arXiv subjects

Thomas A. Witten

Publications and source records attributed to Thomas A. Witten.

At least 37 records · Page 2Linked to original sources

arXiv2016

Hydrodynamic Interactions between Two Forced Objects of Arbitrary Shape: I Effect on Alignment

We study the properties and symmetries governing the hydrodynamic interaction between two identical, arbitrarily shaped objects, driven through a viscous fluid. We treat analytically the leading (dipolar) terms of the pair-mobility matrix, affecting the instantaneous relative linear and angular velocities of the two objects at large separation. We prove that the instantaneous hydrodynamic interaction linearly degrades the alignment of asymmetric objects by an external time-dependent drive [Moths and Witten, Phys. Rev. Lett. 110, 028301 (2013)]. The time-dependent effects of hydrodynamic interactions are explicitly demonstrated through numerically calculated trajectories of model alignable objects composed of four stokeslets. In addition to the orientational effect, we find that the two objects usually repel each other. In this case the mutual degradation weakens as the two objects move away from each other, and full alignment is restored at long times.

physics.flu-dyn↗

arXiv2016

Hydrodynamic Interactions between Two Forced Objects of Arbitrary Shape: II Relative Translation

We study the relative translation of two arbitrarily shaped objects, caused by their hydrodynamic interaction as they are forced through a viscous fluid in the limit of zero Reynolds number. It is well known that in the case of two rigid spheres in an unbounded fluid, the hydrodynamic interaction does not produce relative translation. More generally such an effective pair-interaction vanishes in configurations with spatial inversion symmetry; for example, an enantiomorphic pair in mirror image positions has no relative translation. We show that the breaking of inversion symmetry by boundaries of the system accounts for the interactions between two spheres in confined geometries, as observed in experiments. The same general principle also provides new predictions for interactions in other object configurations near obstacles. We examine the time-dependent relative translation of two self-aligning objects, extending the numerical analysis of our preceding publication [Goldfriend, Diamant and Witten, Phys. Fluids 27, 123303 (2015)]. The interplay between the orientational interaction and the translational one, in most cases, leads over time to repulsion between the two objects. The repulsion is qualitatively different for self-aligning objects compared to the more symmetric case of uniform prolate spheroids. The separation between the two objects increases with time $t$ as $t^{1/3}$ in the former case, and more strongly, as $t$, in the latter.

physics.flu-dyn↗

arXiv2016

Criterion for noise-induced synchronization: application to colloidal alignment

Colloidal bodies of irregular shape rotate as they descend under gravity in solution. This rotational response provides a means of bringing a dispersion of identical bodies into a synchronized rotation with the same orientation using programmed forcing. We use the notion of statistical entropy to derive bounds on the rate of synchronization. These bounds apply generally to dynamical systems with stable periodic motion with a phase $ϕ(t)$, when subjected to an impulsive perturbation. The impulse causes a change of phase expressible as a phase map $ψ(ϕ)$. We derive an upper limit on the average change of entropy $\left<ΔH\right>$ in terms of this phase map; when this limit is negative, alignment must occur. For systems that have achieved a low entropy, the $\left<ΔH\right>$ approaches this upper limit.

cond-mat.soft↗

arXiv2016

Non-affine bending mode of thin cylindrical tubes

We discuss the response of thin cylindrical tubes to small indentations. The stretching-free embedding of these surfaces is completely determined by the embedding of one edge curve, thus reducing their bending response to an effectively one dimensional problem. We obtain that in general thin cylindrical tubes will bend non-uniformly in response to an indentation normal to their surface. As a consequence, their local bending stiffness, as measured by indenting at various locations along their axis, is predicted to peak at the center and decrease by a universal factor of 4 at either end of the tube. This characteristic spatial profile of the bending stiffness variation allows a direct determination of the bending modulus of very thin tubes that are shorter than their pinch persistence length, $l_{p}\propto R^{3/2}/t^{1/2}$, where $R$ is the tube diameter and $t$ its wall thickness. We compare our results with experiments performed on rolled-up stainless steel sheets.

cond-mat.soft↗

arXiv2015

A shapeable material without plastic deformation

Randomly crumpled sheets have shape memory. In order to understand the basis of this form of memory, we simulate triangular lattices of springs whose lengths are altered to create a topography with multiple potential energy minima. We then deform these lattices into different shapes and investigate their ability to retain the imposed shape when the energy is relaxed. The lattices are able to retain a range of curvatures. Under moderate forcing from a state of local equilibrium, the lattices deform by several percent but return to their retained shape when the forces are removed. By increasing the forcing until an irreversible motion occurs, we find that the transitions between remembered shapes show co-operativity among several springs. For fixed lattice structures, the shape memory tends to decrease as the lattice is enlarged; we propose ways to counter this decrease by modifying the lattice geometry. We survey the energy landscape by displacing individual nodes. An extensive fraction of these nodes proves to be bistable; they retain their displaced position when the energy is relaxed. Bending the lattice to a stable curved state alters the pattern of bistable nodes. We discuss this shapeability in the context of other forms of material memory and contrast it with the shapeability of plastic deformation. We outline the prospects for making real materials based on these principles.

cond-mat.soft↗

arXiv2014

Confined disclinations: exterior vs material constraints in developable thin elastic sheets

We examine the shape change of a thin disk with an inserted wedge of material when it is pushed against a plane, using analytical, numerical and experimental methods. Such sheets occur in packaging, surgery and nanotechnology. We approximate the sheet as having vanishing strain, so that it takes a conical form in which straight generators converge to a disclination singularity. Then its shape is that which minimizes elastic bending energy alone. Real sheets are expected to approach this limiting shape as their thickness approaches zero. The planar constraint forces a sector of the sheet to buckle into the third dimension. We find that the unbuckled sector is precisely semicircular, independent of the angle $δ$ of the inserted wedge. We generalize the analysis to include conical as well as planar constraints and thereby establish a law of corresponding states for shallow cones of slope $ε$ and thin wedges. In this regime the single parameter $δ/ε^2$ determines the shape. We discuss the singular limit in which the cone becomes a plane. We discuss the unexpected slow convergence to the semicircular buckling seen experimentally.

cond-mat.soft↗

arXiv2013

Shape and symmetry of a fluid-supported elastic sheet

A connection between the dynamics of a sine-Gordon chain and a certain static membrane folding problem was recently found. The one-dimensional membrane profile is a cross-section of the position-time sine-Gordon amplitude profile. Here we show that when one system is embedded in a higher-dimensional system in this way, obvious symmetries in the larger system can lead to nontrivial symmetries in the embedded system. In particular, a thin buckled membrane on a fluid substrate has a continuous degeneracy that interpolates between a symmetric and an antisymmetric fold. We find the Hamiltonian generator of this symmetry and the corresponding conserved momentum by interpreting the simple translational symmetries of the sine-Gordon chain in terms of the embedded coordinates. We discuss possible extensions to other embedded dynamical systems.

cond-mat.soft↗

arXiv2011

Instability of infinitesimal wrinkles against folding

We analyze the buckling of a rigid thin membrane floating on a dense fluid substrate. The interplay of curvature and substrate energy is known to create wrinkling at a characteristic wavelength $λ$, which localizes into a fold at sufficient buckling displacement $Δ$. By analyzing the regime $Δ<<λ$, we show that wrinkles are unstable to localized folding for {\em arbitrarily small} $Δ$. After observing that evanescent waves at the boundaries can be energetically favored over uniform wrinkles, we construct a localized Ansatz state far from boundaries that is also energetically favored. The resulting surface pressure $P$ in conventional units is $2-(π^2/4)(Δ/λ)^2$, in entire agreement with previous numerical results. The decay length of the amplitude is $κ^{-1}=(2/π^2)λ^2/Δ$. This case illustrates how a leading-order energy expression suggested by the infinitesimal displacement can give a qualitatively wrong configuration.

cond-mat.soft↗

arXiv2011

Compression induced folding of a sheet: an integrable system

The apparently intractable shape of a fold in a compressed elastic film lying on a fluid substrate is found to have an exact solution. Such systems buckle at a nonzero wavevector set by the bending stiffness of the film and the weight of the substrate fluid. Our solution describes the entire progression from a weakly displaced sinusoidal buckling to a single large fold that contacts itself. The pressure decrease is exactly quadratic in the lateral displacement. We identify a complex wavevector whose magnitude remains invariant with compression.

cond-mat.soft↗

arXiv2010

Singular electrostatic energy of nanoparticle clusters

The binding of clusters of metal nanoparticles is partly electrostatic. We address difficulties in calculating the electrostatic energy when high charging energies limit the total charge to a single quantum, entailing unequal potentials on the particles. We show that the energy at small separation $h$ has a strong logarithmic dependence on $h$. We give a general law for the strength of this logarithmic correction in terms of a) the energy at contact ignoring the charge quantization effects and b) an adjacency matrix specifying which spheres of the cluster are in contact and which is charged. We verify the theory by comparing the predicted energies for a tetrahedral cluster with an explicit numerical calculation.

cond-mat.mes-hall↗

arXiv2010

Plugs in rough capillary tubes: enhanced dependence of motion on plug length

We discuss the creeping motion of plugs of negligible viscosity in rough capillary tubes filled with carrier fluids. This extends Bretherton's research work on the infinite-length bubble motion in a cylindrical or smooth tube for small capillary numbers Ca. We first derive the asymptotic dependence of the plug speed on the finite length in the smooth tube case. This dependence on length is exponentially small, with a decay length much shorter than the tube radius R. Then we discuss the effect of azimuthal roughness of the tube on the plug speed. The tube roughness leads to an unbalanced capillary pressure and a carrier fluid flux in the azimuthal plane. This flux controls the relaxation of the plug shape to its infinite-length limit. For long-wavelength roughness, we find that the above decay length is much longer in the rough tube, and even becomes comparable to the tube radius R in some cases. This implies a much-enhanced dependence of the plug speed on the plug length. This mechanism may explain the catch-up effect seen experimentally.

cond-mat.soft↗

arXiv2009

Chiral sedimentation of extended objects in viscous media

We study theoretically the chirality of a generic rigid object's sedimentation in a fluid under gravity in the low Reynolds number regime. We represent the object as a collection of small Stokes spheres or stokeslets, and the gravitational force as a constant point force applied at an arbitrary point of the object. For a generic configuration of stokeslets and forcing point, the motion takes a simple form in the nearly free draining limit where the stokeslet radius is arbitrarily small. In this case, the internal hydrodynamic interactions between stokeslets are weak, and the object follows a helical path while rotating at a constant angular velocity $ω$ about a fixed axis. This $ω$ is independent of initial orientation, and thus constitutes a chiral response for the object. Even though there can be no such chiral response in the absence of hydrodynamic interactions between the stokeslets, the angular velocity obtains a fixed, nonzero limit as the stokeslet radius approaches zero. We characterize empirically how $ω$ depends on the placement of the stokeslets, concentrating on three-stokeslet objects with the external force applied far from the stokeslets. Objects with the largest $ω$ are aligned along the forcing direction. In this case, the limiting $ω$ varies as the inverse square of the minimum distance between stokeslets. We illustrate the prevalence of this robust chiral motion with experiments on small macroscopic objects of arbitrary shape.

cond-mat.soft↗

arXiv2009

Compressing nearly hard sphere fluids increases glass fragility

We use molecular dynamics to investigate the glass transition occurring at large volume fraction, phi, and low temperature, T, in assemblies of soft repulsive particles. We find that equilibrium dynamics in the (phi, T) plane obey a form of dynamic scaling in the proximity of a critical point at T=0 and phi=phi_0, which should correspond to the ideal glass transition of hard spheres. This glass point, `point G', is distinct from athermal jamming thresholds. A remarkable consequence of scaling behaviour is that the dynamics at fixed phi passes smoothly from that of a strong glass to that of a very fragile glass as phi increases beyond phi_0. Correlations between fragility and various physical properties are explored.

cond-mat.stat-mech↗

arXiv2009

The glass transition of dense fluids of hard and compressible spheres

We use computer simulations to study the glass transition of dense fluids made of polydisperse, repulsive spheres. For hard particles, we vary the volume fraction, phi, and use compressible particles to explore finite temperatures, T>0. In the hard sphere limit, our dynamic data show evidence of an avoided mode-coupling singularity near phi_{MCT} ~ 0.592, they are consistent with a divergence of equilibrium relaxation times occurring at phi_0 ~ 0.635, but they leave open the existence of a finite temperature singularity for compressible spheres at volume fraction phi > phi_0. Using direct measurements and a new scaling procedure, we estimate the equilibrium equation of state for the hard sphere metastable fluid up to phi_0, where pressure remains finite, suggesting that phi_0 corresponds to an ideal glass transition. We use non-equilibrium protocols to explore glassy states above phi_0 and establish the existence of multiple equations of state for the unequilibrated glass of hard spheres, all diverging at different densities in the range phi \in [0.642, 0.664]. Glassiness thus results in the existence of a continuum of densities where jamming transitions can occur.

cond-mat.stat-mech↗

arXiv2009

The compensation of Gaussian curvature in developable cones is local

In this paper we use the angular deficit scheme [V. Borrelli, F. Cazals, and J.-M. Morvan, {\sl Computer Aided Geometric Design} {\bf 20}, 319 (2003)] to determine the distribution of Gaussian curvature in developable cones (d-cones) [E. Cerda, S. Chaieb, F. Melo, and L. Mahadevan, {\sl Nature} {\bf 401}, 46 (1999)] numerically. These d-cones are formed by pushing a thin elastic sheet into a circular container. Negative Gaussian curvatures are identified at the rim where the sheet touches the container. Around the rim there are two narrow bands with positive Gaussian curvatures. The integral of the (negative) Gaussian curvature near the rim is almost completely compensated by that of the two adjacent bands. This suggests that the Gauss-Bonnet theorem which constrains the integral of Gaussian curvature globally does not explain the spontaneous curvature cancellation phenomenon [T. Liang and T. A. Witten, {\sl Phys. Rev. E} {\bf 73}, 046604 (2006)]. The locality of the compensation seems to increase for decreasing d-cone thickness. The angular deficit scheme also provides a new way to confirm the curvature cancellation phenomenon.

cond-mat.soft↗

arXiv2007

Microscopic Wrinkles on Supported Surfactant Monolayers

We discuss mechanical buckling instabilities of a rigid film under compression interacting repulsively with a substrate through a thin fluid layer. The buckling occurs at a characteristic wavelength that increases as the 1/4th power of the bending stiffness, like a gravitational instability studied previously by Milner et al. However, the potential can affect the characteristic buckling wavelength strongly, as predicted by Huang and Suo. If the potential changes sufficiently sharply with thickness, this instability is continuous, with an amplitude varying as the square root of overpressure. We discuss three forms of interaction important for the case of Langmuir monolayers transferred to a substrate: Casimir-van der Waals interaction, screened charged double-layer interaction and the Sharma potential. We verify these predictions numerically in the Van der Waals case.

cond-mat.soft↗

arXiv2006

Feasibility of Large Free-standing Liquid Films in Space

We consider the feasibility of large-scale free-standing thin liquid film experiment in the space environment as a new realization to study two-dimensional hydrodynamics. We identify material and environmental criteria necessary to avoid freezing, evaporation, chemical degradation, and spontaneous collapse of the film. These criteria pose no obstacles to achieving films of kilometer scale and lifetime of many months, with attainable Reynolds number up to 10^7. However, impacts from meteoroids pose a serious threat to the film, and require substantial shielding or unproven self-healing properties in the film. Current theoretical and experimental studies of two-dimensional turbulence are briefly reviewed. We also describe a specific candidate liquid for the film.

cond-mat.soft↗

arXiv2006

Spontaneous curvature cancellation in forced thin sheets

In this paper we report numerically observed spontaneous vanishing of mean curvature on a developable cone made by pushing a thin elastic sheet into a circular container. We show that this feature is independent of thickness of the sheet, the supporting radius and the amount of deflection. Several variants of developable cone are studied to examine the necessary conditions that lead to the vanishing of mean curvature. It is found that the presence of appropriate amount of radial stress is necessary. The developable cone geometry somehow produces the right amount of radial stress to induce just enough radial curvature to cancel the conical azimuthal curvature. In addition, the circular symmetry of supporting container edge plays an important role. With an elliptical supporting edge, the radial curvature overcompensates the azimuthal curvature near the minor axis and undercompensates near the major axis. Our numerical finding is verified by a crude experiment using a reflective plastic sheet. We expect this finding to have broad importance in describing the general geometrical properties of forced crumpling of thin sheets.

cond-mat.soft↗