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Th. Stöhlker

Publications and source records attributed to Th. Stöhlker.

50 records · Page 3Linked to original sources

Relativistic calculations of the isotope shifts in highly charged Li-like ions

Relativistic calculations of the isotope shifts of energy levels in highly charged Li-like ions are performed. The nuclear recoil (mass shift) contributions are calculated by merging the perturbative and large-scale configuration-interaction Dirac-Fock-Sturm (CI-DFS) methods. The nuclear size (field shift) contributions are evaluated by the CI-DFS method including the electron-correlation, Breit, and QED corrections. The nuclear deformation and nuclear polarization corrections to the isotope shifts in Li-like neodymium, thorium, and uranium are also considered. The results of the calculations are compared with the theoretical values obtained with other methods.

physics.atom-ph↗

Relativistic calculations of the x-ray emission following the Xe-Bi$^{83+}$ collision

We study the x-ray emission following the collision of a Bi$^{83+}$ ion with a neutral Xe atom at the projectile energy 70 MeV/u. The collisional and post-collisional processes are treated separately. The probabilities of various many-electron processes at the collision are calculated within a relativistic independent electron model using the coupled-channel approach with atomic-like Dirac-Fock-Sturm orbitals. The analysis of the post-collisional processes resulting in the x-ray emission is based on the fluorescence yields, the radiation and Auger decay rates, and allows to derive intensities of the x-ray emission and compare them with experimental data. A reasonable agreement between the theoretical results and the recent experimental data is observed. The role of the relativistic effects is investigated.

physics.atom-ph↗

High-resolution measurement of the time-modulated orbital electron capture and of the $β^+$ decay of hydrogen-like $^{142}$Pm$^{60+}$ ions

The periodic time modulations, found recently in the two-body orbital electron-capture (EC) decay of both, hydrogen-like $^{140}$Pr$^{58+}$ and $^{142}$Pm$^{60+}$ ions, with periods near to 7s and amplitudes of about 20%, were re-investigated for the case of $^{142}$Pm$^{60+}$ by using a 245 MHz resonator cavity with a much improved sensitivity and time resolution. We observed that the exponential EC decay is modulated with a period $T = 7.11(11)$s, in accordance with a modulation period $T = 7.12(11)$ s as obtained from simultaneous observations with a capacitive pick-up, employed also in the previous experiments. The modulation amplitudes amount to $a_R = 0.107(24)$ and $a_P = 0.134(27)$ for the 245 MHz resonator and the capacitive pick-up, respectively. These new results corroborate for both detectors {\it exactly} our previous findings of modulation periods near to 7s, though with {\it distinctly smaller} amplitudes. Also the three-body $β^+$ decays have been analyzed. For a supposed modulation period near to 7s we found an amplitude $a = 0.027(27)$, compatible with $a = 0$ and in agreement with the preliminary result $a = 0.030(30)$ of our previous experiment. These observations could point at weak interaction as origin of the observed 7s-modulation of the EC decay. Furthermore, the data suggest that interference terms occur in the two-body EC decay, although the neutrinos are not directly observed.

nucl-ex↗

Schottky mass measurements of heavy neutron-rich nuclides in the element range $70\leZ \le79$ at the ESR

Storage-ring mass spectrometry was applied to neutron-rich $^{197}$Au projectile fragments. Masses of $^{181,183}$Lu, $^{185,186}$Hf, $^{187,188}$Ta, $^{191}$W, and $^{192,193}$Re nuclei were measured for the first time. The uncertainty of previously known masses of $^{189,190}$W and $^{195}$Os nuclei was improved. Observed irregularities on the smooth two-neutron separation energies for Hf and W isotopes are linked to the collectivity phenomena in the corresponding nuclei.

nucl-ex↗

PEBSI - A Monte Carlo simulator for bremsstrahlung arising from electrons colliding with thin solid-state targets

We present a Monte Carlo code dedicated to the simulation of bremsstrahlung arising in collisions of polarized electrons with thin target foils. The program consists of an electron transport algorithm taking into account elastic electron-nucleus scattering and inelastic collisions with target electrons as well as a treatment of polarized-electron bremsstrahlung emission. Good agreement is found between the predictions of the electron transport code and data stemming from other simulation programs and experiments. In addition, we present first results from the bremsstrahlung simulation which indicate a significant decrease in the degree of linear polarization of bremsstrahlung even for the thinnest gold targets considered.

physics.atom-ph↗

Magnetic Sublevel Population and Alignment for the Excitation of H- and He-like Uranium in Relativistic Collisions

We have measured the alignment of the L-shell magnetic-substates following the K-shell excitation of hydrogen- and helium-like uranium in relativistic collisions with a low-Z gaseous target. Within this experiment the population distribution for the L-shell magnetic sublevels has been obtained via an angular differential study of the decay photons associated with the subsequent de-excitation process. The results show a very distinctive behavior for the H- and He-like heavy systems. In particular for $K \rightarrow L$ excitation of He-like uranium, a considerable alignment of the L-shell levels was observed. A comparison of our experimental findings with recent rigorous relativistic predictions provides a good qualitative and a reasonable quantitative agreement, emphasizing the importance of the magnetic-interaction and many-body effects in the strong-field domain of high-Z ions.

physics.atom-ph↗

Angular correlations in the two--photon decay of helium--like heavy ions

The two-photon decay of heavy, helium-like ions is investigated based on second-order perturbation theory and Dirac's relativistic equation. Special attention has been paid to the angular emission of the two photons, i.e., how the angular correlation function depends on the shell structure of the ions in their initial and final states. Moreover, the effects from the (electric and magnetic) non-dipole terms in the expansion of the electron-photon interaction are discussed. Detailed calculations have been carried out for the two-photon decay of the $1s2s \, ^1S_0$, $1s2s \, ^3S_1$ and $1s2p \, ^3P_0$ states of helium-like xenon Xe$^{52+}$, gold Au$^{77+}$ and uranium U$^{90+}$ ions.

quant-ph↗

Electron loss of fast heavy projectiles in collision with neutral targets

The multiple electron loss of heavy projectiles in fast ion-atom collisions has been studied in the framework of the sudden perturbation approximation. Especially, a model is developed to calculate the cross sections for the loss of any number of electrons from the projectile ion, including the ionization of a single electron and up to the complete stripping of the projectile. For a given collision system, that is specified by the (type and charge state of the) projectile and target as well as the collision energy, in fact, the experimental cross sections for just three final states of the projectile are required by this model in order to predict the loss of any number, $N$, of electrons for the same collision system, or for any similar system that differs only in the energy or the initial charge state of the projectile ion. The model is simple and can be utilized for both, the projectile and target ionization, and without that large computer resources are requested. Detailed computation have been carried out for the multiple electron loss of Xe$^{18+}$ and U$^{6+,\, 10+,\, 28+}$ projectiles in collision with neutral Ar and Ne gas targets.

physics.atom-ph↗

Relativistic calculations of the charge-transfer probabilities and cross sections for low-energy collisions of H-like ions with bare nuclei

A new method for solving the time-dependent two-center Dirac equation is developed. The time-dependent Dirac wave function is represented as a sum of atomic-like Dirac-Sturm orbitals, localized at the ions. The atomic orbitals are obtained by solving numerically the finite-difference one-center Dirac and Dirac-Sturm equations with the potential which is the sum of the exact reference-nucleus potential and a monopole-approximation potential from the other nucleus. An original procedure to calculate the two-center integrals with these orbitals is proposed. The approach is tested by calculations of the charge transfer and ionization cross sections for the H(1s)--proton collisions at proton energies from 1 keV to 100 keV. The obtained results are compared with related experimental and other theoretical data. To investigate the role of the relativistic effects, the charge transfer cross sections for the Ne^{9+}(1s)--Ne^{10+} (at energies from 0.1 to 10 MeV/u) and U^{91+}(1s)--U^{92+} (at energies from 6 to 10 MeV/u) collisions are calculated in both relativistic and nonrelativistic cases.

physics.atom-ph↗

Parity nonconservation effect with laser-induced 2^3S_1 - 2^1S_0 transition in heavy heliumlike ions

The parity nonconservation (PNC) effect on the laser-induced 2^3S_1 - 2^1S_0 transition in heavy heliumlike ions is considered. A simple analytical formula for the PNC correction to the cross section is derived for the case, when the opposite-parity 2^1S_0 and 2^3P_0 states are almost degenerate and, therefore, the PNC effect is strongly enhanced. Numerical results are presented for heliumlike gadolinium and thorium, which seem most promising candidates for such kind of experiments. In both Gd and Th cases the photon energy required will be anticipated with a high-energy laser built at GSI. Alternatively, it can be gained with ultraviolet lasers utilizing relativistic Doppler tuning at FAIR facilities in Darmstadt.

physics.atom-ph↗

Relativistic recoil, electron-correlation, and QED effects on the 2p_j-2s transition energies in Li-like ions

The relativistic nuclear recoil, higher-order interelectronic-interaction, and screened QED corrections to the transition energies in Li-like ions are evaluated. The calculation of the relativistic recoil effect is performed to all orders in 1/Z. The interelectronic-interaction correction to the transition energies beyond the two-photon exchange level is evaluated to all orders in 1/Z within the Breit approximation. The evaluation is carried out employing the large-scale configuration-interaction Dirac-Fock-Sturm method. The rigorous calculation of the complete gauge invariant sets of the screened self-energy and vacuum-polarization diagrams is performed utilizing a local screening potential as the zeroth-order approximation. The theoretical predictions for the 2p_j-2s transition energies are compiled and compared with available experimental data in the range of the nuclear charge number Z=10-60.

physics.atom-ph↗

Negative-continuum dielectronic recombination into excited states of highly-charged ions

The recombination of a free electron into a bound state of bare, heavy nucleus under simultaneous production of bound-electron--free-positron pair is studied within the framework of relativistic first--order perturbation theory. This process, denoted as "negative-continuum dielectronic recombination" leads to a formation of not only the ground but also the singly- and doubly-excited states of the residual helium-like ion. The contributions from such an excited--state capture to the total as well as angle-differential cross-sections are studied in detail. Calculations are performed for the recombination of (initially) bare uranium U$^{92+}$ ions and for a wide range of collision energies. From these calculations, we find almost 75 % enhancement of the total recombination probability if the excited ionic states are taken into account.

physics.atom-ph↗

Isotope shift in the dielectronic recombination of three-electron ^{A}Nd^{57+}

Isotope shifts in dielectronic recombination spectra were studied for Li-like ^{A}Nd^{57+} ions with A=142 and A=150. From the displacement of resonance positions energy shifts δE^{142,150}(2s-2p_1/2)= 40.2(3)(6) meV (stat)(sys)) and δE^{142,150}(2s-2p_3/2) = 42.3(12)(20) meV of 2s-2p_j transitions were deduced. An evaluation of these values within a full QED treatment yields a change in the mean-square charge radius of ^{142,150}δ = -1.36(1)(3) fm^2. The approach is conceptually new and combines the advantage of a simple atomic structure with high sensitivity to nuclear size.

physics.atom-ph↗

Electron gas polarization effect induced by heavy H-like ions of moderate velocities channeled in a silicon crystal

We report on the observation of a strong perturbation of the electron gas induced by 20 MeV/u U$^{91+}$ ions and 13 MeV/u Pb$^{81+}$ ions channeled in silicon crystals. This collective response (wake effect) in-duces a shift of the continuum energy level by more than 100 eV, which is observed by means of Radiative Electron Capture into the K and L-shells of the projectiles. We also observe an increase of the REC probability by 20-50% relative to the probability in a non-perturbed electron gas. The energy shift is in agreement with calculations using the linear response theory, whereas the local electron density enhancement is much smaller than predicted by the same model. This shows that, for the small values of the adiabaticity parameter achieved in our experiments, the density fluctuations are not strongly localized at the vicinity of the heavy ions.

physics.atom-ph↗