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Tamara Nikšić

Publications and source records attributed to Tamara Nikšić.

14 recordsLinked to original sources

Pairing correlations, orientations and quantum fluctuations in one- and two-nucleon transfer reactions at sub-barrier energies

This work investigates one- and two-neutron transfer in the $^{96}\text{Zr} + {}^{40}\text{Ca}$ reaction at sub-barrier energies using a microscopic framework based on time-dependent covariant density functional theory (TD-CDFT). Pairing correlations are incorporated via the time-dependent BCS approximation, which is shown to significantly enhance pair transfer, as evidenced by an increased two-neutron transfer probability. The oblate deformation of $^{96}$Zr causes the transfer probabilities to vary by orders of magnitude with orientation; a direct comparison with experiment is enabled by averaging results over thirteen systematically chosen orientations. While the orientation-averaged one-neutron transfer probabilities agree well with data, the two-neutron channel is suppressed below the Coulomb barrier. This suppression is attributed to missing quantum fluctuations in the semiclassical TD-CDFT approach. To test this, we employ the generalized time-dependent generator coordinate method (TDGCM), which confirms that quantum fluctuations are essential for an accurate description of sub-barrier two-neutron transfer dynamics.

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Intrinsic spin distributions in multinucleon transfer reactions

Time-dependent covariant density functional theory (TD-CDFT) combined with angular momentum projection is developed and applied to study multinucleon transfer (MNT) reactions, with a focus on the intrinsic angular momentum distributions of the final fragments. Using the illustrative reaction $^{40}$Ca + $^{208}$Pb across a range of impact parameters, we find that the MNT process generates broad distributions of intrinsic spins. These distributions arise from the conversion of relative orbital angular momentum into intrinsic spin due to frictional interactions between the colliding nuclei. Additionally, mutual information (entanglement Shannon entropy) is employed to analyze correlations between the intrinsic spins of the fragments.

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Nuclear Physics Confronts Relativistic Collisions Of Isobars

High-energy collisions involving the $A=96$ isobars $^{96}$Zr and $^{96}$Ru have been performed in 2018 at Brookhaven National Laboratory's Relativistic Heavy Ion Collider (RHIC) as a means to search for the chiral magnetic effect in QCD. This would manifest itself as specific deviations from unity in the ratio of observables taken between $^{96}$Zr+$^{96}$Zr and $^{96}$Ru+$^{96}$Ru collisions. Measurements of such ratios (released at the end of 2021) indeed reveal deviations from unity, but these are primarily caused by the two collided isobars having different radial profiles and intrinsic deformations. To make progress in understanding RHIC data, nuclear physicists across the energy spectrum gathered in Heidelberg in 2022 as part of an EMMI Rapid Reaction Task Force (RRTF) to address the following question. Does the combined effort of low-energy nuclear structure physics and high-energy heavy-ion physics enable us to understand the observations made in isobar collisions at RHIC?

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Global properties of nuclei at finite-temperature within the covariant energy density functional theory

In stellar environments nuclei appear at finite temperatures, becoming extremely hot in core-collapse supernovae and neutron star mergers. However, due to theoretical and computational complexity, most model calculations of nuclear properties are performed at zero temperature, while those existing at finite temperatures are limited only to selected regions of the nuclide chart. In this study we perform the global calculation of nuclear properties for even-even $8 \leq Z \leq 104$ nuclei at temperatures in range $0\le T \le 2$ MeV. Calculations are based on the finite temperature relativistic Hartree-Bogoliubov model supplemented by the Bonche-Levit-Vautherin vapor subtraction procedure. We find that near the neutron-drip line the continuum states have significant contribution already at moderate temperature $T\approx 1$ MeV, thus emphasising the necessity of the vapor subtraction procedure. Results include neutron emission lifetimes, quadrupole deformations, neutron skin thickness, proton and neutron pairing gaps, entropy and excitation energy. Up to the temperature $T\approx 1$ MeV nuclear landscape is influenced only moderately by the finite-temperature effects, mainly by reducing the pairing correlations. As the temperature increases further, the effects on nuclear structures become pronounced, reducing both the deformations and the shell effects.

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Influence of the symmetry energy on the nuclear binding energies and the neutron drip line position

A clear connection can be established between properties of nuclear matter and finite-nuclei observables, such as the correlation between the slope of the symmetry energy and dipole polarizability, or between compressibility and the isoscalar monopole giant resonance excitation energy. Establishing a connection between realistic atomic nuclei and an idealized infinite nuclear matter leads to a better understanding of underlying physical mechanisms that govern nuclear dynamics. In this work, we aim to study the dependence of the binding energies and related quantities (e.g. location of drip lines, the total number of bound even-even nuclei) on the symmetry energy $S_2(ρ)$. The properties of finite nuclei are calculated by employing the relativistic Hartree-Bogoliubov (RHB) model, assuming even-even axial and reflection symmetric nuclei. Calculations are performed by employing two families of relativistic energy density functionals (EDFs), based on different effective Lagrangians, constrained to a specific symmetry energy at saturation density $J$ within the interval of $30$--$36$ MeV. Nuclear binding energies and related quantities of bound nuclei are calculated between $8 \leq Z \leq 104$ from the two-proton to the two-neutron drip line. As the neutron drip line is approached, the interactions with stiffer $J$ tend to predict more bound nuclei, resulting in a systematic shift of the two-neutron drip line towards more neutron-rich nuclei. Consequentially, a correlation between the number of bound nuclei $N_{nucl}$ and $S_2(ρ)$ is established for a set of functionals constrained using the similar optimization procedures. The direction of the relationship between the number of bound nuclei and symmetry energy highly depends on the density under consideration.

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Many-body approach to superfluid nuclei in axial geometry

Starting from a general many-body fermionic Hamiltonian, we derive the equations of motion (EOM) for nucleonic propagators in a superfluid system. The resulting EOM is of the Dyson type formulated in the basis of Bogoliubov's quasiparticles. As the leading contributions to the dynamical kernel of this EOM in strongly-coupled regimes contain phonon degrees of freedom in various channels, an efficient method of calculating phonon's characteristics is required to successfully model these kernels. The traditional quasiparticle random phase approximation (QRPA) solvers are typically used for this purpose in nuclear structure calculations, however, they become very prohibitive in non-spherical geometries. In this work, by linking the notion of the quasiparticle-phonon vertex to the variation of the Bogoliubov's Hamiltonian, we show that the recently developed finite-amplitude method (FAM) can be efficiently employed to compute the vertices within the FAM-QRPA. To illustrate the validity of the method, calculations based on the relativistic density-dependent point-coupling Lagrangian are performed for the single-nucleon states in heavy and medium-mass nuclei with axial deformations. The cases of $^{38}$Si and $^{250}$Cf are presented and discussed.

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Time-dependent generator coordinate method study of fission: dissipation effects

Starting from a quantum theory of dissipation for nuclear collective motion, the time-dependent generator coordinate method (TDGCM) is extended to allow for dissipation effects in the description of induced fission dynamics. The extension is based on a generalization of the GCM generating functions that includes excited states, and the resulting equation of motion in the collective coordinates and excitation energy. With the assumption of a narrow hamiltonian kernel, an expansion in a power series in collective momenta leads to a Schrödinger-like equation that explicitly includes a dissipation term, proportional to the momentum of the statistical wave function. An illustrative calculation is performed for induced fission of $^{228}$Th. The three-dimensional model space includes the axially-symmetric quadrupole and octupole shape variables, and the nuclear temperature. When compared to data for photo-induced fission of $^{228}$Th, the calculated fission yields demonstrate the important role of the additional term in the hamiltonian that explicitly takes into account the dissipation of energy of collective motion into intrinsic degrees of freedom.

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Microscopic self-consistent description of induced fission: dynamical pairing degree of freedom

The role of dynamical pairing in induced fission dynamics is investigated using the time-dependent generator coordinate method in the Gaussian overlap approximation, based on the microscopic framework of nuclear energy density functionals. A calculation of fragment charge yields for induced fission of $^{228}$Th is performed in a three-dimensional space of collective coordinates that, in addition to the axial quadrupole and octupole intrinsic deformations of the nuclear density, also includes an isoscalar pairing degree of freedom. It is shown that the inclusion of dynamical pairing has a pronounced effect on the collective inertia, the collective flux through the scission hyper-surface, and the resulting fission yields, reducing the asymmetric peaks and enhancing the contribution of symmetric fission, in better agreement with the empirical trend.

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Microscopic model for the collective enhancement of nuclear level densities

A microscopic method for calculating nuclear level densities (NLD) is developed, based on the framework of energy density functionals. Intrinsic level densities are computed from single-quasiparticle spectra obtained in a finite-temperature self-consistent mean-field (SCMF) calculation that takes into account nuclear deformation, and is specified by the choice of the energy density functional (EDF) and pairing interaction. The total level density is calculated by convoluting the intrinsic density with the corresponding collective level density, determined by the eigenstates of a five-dimensional quadrupole or quadrupole plus octupole collective Hamiltonian. The parameters of the Hamiltonian (inertia parameters, collective potential) are consistently determined by deformation-constrained SCMF calculations using the same EDF and pairing interaction. The model is applied in the calculation of NLD of $^{94,96,98}$Mo, $^{106,108}$Pd, $^{106,112}$Cd, $^{160,162,164}$Dy, $^{166}$Er, and $^{170,172}$Yb, in comparison with available data. It is shown that the collective enhancement of the intrinsic level density, consistently computed from the eigenstates of the corresponding collective Hamiltonian, leads to total NLDs that are in excellent agreement with data over the whole energy range of measured values.

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Time-dependent generator coordinate method study of fission: mass parameters

Collective mass tensors derived in the cranking approximation to the adiabatic time-dependent Hartree-Fock-Bogoliubov (ATDHFB) method are employed in a study of induced fission dynamics. Together with a collective potential determined in deformation-constrained self-consistent mean-field calculations based on nuclear energy density functionals, the mass tensors specify the collective Hamiltonian that governs the time evolution of the nuclear wave function from an initial state at equilibrium deformation, up to scission and the formation of fission fragments. In an illustrative calculation of low-energy induced fission of $^{228}$Th, $^{230}$Th, $^{234}$U, and $^{240}$Pu, we compare the non-perturbative and perturbative cranking ATDHFB mass tensors in the plane of axially-symmetric quadrupole and octupole deformations, as well as the resulting charge yields.

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Cluster structures in $^{12}$C from global energy density functionals

Spectroscopic properties of low-lying states and cluster structures in $^{12}$C are analyzed in a "beyond mean-field framework" based on global energy density functionals (EDFs). To build symmetry-conserving collective states, axially-symmetric and reflection-asymmetric solutions of the relativistic Hartree-Bogoliubov equations are first projected onto good values of angular momentum, particle number, and parity. Configuration mixing is implemented using the generator coordinate method formalism. It is shown that such a global microscopic approach, based on a relativistic EDF, can account for the main spectroscopic features of $^{12}$C, including the ground-state and linear-chain bands as well as, to a certain approximation, the excitation energy of the Hoyle state. The calculated form factors reproduce reasonably well the available experimental values, and display an accuracy comparable to that of dedicated microscopic cluster models.

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Time-dependent generator coordinate method study of mass-asymmetric fission of actinides

Low-energy positive and negative parity collective states in the equilibrium minimum, and the dynamics of induced fission of actinide nuclei are investigated in a unified theoretical framework based on the generator coordinate method (GCM) with the Gaussian overlap approximation (GOA). The collective potential and inertia tensor, both at zero and finite temperature, are computed using the self-consistent multidimensionally constrained relativistic mean field (MDC-RMF) model, based on the energy density functional DD-PC1. Pairing correlations are treated in the BCS approximation with a separable pairing force of finite range. A collective quadrupole-octupole Hamiltonian characterized by zero-temperature axially-symmetric deformation energy surface and perturbative cranking inertia tensor, is used to model the low-lying excitation spectrum. The fission fragment charge distributions are obtained by propagating the initial collective states in time with the time-dependent GCM+GOA that uses the same quadrupole-octupole Hamiltonian, but with the collective potential and inertia tensor computed at finite temperature. The illustrative charge yields of $^{228}$Th, $^{234}$U, $^{240}$Pu, $^{244}$Cm, and $^{250}$Cf are in very good agreement with experiment, and the predicted mass asymmetry is consistent with the result of a recent microscopic study that has attributed the distribution (peak) of the heavier-fragment nuclei to shell-stabilized octupole deformations.

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Microscopic self-consistent description of induced fission dynamics: finite temperature effects

The dynamics of induced fission of $^{226}$Th is investigated in a theoretical framework based on the finite-temperature time-dependent generator coordinate method (TDGCM) in the Gaussian overlap approximation (GOA). The thermodynamical collective potential and inertia tensor at temperatures in the interval $T=0 - 1.25$ MeV are calculated using the self-consistent multidimensionally constrained relativistic mean field (MDC-RMF) model, based on the energy density functional DD-PC1. Pairing correlations are treated in the BCS approximation with a separable pairing force of finite range. Constrained RMF+BCS calculations are carried out in the collective space of axially symmetric quadrupole and octupole deformations for the asymmetric fissioning nucleus $^{226}$Th. The collective Hamiltonian is determined by the temperature-dependent free energy surface and perturbative cranking inertia tensor, and the TDGCM+GOA is used to propagate the initial collective state in time. The resulting charge and mass fragment distributions are analyzed as functions of the internal excitation energy. The model can qualitatively reproduce the empirical triple-humped structure of the fission charge and mass distributions already at $T=0$, but the precise experimental position of the asymmetric peaks and the symmetric-fission yield can only be accurately reproduced when the potential and inertia tensor of the collective Hamiltonian are determined at finite temperature, in this particular case between $T=0.75$ MeV and $T=1$ MeV.

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"Sloppy" nuclear energy density functionals (II): Finite nuclei

A study of parameter sensitivity of nuclear energy density functionals, initiated in the first part of this work \cite{NV.16}, is extended by the inclusion of data on ground-state properties of finite nuclei in the application of the manifold boundary approximation method (MBAM). Density functionals used in self-consistent mean-field calculations, and nuclear structure models based on them, are generally "sloppy" and exhibit an exponential range of sensitivity to parameter variations. Concepts of information geometry are used to identify the presence of effective functionals of lower dimension in parameter space associated with parameter combinations that can be tightly constrained by data. The MBAM is used in an iterative procedure that systematically reduces the complexity and the dimension of parameter space of a sloppy functional, with properties of nuclear matter and data on finite nuclei determining not only the values of model parameters, but also the optimal functional form of the density dependence.

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