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Taro Nakajima

Publications and source records attributed to Taro Nakajima.

At least 19 recordsLinked to original sources
arXiv2026

Anomalous metallic states at magnetic interfaces in an antiferromagnetic topological insulator candidate DyPtBi with ferroquadrupolar order

Antiferromagnetic topological insulators provide a fertile platform where symmetry-breaking magnetic order is intertwined with topological electronic states. In particular, magnetic domain walls have attracted much attention, as they can be easily controlled by external fields as in general magnets, and moreover, host nontrivial electronic states distinct from those in bulks and sample surfaces. Here, we report a new antiferromagnetic topological insulator candidate DyPtBi, which hosts conductive magnetic domain walls controllable by uniaxial stress and magnetic field. We find that the resistivity exhibits abrupt increase upon the magnetic and structural phase transition. Concomitantly, the transverse ultrasonic mode shows remarkable softening of 6 %, indicating that the Dy 4f ferroquadrupolar order plays a vital role in the phase transition. Furthermore, we reveal by neutron experiments that applying compressive uniaxial stress aligns the magnetic domain state, leading to the strong resistivity enhancement of 14 % while eliminating the conductive magnetic domain walls. These findings demonstrate that DyPtBi exhibits topological electronic states entangled with multipolar degrees of freedom, providing a promising route for in situ control of topological properties.

cond-mat.str-el↗
arXiv2026

Carrier-tunable RKKY magnetism in a crystalline magnet

In itinerant magnets governed by the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction, the exchange coupling depends on both the moment-moment distance $r$ and the Fermi wavevector $k_{\mathrm{F}}$, yet in bulk synthesis the two are tightly coupled: a change in composition typically alters both. Here, we use a thin-film approach to tune these two variables independently in a single crystalline host. Using molecular-beam epitaxy (MBE), we stabilize either $2\times2\mathrm{R}0^\circ$ Cr$_{1/4}$NbSe$_2$ or $\sqrt{3}\times\sqrt{3}\mathrm{R}30^\circ$ Cr$_{1/3}$NbSe$_2$ within the same NbSe$_2$ host through separate growth windows. Controlled post-growth annealing performed across a series of temperatures then modifies the carrier density while leaving the Cr superstructure intact below a structural-transition threshold. The two as-grown phases are distinct in electronic structure, magnetic ground state, and transport. Along this annealing series, the Hall response evolves systematically while the magnetic response changes in a structurally insensitive manner, with ferromagnetic order emerging within the same $\sqrt{3}\times\sqrt{3}\mathrm{R}30^\circ$ structural class only above a critical annealing temperature, experimentally disentangling carrier density and moment geometry. The Hall magnitude and sign evolution point to a low-carrier-density system in which $k_{\mathrm{F}}$ is susceptible to modest external tuning. Cr-NbSe$_2$ thus realizes carrier-sensitive RKKY magnetism in a single crystalline host, within an MBE-plus-annealing approach extensible across the intercalated transition-metal dichalcogenide family.

cond-mat.str-el↗
arXiv2026

Uniaxial stress effects on magnetic and electric properties of the ground state in a centrosymmetric magnetic skyrmion host Gd$_2$PdSi$_3$

We investigate effects of uniaxial stress to magnetic orders and electrical resistivity of the centrosymmetric magnetic skyrmion compound Gd$_2$PdSi$_3$, which has a hexagonal crystal structure composed of triangular lattice layers of magnetic Gd$^{3+}$ ions. This compound is known to exhibit the triple-$q$ magnetic skyrmion lattice phase with a giant topological Hall effect in the first field induced phase [T. Kurumaji $\textit{et al}$. Science $\textbf{365}$, 914-918 (2019)]. In contrast to the established picture of the field-induced phase, the ground state of this system still remains to be studied. Although previous studies reported the existence of the incommensurate magnetic modulations described by a magnetic modulation wave vector ${\bf q}=(q,0,0)$ where $q\sim 0.14$ and its equivalents, it is still unclear whether the magnetic structure is a single-$q$ structure or a multiple-$q$ structure. In the present study, we performed magnetization, resistivity and neutron diffraction measurements with a compressive uniaxial stress applied perpendicular to the $c$ axis. The observed data revealed that the system did not exhibit anisotropic magnetic and electric properties expected from a single-$q$ magnetic order, suggesting that the magnetic ground state of this system is a multi-$q$ magnetic order.

cond-mat.str-el↗
arXiv2026

Observation of an emergent energy scale close to dimensional reduction in a quasi-two-dimensional quantum magnet

By appropriately perturbing a critical transverse-field Ising chain away from its critical point, the system can develop a finite correlation length with a characteristic purely massive spectrum, whose ratios and correlations are precisely described by an integrable field theory and an infinite set of integrals of motion corresponding to the $E_8$ Lie algebra. In this work, we report on experimental observation of a characteristic massive spectrum close to transverse field-induced dimensional reduction in a quasi-two-dimensional quantum magnet Cu$_2$(OH)$_3$Br, providing evidence for an emergent $E_8$ symmetry and the corresponding excitations of bound states in the sublattice of its ferromagnetic chains. These results demonstrate the power of integrable field theory in describing emergent many-body quantum critical phenomena in condensed matter systems.

cond-mat.str-el↗
arXiv2026

Zero-field magnetic structure of the antiferromagnetic metal EuSnP

We investigated the zero-field magnetic structure of the antiferromagnetic metal EuSnP through single-crystal neutron diffraction experiments. The magnetic propagation vector in the magnetically ordered phase was determined to be $(0,0,1/2)$, indicating that commensurate antiferromagnetic ordering is realized in this material. The detailed magnetic structure analysis revealed a collinear A-type antiferromagnetic structure with ferromagnetic alignment of Eu$^{2+}$ moments within the Eu--P layer. The present findings provide a microscopic basis for understanding the intriguing magnetic behaviors of EuSnP, as exemplified by the multiple metamagnetic transitions in the antiferromagnetic state and the strong pressure dependence of the magnetic transition temperature.

cond-mat.str-el↗
arXiv2026

Dominant in-plane anomalous Hall effect in a monoclinic room-temperature ferromagnet

Ferromagnetic metals are characterized by enhanced dissipationless transverse transport responses via the anomalous Hall effect, offering a route towards magnetic sensing and spintronic readout functionalities. In most ferromagnets, the anomalous Hall current is constrained to lie in the plane perpendicular to the magnetization (or applied magnetic field). Recently, it has been recognized that selected symmetries can also permit a Hall response in a traditionally forbidden configuration, where the Hall current lies in the same plane as the magnetization, realizing an in-plane anomalous Hall effect. Reported realizations of this effect, however, are typically much weaker than the conventional Hall response in the same material. Here, through engineering specific crystallographic mirror symmetry-breaking, we realize a strongly enhanced in-plane anomalous Hall response in monoclinic Cr3Te4 with room-temperature ferromagnetism. Remarkably, the in-plane anomalous Hall signal exceeds the out-of-plane response by a factor of five, with which we demonstrate a unique in-plane field and current sensing functionality. Combined with density functional theory calculations, our results establish low-crystalline-symmetry ferromagnets with near-Fermi-level Weyl points as a practical platform for symmetry-engineered Hall responses, and point to a route towards room-temperature, geometry-flexible sensing devices.

cond-mat.mtrl-sci↗
arXiv2026

Magnetoelastic mapping of the high-field phase diagram in the topological cubic helimagnet SrFeO$_{3}$

The cubic perovskite SrFeO$_{3}$ is a prototypical centrosymmetric itinerant magnet that hosts a quadruple-${\mathbf Q}$ hedgehog-antihedgehog lattice and exhibits a complex magnetic-field-temperature phase diagram. Yet, the microscopic mechanism underlying the emergence of its versatile multiple-${\mathbf Q}$ phases remains unresolved. Here, we reveal the field-orientation dependence of the magnetic phase diagram and establish an effective spin Hamiltonian for SrFeO$_{3}$ that incorporates a cubic single-ion anisotropy together with bilinear and biquadratic interactions in momentum space, which originate from the spin-charge coupling. In addition, we observe magnetoelastic signatures of a redistribution of the ligand-hole density upon entering the forced ferromagnetic phase. These findings emphasize the pivotal importance of electronic itinerancy arising from the formation of a ligand-hole band in stabilizing multiple-${\mathbf Q}$ phases.

cond-mat.str-el↗
arXiv2026

Observation of Altermagnetic Order Switching in Bulk MnTe by Polarized Neutron Diffraction

Altermagnetic order, characterized by the Néel vector, breaks time-reversal symmetry (TRS) even in the nonrelativistic limit. Although spin-polarized and anomalous transport phenomena emerge with this order, they are mutually compensated by TRS-connected antiphase domains with opposite Néel vectors. Here we employ polarized neutron diffraction to directly probe the altermagnetic order in MnTe. Pronounced nuclear-magnetic interference terms were observed, providing direct evidence of a net Néel vector in the bulk crystal. Moreover, a weak ferromagnetic moment (WFM), originating from relativistic spin-orbit coupling, was found to be coupled with the altermagnetic order. Both the altermagnetic order and the WFM can be switched by milli-Tesla-scale magnetic field cooling.

cond-mat.str-el↗
arXiv2026

Collinear ferromagnetism with reduced moment length in kagome magnet Nd3Ru4Al12

We determine the magnetic ground state of the kagome lattice magnet Nd3Ru4Al12 by single-crystal neutron diffraction, supported by experiments with polarized neutrons. We identify this material as a collinear ferromagnet ("hex-FM") with uniform moment length mc = 2.1 {\mu}B/Nd and ordering vector Q = 0, in contrast to a previous, seminal report that proposed unequal moment lengths on two Nd sites, here called the "ortho-FM" state. Our analysis of the flipping ratio in polarized neutron scattering is consistent with the hex-FM state. The results provide a microscopic basis for understanding the large fluctuation-induced Hall and Nernst responses near TC = 41 K, as previously reported for Nd3Ru4Al12.

cond-mat.str-el↗
arXiv2026

Probing the real-space density of spin-entangled electrons

On the textbook example of an isolated antiferromagnetic Heisenberg dimer, we demonstrate that the magnetic form factor and the magnetic electron density distribution can be extracted from the momentum-dependence of the inelastic neutron scattering (INS) intensity of a magnetic excitation. We measure the three-dimensional (3D) magnetic structure factor of the singlet-to-triplet excitation in Cu(II) acetate monohydrate with INS. Using a minimal parametrization of the magnetic electron density, we deduce the real-space density of the spin-entangled electrons and the transfer of magnetic electron density between metal and ligand atoms from the experimental data. Density functional theory (DFT) calculations reproduce the measured structure factor quantitatively, providing a direct validation of DFT broken-symmetry spin densities against full 3D INS data. The quantitative agreement between experiment, parametrization, and theory establishes a robust framework for determining magnetic form factors and the magnetic electron density in a broad range of magnetic materials and demonstrates INS as a probe of the envelope of spatial electronic wavefunctions.

cond-mat.str-el↗
arXiv2026

Magnetic order and excitations in the magnetically intercalated van der Waals material Cr$_{\frac{1}{4}}$NbSe$_2$

Cr$_{\frac{1}{4}}$NbSe$_2$ is a triangular lattice magnet in which magnetic Cr$^{3+}$ ions are intercalated to form triangular lattices between NbSe$_2$ van der Waals layers stacked along the c axis. By unpolarized and polarized neutron scattering experiments, we have revealed that the magnetic ground state of this system is a 120$^{\circ}$-type antiferromagnetic order characterized by the magnetic propagation wave vector of $q=(\frac{1}{3}, \frac{1}{3}, 0)$. We also performed inelastic neutron scattering measurements using co-aligned single crystals, and determined dispersion relations of magnetic excitations at low temperatures. Comparing the observed spectra with calculations based on the linear spin-wave theory, we revealed that the out-of-plane ferromagnetic interaction is fairly strong as compared to the in-plane nearest neighbor antiferromagnetic interaction. Although the crystal structure of this system is composed of two-dimensional van der Waals layers, the magnetic order has a three dimensional character, which would be attributed to long-range magnetic interactions mediated by conduction electrons.

cond-mat.str-el↗
arXiv2026

Stripe antiferromagnetism in van der Waals metal HoTe3 decoupled from charge density wave order

The $R\mathrm{Te}_3$ ($R = \text{rare earth}$) family of layered van der Waals (vdW) compounds hosts coexisting magnetic and charge density wave (CDW) orders, yet the interplay between these degrees of freedom remains little explored. Combining polarized and unpolarized neutron diffraction on single-crystal $\mathrm{HoTe}_3$, we identify two distinct antiferromagnetic (AFM) phases, both exhibiting a collinear $\uparrow\uparrow\downarrow\downarrow$ motif within individual vdW layers. The two phases are distinguished by the vdW stacking of magnetic layers: ferromagnetic (FM) stacking in the higher-temperature AFM-II phase, here termed ``vertical-stripe'', and AFM stacking in the AFM-I ground state, here termed ``tilted-stripe''; the two phases have propagation vectors $\boldsymbol{q}_{\mathrm{m2}} = (0.48, 0, 0)$ and $\boldsymbol{q}_{\mathrm{m1}} = (0.5, 0.5, 0)$, respectively. In contrast to the CDW-driven exotic magnetism in $\mathrm{DyTe}_3$, $\mathrm{TbTe}_3$, and $\mathrm{GdTe}_3$, we find no evidence for coupling between magnetism and CDW in $\mathrm{HoTe}_3$. The relative alignment between AFM and CDW propagation vectors, as well as single-ion anisotropy, are likely essential for generating coupled spin/charge orders in layered vdW systems.

cond-mat.str-el↗
arXiv2026

Effect of uniaxial stress on helimagnetic phases in the square-lattice itinerant magnet EuAl$_{4}$

We investigate uniaxial-stress effects on the magnetic phase diagram of the square-lattice itinerant magnet EuAl$_{4}$, where strong coupling among spin, lattice, and charge produces a variety of helimagnetic phases, including rhombic and square skyrmion lattices. Combining resistivity and magnetization measurements with neutron scattering, we find that compressive stresses of only several tens of megapascal along [010] enhance antiferromagnetic character and shorten the magnetic modulation period in the lowest-temperature single-Q spiral state, thereby driving the critical temperatures and fields of multiple phases to higher values. First-principles calculations show that increasing orthorhombic lattice distortion deforms the Fermi surface relevant to the magnetism, providing compelling evidence that Fermi-surface nesting plays a crucial role in stabilizing the helical magnetic modulations in EuAl$_{4}$.

cond-mat.str-el↗
arXiv2026

Emergent electric field induced by dissipative sliding dynamics of domain walls in a Weyl magnet

The dynamic motion of topological defects in magnets induces an emergent electric field, as exemplified by the continuous flow of skyrmion vortices. However, the electrodynamics underlying this emergent field remains poorly understood. In this context, magnetic domain walls - one dimensional topological defects with two collective modes, sliding and spin tilt - offer a promising platform for exploration. Here, we demonstrate that the dissipative motion of domain walls under oscillatory current excitation generates an emergent electric field. We image domain patterns and quantify domain wall length under applied magnetic fields in mesoscopic devices based on the magnetic Weyl semimetal NdAlSi. These devices exhibit exceptionally strong domain wall scattering and a pronounced emergent electric field, observed in the imaginary component of the complex impedance. Spin dynamics simulations reveal that domain wall sliding dominates over spin tilting, where the phase delay of the domain wall motion with respect to the driving force impacts the emergent electric field. Our findings establish domain-wall dynamics as a platform for studying emergent electromagnetic fields and motivate further investigations on the coupled motion of magnetic solitons and conduction electrons.

cond-mat.mes-hall↗
arXiv2025

Skyrmion and Meron Crystals in Intermetallic Gd$_3$Ru$_4$Al$_{12}$: Microscopic Model Insights into Chiral Phases

Topological spin textures in frustrated intermetallics hold great promise for spintronics applications. However, understanding their origin and properties remains a significant challenge due to competing and often long-range interactions mediated by conduction electrons. Here, by combining neutron scattering experiments with theoretical modeling via unprecedented multi-target fits that further incorporate the ferromagnentic resonance data and magnetization curve, we construct a realistic microscopic model for the prototypical intermetallic skyrmion host \text{Gd}$_3$\text{Ru}$_4$\text{Al}$_{12}$. Beyond magnetic frustration, we identify the competition between dipolar interactions and easy-plane single-ion anisotropy as a key ingredient for stabilizing the rich chiral magnetic phases observed in this compound -- including a hexagonal skyrmion crystal and two distinct meron crystals. Remarkably, the meron crystal in lower field is revealed to be commensurate with the underlying lattice, and its unique three-meron-one-antimeron spin texture is verified by the polarized x-ray diffraction data. At elevated temperatures, the short-range spin correlations in \text{Gd}$_3$\text{Ru}$_4$\text{Al}$_{12}$ are well described by a codimension-two spiral spin-liquid. Perturbations from staggered Dzyaloshinskii-Moriya interactions give rise to chiral fluctuations that account for the temperature and field dependence of the anomalous Hall response. Our results highlight the unique power of neutron scattering, especially when combined with complementary experimental techniques, to unravel complex magnetic phase transitions and provide new insights into the rich variety of topological spin textures in frustrated systems.

cond-mat.str-el↗
arXiv2025

Metallic $p$-wave magnet with commensurate spin helix

Antiferromagnetic states with spin-split electronic structure give rise to novel spintronic, magnonic, and electronic phenomena despite (near-) zero net magnetization. The simplest odd-parity spin splitting - $p$-wave - was originally proposed to emerge from a collective instability in interacting electron systems. Recent theory identifies a distinct route to realise $p$-wave spin-split electronic bands without strong correlations, termed $p$-wave magnetism. Here we demonstrate an experimental realisation of a metallic $p$-wave magnet. The odd-parity spin splitting of delocalised conduction electrons arises from their coupling to an antiferromagnetic texture of localised magnetic moments: a coplanar spin helix whose magnetic period is an even multiple of the chemical unit cell, as revealed by X-ray scattering experiments. This texture breaks space inversion symmetry but preserves time-reversal ($T$) symmetry up to a half-unit-cell translation - thereby fulfilling the symmetry conditions for $p$-wave magnetism. Consistent with theoretical predictions, our $p$-wave magnet exhibits a characteristic anisotropy in the electronic conductivity. Relativistic spin-orbit coupling and a tiny spontaneous net magnetization further break $T$ symmetry, resulting in a giant anomalous Hall effect (AHE, $σ_{xy}>600\,$S/cm, Hall angle $>3\,\%$), for an antiferromagnet. Our model calculations show that the spin nodal planes found in the electronic structure of $p$-wave magnets are readily gapped by a small perturbation to induce the AHE.

cond-mat.str-el↗
arXiv2024

Giant Hall effect in a highly conductive frustrated magnet GdCu$_2$

The Hall effect is one of the most fundamental but elusive phenomena in condensed matter physics due to the rich variety of underlying mechanisms. Here we report an exceptionally large Hall effect in a frustrated magnet GdCu$_2$ with high conductivity. The Hall conductivity at the base temperature is as high as 4 x 10$^4$ $Ω^{-1}$cm$^{-1}$ and shows abrupt sign changes under magnetic fields. Remarkably, the giant Hall effect is rapidly suppressed as the longitudinal conductivity is lowered upon increasing temperature or introducing tiny amount of quenched disorder. Our systematic transport measurements together with neutron scattering measurements and ab initio band calculations indicate that the unusual Hall effect can be understood in terms of spin-splitting induced emergence/disappearance of Fermi pockets as well as skew scattering from spin-chiral cluster fluctuations in a field-polarized state. The present study demonstrates complex interplay among magnetization, spin-dependent electronic structure, and spin fluctuations in producing the giant Hall effect in highly conductive frustrated magnets.

cond-mat.str-el↗
arXiv2024

Spin-lattice-coupled helical magnetic order in breathing pyrochlore magnets, CuAlCr$_{4}$S$_{8}$ and CuGaCr$_{4}$S$_{8}$

We report low-temperature powder X-ray and neutron diffraction studies on breathing pyrochlore magnets Cu$M$Cr$_{4}$S$_{8}$ ($M$ = Al, Ga), which undergo a magnetic transition at $T_{\rm N} \approx$ 21 and 31 K for {$M$ = Al and Ga, respectively. X-ray diffraction reveals that the magnetic transition accompanies a structural transition from cubic $F{\overline 4}3m$ to polar orthorhombic $Imm2$ symmetry for both the compounds, with larger distortion observed for $M$ = Ga at low temperatures. Neutron diffraction reveals incommensurate magnetic modulation ${\mathbf Q} = (q_{\rm IC}, 0.5, 0)$ in the orthorhombic setting, where $q_{\rm IC} \approx$ 0.39 and 0.31 for $M$ = Al and Ga, respectively. Our magnetic-structure analysis suggests cycloid-type magnetic order but not proper-screw type for both the compounds. We find strong correlation between the local spin configuration and Cr-Cr bond lengths, indicating that the spin-lattice coupling as well as the magnetic frustration play an important role in determining the ground state. Cu$M$Cr$_{4}$S$_{8}$ potentially offers a platform to explore magnetoelectric effects arising from the helimagnet driven electric polarity.

cond-mat.mtrl-sci↗