompatibilities in optimal estimation strategies. At its most extreme, this incompatibility culminates in a fundamental impossibility when the quantum Fisher information matrix (QFIM) becomes singular, rendering joint estimation unattainable. This is the case for a canonical problem: estimating the amplitude and frequency of an AC magnetic field, where the generators are parallel to each other. Here, we introduce a quantum control protocol that resolves this singularity. Our control protocol strategically engineers the sensor's time evolution so the generators for the two parameters become orthogonal. It not only removes the singularity but also restores the optimal scaling of precision with interrogation time for both parameters simultaneously. We experimentally validate this protocol using a nitrogen-vacancy center in diamond at room temperature, demonstrating the concurrent achievement of the optimal scaling for both parameters under realistic conditions.

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arXiv2025

Optimal Control of Coupled Sensor-Ancilla Qubits for Multiparameter Estimation

Designing optimal control for multiparameter quantum sensing is essential for approaching the ultimate precision limits. However, analytical solutions are generally available only for simple systems, while realistic scenarios often involve coupled qubits and time-dependent Hamiltonians. Here we numerically investigate optimal control of a two-qubit sensor-ancilla system coupled via an Ising term using Gradient Ascent Pulse Engineering (GRAPE) to minimize the objective function. By seeding the optimization recursively with solutions obtained for smaller coupling strengths and selecting a suitable initial guess, we achieve robust convergence and high precision across a wide range of interaction strengths and field configurations. The proposed approach offers a practical route toward high-sensitivity, robust multiparameter magnetometry and it is applicable to solid-state quantum sensors such as nitrogen-vacancy (NV) centers in realistic experimental settings.

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arXiv2025

Entanglement-assisted multiparameter estimation with a solid-state quantum sensor

Quantum multiparameter estimation promises to extend quantum advantage to the simultaneous high-precision measurements of multiple physical quantities. However, realizing this capability in practical quantum sensors under realistic conditions remains challenging due to intrinsic system imperfections. Here, we experimentally demonstrate multiparameter estimation using a nitrogen-vacancy (NV) center in diamond, a widely adopted solid-state quantum sensor. Leveraging electronic-nuclear spin entanglement and optimized Bell state measurement at room temperature, we simultaneously estimate the amplitude, detuning, and phase of a microwave drive from a single measurement sequence. Despite practical constraints, our results achieve linear sensitivity scaling for all parameters with respect to interrogation time. This work bridges the gap between foundational quantum estimation theory and real-world quantum sensing, opening pathways toward enhanced multiparameter quantum sensors suitable for diverse scientific and technological applications.

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arXiv2024

Control incompatibility in multiparameter quantum metrology

In practical applications like quantum sensing and quantum imaging, there is often a necessity to estimate multiple parameters simultaneously. Although the ultimate precision limits for single-parameter estimation are well established, the precision limit of multi-parameter estimation is much less understood. This is primarily due to the inherent incompatibility of the optimal strategies for the estimation of different parameters, particularly those pertaining to optimal control.In this study, we tackle the critical issue of control incompatibility in multi-parameter estimation by presenting explicit cases that expose this challenge. Our research not only pioneers the exploration of control incompatibility but also highlights its pivotal role in the field. Furthermore, our work offers valuable insights into how to minimize trade-offs induced by control incompatibility and enhance precision. This paves the way for future investigations into control strategies that enable optimal estimation of multiple parameters that are incompatible.

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arXiv2024

Optimal Quantum Purity Amplification

Quantum purity amplification (QPA) provides a novel approach to counteracting the pervasive noise that degrades quantum states. We present the optimal QPA protocol for general quantum systems and global noise, resolving a two-decade open problem. Under strong depolarization, our protocol achieves an exponential reduction in sample complexity over the best-known methods. We provide an efficient implementation of the protocol based on generalized quantum phase estimation. Additionally, we introduce SWAPNET, a sparse and shallow circuit that enables QPA for near-term experiments. Simulations in both digital and analog quantum settings, along with experiments on superconducting quantum processors, confirm the protocol's robustness and practical utility. Our findings suggest that QPA could improve the performance of quantum information processing tasks, particularly in the context of Noisy Intermediate-Scale Quantum (NISQ) devices, where reducing the effect of noise with limited resources is critical.

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arXiv2024

Interferometry of quantum correlation functions to access quasiprobability distribution of work

The Kirkwood-Dirac quasiprobability distribution, intimately connected with the quantum correlation function of two observables measured at distinct times, is becoming increasingly relevant for fundamental physics and quantum technologies. This quasiprobability distribution can take non-positive values, and its experimental reconstruction becomes challenging when expectation values of incompatible observables are involved. Here, we use an interferometric scheme aided by an auxiliary system to reconstruct the Kirkwood-Dirac quasiprobability distribution. We experimentally demonstrate this scheme in an electron-nuclear spin system associated with a nitrogen-vacancy center in diamond. By measuring the characteristic function, we reconstruct the quasiprobability distribution of work and analyze the behavior of its first and second moments. Our results clarify the physical meaning of the work quasiprobability distribution in the context of quantum thermodynamics. Finally, we study the uncertainty of measuring the Hamiltonian of the system at two times, via the Robertson-Schr{\"o}dinger uncertainty relation, for different initial states.

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arXiv2023

A many-body singlet prepared by a central spin qubit

Controllable quantum many-body systems are platforms for fundamental investigations into the nature of entanglement and promise to deliver computational speed-up for a broad class of algorithms and simulations. In particular, engineering entanglement within a dense spin ensemble can turn it into a robust quantum memory or a computational platform. Recent experimental progress in dense central spin systems motivates the design of algorithms that use a central-spin qubit as a convenient proxy for the ensemble. Here we propose a protocol that uses a central spin to initialize two dense spin ensembles into a pure anti-polarized state and from there creates a many-body entangled state -- a singlet -- from the combined ensemble. We quantify the protocol performance for multiple material platforms and show that it can be implemented even in the presence of realistic levels of decoherence. Our protocol introduces an algorithmic approach to preparation of a known many-body state and to entanglement engineering in a dense spin ensemble, which can be extended towards a broad class of collective quantum states.

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arXiv2021

Vector DC magnetic-field sensing with reference microwave field using perfectly aligned nitrogen-vacancy centers in diamond

The measurement of vector magnetic fields with high sensitivity and spatial resolution is important for both fundamental science and engineering applications. In particular, magnetic-field sensing with nitrogen-vacancy (NV) centers in diamond is a promising approach that can outperform existing methods. Recent studies have demonstrated vector DC magnetic-field sensing with perfectly aligned NV centers, which showed a higher readout contrast than NV centers having four equally distributed orientations. However, to estimate the azimuthal angle of the target magnetic field with respect to the NV axis in these previous approaches, it is necessary to apply a strong reference DC magnetic field, which can perturb the system to be measured. This is a crucial problem, especially when attempting to measure vector magnetic fields from materials that are sensitive to applied DC magnetic fields. Here, we propose a method to measure vector DC magnetic fields using perfectly aligned NV centers without reference DC magnetic fields. More specifically, we used the direction of linearly polarized microwave fields to induce Rabi oscillation as a reference and estimated the azimuthal angle of the target fields from the Rabi frequency. We further demonstrate the potential of our method to improve sensitivity by using entangled states to overcome the standard quantum limit. Our method of using a reference microwave field is a novel technique for sensitive vector DC magnetic-field sensing.

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