arXiv subjects

Themistoklis Sidiropoulos

Publications and source records attributed to Themistoklis Sidiropoulos.

6 recordsLinked to original sources

arXiv2025

Picosecond localization dynamics following ultrafast nanoscale magnetic switching

Ultrashort laser pulses provide the fastest known way to switch magnetic order. Such excitation commonly creates nanometer-scale domains, even after homogeneous illumination when the position of nucleated domains is not externally defined. However, the physics of domain localization during such ultrafast phase transitions remains unresolved. Here, we use shot-resolved pump-probe resonant x-ray scattering together with a material featuring a periodically modulated magnetic anisotropy landscape to track, in real time, the laser-driven nucleation and localization of nanometer-scale spin textures. We find that nucleation and localization are two distinct processes. Nucleation occurs homogeneously via fluctuations at early times, whereas spatially periodic structures emerge only later and, under suitable conditions, localize in less than one nanosecond. Real-space simulations show that this localization is governed by strong lateral variations in spin-texture lifetimes. Our results demonstrate that ultrafast phase-transition dynamics fundamentally differ from conventional transitions, yet still can be controlled through moderate nanometer-scale tailoring of the energy landscape.

cond-mat.mes-hall↗

arXiv2025

Soft X-ray imaging with coherence tomography in the water window spectral range using high-harmonic generation

High-harmonic generation (HHG) is used as a source for various imaging applications in the extreme ultraviolet spectral range. It offers spatially coherent radiation and unique elemental contrast with the potential for attosecond time resolution. The unfavorable efficiency scaling to higher photon energies prevented the imaging application in the soft X-ray range so far. In this work we demonstrate the feasibility of using harmonics for imaging in the water window spectral region (284$\,$eV to 532$\,$eV). We achieve nondestructive depth profile imaging in a heterostructure by utilizing a broadband and noise-resistant technique called soft X-ray Coherence Tomography (SXCT) at a high-flux lab-scale HHG source. SXCT is derived from Optical Coherence Tomography, a Fourier based technique, that can use the full bandwidth of the source to reach an axial resolution of 12$\,$nm in this demonstration. The employed source covers the entire water window, with a photon flux exceeding 10$^\text{6}\,$photons/eV/s at a photon energy of 500$\,$eV. We show local cross sections of a sample consisting of Aluminium oxide and Platinum layers of varying thickness on a Zinc oxide substrate. We validate the findings with scanning and transmission electron microscopy after preparation with focused ion beam milling.

physics.optics↗

arXiv2024

Sub-wavelength localized all-optical helicity-independent magnetic switching using plasmonic gold nanostructures

All-optical helicity-independent switching (AO-HIS) is of interest for ultrafast and energy efficient magnetic switching in future magnetic data storage approaches. Yet, to achieve high bit density magnetic recording it is necessary to reduce the size of the magnetic bits addressed by laser pulses at well-controlled positions. Metallic nanostructures that support localized surface plasmons enable spatial electromagnetic confinement well below the diffraction limit and rare-earth transition metal alloys such as GdTbCo have demonstrated nanometre-sized stable domains. Here, we deposit plasmonic gold nanostructures on a GdTbCo film and probe the magnetic state using magnetic force microscopy. We observe localized AO-HIS down to a critical dimension of 240 nm after excitation of the gold nanostructures by a single 370 fs long laser pulse with a centre wavelength of 1030 nm. We demonstrate that the strong localization of optical fields through plasmonic nanostructures enables reproducible localized nanoscale AO-HIS at sub-wavelength length scales. We study the influence of the localized electromagnetic field enhancement by the plasmonic nanostructures on the required fluence to switch the magnetization.

cond-mat.mtrl-sci↗

arXiv2024

Ultrafast energy-dispersive soft-x-ray diffraction in the water window with a laser-driven source

Time-resolved soft-x-ray-diffraction experiments give access to microscopic processes in a broad range of solid-state materials by probing ultrafast dynamics of ordering phenomena. While laboratory-based high-harmonic generation (HHG) light sources provide the required photon energies, their limited photon flux is distributed over a wide spectral range, rendering typical monochromatic diffraction schemes challenging. Here, we present a scheme for energy-dispersive soft-x-ray diffraction with femtosecond temporal resolution and photon energies across the water window from 200 to 600 eV. The experiment utilizes the broadband nature of the HHG emission to efficiently probe large slices in reciprocal space. As a proof-of-concept, we study the laser-induced structural dynamics of a Mo/Si superlattice in an ultrafast, non-resonant soft-x-ray diffraction experiment. We extract the underlying strain dynamics from the measured shift of its first order superlattice Bragg peak in reciprocal space at photon energies around 500 eV via soft-x-ray scattering simulations.

physics.optics↗

arXiv2022

Tailoring Optical Excitation to Control Magnetic Skyrmion Nucleation

In ferromagnetic multilayers, a single laser pulse with a fluence above an optical nucleation threshold can create magnetic skyrmions, which are randomly distributed over the area of the laser spot. However, in order to study the dynamics of skyrmions and for their application in future data technology, a controllable localization of the skyrmion nucleation sites is crucial. Here, it is demonstrated that patterned reflective masks behind a thin magnetic film can be designed to locally tailor the optical excitation amplitudes reached, leading to spatially controlled skyrmion nucleation on the nanometer scale. Using x-ray microscopy, the influence of nanopatterned back-side aluminum masks on the optical excitation is studied in two sample geometries with varying layer sequence of substrate and magnetic Co/Pt multilayer. Surprisingly, the masks' effect on suppressing or enhancing skymion nucleation reverses when changing this sequence. Moreover, optical near-field enhancements additionally affect the spatial arrangement of the nucleated skyrmions. Simulations of the spatial modulation of the laser excitation, and the following heat transfer across the interfaces in the two sample geometries are employed to explain these observations. The results demonstrate a reliable approach to add nanometer-scale spatial control to optically induced magnetization processes on ultrafast timescales.

cond-mat.mtrl-sci↗

arXiv2022

Ultrafast element- and depth-resolved magnetization dynamics probed by transverse magneto-optical Kerr effect spectroscopy in the soft x-ray range

We report on time- and angle-resolved transverse magneto-optical Kerr effect spectroscopy in the soft x-ray range that, by analysis via polarization-dependent magnetic scattering simulations, allows us to determine the spatio-temporal and element-specific evolution of femtosecond laser-induced spin dynamics in nanostructured magnetic materials. In a ferrimagnetic GdFe thin film system, we correlate a reshaping spectrum of the magneto-optical Kerr signal to depth-dependent magnetization dynamics and disentangle contributions due to non-equilibrium electron transport and nanoscale heat diffusion on their intrinsic time scales. Our work provides a quantitative insight into light-driven spin dynamics occurring at buried interfaces of complex magnetic heterostructures, which can be tailored and functionalized for future opto-spintronic devices.

cond-mat.mtrl-sci↗