Searcharxiv⌕ Search

arXiv subjects

Thiago A. de Assis

Publications and source records attributed to Thiago A. de Assis.

20 records · Page 2Linked to original sources

Nanostructures mechanically stable with desirable characteristic field enhancement factor: a response from scale invariance in electrostatics

This work presents an accurate numerical study of the electrostatics of systems formed by individual nanostructure mounted on support substrate tip, a theoretical prototype for applications in field electron emission or for construction of tips in probe microscopy requiring high resolution. We modeled substrate tip with height $h_1$, radius $r_{1}$ and characteristic field enhancement factor (FEF) $γ_1$, and the top nanostructure with height $h_2$, radius $r_{2}<r_{1}$ and FEF $γ_2$, both hemisphere on post-like structures. Then, nanostructure mounted on support substrate tip has characteristic FEF, $γ_{C}$. Defining the relative difference $η_R \equiv (γ_{C} - γ_{1})/ (γ_{3} - γ_{1})$, where $γ_{3}$ corresponds to reference FEF for a hemisphere on post structure with radius $r_3=r_2$ and height $h_3=h_1 + h_2$, our results suggest, from numerical solution of Laplace's equation using a finite element scheme, a scaling $η_R = f(u\equivλθ^{-1})$, where $λ\equiv h_{2}/h_1$ and $θ\equiv r_1/r_2$. Given a characteristic variable $u_{c}$, we found, for $u \ll u_{c}$, a power law $η_{R} \sim u^κ$ with $κ\approx 0.55$. For $u \gg u_{c}$, $η_{R} \approx 1$ providing conditions where $γ_C \rightarrow γ_3$. As a consequence of scaling invariance, it's possible to derive a simple expression for $γ_C$, being possible to predict conditions to produce related systems with a desirable FEF and that, at the same time, are mechanically stable by presence of substrate tip. Finally, we also discuss the validity of Schottky's conjecture (SC) for these systems showing that, while to obey SC is a indicative of scale invariance, the opposite is not necessarily satisfied. This suggest that a careful analysis must be done before attribute the SC as a origin of giant FEF in experiments.

cond-mat.mes-hall↗

The consequences of dependence between the formal area efficiency and the macroscopic electric field on linearity behavior in Fowler-Nordheim plots

This work presents a theoretical explanation for a crossover in the linear behavior in Fowler-Nordheim (FN) plots based on cold field electron emission (CFE) experimental data. It is characterized by a clear change in the decay rate of usually single-slope FN plots, and has been reported when non-uniform nano-emitters are subject to high macroscopic electric field $F_M$. We assume that the number of emitting spots, which defines an apparent formal area efficiency of CFE surfaces, depends on the macroscopic electric field. Non-uniformity is described by local enhancement factors $\left\{γ_j\right\}$, which are randomly assigned to each distinct emitter of a conducting CFE surface, from a discrete probability distribution $ρ{(γ_{j})}$, with $j=1,2$. It is assumed that $ρ{(γ_{1})} < ρ{(γ_{2})}$, and that $γ_{1} > γ_{2}$. The local current density is evaluated by considering a usual Schottky-Nordheim barrier. The results reproduce the two distinct slope regimes in FN plots when $F_M \in $ $[2,20]$ V/$μ$m and are analyzed by taking into account the apparent formal area efficiency, the distribution $ρ$, and the slopes in the corresponding FN plot. Finally, we remark that our results from numerical solution of Laplace's equation, for an array of conducting nano-emitters with uniform apex radii $50$ nm but different local height, supports our theoretical assumptions and could used in orthodox CFE experiments to test our predictions.

cond-mat.mtrl-sci↗