arXiv subjects

Tatsuya Nagao

Publications and source records attributed to Tatsuya Nagao.

28 records · Page 2Linked to original sources

arXiv2007

Two-magnon excitations in resonant inelastic x-ray scattering from quantum Heisenberg antiferromagnets

We study two-magnon spectra in resonant inelastic x-ray scattering (RIXS) from the Heisenberg antiferromanets by extending the formula of Nomura andIgarashi (Phys. Rev. B 71, 035110 (2005)). The core-hole potential in the intermediate state of RIXS gives rise to a change in the exchange coupling between 3d electrons, leading to an effective interaction between the core hole and spins of 3d electrons. We derive a formula suitable to calculate the two-magnon RIXS intensities, replacing the bare core-hole potential responsible to charge excitations by this effective interaction creating two magnons in our previous formula. It consists of two factors, one of which determines the incident-photon-energy dependence and another is the two-magnon correlation function. We evaluate the former factor for La_{2}CuO_{4} in terms of the density of states of the 4p states obtained by the band calculation. We also calculate the two-magnon correlation function as a function of energy loss ωand momentum transfer \textbf{q} of the Heisenberg model on a square lattice,by summing up the ladder diagrams after transforming the magnon-magnon interaction into a separable form. The calculated spectra form a broad peak around ω=3J for S=1/2 on the magnetic Brillouin zone boundary and vanish at \textbf{q}=(0,0) and (π,π). Such momentum dependence of the RIXS spectra could provide an excellent opportunity to study the dynamics in the Heisenberg model.

cond-mat.str-el↗

arXiv2006

A theory of the electric quadrupole contribution to resonant x-ray scattering: Application to multipole ordering phases in Ce_{1-x}La_{x}B_{6}

We study the electric quadrupole (E2) contribution to resonant x-ray scattering (RXS). Under the assumption that the rotational invariance is preserved in the Hamiltonian describing the intermediate state of scattering, we derive a useful expression for the RXS amplitude. One of the advantages the derived expression possesses is the full information of the energy dependence, lacking in all the previous studies using the fast collision approximation. The expression is also helpful to classify the spectra into multipole order parameters which are brought about. The expression is suitable to investigate the RXS spectra in the localized f electron systems. We demonstrate the usefulness of the formula by calculating the RXS spectra at the Ce L_{2,3} edges in Ce_{1-x}La_{x}B_{6} on the basis of the formula. We obtain the spectra as a function of energy in agreement with the experiment of Ce_{0.7}La_{0.3}B_{6}. Analyzing the azimuthal angle dependence, we find the sixfold symmetry in the σ-σ' channel and the threefold onein the σ-π' channel not only in the antiferrooctupole (AFO) ordering phase but also in the antiferroquadrupole (AFQ) ordering phase, which behavior depends strongly on the domain distribution. The sixfold symmetry in the AFQ phase arises from the simultaneously induced hexadecapole order. Although the AFO order is plausible for phase IV in Ce_{1-x}La_{x}B_{6}, the possibility of the AFQ order may not be ruled out on the basis of azimuthal angle dependence alone.

cond-mat.str-el↗

arXiv2006

Resonant X-Ray Scattering on the M-Edge Spectra from Triple-k Structure Phase in U_{0.75}Np_{0.25}O_{2} and UO_{2}

We derive an expression for the scattering amplitude of resonant x-ray scattering under the assumption that the Hamiltonian describing the intermediate state preserves spherical symmetry. On the basis of this expression, we demonstrate that the energy profile of the RXS spectra expected near U and Np M_4 edges from the triple-k antiferromagnetic ordering phase in UO_{2} and U_{0.75}Np_{0.25}O_{2} agree well with those from the experiments. We demonstrate that the spectra in the σ-σ' and σ-π' channels exhibit quadrupole and dipole natures, respectively.

cond-mat.str-el↗

arXiv2005

Resonant x-ray scattering spectra from multipole orderings: Np M_{4,5} edges in NpO2

We study resonant x-ray scattering (RXS) at Np M_{4,5} edges in the triple-\textbf{k} multipole ordering phase in NpO_{2}, on the basis of a localized electron model. We derive an expression for RXS amplitudes to characterize the spectra under the assumption that a rotational invariance is preserved in the intermediate state of scattering process. This assumption is justified by the fact that energies of the crystal electric field and the intersite interaction is smaller than the energy of multiplet structures. This expression is found useful to calculate energy profiles with taking account of the intra-Coulomb and spin-orbit interactions. Assuming the Γ_{8}-quartet ground state, we construct the triple-\textbf{k} ground state, and analyze the RXS spectra. The energy profiles are calculated in good agreement with the experiment, providing a sound basis to previous phenomenological analyses.

cond-mat.str-el↗

arXiv2005

1/S-expansion study of spin waves in a two-dimensional Heisenberg antiferromagnet

We study the effects of quantum fluctuations on excitation spectra in the two-dimensional Heisenberg antiferromagnet by means of the 1/S expansion. We calculate the spin-wave dispersion and the transverse dynamical structure factor up to the second order of 1/S in comparison with inelastic neutron scattering experiments. The spin-wave energy at momentum $(π,0)$ is found to be about 2% smaller than that at $(π/2,π/2)$ due to the second-order correction. In addition, we study the dimensional crossover from two dimensions to one dimension by weakening exchange couplings in one direction. It is found that the second-order correction becomes large with approaching the quasi-one dimensional situation and makes the spin-wave energy approach to the des Cloizeaux-Pearson boundary for $S=1/2$. The transverse dynamical structure factor is also calculated up to the second order of 1/S. It is shown that the intensity of spin-wave peak is strongly reduced while the intensity of three-spin-wave continuum becomes large and exceeds that of the spin-wave peak in the quasi-one dimensional situation.

cond-mat.str-el↗

arXiv2004

Resonant X-Ray Scattering from URu_{2}Si_{2}

Based on a localized crystal electric field model for the U^{4+} in the (5f)^2-configuration, we analyze the resonant x-ray scattering spectra around U M_{IV} and M_{V} edges in URu_{2}Si_{2}, taking full Coulomb and spin-orbit interactions into account. We consider two level schemes, a singlet model of Santini and Amoretti and a doublet model of Ohkawa and Shimizu, and assume the antiferroquadrupolar order and the antiferromagnetic order as candidates for the ambient pressure phase and the high pressure phase. It is found that the spectral shapes as a function of photon energy are independent of the assumed level scheme, but are quite different between the antiferroquadrupole and antiferromagnetic phases, This may be useful to determine the character of the ordered phase.

cond-mat.str-el↗

arXiv2003

Lattice Distortion and Resonant X-Ray Scattering in DyB2C2

We study the resonant x-ray scattering (RXS) spectra at the Dy $L_{\rm III}$ absorption edge in the quadrupole ordering phase of DyB$_2$C$_2$. Analyzing the buckling of sheets of B and C atoms, we construct an effective model that the crystal field is acting on the $5d$ and $4f$ states with the principal axes different for different sublattices. Treating the $5d$ states as a band and the $4f$ states as localized states, we calculate the spectra within the dipole transition. We take account of processes that (1) the lattice distortion directly modulates the $5d$ states and (2) the charge anisotropy of the quadrupole ordering $4f$ states modulates the $5d$ states through the $5d$-$4f$ Coulomb interaction. Both processes give rise to the RXS intensities on $(00\frac{\ell}{2})$ and $(h0\frac{\ell}{2})$ spots. Both give similar photon-energy dependences and the same azimuthal-angle dependences for the main peak, in agreement with the experiment. The first process is found to give the intensities much larger than the second one in a wide parameter range of crystal field. This suggests that the main-peak of the RXS spectra is not a direct reflection of the quadrupole order but mainly controlled by the lattice distortion.

cond-mat.str-el↗

arXiv2002

Resonant X-Ray Scattering from CeB$_{6}$

We calculate the resonant x-ray scattering (RXS) spectra near the Ce $L_{\rm III}$ absorption edge in CeB$_6$, on the basis of a microscopic model that the $4f$ states of Ce are atomic while the $5d$ states form an energy band with a reasonable density of states. In the initial state, we employ an effective Hamiltonian of Shiina {\it et al}. in the antiferro-quadrupole (AFQ) ordering phase, while we construct the wave function consistent with the neutron scattering experiment in the magnetic ground state. In the intermediate state, we take full account of the intra-atomic Coulomb interaction. Without assuming any lattice distortion, we obtain sufficient RXS intensities on the AFQ superlattice spot. We obtain the spectral shape, the temperature and magnetic field dependences in good agreement with the experiment, thus demonstrating the mechanism that the intensity is brought about by the modulation of $5d$ states through the anisotropic term of the $5d$-$4f$ Coulomb interaction. In the magnetic ground state, a small pre-edge peak is found by the $E_2$ process. On the magnetic superlattice spot, we get a finite but considerably small intensity. The magnetic form factor is briefly discussed.

cond-mat.str-el↗

arXiv2001

Resonant X-Ray Scattering from the Quadrupolar Ordering Phase of CeB_6

We theoretically investigate the origin of the resonant x-ray scattering (RXS) signal near the Ce $L_{III}$ absorption edge in the quadrupolar ordering phase of CeB$_6$, considering the intersite interaction between the $Γ_8$ states in the initial state. The anisotropic charge distribution of the $4f$ states modulates the $5d$ states through the intra-atomic Coulomb interaction and thereby generates a large RXS superlattice intensity. The temperature and magnetic field dependence indicates that the induced dipolar and octupolar orders have little influence on the RXS spectra, in good agreement with the recent experiment.

cond-mat.str-el↗

arXiv1999

Three-body correlations in the Nagaoka state on the square lattice

A three-body scattering theory previously proposed by one of the present authors is developed to be applied to the saturated ferromagnetic state in the two-dimensional Hubbard model. The single-particle Green's function is calculated by taking account of the multiple scattering between two electrons and one hole. Several limiting cases are discussed and the relation to the variational principle is examined. The importance of the three-body correlation is demonstrated in comparison with the results of the ladder approximation. A possible phase boundary for the Nagaoka ground state is presented for the square lattice, which improves the previous variational results.

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