arXiv subjects

Tatsuro Yuge

Publications and source records attributed to Tatsuro Yuge.

At least 19 recordsLinked to original sources

arXiv2026

Electron-Photon Spatial Entanglement in Coherent Cathodoluminescence

Electron--photon quantum entanglement in an electron microscope paves the way for a new quantum platform, enabling the integration of quantum functionalities into electron microscopy and opening opportunities for quantum imaging and quantum sensing at the nanoscale. To realize such a platform, it is crucial to understand the degree and nature of electron--photon entanglement in cathodoluminescence (CL). However, its dependence on electron-beam properties, particularly transverse coherence, remains unclear. Here, we present a theoretical framework describing the quantum state of an electron--photon pair generated in coherent CL from a system with translational invariance in the plane perpendicular to the electron beam, as can be realized, for example, in transition radiation at a planar interface. By expressing the scattered state directly in terms of the luminescence spectrum, we evaluate the entanglement using both subsystem purity and an Einstein--Podolsky--Rosen-type criterion. These two measures enable a clear distinction among wave-like, particle-like, and classical regimes in terms of spatial and momentum entanglement in the electron--photon system. Our analysis identifies the roles of the electron's transverse and longitudinal coherence, as well as the photon's spectral width, and reveals the conditions under which strong spatial entanglement emerges. This unified perspective clarifies the nature of electron--photon quantum correlations in coherent CL and advances the development of quantum-enabled functionalities in electron microscopy.

quant-ph↗

arXiv2026

Pseudomode approach to Fano effect in dissipative cavity quantum electrodynamics

We study the Fano effect in dissipative cavity quantum electrodynamics (QED), which originates from the interference between the emitter's direct radiation and that mediated by a cavity mode. Starting from a two-level system coupled to a structured reservoir, we show that a quantum master equation previously derived within the Born-Markov approximation can be rederived by introducing a single auxiliary mode through the pseudomode approach. We identify the corresponding spectral function of the system--environment interaction and show that it consists of a constant contribution and a non-Lorentzian contribution, whose interplay gives rise to a spectral profile of the Fano form. The constant contribution represents a Markovian background and is essential for obtaining a Lindblad master equation. Furthermore, by applying Fano diagonalization to an atom--cavity system coupled to common and independent reservoirs, we independently derive the same spectral function and clarify its physical origin. Our results provide a unified description of the Fano effect in single-mode cavity QED systems and reveal its non-Markovian origin encoded in the spectral function of the structured reservoir.

quant-ph↗

arXiv2025

Deep learning of thermodynamic laws from microscopic dynamics

We numerically show that a deep neural network (DNN) can learn macroscopic thermodynamic laws purely from microscopic data. Using molecular dynamics simulations, we generate the data of snapshot images of gas particles undergoing adiabatic processes. We train a DNN to determine the temporal order of input image pairs. We observe that the trained network induces an order relation between states consistent with adiabatic accessibility, satisfying the axioms of thermodynamics. Furthermore, the internal representation learned by the DNN act as an entropy. These results suggest that machine learning can discover emergent physical laws that are valid at scales far larger than those of the underlying constituents -- opening a pathway to data-driven discovery of macroscopic physics.

cond-mat.stat-mech↗

arXiv2025

Unveiling the nature of cathodoluminescence from photon statistics

Cathodoluminescence (CL), the emission of light induced by accelerated free electrons, has been extensively utilized in various applications, such as displays, streak cameras, and high-spatial-resolution analysis of optical material, surpassing the diffraction limit of light. Despite its long history, the photon statistics of CL have only recently been examined, revealing unexpectedly large bunching of photons. Here we find that this peculiar photon bunching contains information of intervening excitation processes before the photon emission, which can be extracted from the photon statistics within each excitation event by a single free electron. Using this approach, we experimentally unveiled the statistical differences of coherent CL involving a single electromagnetic interaction process and incoherent CL involving multiple excitation processes. The developed formulation is universally applicable for particle generation processes in general to investigate the nature of cascade reactions.

physics.optics↗

arXiv2023

Time-correlated electron and photon counting microscopy

Electron microscopy based on high-energy electrons allows nanoscopic analytical imaging taking advantage of secondarily generated particles. Especially for cathodoluminescence, the correlation between primary incident electrons and emitted photons includes information on the entire interaction process. However, electron-photon time correlation tracking the relaxation dynamics of luminescent materials has so far not been achieved. In this work, we propose time-correlated electron and photon counting microscopy, where coincidence events of primary electrons and generated photons are counted after interaction. The electron-photon time correlation enables extracting a unique lifetime of the emitter independent of the photon state, accounting for coherent and incoherent photon generation processes. We also introduce a correlation factor and discuss the correlation between electrons and generated coherent photons. Through momentum selection, we observe correlation changes indicating the presence of pair correlation originated from the electron-photon entanglement. The present work lays the foundation for developing next-generation electron microscopy based on quantum correlation.

physics.ins-det↗

arXiv2023

Superbunching in cathodoluminescence: a master equation approach

We propose a theoretical model of a master equation for cathodoluminescence (CL). The master equation describes simultaneous excitation of multiple emitters by an incoming electron and radiative decay of individual emitters. We investigate the normalized second-order correlation function, $g^{(2)}(τ)$, of this model. We derive the exact formula for the zero-time delay correlation, $g^{(2)}(0)$, and show that the model successfully describes giant bunching (superbunching) in the CL. We also derive an approximate form of $g^{(2)}(τ)$, which is valid for small excitation rate. Furthermore, we discuss the state of the radiation field of the CL. We reveal that the superbunching results from a mixture of an excited photon state and the vacuum state and that this type of state is realized in the CL.

cond-mat.mes-hall↗

arXiv2022

Time-resolved physical spectrum in cavity quantum electrodynamics

The time-resolved physical spectrum of luminescence is theoretically studied for a standard cavity quantum electrodynamics system. In contrast to the power spectrum for the steady state, the correlation functions up to the present time are crucial for the construction of the time-resolved spectrum, while the correlations with future quantities are inaccessible because of the causality, i.e., the future quantities cannot be measured until the future comes. We find that this causality plays a key role to understand the time-resolved spectrum, in which the Rabi doublet can never be seen during the time of the first peak of the Rabi oscillation. Furthermore, the causality can influence on the transient magnitude of the Rabi doublet in some situations. We also study the dynamics of the Fano anti-resonance, where the difference from the Rabi doublet can be highlighted.

quant-ph↗

arXiv2021

Theory of Fano effect in cavity quantum electrodynamics

We propose a Markovian quantum master equation that can describe the Fano effect directly, by assuming a standard cavity quantum electrodynamics system. The framework allows us to generalize the Fano formula, applicable over the weak and strong coupling regimes with pure dephasing. A formulation of its emission spectrum is also given in a consistent manner. We then find that the interference responsible for the Fano effect is robust against pure dephasing. This is counterintuitive because the impact of interference is, in general, severely reduced by decoherence processes. Our approach thus provides a basis for theoretical treatments of the Fano effect and new insights into the quantum interference in open quantum systems.

quant-ph↗

arXiv2019

Fluctuation theorem in cavity quantum electrodynamics systems

We derive an integral fluctuation theorem (FT) in a general setup of cavity quantum electrodynamics systems. In the derivation, a key difficulty lies in a diverging behavior of entropy change arising from the zero-temperature limit of an external bath, which is required to describe the cavity loss. We solve this difficulty from the viewpoint of absolute irreversibility and find that two types of absolute irreversibility contribute to the integral FT. Furthermore, we show that, in a stationary and small cavity-loss condition, these contributions have simple relationships to the average number of photons emitted out of the cavity, and the integral FT yields an approximate form independent of the setup details. We illustrate the general results with a numerical simulation in a model of quantum heat engine.

cond-mat.stat-mech↗

arXiv2019

1/f^2 spectra of decoherence noise on ^75^As nuclear spins in bulk GaAs

To identify the decoherence origin, frequency spectra using multiple π-pulses have been extensively studied. However, little has been discussed on how to define the spectral intensities from multiple-echo decays and how to incorporate the Hahn-echo T_2 in the noise spectra. Here, we show that experiments based on two theories solve these issues. With the previous theory clarifying that the spectral intensity should be given as the decay in the long-time limit, the intensity can be deduced without experimental artifacts usually entailed in the initial process. The other is the fluctuation-dissipation theory, with which the Hahn-echo T_2 is utilized as the zero-frequency limit of the noise spectrum and as an answer to the divergent issue on the 1/f^n noises. As a result, arsenic nuclear spins are found to exhibit 1/f2 dependences over two orders of magnitude in all the substrates of un-doped, Cr-doped semi-insulating and Si-doped metallic GaAs at 297 K. The 1/f^2 dependence indicates single noise source that is characterized by the characteristic frequency f_c_^un^=170 Hz, f_c_^Cr^=210 Hz and f_c_^Si^ =460 Hz. These f_c values are explained by a model that the decoherence is caused by the fluctuations of next-nearest-neighboring nuclear spins.

cond-mat.mes-hall↗

arXiv2017

Superposition of Macroscopically Distinct States in Adiabatic Quantum Computation

What are the conditions for adiabatic quantum computation (AQC) to outperform classical computation? Although there exist several quantum adiabatic algorithms achieving the strong quantum speedup, the essential keys to their speedups are still unclear. Here, we investigate the connection between superpositions of macroscopically distinct states and known examples of the speedup in AQC. To formalize this notion we consider an index $p$ that quantifies a superposition of macroscopically distinct states from the asymptotic behaviors of fluctuations of additive observables. We determine this index for five examples of adiabatic algorithms exhibiting various degrees of the speedup. The results suggest that the superposition of macroscopically distinct states is an appropriate indicator of entanglement crucial to the strong quantum speedup in AQC.

quant-ph↗

arXiv2017

Decomposition of radiation energy into work and heat

We investigate energy transfer by the radiation from a cavity quantum electrodynamics (QED) system in the context of quantum thermodynamics. We propose a method of decomposing it into work and heat within the framework of quantum master equations. We find that the work and heat correspond respectively to the coherent and incoherent parts of the radiation. In the derivation of the method, it is crucial to investigate the dynamics of the system that receives the radiation from the cavity.

cond-mat.stat-mech↗

arXiv2017

Markovian Quantum Master Equation beyond Adiabatic Regime

By introducing a temporal change timescale $τ_{\text{A}}(t)$ for the time-dependent system Hamiltonian, a general formulation of the Markovian quantum master equation is given to go well beyond the adiabatic regime. In appropriate situations, the framework is well justified even if $τ_{\text{A}}(t)$ is faster than the decay timescale of the bath correlation function. An application to the dissipative Landau-Zener model demonstrates this general result. The findings are applicable to a wide range of fields, providing a basis for quantum control beyond the adiabatic regime.

cond-mat.stat-mech↗

arXiv2015

Liquid is More Rigid than Solid in a High-Frequency Region

We compare rigidity of materials in two phases, liquid and solid phases. As a measure of the rigidity, we employ the one characterizing how firmly the material is fixed by low density of pinning centers, such as impurities and rough surfaces of walls, against a weak force. Although a solid is more rigid than a liquid against a low-frequency force, we find that against a high-frequency force the liquid becomes more rigid than the solid of the same material. Since this result is derived from universal properties of a response function, it is valid for wide classes of materials, including quantum and classical systems and crystalline and amorphous solids. An instructive example is studied using nonequilibrium molecular dynamics simulations. We find that the frequency region in which a solid is more flexible than a liquid is not purely determined by intrinsic properties of the solid. It depends also on extrinsic factors such as the density of pinning centers.

cond-mat.stat-mech↗

arXiv2014

An expression of excess work during transition between nonequilibrium steady states

Excess work is a non-diverging part of the work during transition between nonequilibrium steady states (NESSs). It is a central quantity in the steady state thermodynamics (SST), which is a candidate for nonequilibrium thermodynamics theory. We derive an expression of excess work during quasistatic transitions between NESSs by using the macroscopic linear response relation of NESS. This expression is a line integral of a vector potential in the space of control parameters. We show a relationship between the vector potential and the response function of NESS, and thus obtain a relationship between the SST and a macroscopic quantity. We also connect the macroscopic formulation to microscopic physics through a microscopic expression of the nonequilibrium response function, which gives a result consistent with the previous studies.

cond-mat.stat-mech↗

arXiv2014

A perturbative method for nonequilibrium steady state of open quantum systems

We develop a method of calculating the nonequilibrium steady state (NESS) of an open quantum system that is weakly coupled to reservoirs in different equilibrium states. We describe the system using a Redfield-type quantum master equation (QME). We decompose the Redfield QME into a Lindblad-type QME and the remaining part $\mathcal{R}$. Regarding the steady state of the Lindblad QME as the unperturbed solution, we perform a perturbative calculation with respect to $\mathcal{R}$ to obtain the NESS of the Redfield QME. The NESS thus determined is exact up to the first order in the system-reservoir coupling strength (pump/loss rate), which is the same as the order of validity of the QME. An advantage of the proposed method in numerical computation is its applicability to systems larger than those in methods of directly solving the original Redfield QME. We apply the method to a noninteracting fermion system to obtain an analytical expression of the NESS density matrix. We also numerically demonstrate the method in a nonequilibrium quantum spin chain.

cond-mat.stat-mech↗

arXiv2014

Cavity-loss induced plateau in coupled cavity QED array

Nonequilibrium steady states are investigated in a coupled cavity QED array system which is pumped by a thermal bath and dissipated through cavity loss. In the coherent (non-zero photon amplitude) phase, plateau regions appear, where the steady states become unchanged against the variation of the chemical potential of the thermal bath. The cavity loss plays a crucial role for the plateaus: the plateaus appear only if the cavity loss exists, and the photon leakage current, which is induced by the loss, is essential to the mechanism of the plateaus.

quant-ph↗

arXiv2013

Geometrical Excess Entropy Production in Nonequilibrium Quantum Systems

For open systems described by the quantum Markovian master equation, we study a possible extension of the Clausius equality to quasistatic operations between nonequilibrium steady states (NESSs). We investigate the excess heat divided by temperature (i.e., excess entropy production) which is transferred into the system during the operations. We derive a geometrical expression for the excess entropy production, which is analogous to the Berry phase in unitary evolution. Our result implies that in general one cannot define a scalar potential whose difference coincides with the excess entropy production in a thermodynamic process, and that a vector potential plays a crucial role in the thermodynamics for NESSs. In the weakly nonequilibrium regime, we show that the geometrical expression reduces to the extended Clausius equality derived by Saito and Tasaki (J. Stat. Phys. {\bf 145}, 1275 (2011)). As an example, we investigate a spinless electron system in quantum dots. We find that one can define a scalar potential when the parameters of only one of the reservoirs are modified in a non-interacting system, but this is no longer the case for an interacting system.

cond-mat.stat-mech↗