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Tanmoy Das

Publications and source records attributed to Tanmoy Das.

At least 19 recordsLinked to original sources

Comparative Assessment of Thermal Transport Theories: Dual-Channel Mechanism Dictates Heat Transport in Ultralow-$\kappa$ Materials

Anomalous heat transport in strongly anharmonic crystalline solids poses both a fundamental challenge to the theoretical understanding and an opportunity for thermoelectric and thermal barrier coating applications. Although Green-Kubo theory reproduces experimental thermal conductivity ($\kappa$) at high temperatures, it lacks microscopic insight and neglects the Bose-Einstein statistics of lattice vibrations. On the other hand, the conventional Boltzmann transport equation (BTE) framework, based on a phonon-gas picture, fails due to strong anharmonicity-induced overdamped phonons. Herein, the thermal transport properties in TlAgSe, a metal chalcogenide, and Cs$_2$PbI$_2$C$_2$, an all-inorganic layered Ruddlesden-Popper perovskite, are investigated by explicitly accounting for temperature-dependent lattice dynamics through machine learning interatomic potentials and employing the Wigner transport equation (WTE) framework. Crucially, heat conduction is governed not only by higher-order phonon scattering-dominated populations' transport channel described within the BTE, but also by a coherences' channel in the WTE framework arising from wave-like interbranch coherence between eigenstates. Incorporating four-phonon scattering, WTE predicts average room-temperature $\kappa$ values of 0.31 Wm$^{-1}$K$^{-1}$ (TlAgSe) and 0.38 Wm$^{-1}$K$^{-1}$ (Cs$_2$PbI$_2$C$_2$), in excellent agreement with experiments. Phonon scattering-rate analysis reveals strong coherences' contributions and prevalent overdamped phonon modes, demonstrating the breakdown of the conventional BTE framework based on the phonon quasiparticle picture with only first-order anharmonic perturbation. This computational approach provides a unified description of heat transport in ultralow-$\kappa$ materials, offering a basis for the rational design of phononic and thermoelectric devices.

cond-mat.mtrl-sci

Second quantization of anyons and spin-anyon duality

Anyons exhibit a non-trivial interplay between local exclusion rules and non-local braiding and exchange phases, making a consistent commutation algebra and second-quantized formulation challenging. We develop an algebraic framework for Abelian anyons in one dimension with statistical phase $\theta$ = $\pi$/N that enforces a finite on-site occupancy of N-1 anyons with the exchange phase $\theta$ between different sites. Moreover, we introduce an exact Jordan-Wigner duality between $\pi$/3 anyons and spin-1 operators, allowing us to map a tight-binding anyon model to an XY-like spin-1 model. The model exhibits anyon-density-dependent flux, incompressible or gapless regions, and critical points with level crossings that appear as discontinuities in ground-state currents, momenta, fidelities, and correlation functions. Our second-quantization formalism establishes a novel spin anyon duality, offering a conceptually new route to realize anyons from spin Hamiltonians and to engineer corresponding device architectures.

cond-mat.str-el

Coherent magnetic excitations in a topological Kondo semimetal

In Kondo insulators the many-body Kondo lattice effect drives the formation of bands containing heavy charge carriers with a hybridization gap, leading to insulating properties. These renormalized bands can host non-trivial topologies driven by strong electron-electron interactions, but probing narrow heavy bands at low temperatures is challenging. We use inelastic neutron scattering (INS) to probe the Kondo lattice CeNiSn, which hosts both semimetallic transport properties and a hybridization gap. The INS response exhibits momentum-dependent magnetic excitations and a spin-gap in the low-temperature Kondo coherent state, which electronic structure calculations corroborate as arising from the renormalized heavy band structure. Dynamical-mean field theory demonstrates that this renormalized band structure corresponds to a topological Kondo insulating state, and hence the INS probes bulk excitations of heavy topological bands. This identification of a Kondo insulator addresses the long-standing mystery of the electronic properties of CeNiSn, and demonstrates the manifestation of a topological many-body coherent state in spectroscopic measurements of strongly correlated narrow band materials.

cond-mat.str-el

Coexistence of Rashba and Ising Spin-Singlet Pairings in Two-Dimensional IrTe$_{2}$

Symmetry offers a useful approach to unfold the intertwined degrees of freedom. Thus it paves the way to resolve coexisting quantum orders into distinct symmetry sectors. Motivated by the recent observation of superconductivity in nano-flaked IrTe$_2$, we investigate the superconductivity in strain-stabilized two-dimensional (2D) limit of IrTe$_2$ by combining density-functional theory with mean-field solution of spin-fluctuation mediated pairing interaction on a symmetry-constrained ${\bf k}\cdot{\bf p}$ model. The spin-orbit coupled band structure shows $\Gamma$-centred Fermi sheets with coexistence of band-selective Rashba-like (in-plane) and Ising-like (out-of-plane) superconductivity. Remarkably, the superconducting gaps are odd in spin, orbital, and momentum channels despite the presence of global inversion symmetry. Fermi surface topologies and little-group symmetry enforce distinct irreducible representations to the Rashba and Ising channels, forbidding their mixing. Our findings open up a symmetry-based route to multichannel superconductivity in 2D transition-metal dichalcogenides with unique functionalities.

cond-mat.supr-con

Sedimentation of particulate suspensions under stagnant conditions in horizontal pipes

Sedimentation of particulate suspensions in horizontal pipes can lead to formation, growth and consolidation of a solid-like bed which can severely retard pipeline performance. As stagnant flow conditions frequently arise during industrial processes, critical operational questions are: (i) at what rate and extent does sedimentation proceed, and (ii) can the sedimentation dynamics be predicted from conventional suspension characterisation methods? We address these questions by characterising the sedimentation properties of an aqueous Kaolin suspension via batch settling tests and comparing predictions from 1D sedimentation theory with experiments in a horizontally oriented cylindrical pipe. We show that particulate sedimentation can be accurately predicted, indicating that the estimated sedimentation properties are representative material properties, and that transient effects such as gravity currents are not significant. Conversely, we find that the consolidation of the sediment is not well predicted by 1D theory, suggesting that the stress state is not 1D and likely involves contributions from the pipe walls. These stagnant cylindrical pipe results provide a basis for the development of methods to predict pipeline sedimentation under more general (laminar and turbulent) flow conditions.

physics.flu-dyn

Phase-Space Approach to Wannier Pairing and Bogoliubov Orbitals in Square-Octagon Lattices

Low-energy lattice models are the cornerstone for studying many-body physics and interactions between the system and measurement fields. A key challenge is identifying appropriate quasiparticle states that canonically transform between momentum and real space while retaining the correlation, entanglement, and geometric properties - generally called the Wannier obstruction. Here, we introduce a phase-space approach to bypass these obstructions. Instead of treating the phase space as a manifold, we embed a real space through a Bloch vector space at each momentum. Orbital and spin states are introduced through product states with the Bloch vector, while quantum statistics, correlations, topology, and entanglements are inherited from the Hamiltonian. We apply this framework to explore the unconventional pairing symmetry and the Bogoliubov-de Gennes (BdG) equation in phase space. Our findings demonstrate that while superconductivity exhibits global coherence, the local Wannier orbital symmetry primarily determines the pairing symmetry. We analytically solve the spin-fluctuation-mediated pairing symmetry on the phase space by engineering a flat band with artificial gauge fields. We validate the model on the square-octagon superconductor Lu$_2$Fe$_3$Si$_5$ using density functional theory (DFT), revealing the coexistence of nodeless $s^{\pm}$ and nodal $s_{z^2}$ pairing symmetries. This phase-space framework provides a robust, obstruction-free lattice model for complex many-body systems and their exotic excitations.

cond-mat.supr-con

Improving precision of A/B experiments using trigger intensity

In industry, online randomized controlled experiment (a.k.a. A/B experiment) is a standard approach to measure the impact of a causal change. These experiments have small treatment effect to reduce the potential blast radius. As a result, these experiments often lack statistical significance due to low signal-to-noise ratio. A standard approach for improving the precision (or reducing the standard error) focuses only on the trigger observations, where the output of the treatment and the control model are different. Although evaluation with full information about trigger observations (full knowledge) improves the precision, detecting all such trigger observations is a costly affair. In this paper, we propose a sampling based evaluation method (partial knowledge) to reduce this cost. The randomness of sampling introduces bias in the estimated outcome. We theoretically analyze this bias and show that the bias is inversely proportional to the number of observations used for sampling. We also compare the proposed evaluation methods using simulation and empirical data. In simulation, bias in evaluation with partial knowledge effectively reduces to zero when a limited number of observations (<= 0.1%) are sampled for trigger estimation. In empirical setup, evaluation with partial knowledge reduces the standard error by 36.48%.

econ.EM

Experimental detection of topological electronic state and large linear magnetoresistance in $SrSn_{4}$ superconductor

While recent experiments confirm the existence of hundreds of topological electronic materials, only a few exhibit the coexistence of superconductivity and a topological electronic state. These compounds attract significant attention in forefront research because of the potential for the existence of topological superconductivity, paving the way for future technological advancements. $SrSn_{4}$ is known for exhibiting unusual superconductivity below the transition temperature ($T_{C}$) of 4.8 K. Recent theory predicts a topological electronic state in this compound, which is yet to be confirmed by experiments. Systematic and detailed studies of the magnetotransport properties of $SrSn_{4}$ and its Fermi surface characterizations are also absent. For the first time, a quantum oscillation study reveals a nontrivial $\pi$ Berry phase, very light effective mass, and high quantum mobility of charge carriers in $SrSn_{4}$. Magnetotransport experiment unveils large linear transverse magnetoresistance (TMR) of more than 1200% at 5 K and 14 T. Angle-dependent transport experiments detect anisotropic and four-fold symmetric TMR, with the maximum value ($\sim$ 2000%) occurring when the angle between the magnetic field and the crystallographic b-axis is 45 degree. Our results suggest that $SrSn_{4}$ is the first topological material with superconductivity above the boiling point of helium that displays such high magnetoresistance.

cond-mat.mtrl-sci

Fractional Wannier Orbitals and Tight-Binding Gauge Fields for Kitaev Honeycomb Superlattices with Flat Majorana Bands

Fractional excitations hold immense promise for both fundamental physics and quantum technologies. However, constructing lattice models for their dynamics under gauge fields remains a formidable challenge due to inherent obstructions. Here, we introduce a novel and systematic framework for deriving low-energy lattice models of fractional orbitals coupled to tight-binding gauge fields. Departing from conventional geometric approaches, our method systematically eliminates the high-energy states via virtual hopping, thereby deriving the gauge potential and quantum metric through a superexchange-like mechanism. We demonstrate the framework by constructing Wannier orbitals for Majorana states and a tight-binding $Z_2$ gauge field across various flux crystalline phases in the Kitaev spin model on a honeycomb lattice. Our study reveals a striking phase transition between two non-trivial topological phases characterized by gapless flat-band with extensive degeneracy. Furthermore, we develop a gauge-invariant mean-field theory for interacting Majorana orbitals, leading to a correlation-induced fractional Chern state. Our work establishes a general framework for gauge-mediated tight-binding models and a gauge-invariant mean-field theory for interacting fractional orbitals that can be readily extended to $U(1)$, $SU(N)$ lattice gauge theories.

cond-mat.str-el

Symmetry, Superposition and Fragmentation in Classical Spin Liquids: A General Framework and Applications to Square Kagome Magnets

Classical magnets exhibit exotic ground state properties such as spin liquids and fractionalization, promising a manifestation of superposition and projective symmetry construction in classical theory. While system-specific spin-ice or soft-spin models exist, a formal theory for general classical magnets remains elusive. Here, we introduce a generic symmetry group construction built from a vector field in a plaquette of classical spins, demonstrating how classical spins superpose in irreducible representations (irreps) of the symmetry group. The corresponding probability amplitudes serve as order parameters and local spins as fragmented excitations. The formalism offers a many-body vector field representation of diverse ground states, including spin liquids and fragmented phases described as degenerate ensembles of irreps. We apply the theory to a frustrated square Kagome lattice, where spin-ice or soft spin rules are inapt, to describe spin liquids and fragmented phases, all validated through irreps ensembles and unbiased Monte Carlo simulation. Our generic theory sheds light on previously unknown aspects of spin-liquid phases and fragmentation and broadens their applications to other branches of field theory.

cond-mat.str-el

A Hermitian bypass to the non-Hermitian quantum theory

Describing systems with non-Hermitian (NH) operators remains a challenge in quantum theory due to instabilities (e.g., exceptional points and decoherence) arising from interactions with the environment. We propose a framework to express the energy states of NH Hamiltonians using a well-defined basis (dub computational basis) derived from a related Hermitian operator. This suitably shifts the singularities from the basis states to the expansion coefficients, allowing for their easier mathematical treatment and parametric control. Furthermore, we introduce a `space-time' transformation on the computational basis that defines a generic dual space map for the energy states. Interestingly, this transformation leads to a symmetry for real/imaginary energy values, revealing the existence of weaker condition than hermiticity or the $\mathcal{PT}$ symmetry. This leads to clearer understanding and novel interpretations of key features like exceptional points, dual space, and weaker symmetry-enforced real eigenvalues. The applicability of our framework extends to various branches of physics where NH operators manifest as ladder operators, order parameters, self-energies, projectors, and other entities.

quant-ph

Emergent glassiness in disorder-free Kitaev model: Density matrix renormalization group study on a one-dimensional ladder setting

The complete phase diagram of the Kitaev model with a magnetic field remains elusive, as do the experimental results in the candidate material α-RuCl3. Here, we study the Kitaev model on a one-dimensional ladder setting within the density-matrix renormalization group method in the presence of a magnetic field at zero temperature. We find five distinct phases with increasing magnetic field, which are characterized by a homogeneous flux phase, the Z2 vortex gas, solid and emergent glass phase, and finally, a spin-polarized phase. The emergent glassiness is confirmed by calculating correlation functions showing quasi-long-range behavior and ground state fidelity, showing a plethora of energetically accessible orthogonal saddle points corresponding to different flux configurations. This glassy behavior seems to arise from the slow dynamics of the Z2 fluxes, which is a consequence of the local constraints present in the underlying Hilbert space. This phenomenon can also be explored in other spin-liquid systems where the corresponding low-energy excitations are similarly retarded due to constraints.

cond-mat.str-el

Charge density wave induced nodal lines in LaTe$_3$

LaTe$_3$ is a noncentrosymmetric (NC) material with time reversal (TR) symmetry in which the charge density wave (CDW) is hosted by the Te bilayers. Here, we show that LaTe$_3$ hosts a Kramers nodal line (KNL), a twofold degenerate nodal line that connects the TR invariant momenta in NC achiral systems, using angle resolved photoemission spectroscopy (ARPES), density functional theory (DFT), effective band structure (EBS) calculated by band unfolding, and symmetry arguments. DFT incorporating spin-orbit coupling (SOC) reveals that the KNL -- protected by the TR and lattice symmetries -- imposes gapless crossings between the bilayer-split CDW-induced shadow bands and the main bands. In excellent agreement with the EBS, ARPES data corroborate the presence of the KNL and show that the crossings traverse the Fermi level. Furthermore, spinless nodal lines - entirely gapped out by the SOC - are formed by the linear crossings of the shadow and main bands with a high Fermi velocity.

cond-mat.mtrl-sci

Spectroscopic evidence of multi-gap superconductivity in non-centrosymmetric AuBe

AuBe is a chiral, non-centrosymmetric superconductor with transition temperature $T_C$ $\simeq$ 3.25 K. The broken inversion symmetry in its crystal structure makes AuBe a possible candidate to host a mixed singlet-triplet pairing symmetry in its superconducting order parameter ($Δ$). This possibility was investigated by transport, thermodynamic, and muon-spin rotation/relaxation experiments in AuBe. However, this issue was not addressed using direct spectroscopic probes so far. In addition, certain ambiguities exist in the description of superconductivity in AuBe based on $μ$SR experiments reported earlier. Here we report scanning tunneling spectroscopy (STS) on AuBe down to 300 mK. We found a signature of two superconducting gaps (with 2$Δ_1/k_{B}T_{C}$ = 4.37 and 2$Δ_2/k_{B}T_{C}$ = 2.46 respectively) and a clean BCS-like temperature dependence of both the gaps. We have also performed band structure calculations to identify the different bands that might give rise to the observed two-gap superconductivity in AuBe.

cond-mat.supr-con

Time-reversal symmetry breaking in frustrated superconductor Re$_2$Hf

Geometrical frustration leads to novel quantum phenomena such as the spin-liquid phase in triangular and Kagomé lattices. Intra-band and inter-band Fermi surface (FS) nesting can drive unique superconducting (SC) ground states with $d$-wave and $s^{\pm}$ pairing symmetries, respectively, according to the criterion that the SC gap changes sign across the nesting wavevector. For an odd number of FSs, when multiple inter-band nesting is of comparable strength, the sign-reversal criterion between different FS sheets can leads to frustration, which promotes novel SC order parameters. Here we report the experimental observation of a time-reversal symmetry breaking pairing state in Re$_2$Hf resulting from FS nesting frustration. Furthermore, our electronic specific heat and transverse-field $μ$SR experiments suggest a fully gaped pairing symmetry. The first-principle electronic structure calculation reveals multiple Fermi surface sheets with comparable inter-band nesting strength. Implementing the {\it ab-initio} band structure, we compute spin-fluctuation mediated SC pairing symmetry which reveals a $s+is'$-pairing state - consistent with experimental observations. Our investigation demonstrates a novel SC state which provides a putative setting for both applied and fundamental study.

cond-mat.supr-con

Coexisting charge-ordered states with distinct driving mechanisms in monolayer VSe$_2$

Thinning crystalline materials to two dimensions (2D) creates a rich playground for electronic phases, including charge, spin, superconducting, and topological order. Bulk materials hosting charge density waves (CDWs), when reduced to ultrathin films, have shown CDW enhancement and tunability. However, charge order confined to only 2D remains elusive. Here we report a distinct charge ordered state emerging in the monolayer limit of $1T$-VSe$_2$. Systematic scanning tunneling microscopy experiments reveal that bilayer VSe$_2$ largely retains the bulk electronic structure, hosting a tri-directional CDW. However, monolayer VSe$_2$ -- consistently across distinct substrates -- exhibits a dimensional crossover, hosting two CDWs with distinct wavelengths and transition temperatures. Electronic structure calculations reveal that while one CDW is bulk-like and arises from the well-known Peierls mechanism, the other is decidedly unconventional. The observed CDW-lattice decoupling and the emergence of a flat band suggest that the new CDW could arise from enhanced electron-electron interactions in the 2D limit. These findings establish monolayer-VSe$_2$ as a host of coexisting charge orders with distinct origins, and enable the tailoring of electronic phenomena via emergent interactions in 2D materials.

cond-mat.str-el

$μ$SR study of unconventional pairing symmetry in the quasi-1D Na$_2$Cr$_3$As$_3$ superconductor

We report the finding of a novel pairing state in a newly discovered superconductor Na$_2$Cr$_3$As$_3$. This material has a noncentrosymmetric quasi-one-dimensional crystal structure and is superconducting at $T_{\mathrm{C}}\sim$ 8.0 K. We find that the magnetic penetration depth data suggests the presence of a nodal line $p_z$-wave pairing state with zero magnetic moment using transverse-field muon-spin rotation (TF-$μ$SR) measurements. The nodal gap observed in Na$_2$Cr$_3$As$_3$ compound is consistent with that observed in isostructural (K,Cs)$_2$Cr$_3$As$_3$ compounds using TF-$μ$SR measurements. The observed pairing state is consistent with a three-band model spin-fluctuation calculation, which reveals the $S_z=0$ spin-triplet pairing state with the $\sin k_z$ pairing symmetry. The long-sought search for chiral superconductivity with topological applications could be aided by such a novel triplet $S_z=0$ $p$-wave pairing state.

cond-mat.supr-con

Enhanced electron-phonon coupling in doubly aligned hexagonal boron nitride bilayer graphene heterostructure

The relative twist angle in heterostructures of two-dimensional (2D) materials with similar lattice constants result in a dramatic alteration of the electronic properties. Here, we investigate the electrical and magnetotransport properties in bilayer graphene (BLG) encapsulated between two hexagonal boron nitride (hBN) crystals, where the top and bottom hBN are rotationally aligned with bilayer graphene with a twist angle $θ_t\sim 0^{\circ} \text{and}~ θ_b < 1^{\circ}$, respectively. This results in the formation of two moiré superlattices, with the appearance of satellite resistivity peaks at carrier densities $n_{s1}$ and $n_{s2}$, in both hole and electron doped regions, together with the resistivity peak at zero carrier density. Furthermore, we measure the temperature(T) dependence of the resistivity ($ρ$). The resistivity shows a linear increment with temperature within the range 10K to 50K for the density regime $n_{s1} <n<n_{s2}$ with a large slope d$ρ$/dT $\sim$ 8.5~$Ω$/K. The large slope of d$ρ$/dT is attributed to the enhanced electron-phonon coupling arising due to the suppression of Fermi velocity in the reconstructed minibands, which was theoretically predicted, recently in doubly aligned graphene with top and bottom hBN. Our result establishes the uniqueness of doubly aligned moire system to tune the strength of electron-phonon coupling and to modify the electronic properties of multilayered heterostructures.

cond-mat.mes-hall