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Tanmoy Das

Publications and source records attributed to Tanmoy Das.

At least 55 records · Page 3Linked to original sources

Generation of strain-induced pseudo-magnetic field in a doped type-II Weyl semimetal

In Weyl semimetals, there is an intriguing possibility of realizing a pseudo-magnetic field in presence of small strain due to certain special cases of static deformations. This pseudo-magnetic field can be large enough to form quantized Landau levels and thus become observable in Weyl semimetals. In this paper, we experimentally show the emergence of a pseudo-magnetic field (~ 3 Tesla) by Scanning Tunneling Spectroscopy (STS) on the doped Weyl semimetal Re-MoTe2, where distinct Landau level oscillations in the tunneling conductance are clearly resolved. The crystal lattice is intrinsically strained where large area STM imaging of the surface reveals differently strained domains where atomic scale deformations exist forming topographic ripples with varying periodicity in the real space. The effect of pseudo-magnetic field is clearly resolved in areas under maximum strain.

cond-mat.mes-hall↗

Higgs-Axion interplay and anomalous magnetic phase diagram in TlCuCl$_3$

What is so unique in TlCuCl3 which drives so many unique magnetic features in this compound? To study these properties, here we employ a combination of ab-initio band structure, tight-binding model, and an effective quantum field theory. Within a density-functional theory (DFT) calculation, we find an unexpected bulk Dirac cone without spin-orbit coupling (SOC). Tracing back to its origin, we identify, for the first time, the presence of a Su-Schrieffer-Heeger (SSH) like dimerized Cu chain lying in the 3D crystal structure. The SSH chain, combined with SOC, stipulates an anisotropic 3D Dirac cone where chiral and helical states are intertwined. As a Heisenberg interaction is introduced, we show that the dimerized Cu sublattices of the SSH chain condensate into spin-singlet, dimerized magnets. In the magnetic ground state, we also find a topological phase, distinguished by the axion angle. Finally, to study how the topological axion term couples to magnetic excitations, we derive a Chern-Simons-Ginzburg-Landau action from the 3D SSH Hamiltonian. We find that axion term provides an additional mass term to the Higgs mode, and a lifetime to paramagnons, which are independent of the quantum critical physics. The axion-Higgs interplay can be probed with electric and magnetic field applied parallel or anti-parallel to each other.

cond-mat.str-el↗

Evidence of Nodal Line in the Superconducting Gap Symmetry of Noncentrosymmetric ThCoC$_{2}$

The newly discovered noncentrosymmetric superconductor ThCoC$_{2}$ exhibits numerous unconventional behavior in the field dependent heat capacity data. Here we present the first measurement of the gap symmetry of ThCoC$_{2}$ by muon spin rotation/relaxation $(μ$SR) measurements. Temperature dependence of the magnetic penetration depth measured using the transverse field $μ$SR measurement reveal the evidence of nodal pairing symmetry. To understand these findings, we carry out the calculations of superconducting pairing eigenvalue and eigenfunction symmetry due to the spin-fluctuation mechanism, by directly implemented the {\it ab-initio} band structures. We find that the system possesses a single Fermi surface with considerable three-dimensionality, and hence a strong nesting along the $k_z$-direction. Such a nesting promotes a superconducting pairing with a $\cos{k_z}$-like symmetry with a prominent nodal line on the $k_z=\pmπ/2$ plane. The result agrees well with the experimental data.

cond-mat.supr-con↗

Multi-band superconductivity driven by a site-selective mechanism in Mo$_8$Ga$_{41}$

The family of the endohedral gallide cluster compounds recently emerged as a new family of superconductors which is expected to host systems displaying unconventional physics. Mo$_8$Ga$_{41}$ is an important member of this family which shows relatively large $T_c \sim$ 10 K and has shown indications of strong electron-phonon coupling and multi-band superconductivity. Here, through direct measurement of superconducting energy gap by scanning tunneling spectroscopy (STS) we demonstrate the existence of two distinct superconducting gaps of magnitude 0.85 meV and 1.6 meV respectively in Mo$_8$Ga$_{41}$. Both the gaps are seen to be conventional in nature as they evolve systematically with temperature as per the predictions of BCS theory. Our band structure calculations reveal that only two specific Mo sites in an unit cell contribute to superconductivity where only $d_{xz}$/$d_{yz}$ and $d_{x^2-y^2}$ orbitals have strong contributions. Our analysis indicates that the site-elective contribution govern the two-gap nature of superconductivity in Mo$_8$Ga$_{41}$.

cond-mat.supr-con↗

Coexistence of non-Fermi liquid and Fermi liquid self-energies at all dopings in cuprates

Various angle-dependent measurements in hole-doped cuprates suggested that Non-Fermi liquid (NFL) and Fermi-liquid (FL) self-energies coexist in the Brillouin zone. Moreover, it is also found that NFL self-energies survive up to the overdoped region where the resistivity features a global FL-behavior. To address this problem, here we compute the momentum dependent self-energy from a single band Hubbard model. The self-energy is calculated self-consistently by using a momentum-dependent density-fluctuation (MRDF) method. One of our main result is that the computed self-energy exhibits a NFL-like frequency dependence only in the antinodal region, and FL-like behavior elsewhere, and retains its analytic form at all momenta and dopings. The dominant source of NFL self-energy in the antinodal region stems from the self-energy-dressed fluctuations between the itinerant and localized densities as self-consistency is invoked. We also calculate the DC conductivity by including the full momentum dependent self-energy. We find that the resistivity-temperature exponent n becomes 1 near the optimal doping, while the NFL self-energy occupies largest momentum-space volume. Surprisingly, even in the NFL state near the optimal doping, the nodal region contains FL-like self-energies; while in the under- and over-dopings (n ~ 2), the antinodal region remains NFL-like. These results highlight the non-local correlation physics in cuprates and in other similar intermediately correlated materials, where a direct link between the microscopic single-particle spectral properties and the macroscopic transport behavior can not be well established.

cond-mat.str-el↗

Direct Evidence for Time-Reversal Symmetry Breaking in Topological Superconductor Sr0.1Bi2Se3

The single helical Fermi surface on the surface state of three-dimensional topological insulator Bi2Se3 is constrained by the time-reversal invariant bulk topology to possess a spin-singlet superconducting pairing symmetry. In fact, the Cu-doped, and pressure-tuned superconducting Bi2Se3 show no evidence of the time reversal symmetry breaking. We report on the detection of the time reversal symmetry (TRS) breaking in the topological superconductor Sr0.1Bi2Se3 , probed by zero-field (ZF) μSR measurements. The TRS breaking provides strong evidence for the existence of spin-triplet pairing state. The temperature dependent super-fluid density deduced from transverse-field (TF) μSR measurement yields nodeless superconductivity with low superconducting carrier density and penetration depth λ = 1622(134) nm. From the microscopic theory of unconventional pairing, we find that such a fully gapped spin triplet pairing channel is promoted by the complex interplay between the structural hexagonal warping and higher order Dresselhaus spin-orbit coupling terms. Based on Ginzburg-Landau analysis, we delineate the mixing of singlet to triplet pairing symmetry as the chemical potential is tuned far above from the Dirac cone. Our observation of such spontaneous TRS breaking chiral superconductivity on a helical surface state, protected by the TRS invariant bulk topology, can open new avenues for interesting research and applications.

cond-mat.supr-con↗

Large Landau level splitting with tunable one-dimensional graphene superlattice probed by magneto capacitance measurements

The unique zero energy Landau Level of graphene has a particle-hole symmetry in the bulk, which is lifted at the boundary leading to a splitting into two chiral edge modes. It has long been theoretically predicted that the splitting of the zero-energy Landau level inside the {\it bulk} can lead to many interesting physics, such as quantum spin Hall effect, Dirac like singular points of the chiral edge modes, and others. However, so far the obtained splitting with high-magnetic field even on a hBN substrate are not amenable to experimental detection, and functionality. Guided by theoretical calculations, here we produce a large gap zero-energy Landau level splitting ($\sim$ 150 meV) with the usage of a one-dimensional (1D) superlattice potential. We have created tunable 1D superlattice in a hBN encapsulated graphene device using an array of metal gates with a period of $\sim$ 100 nm. The Landau level spectrum is visualized by measuring magneto capacitance spectroscopy. We monitor the splitting of the zeroth Landau level as a function of superlattice potential. The observed splitting energy is an order higher in magnitude compared to the previous studies of splitting due to the symmetry breaking in pristine graphene. The origin of such large Landau level spitting in 1D potential is explained with a degenerate perturbation theory. We find that owing to the periodic potential, the Landau level becomes dispersive, and acquires sharp peaks at the tunable band edges. Our study will pave the way to create the tunable 1D periodic structure for multi-functionalization and device application like graphene electronic circuits from appropriately engineered periodic patterns in near future.

cond-mat.mes-hall↗

Quantum phase transition in few-layer NbSe$_2$ probed through quantized conductance fluctuations

We present the first observation of dynamically modulated quantum phase transition (QPT) between two distinct charge density wave (CDW) phases in 2-dimensional 2H-NbSe$_2$. There is recent spectroscopic evidence for the presence of these two quantum phases, but its evidence in bulk measurements remained elusive. We studied suspended, ultra-thin \nbse devices fabricated on piezoelectric substrates - with tunable flakes thickness, disorder level and strain. We find a surprising evolution of the conductance fluctuation spectra across the CDW temperature: the conductance fluctuates between two precise values, separated by a quantum of conductance. These quantized fluctuations disappear for disordered and on-substrate devices. With the help of mean-field calculations, these observations can be explained as to arise from dynamical phase transition between the two CDW states. To affirm this idea, we vary the lateral strain across the device via piezoelectric medium and map out the phase diagram near the quantum critical point (QCP). The results resolve a long-standing mystery of the anomalously large spectroscopic gap in NbSe$_2$.

cond-mat.str-el↗

Localization physics in graphene Moire superlattices

Non-trivial Berry phase of graphene leads to unusual quantum correction to the conductivity. Berry phase of pi in single layer graphene (SLG) and 2pi in bi-layer graphene (BLG) is expected to reveal weak anti-localization (WAL) and weak localization (WL), respectively. However, experimentally both WAL and WL have been observed in graphene devices depending on the strength of different scattering mechanisms. Graphene superlattice having multiple Dirac cones is expected to exhibit pi to 2pi Berry phase transition from primary Dirac cone (PDC) to cloned Dirac cone (CDC). However, its effect on localization physics has not been explored yet. In this letter we present the magneto-conductance study in a hexagonal Boron-nitride (hBN)-graphene moire superlattice. Our results reveal a transition from WAL at PDC to WL at CDC in a single device by tuning the Fermi energy. The transition is supported by the quantum oscillation measurements showing a shift of pi phase from PDC to CDC and corresponding theoretical calculation capturing the Berry phase transition. Thus, our studies on localization physics in graphene superlattice pave the way to understand the carrier dynamics at multiple Dirac cones.

cond-mat.mes-hall↗

Theory of superconductivity with non-Hermitian and parity-time reversal symmetric cooper pairing symmetry

Recently developed parity (P) and time-reversal (T) symmetric non-Hermitian systems govern a rich variety of new and characteristically distinct physical properties, which may or may not have a direct analog in their Hermitian counterparts. We study here a non-Hermitian, PT-symmetric superconducting Hamiltonian that possesses real quasiparticle spectrum in the PT-region of the Brillouin zone. Within a single-band mean-field theory, we find that real quasiparticle energies are possible when the superconducting order parameter itself is either Hermitian or anti-Hermitian. Within the corresponding Bardeen-Cooper-Schrieffer (BCS) theory, we find that several properties are characteristically distinct and novel in the non-Hermitian pairing case than its Hermitian counterpart. One of our significant findings is that while a Hermitian superconductor gives a second order phase transition, the non-Hermitian one produces a robust first order phase transition. The corresponding thermodynamic properties, and the Meissner effect are also modified accordingly. Finally, we discuss how such a PT-symmetric pairings can emerge from an anti-symmetric potential, such as the Dzyloshinskii-Moria interaction, but with an external external bath, or complex potential, among others.

cond-mat.supr-con↗

Probing the Fermi surface and magnetotransport properties in MoAs$_{2}$

Transition metal dipnictides (TMDs) have recently been identified as possible candidates to host topology protected electronic band structure. These materials belong to an isostructural family and show several exotic transport properties. Especially, the large values of magnetoresistance (MR) and carrier mobility have drawn significant attention from the perspective of technological applications. In this report, we have investigated the magnetotransport and Fermi surface properties of single crystalline MoAs$_{2}$, another member of this group of compounds. Field induced resistivity plateau and a large MR have been observed, which are comparable to several topological systems. Interestingly, in contrast to other isostructural materials, the carrier density in MoAs$_{2}$ is quite high and shows single-band dominated transport. The Fermi pockets, which have been identified from the quantum oscillation, are largest among the members of this group and have significant anisotropy with crystallographic direction. Our first-principles calculations reveal a substantial difference between the band structures of MoAs$_{2}$ and other TMDs. The calculated Fermi surface consists of one electron pocket and another 'open-orbit' hole pocket, which has not been observed in TMDs so far.

cond-mat.mtrl-sci↗

Quantum spin Hall density wave insulator of correlated fermions

We present the theory of a new type of topological quantum order which is driven by the spin-orbit density wave order parameter, and distinguished by $Z_2$ topological invariant. We show that when two oppositely polarized chiral bands [resulting from the Rashba-type spin-orbit coupling $α_k$, $k$ is crystal momentum] are significantly nested by a special wavevector ${\bf Q}\sim(π,0)/(0,π)$, it induces a spatially modulated inversion of the chirality ($α_{k+Q}=α_k^*$) between different sublattices. The resulting quantum order parameters break translational symmetry, but preserve time-reversal symmetry. It is inherently associated with a $Z_2$-topological invariant along each density wave propagation direction. Hence it gives a weak topological insulator in two dimensions, with even number of spin-polarized boundary states. This phase is analogous to the quantum spin-Hall state, except here the time-reversal polarization is spatially modulated, and thus it is dubbed quantum spin-Hall density wave (QSHDW) state. This order parameter can be realized or engineered in quantum wires, or quasi-2D systems, by tuning the spin-orbit couping strength and chemical potential to achieve the special nesting condition.

cond-mat.mes-hall↗

Photo-induced SU(3) topological material of spinless fermions

Generation of topological phases of matter with SU(3) symmetry in a condensed matter setup is challenging due to the lack of an intrinsic three-fold chirality of quasiparticles. We uncover two salient ingredients required to express a three-component lattice Hamiltonian in a SU(3) format with non-trivial topological invariant. We find that all three SU(3) components must be entangled via a gauge field, with opposite chirality between any two components, and there must be band inversions between all {\it three} components in a given eigenstate. For spinless particles, we show that such chiral states can be obtained in a tripartite lattice with three inequivalent lattice sites in which the Bloch phase associated with the nearest neighbor hopping acts as $k$-space gauge field. The second and a more crucial criterion is that there must also be an odd-parity Zeeman-like term, i.e. $\sin(k)σ_z$ term where $σ_z$ is the third Pauli matrix defined in any two components of the SU(3) basis. Solving the electron-photon interaction term in a periodic potential with a modified tight-binding model, we show that such a term can be engineered with site-selective photon polarization. Such site selective polarization can be obtained in multiple ways, such as using Sisyphus cooling technique, polarizer plates, etc. With the $k$-resolved Berry curvature formalism, we delineate the relationship between the SU(3) chirality, band inversion, and $k$-space monopoles, governing finite Chern number without breaking the time-reversal symmetry. The topological phase is affirmed by edge state calculation, obeying the bulk-boundary correspondence.

cond-mat.mes-hall↗

Unusual Dirac fermions on the surface of noncentrosymmetric $α$ - BiPd superconductor

Combining multiple emergent correlated properties such as superconductivity and magnetism within the topological matrix can have exceptional consequences in garnering new and exotic physics. Here, we study the topological surface states from a noncentrosymmetric $α$-BiPd superconductor by employing angle-resolved photoemission spectroscopy (ARPES) and first principle calculations. We observe that the Dirac surface states of this system have several interesting and unusual properties, compared to other topological surface states. The surface state is strongly anisotropic and the in-plane Fermi velocity varies rigorously on rotating the crystal about the $y$-axis. Moreover, it acquires an unusual band gap as a function of $k_y$, possibly due to hybridization with bulk bands, detected upon varying the excitation energy. Coexistence of all the functional properties, in addition to the unusual surface state characteristics make this an interesting material.

cond-mat.supr-con↗

Intra-layer doping effects on the high-energy magnetic correlations in NaFeAs

We have used Resonant Inelastic X-ray Scattering (RIXS) and dynamical susceptibility calculations to study the magnetic excitations in NaFe$_{1-x}$Co$_x$As (x = 0, 0.03, and 0.08). Despite a relatively low ordered magnetic moment, collective magnetic modes are observed in parent compounds (x = 0) and persist in optimally (x = 0.03) and overdoped (x = 0.08) samples. Their magnetic bandwidths are unaffected by doping within the range investigated. High energy magnetic excitations in iron pnictides are robust against doping, and present irrespectively of the ordered magnetic moment. Nevertheless, Co doping slightly reduces the overall magnetic spectral weight, differently from previous studies on hole-doped BaFe$_{2}$As$_{2}$, where it was observed constant. Finally, we demonstrate that the doping evolution of magnetic modes is different for the dopants being inside or outside the Fe-As layer.

cond-mat.supr-con↗

Two types of superconducting domes in unconventional superconductors

Uncovering the origin of unconventional superconductivity is often plagued by the overwhelming material diversity with varying normal and superconducting (SC) properties. In this article, we deliver a comprehensive study of the SC properties and phase diagrams using multiple tunings (such as disorder, pressure or magnetic field in addition to doping and vice versa) across several families of unconventional superconductors, including the copper-oxides, heavy-fermions, organics and the recently discovered iron-pnictides, iron-chalcogenides, and oxybismuthides. We discover that all these families often possess two types of SC domes, with lower and higher superconducting transition temperatures Tc, both unconventional but with distinct SC and normal states properties. The lower Tc dome arises with or without a quantum critical point (QCP), and not always associated with a non-Fermi liquid (NFL) background. On the contrary, the higher-Tc dome clearly stems from a NFL or strange metal phase, without an apparent intervening phase transition or a QCP. The two domes appear either fully separated in the phase diagram, or merged into one, or arise independently owing to their respective normal state characteristics. Our findings suggest that a QCP-related mechanism is an unlikely scenario for the NFL phase in these materials, and thereby narrows the possibility towards short-range fluctuations of various degrees of freedom in the momentum and frequency space. We also find that NFL physics may be a generic route to higher-Tc superconductivity.

cond-mat.supr-con↗

Intrinsic large gap quantum anomalous Hall insulators in La$X$ ($X$=Br, Cl, I)

We report a theoretical prediction of a new class of bulk and intrinsic quantum Anomalous Hall (QAH) insulators La$X$ ($X$=Br, Cl, and I) via relativistic first-principle calculations. We find that these systems are innate long-ranged ferromagnets which, with the help of intrinsic spin-orbit coupling, become QAH insulators. A low-energy multiband tight binding model is developed to understand the origin of the QAH effect. Finally integer Chern number is obtained via Berry phase computation for each two-dimensional plane. These materials have the added benefit of a sizable band gap of as large as $\sim$ 25 meV, with the flexibility of enhancing it to above 75 meV via strain engineering. The synthesis of La$X$ materials will provide the impurity-free single crystals and thin-film QAH insulators for versatile experiments and functionalities.

cond-mat.mes-hall↗

Assembling topological insulators with lasers

Despite the realizations of spin-orbit (SO) coupling and synthetic gauge fields in optical lattices, the associated time-reversal symmetry breaking, and 1D nature of the observed SO coupling pose challenges to obtain intrinsic $Z_2$ topological insulator. We propose here a model optical device for engineering intrinsic $Z_2$ topological insulator which can be easily set up with the existing tools. The device is made of a periodic lattice of quantum mechanically connected atomic wires (dubbed SO wires) in which the laser generated SO coupling ($α_{\bf k}$, with ${\bf k}$ being the momentum) is reversed in every alternating wires as $\pmα_{\bf k}$. The associated small Zeeman terms are also automatically reversed in any two adjacent SO wires, which allow to effectively restore the global time-reversal (TR) symmetry. Therefore, the two SO wires serve as the TR partner to each other which is an important ingredient for $Z_2$ topological insulators according to the Kane-Mele model. These properties ensure a non-trivial $Z_2$ invariant topological insulator phase with protected edge states. We also discuss that a non-local current measurement can be used to detect the chiral edge states.

cond-mat.mes-hall↗