arXiv subjects

Tariq Leinen

Publications and source records attributed to Tariq Leinen.

3 recordsLinked to original sources

arXiv2026

Profiling THz Beams With Off-Label Use of Infrared Microbolometric Cameras

Visualizing the spatial profile of light beams is essential for evaluating irradiance, characterizing beam quality, and achieving precise alignment. In the optical spectral range, this is readily performed using silicon-based CCD and CMOS cameras. In the terahertz (THz) range, however, it typically requires specialized detectors with prohibitive costs. Here, we show that an infrared (IR) camera can be used outside of its labeled specifications to achieve similar performance as a dedicated microbolometric THz camera, at under 1% of the THz camera's cost. We compared the cameras by characterizing THz beam profiles from two sources: a pulsed broadband THz beam produced through optical rectification in organic crystals, and a narrowband quasi-continuous-wave (quasi-CW) THz beam emitted by a quantum cascade laser. For the broadband THz radiation, the beam width measured by the two cameras differed by only ~ 6%, well within the pixel resolution limit, and in the narrowband quasi-CW case by just ~ 1.3%. Additionally, the IR camera exhibits a lower minimum detectable power (down to 1.5 THz) than the THz camera, while also maintaining a linear and polarization-independent responsivity. These results expand the applicability of conventional IR cameras to the THz range, suggesting that they will become routine tools for high-fidelity THz beam diagnostics and imaging in scientific and industrial applications.

physics.optics↗

arXiv2026

Electronic excitations in the Shastry-Sutherland compound SrCu$_2$(BO$_3$)$_2$

SrCu2(BO3)2 (SCBO) is a paradigmatic realization of the Shastry-Sutherland model, hosting geometrically frustrated spin dimers and a variety of quantum magnetic phases and phenomena. Although its magnetic properties have been extensively studied, the high-energy electronic excitations that determine the crystal-field environment and Cu-O hybridization have remained largely unexplored. Here we combine Cu L3-edge resonant inelastic x-ray scattering (RIXS), broadband optical spectroscopy, and electronic-structure calculations to determine the relevant local and interband excitation energy scales in SCBO. RIXS resolves a well-defined manifold of localized Cu2+ d-d excitations between 1.8 and 2.4 eV, whose energies and polarization dependence are well reproduced by multireference quantum-chemistry calculations. In contrast, optical spectroscopy identifies charge-transfer excitations with an absorption onset near 1.2-1.6 eV and a broader higher-energy structure around 4.5 eV, which are qualitatively captured by DFT+U calculations. Taken together, these results define the characteristic energy scales of d-d and CT excitations, offering quantitative benchmarks for computational frameworks and providing essential input for refining superexchange-based magnetic models of this prototypical frustrated quantum antiferromagnet.

cond-mat.str-el↗

arXiv2020

Role of the ferroelastic strain in the optical absorption of BiVO4

Bismuth vanadate (BiVO4) has recently been under focus for its potential use in photocatalysis thanks to its well-suited absorption edge in the visible light range. Here, we characterize the optical absorption of a BiVO4 single crystal as a function of temperature and polarization direction by reflectance and transmittance spectroscopy. The optical band gap is found to be very sensitive to temperature, and to the monoclinic-to-tetragonal ferroelastic transition at 523K. The anisotropy, as measured by the difference in absorption edge for light polarized parallel and perpendicular to the principal axis, is reduced from 0.2 eV in the high-temperature tetragonal phase to 0.1 eV at ambient temperature. We show that this evolution is dominantly controlled by the ferroelastic shear strain. These findings provide a route for further optimization of bismuth-vanadate-based light absorbers in photocatalytic devices.

cond-mat.mtrl-sci↗