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Tatsuma D. Matsuda

Publications and source records attributed to Tatsuma D. Matsuda.

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High-Field Fermi Surface Properties in the Low Carrier Heavy Fermion Compound URu2Si2

We performed the Shubnikov-de Haas (SdH) experiments of the low carrier heavy fermion compound URu2Si2 at high fields up to 34T and at low temperatures down to 30mK. All main SdH branches named alpha, beta and gamma were observed for all the measured field-directions (H // [001] -> [100], [100] -> [110] and [001] -> [110]), indicating that these are attributed to the closed Fermi surfaces with nearly spherical shapes. Anomalous split of branch alpha was detected for the field along the basal plane, and the split immediately disappears by tilting the field to [001] direction, implying a fingerprint of the hidden order state. High field experiments reveal the complicated field-dependence of the SdH frequencies and the cyclotron masses due to the Zeeman spin-splitting associated with the Fermi surface reconstruction in the hidden order state with small carrier numbers. A new SdH branch named omega with large cyclotron mass of 25m0 was detected at high fields above 23T close to the hidden order instabilities.

cond-mat.str-el↗

Field-induced Phenomena in Ferromagnetic Superconductors UCoGe and URhGe

We review our recent studies on ferromagnetic superconductors, UGe2, URhGe and UCoGe, where the spin-triplet state with the so-called equal spin pairing is realized. We focus on experimental results of URhGe and UCoGe in which the superconductivity occurs already at ambient pressure. The huge upper critical field Hc2 on UCoGe for the field along the hard magnetization axis (b-axis) is confirmed by the AC susceptibility measurements by the fine tuning of field angle. Contrary to the huge Hc2 along the hard-magnetization axis, Hc2 along the easy-magnetization axis (c-axis) is relatively small in value. However, the initial slope of Hc2, namely dHc2/dT (H -> 0) both in UCoGe and in URhGe indicates the large value, which can be explained by the magnetic domain effect detected in the magnetization measurements. The specific heat measurements using a high quality single crystal of UCoGe demonstrate the bulk superconductivity, which is extended under magnetic field for the field along c-axis.

cond-mat.str-el↗

Details of Sample Dependence and Transport Properties of URu2Si2

Resistivity and specific heat measurements were performed in the low carrier unconventional superconductor URu2Si2 on various samples with very different qualities. The superconducting transition temperature (TSC) and the hidden order transition temperature (THO) of these crystals were evaluated as a function of the residual resistivity ratio (RRR). In high quality single crystals the resistivity does not seem to follow a T2 dependence above TSC, indicating that the Fermi liquid regime is restricted to low temperatures. However, an analysis of the isothermal longitudinal magnetoresistivity points out that the T2 dependence may be "spoiled" by residual inhomogeneous superconducting contribution. We discuss a possible scenario concerning the distribution of TSC related with the fact that the hidden order phase is very sensitive to the pressure inhomogeneity.

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Strong Longitudinal Magnetic Fluctuations near Critical End Point in UCoAl: A ^59Co-NMR Study

We report ^59Co-NMR measurements in UCoAl where a metamagnetism occurs due to enhancement of ferromagnetism by magnetic field. The metamagnetic transition from a paramagnetic (PM) state to a ferromagnetic state is a first order transition at low temperatures, but it changes to a crossover at high temperatures on crossing the critical end pint (CEP) at T_CEP ~ 12 K. The contrasting behavior between the relaxation rates 1/T_1 and 1/T_2 suggests that the longitudinal magnetic fluctuation of U moment is strongly enhanced especially near the CEP. A wide diffusion of the fluctuation from the CEP can be confirmed even in the PM state where the magnetic transition does not occur.

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Ferromagnetic Quantum Critical Endpoint in UCoAl

Resistivity and magnetostriction measurements were performed at high magnetic fields and under pressure on UCoAl. At ambient pressure, the 1st order metamagnetic transition at H_m ~ 0.7 T from the paramagnetic ground state to the field-induced ferromagnetic state changes to a crossover at finite temperature T_0 ~11 K. With increasing pressure, H_m linearly increases, while T_0 decreases and is suppressed at the quantum critical endpoint (QCEP, P_QCEP ~ 1.5 GPa, H_m ~ 7 T). At higher pressure, the value of H_m identified as a crossover continuously increases, while a new anomaly appears above P_QCEP at higher field H* in resistivity measurements. The field dependence of the effective mass (m*) obtained by resistivity and specific heat measurements exhibits a step-like drop at H_m at ambient pressure. With increasing pressure, it gradually changes into a peak structure and a sharp enhancement of m* is observed near the QCEP. Above P_QCEP, the enhancement of m* is reduced, and a broad plateau is found between H_m and H*. We compare our results on UCoAl with those of the ferromagnetic superconductor UGe2 and the itinerant metamagnetic ruthenate Sr3Ru2O7.

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Properties of Ferromagnetic Superconductors

Thanks to the discovery in the last decade of three uranium ferromagnetic superconductors, UGe2, URhGe and UCoGe, the fascinating aspects of the interplay between the triplet state of Cooper pairing and ferromagnetism have emerged. Furthermore, as the ferromagnetic properties in the normal state are quite different with respect to the proximity of the ferromagnetic-paramagnetic instabilities, the feedback with the coexistence of superconductivity gives rise to quite different boundaries in pressure and magnetic field. Special attention is given on the location of the materials with respect to the tricriticality and on the reinforcement of superconductivity in a transverse field response with respect to the direction of the ferromagnetic sublattice magnetization. The other facts of the interplay between ferromagnetism and superconductivity is briefly mentioned.

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Pressure Evolution of the Magnetic Field induced Ferromagnetic Fluctuation through the Pseudo-Metamagnetism of CeRu2Si2

Resistivity measurements performed under pressure in the paramagnetic ground state of CeRu2Si2 are reported. They demonstrate that the relative change of effective mass through the pseudo metamagnetic transition is invariant under pressure. The results are compared with the first order metamagnetic transition due to the antiferromagnetism of Ce0.9La0.1Ru2Si2 which corresponds to the "negative" pressure of CeRu2Si2 by volume expansion. Finally, we describe the link between the spin-depairing of quasiparticles on CeRu2Si2 and that of Cooper pairs on the unconventional heavy fermion superconductor CeCoIn5.

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Magnetic Field and Pressure Phase Diagrams of Uranium Heavy-Fermion Compound U$_2$Zn$_{17}$

We have performed magnetization measurements at high magnetic fields of up to 53 T on single crystals of a uranium heavy-fermion compound U$_2$Zn$_{17}$ grown by the Bridgman method. In the antiferromagnetic state below the Néel temperature $T_{\rm N}$ = 9.7 K, a metamagnetic transition is found at $H_c$ $\simeq$ 32 T for the field along the [11$\bar{2}$0] direction ($a$-axis). The magnetic phase diagram for the field along the [11$\bar{2}$0] direction is given. The magnetization curve shows a nonlinear increase at $H_m$ $\simeq$ 35 T in the paramagnetic state above $T_{\rm N}$ up to a characteristic temperature $T_{χ{\rm max}}$ where the magnetic susceptibility or electrical resistivity shows a maximum value. This metamagnetic behavior of the magnetization at $H_m$ is discussed in comparison with the metamagnetic magnetism of the heavy-fermion superconductors UPt$_3$, URu$_2$Si$_2$, and UPd$_2$Al$_3$. We have also carried out high-pressure resistivity measurement on U$_2$Zn$_{17}$ using a diamond anvil cell up to 8.7 GPa. Noble gas argon was used as a pressure-transmitting medium to ensure a good hydrostatic environment. The Néel temperature $T_{\rm N}$ is almost pressure-independent up to 4.7 GPa and starts to increase in the higher-pressure region. The pressure dependences of the coefficient of the $T^2$ term in the electrical resistivity $A$, the antiferromagnetic gap $Δ$, and the characteristic temperature $T_{ρ{\rm max}}$ are discussed. It is found that the effect of pressure on the electronic states in U$_2$Zn$_{17}$ is weak compared with those in the other heavy fermion compounds.

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Superconductivity Reinforced by Magnetic Field and the Magnetic Instability in Uranium Ferromagnets

We review our recent results on ferromagnetic superconductors, URhGe and UCoGe. High quality single crystals of both compounds were successfully grown. The specific heat shows a clear jump related to the superconducting transition in UCoGe. The finite values of C/T at 0K are discussed in terms of the self-induced vortex state and the value of the ordered moment. With increasing fields for H // b-axis in URhGe, the jump of thermal expansion increases and shifts to lower temperature. The re-entrant and S-shaped superconducting phases for URhGe and UCoGe respectively are explained by the unusual field dependence of the effective mass, which is induced by the ferromagnetic instability when the field is applied along the hard magnetization b-axis. The magnetic fluctuations are very sensitive to the field orientation. This is reflected in the Hc2 and the anisotropy of the effective mass.

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First Observation of Quantum Oscillations in the Ferromagnetic Superconductor UCoGe

We succeeded in growing high quality single crystals of the ferromagnetic superconductor UCoGe and measured the magnetoresistance at fields up to 34T. The Shubnikov-de Haas signal was observed for the first time in a U-111 system (UTGe, UTSi, T: transition metal). A small pocket Fermi surface (F~1kT) with large cyclotron effective mass 25m0 was detected at high fields above 22T, implying that UCoGe is a low carrier system accompanyed with heavy quasi-particles. The observed frequency decreases with increasing fields, indicating that the volume of detected Fermi surface changes nonlinearly with field. The cyclotron mass also decreases, which is consistent with the decrease of the A coefficient of resistivity.

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Extremely Large and Anisotropic Upper Critical Field and the Ferromagnetic Instability in UCoGe

Magnetoresistivity measurements with fine tuning of the field direction on high quality single crystals of the ferromagnetic superconductor UCoGe show anomalous anisotropy of the upper critical field H_c2. H_c2 for H // b-axis (H_c2^b) in the orthorhombic crystal structure is strongly enhanced with decreasing temperature with an S-shape and reaches nearly 20 T at 0 K. The temperature dependence of H_c2^a shows upward curvature with a low temperature value exceeding 30 T, while H_c2^c at 0 K is very small (~ 0.6 T). Contrary to conventional ferromagnets, the decrease of the Curie temperature with increasing field for H // b-axis marked by an enhancement of the effective mass of the conduction electrons appears to be the origin of the S-shaped H_c2^b curve. These results indicate that the field-induced ferromagnetic instability or magnetic quantum criticality reinforces superconductivity.

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Thermodynamic Studies on Non Centrosymmetric Superconductors by AC Calorimetry under High Pressures

We investigated the non centrosymmetric superconductors CePt$_3$Si and UIr by the ac heat capacity measurement under pressures. We determined the pressure phase diagrams of these compounds. In CePt$_3$Si, the Néel temperature $T_{\rm N}$ = 2.2 K decreases with increasing pressure and becomes zero at the critical pressure $P_{\rm AF}$ $\simeq$ 0.6 GPa. On the other hand, the superconducting phase exists in a wider pressure region from ambient pressure to $P_{\rm AF}$ $\simeq$ 1.5 GPa. The phase diagram of CePt$_3$Si is very unique and has never been reported before for other heavy fermion superconductors. In UIr, the heat capacity shows an anomaly at the Curie temperature $T_{\rm C1}$ = 46 K at ambient pressure, and the heat capacity anomaly shifts to lower temperatures with increasing pressure. The present pressure dependence of $T_{\rm C1}$ was consistent with the previous studies by the resistivity and magnetization measurements. Previous ac magnetic susceptibility and resistivity measurements suggested the existence of three ferromagnetic phases, FM1-3. $C_{\rm ac}$ shows a bending structure at 1.98, 2.21, and 2.40 GPa .The temperatures where these anomalies are observed are close to the phase boundary of the FM3 phase.

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High pressure study on the strong-coupling superconductivity in non-centrosymmetric compound CeIrSi_3

We have carried out high pressure experiment on the pressure-induced superconductor CeIrSi$_3$ without inversion center. The electrical resistivity and ac heat capacity were measured in the same run for the same sample. The critical pressure of the antiferromagnetic state was determined to be $P_{\rm c}$ = 2.25 GPa. The heat capacity $C_{\rm ac}$ shows both antiferromagnetic and superconducting transitions at pressures close to $P_{\rm c}$. The superconducting transition temperature $T_{\rm sc}$ shows a maximum value of 1.6 K around $2.5-2.7$ GPa. At 2.58 GPa, a large heat capacity anomaly was observed at $T_{\rm sc}$ = 1.59 K. The jump of the heat capacity in the form of $Δ{C_{\rm ac}}/C_{\rm ac}(T_{\rm sc})$ is 5.7 $\pm$ 0.1. This is the largest value observed among all superconductors studied previously, suggesting the strong-coupling superconductivity in CeIrSi$_3$. The large magnitude and anisotropy of the upper critical field $B_{\rm c2}$ at 2.65 GPa is discussed from view points of the strong-coupling superconductivity and the reduced paramagnetic effect in the non-centrosymmetric superconductor. Above $P_{\rm c}$, the electrical resistivity shows the anomalous $T$-linear dependence in the wide temperature region from $T_{\rm sc}$ to 30 K, which is different from the Fermi liquid theory. Meanwhile, the heat capacity $C_{\rm ac}/T$ shows a simple temperature dependence in the normal state above $T_{\rm sc}$. These features do not seem to be explained simply by the spin fluctuation theory. The electronic specific heat coefficient at $T_{\rm sc}$ is approximately unchanged as a function of pressure, even at $P_{\rm c}$.

cond-mat.supr-con↗

Strong-Coupling Superconductivity of CeIrSi$_3$ with the Non-centrosymmetric Crystal Structure

We studied the pressure-induced superconductor CeIrSi$_3$ with the non-centrosymmetric tetragonal structure under high pressure. The electrical resistivity and ac heat capacity were measured in the same run for the same sample. The critical pressure was determined to be $P_{\rm c}$ = 2.25 GPa, where the antiferromagnetic state disappears. The heat capacity $C_{\rm ac}$ shows both antiferromagnetic and superconducting transitions at pressures close to $P_{\rm c}$. On the other hand, the superconducting region is extended to high pressures of up to about 3.5 GPa, with the maximum transition temperature $T_{\rm sc}$ = 1.6 K around $2.5-2.7$ GPa. At 2.58 GPa, a large heat capacity anomaly was observed at $T_{\rm sc}$ = 1.59 K. The jump of the heat capacity in the form of $Δ{C_{\rm ac}}/C_{\rm ac}(T_{\rm sc})$ is 5.7 $\pm$ 0.1. This is the largest observed value among previously reported superconductors, indicating the strong-coupling superconductivity. The electronic specific heat coefficient at $T_{\rm sc}$ is, however, approximately unchanged as a function of pressure, even at $P_{\rm c}$.

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Itinerant U 5f band states in the layered compound UFeGa5 observed by soft X-ray angle-resolved photoemission spectroscopy

We have performed angle-resolved photoemission spectroscopy (ARPES) experiments on paramagnetic UFeGa5 using soft X-ray synchrotron radiation (hn=500eV) and derived the bulk- and U 5f-sensitive electronic structure of UFeGa5. Although the agreement between the experimental band structure and the LDA calculation treating U 5f electrons as being itinerant is qualitative, the morphology of the Fermi surface is well explained by the calculation, suggesting that the U 5f states can be essentially understood within the itinerant-electron model.

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Novel Pressure Phase Diagram of Heavy Fermion Superconductor CePt$_{3}$Si Investigated by ac Calorimetry

The pressure dependences of the antiferromagnetic and superconducting transition temperatures have been investigated by ac heat capacity measurement under high pressures for the heavy-fermion superconductor CePt$_3$Si without inversion symmetry in the tetragonal structure. The Néel temperature $T_{\rm N}$ = 2.2 K decreases with increasing pressure and becomes zero at the critical pressure $P_{\rm AF}$ $\simeq$ 0.6 GPa. On the other hand, the superconducting phase exists in a wider pressure region from ambient pressure to about 1.5 GPa. The pressure phase diagram of CePt$_3$Si is thus very unique and has never been reported before for other heavy fermion superconductors.

cond-mat.supr-con↗