arXiv subjects

Tan Shi

Publications and source records attributed to Tan Shi.

15 recordsLinked to original sources

arXiv2026

Unveiling Nanoscale Surface Damage Dynamics in Swift Heavy Ion Irradiated Gallium Nitride

This work systematically unveils the nanoscale surface damage dynamics in gallium nitride by investigating the atomistic mechanisms of hillock formation. The results identify two distinct hillock morphologies dependent on electronic energy loss (Se) values. Bell-shaped hillocks form under 18.2 keV/nm Kr irradiation, whereas crater-rim hillocks with central holes emerge under 40.2 keV/nm Ta irradiation. Microstructural analysis reveals that Ga-rich hillocks are accompanied by the generation of metastable zincblende nanodomains. These nanodomains preferentially aggregate around the periphery or sidewalls of the hillocks and exhibit a high spatial correlation with screw dislocations. Further temperature-dependent studies indicate that elevated temperatures significantly enlarge the overall dimensions of the hillock structures without altering their fundamental morphologies. Notably, under Ta irradiation above 1200 K, the high temperatures drastically reduce the viscosity and surface tension of liquid gallium. This enhanced fluidity of the transient molten phase promotes the formation of penetrating nanochannels.

cond-mat.mtrl-sci↗

arXiv2026

Atomistic Mechanisms of Temperature-Dependent Ion Track Formation in Gallium Nitride under Swift Heavy Ion Irradiation

The radiation tolerance of gallium nitride under extreme conditions is critical for its deployment in next-generation electronic and optoelectronic devices, yet the microscopic mechanisms governing swift heavy ion induced damage at elevated temperatures remain poorly understood. Therefore, this study employs a coupled approach including the two-temperature model and molecular dynamics simulations to resolve the entire processes of ion track generation induced by swift heavy ions irradiation across a wide temperature range. A temperature-driven morphological transition of ion tracks, evolving from discontinuous segments to continuous tracks composed of isolated nanobubbles, and ultimately to fully continuous channels is observed. Under lower electronic stopping loss of 430 MeV Kr irradiation, increasing temperature significantly enhances track visibility, enlarges track radii and promotes nanobubble formation. For higher electronic stopping conditions of 1171 MeV Ta irradiation, continuous ion tracks consisting of discontinuous nanobubbles (~1.5 nm radius) emerge already at 300 K, followed by a thermally activated transition into continuous channels with further radial expansion. At the atomic scale, SHI irradiation induces decomposition of wurtzite GaN into Ga clusters and N2 molecules along the ion trajectory, with Ga-rich regions and recrystallized wurtzite phases accumulating near bubble interfaces, while N2 preferentially segregates within bubble cores. Additionally, zincblende nanodomains nucleate around ion tracks and exhibit strong spatial correlation with radiation-induced dislocation networks, particularly screw dislocations, providing potential pathways for leakage current and increased susceptibility to single-event burnout.

cond-mat.mtrl-sci↗

arXiv2026

Anisotropic Core-Shell Swift Heavy Ion Tracks in beta-Ga2O3

Swift heavy ion (SHI) irradiation generates nanoscale ion tracks through intense electronic excitation, yet the microscopic mechanisms governing their morphology and phase stability in low symmetry oxides remain poorly understood. Here, a multiscale atomistic simulation framework is used to investigate the formation and recovery of SHI-induced tracks in monoclinic $\beta$-Ga2O3 over a wide range of electronic energy losses (Se) and crystallographic orientations. A sequence of distinct structural responses is identified with increasing Se: (i) complete lattice recovery at low Se; (ii) recrystallization into a metastable $\gamma$-Ga2O3 phase at intermediate Se; and (iii) the formation of core-shell ion tracks at high Se, consisting of an amorphous core surrounded by a recrystallized $\gamma$-phase shell. Despite the essentially isotropic initial energy deposition, the final ion-track morphology exhibits pronounced crystallographic anisotropy, governed by orientation-dependent recovery dynamics. The superior recrystallization along the [010] direction is attributed to its exceptionally high elastic stiffness. Notably, SHI irradiation perpendicular to the (100) plane induces a more severe structural response at low Se ($\le$ 10 keV/nm), however, at higher Se, it yields a smaller residual ion track compared to the other orientations. The simulated ion-track sizes show excellent quantitative agreement with the available experimental measurements over a wide range of Se values. These findings establish a unified atomic-scale picture of core-shell track formation and anisotropic recovery in $\beta$-Ga2O3.

cond-mat.mtrl-sci↗

arXiv2023

Dual-band polarized upconversion photoluminescence enhanced by resonant dielectric metasurfaces

Lanthanide-doped upconversion nanoparticles emerged recently as an attractive material platform underpinning a broad range of innovative applications such as optical cryptography, luminescent probes, and lasing. However, the intricate 4f-associated electronic transition in upconversion nanoparticles leads only to a weak photoluminescence intensity and unpolarized emission, hindering many applications that demand ultrabright and polarized light sources. Here, we uncover a new strategy for achieving ultrabright and dual-band polarized upconversion photoluminescence. We employ resonant dielectric metasurfaces supporting high-quality resonant modes at dual upconversion bands enabling two-order-of-magnitude amplification of upconversion emissions. We demonstrate that dual-band resonances can be selectively switched on polarization, endowing cross-polarization controlled upconversion luminescence with ultra-high degrees of polarization, reaching approximately 0.86 and 0.91 at dual emission wavelengths of 540 nm and 660 nm, respectively. Our strategy offers an effective approach for enhancing photon upconversion processes paving the way toward efficient low-threshold polarization upconversion lasers.

physics.optics↗

arXiv2021

Planar chiral metasurfaces with maximal tunable chiroptical response driven by bound states in the continuum

Optical metasurfaces with high-Q chiral resonances can boost light-matter interaction for various applications of chiral response for ultrathin, active, and nonlinear metadevices. Usually, such metasurfaces require sophisticated depth-resolved nanofabrication to realize subwavelength stereo-nanostructures, posing overwhelming challenges, especially in the short-wavelength range. Here, we suggest a novel planar design for chiral metasurfaces supporting bound states in the continuum (BICs) and demonstrate experimentally chiroptical responses with record-high Q-factors (Q=390) and near-perfect circular dichroism (CD=0.93) at optical frequencies. The symmetry-reduced meta-atoms are highly birefringent and support winding elliptical eigen-polarizations with opposite helicity surrounding the BIC polarization singularity, providing a convenient way for achieving maximal planar chirality tuned by either breaking in-plane symmetry or changing illumination direction. Such sharply resonant chirality realized in planar metasurfaces promises various practical applications in classical and quantum optics including chiral sensing, enantiomer selection, and chiral quantum emitters.

physics.optics↗

arXiv2021

Observation of Topologically Robust Localized Magnetic Plasmon Skyrmions

Optical skyrmions have recently been constructed by tailoring electric or spin field distributions through the interference of multiple surface plasmon polaritons, offering promising features for advanced information processing, transport and storage. Here, we construct topologically robust plasmonic skyrmions in a wisely tailored space-coiling meta-structure supporting magnetic localized spoof plasmons (LSPs), which are strongly squeezed down to {\lambda}3/106 and do not require stringent external interference conditions. By directly measuring the spatial profile of all three vectorial magnetic fields, we reveal multiple {\pi}-twist target skyrmion configurations mapped to multi-resonant near-equidistant LSP eigen-modes. The real-space topological robustness of these skyrmion configurations is confirmed by arbitrary deformations of the meta-structure, demonstrating flexible skyrmionic textures with arbitrary shapes. The observed magnetic LSP skyrmions pave the way to ultra-compact and topologically robust plasmonic devices, such as flexible sensors, wearable electronics and ultra-compact antennas.

physics.optics↗

arXiv2021

Radiation-tolerant high-entropy alloys via interstitial-solute-induced chemical heterogeneities

High-entropy alloys (HEAs) composed of multiple principal elements have been shown to offer improved radiation resistance over their elemental or dilute-solution counterparts. Using NiCoFeCrMn HEA as a model, here we introduce carbon and nitrogen interstitial alloying elements to impart chemical heterogeneities in the form of the local chemical order (LCO) and associated compositional variations. Density functional theory simulations predict chemical short-range order (CSRO) (nearest neighbors and the next couple of atomic shells) surrounding C and N, due to the chemical affinity of C with (Co, Fe) and N with (Cr, Mn). Atomic-resolution chemical mapping of the elemental distribution confirms marked compositional variations well beyond statistical fluctuations. Ni+ irradiation experiments at elevated temperatures demonstrate a remarkable reduction in void swelling by at least one order of magnitude compared to the base HEA without C and N alloying. The underlying mechanism is that the interstitial-solute-induced chemical heterogeneities roughen the lattice as well as the energy landscape, impeding the movements of, and constraining the path lanes for, the normally fast-moving self-interstitials and their clusters. The irradiation-produced interstitials and vacancies therefore recombine more readily, delaying void formation. Our findings thus open a promising avenue towards highly radiation-tolerant alloys.

cond-mat.mtrl-sci↗

arXiv2020

Transmissive Metagrating for Arbitrary Wavefront Shaping Over the Full Visible Spectrum

Metagratings have been shown to form an agile and efficient platform for extreme wavefront manipulation, going beyond the limitations of gradient metasurfaces. Previous approaches for transmissive metagratings have resorted on compound asymmetric inclusions to achieve single-channel near-perfect diffraction. However, such complex inclusions are sensitive to geometric parameters and lack the flexibility for arbitrary phase modulation, restricting applications to beam deflection. Here, we show perfect unitary diffraction in all-dielectric transmissive metagratings using rectangular inclusions by tailoring their multipole interferences. Using this principle, we experimentally demonstrate analog phase profile encoding of a hologram through displacement modulation of CMOS-compatible silicon nitride nanobars, manifesting broadband and wide-angle high diffraction efficiencies for both polarizations and across the entire visible range. Featured with extreme angle/wavelength/polarization tolerance and alleviated structural complexity for both design and fabrication, our demonstration unlocks the full potential of metagrating-based wavefront manipulation for a variety of practical applications.

physics.optics↗

arXiv2019

Full-color complex-amplitude vectorial holograms based on multi-freedom metasurfaces

Phase, polarization, amplitude and frequency represent the basic dimensions of light, playing crucial roles for both fundamental light-mater interactions and all major optical applications. Metasurface emerges as a compact platform to manipulate these knobs, but previous metasurfaces have limited flexibility to simultaneous control them. Here, we introduce a multi-freedom metasurface that can simultaneously and independently modulate phase, polarization and amplitude in an analytical form, and further realize frequency multiplexing by a k-space engineering technique. The multi-freedom metasurface seamlessly combine geometric Pancharatnam-Berry phase and detour phase, both of which are frequency-independent. As a result, it allows complex-amplitude vectorial hologram at various frequencies based on the same design strategy, without sophisticated nanostructure searching of massive size parameters. Based on this principle, we experimentally demonstrate full-color complex-amplitude vectorial meta-holograms in the visible with a metal-insulator metal architecture, unlocking the long-sought full potential of advanced light field manipulation through ultrathin metasurfaces.

physics.optics↗

arXiv2019

Modeling of Electro-deposition and Mechanical Stability at Li Metal/Solid Electrolyte Interface during Plating in Solid-State Batteries

Interfacial deposition stability between Li metal and a solid electrolyte (SE) is important in preventing interfacial contact loss, mechanical fracture, and dendrite growth in Li-metal solid-state batteries (SSB). In this work, we investigate the deposition and mechanical stability at the Li metal/SE interface and its consequences (such as SE fracture and contact loss). A wide range of contributing factors are investigated, such as charge and mass transfer kinetics, the plasticity of Li metal and fracture of the SE, and the applied stack pressure. We quantify the effect of the ionic conductivity of the SE, the exchange current density of the interfacial charge-transfer reaction and SE surface roughness on the Li deposition stability at the Li metal/SE interface. We also propose a mechanical stability window for the applied stack pressure that can prevent both contact loss and SE fracture, which can be extended to other metal-electrode (such as Sodium) SSB systems.

physics.app-ph↗

arXiv2018

Hidden structural order controls Li-ion transport in cation-disordered oxides for rechargeable lithium batteries

Crystal structures play a vital role in determining materials properties. In Li-ion cathodes, the crystal structure defines the dimensionality and connectivity of interstitial sites, thus determining Li-ion diffusion kinetics. While a perfect crystal has infinite structural coherence, a class of recently discovered high-capacity cathodes, Li-excess cation-disordered rocksalts, falls on the other end of the spectrum: Their cation sublattices are assumed to be randomly populated by Li and transition metal ions with zero configurational coherence based on conventional X-ray diffraction, such that the Li transport is purely determined by statistical effects. In contrast to this prevailing view, we reveal that cation short-range order, hidden in diffraction, is ubiquitous in these long-range disordered materials and controls the local and macroscopic environments for Li-ion transport. Our work not only discovers a crucial property that has previously been overlooked, but also provides new guidelines for designing and engineering disordered rocksalts cathode materials.

cond-mat.mtrl-sci↗

arXiv2015

Multi-channel exchange-scattering spin polarimetry

Electron spin takes critical role in almost all novel phenomena discovered in modern condensed matter physics (High-temperature superconductivity, Kondo effect, Giant Magnetoresistance, topological insulator, quantum anomalous Hall effect, etc.). However, the measurements for electron spin is of poor quality which blocks the development of material sciences because of the low efficiency of spin polarimeter. Here we show an imaging type exchange-scattering spin polarimeter with 5 orders more efficiency compared with a classical Mott polarimeter. As a demonstration, the fine spin structure of electronic states in bismuth (111) is investigated, showing the strong Rashba type spin splitting behavior in both bulk and surface states. This improvement pave the way to study novel spin related phenomena with unprecedented accuracy.

cond-mat.mtrl-sci↗

arXiv2015

3D Scaffolded Nickel-Tin Li-Ion Anodes with Enhanced Cyclability

A 3D mechanical stable scaffold is shown to accommodate the volume change of a high specific capacity nickel-tin nanocomposite Li-ion battery anode. When the nickel-tin anode is formed on an electrochemically inactive conductive scaffold with an engineered free volume and controlled characteristic dimensions, it exhibits significantly improved the cyclability.

cond-mat.mtrl-sci↗

arXiv2014

The design of a high flux VUV beamline for low energy photons

A VUV beamline at SSRF for ARPES measurements are designed. To increase the resolution and bulk sensitivity, the photon energy as low as 7 eV is desired. Because the reflectivity for p-polarized photons strongly decreases when the photon energy is below 30 eV, the design of high flux beamline for low energy VUV photons is a challenge. This work shows a variable including angle VLPGM with varied grating depth (VGD) which can achieve both high resolution and high flux with broad energy coverage.

physics.ins-det↗

arXiv2014

The design of a multi-channel spin polarimeter

All commercial electron spin polarimeters work in single channel mode, which is the bottleneck of researches by spin-resolved photoelectron spectroscopy. By adopting the time inversion antisymmetry of magnetic field, we developed a multichannel spin polarimeter based on normal incident VLEED. The key point to achieve the multi-channel measurements is the spatial resolution of the electron optics. The test of the electron optics shows that the designed spatial resolution can be achieved and an image type spin polarimeter with 100 times 100, totally ten thousand channels is possible to be realized.

physics.ins-det↗