arXiv subjects

Thomas Brabec

Publications and source records attributed to Thomas Brabec.

At least 19 recordsLinked to original sources

arXiv2026

Toroidal pulse enhanced XUV generation

Extreme ultraviolet (XUV) radiation plays a central role in a wide range of applications. Despite being a cornerstone of attosecond science, efficient XUV generation remains highly challenging. Here, we investigate XUV generation via nonlinear Thomson scattering driven by a toroidal pulse. Unlike conventional laser pulses, toroidal pulses possess intrinsically non-separable spatiotemporal field distributions. This unique field structure produces strongly asymmetric electron acceleration, resulting in substantially enhanced XUV emission that is 2-4 orders of magnitude stronger than that generated by a Gaussian pulse. Our results identify toroidal pulses as a promising route toward compact ultrafast XUV sources and advanced strong-field light-matter interaction studies.

physics.optics↗

arXiv2026

Roadmap on Attosecond Science

Twenty-five years have passed since the first experimental demonstration of attosecond pulses, marking the advent of our ability to resolve and control electron motion in real time. What began as a technological breakthrough - generating the shortest flashes ever produced - has evolved into a powerful approach for probing and steering electronic dynamics in atoms, molecules, and solids. This roadmap, authored by leading experts in the field, surveys the recent rapid progress in the generation and characterization of attosecond pulses, emerging attosecond measurement and control techniques, and their expanding range of applications. It reviews current and future developments in attosecond light sources, including novel laser technologies, waveform synthesizers, new schemes for high-order harmonic generation, attosecond pulse generation at free-electron lasers, and structured light. Advances in attosecond measurement methodologies are also discussed, encompassing all-attosecond pump-probe spectroscopy, attosecond four-wave mixing, attosecond microscopy, spectroscopy with light transients, and attosecond interferometry. Furthermore, the roadmap addresses applications of attosecond spectroscopy to reveal electron dynamics in molecules and condensed matter systems from both theoretical and experimental perspectives, and highlights emerging directions at the interface with quantum optics and quantum entanglement. Overall, this work aims to serve as a comprehensive resource for navigating the evolving landscape of attosecond science.

physics.optics↗

arXiv2025

Quantum Dial for High-Harmonic Generation

High-harmonic generation (HHG) is a highly nonlinear optical process that typically requires an intense laser to trigger emissions at integer multiples of the driving field frequency. However, the strong fields required for conventional HHG inevitably perturb the system, limiting its use as a nondestructive spectroscopic probe. Recent advances in bright squeezed vacuum (BSV) sources have created opportunities to drive HHG with quantum fields alone. In this work, we demonstrate a regime in which the light-matter interactions can be controlled and tuned using a weak classical field, whose pulse energy is two orders of magnitude lower than that in standard HHG-perturbed by an even weaker quantum field such as BSV. This approach opens new avenues for nonlinear spectroscopy of materials while substantially suppressing strong laser-induced damage, distortions, and heating. We show that a BSV pulse containing less than 5% of the classical driving energy can act as an 'optical dial', allowing tuning of the nonlinear emission spectrum, emission angular dependence, and ionization.

physics.optics↗

arXiv2025

A unified perspective of high-harmonic generation in gases and solids

We present a quantum optical generalization of the quantum-matter Lewenstein model of high-harmonic generation (HHG) in gases that contains two channels corresponding to the inter- and intraband HHG in solids. Both channels can be presented as a semiclassical current multiplied by the vacuum field strength, resulting in a quantitative correction and a faster roll-off of the harmonic power with order than in previous theories. In gases, like in solids, intraband HHG dominates at low orders; the switchover harmonic corresponds to a specific photon energy, independent of pump wavelength.

physics.atom-ph↗

arXiv2025

Quantum engineering of high harmonic generation

In quantum sideband high harmonic generation (QSHHG), high harmonic generation is perturbed by a bright quantum field resulting in harmonic sidebands, with the intent to transfer non-classical properties from the quantum perturbation to the harmonic sidebands. So far, non-classical features have not been found in QSHHG yet. The closed form theory of QSHHG in atoms and solids developed here answers the question under which conditions non-classical features can be realized. QSHHG results in a multi-mode entanglement between harmonic sideband modes and perturbative quantum mode. A projective measurement on either creates a variety of non-classical states commonly used in quantum information science. This opens a pathway towards quantum engineering high harmonic generation as a short wavelength source for quantum information science.

quant-ph↗

arXiv2025

Strong field physics in open quantum systems

Dephasing is the loss of phase coherence due to the interaction of an electron with the environment. The most common approach to model dephasing in light-matter interaction is the relaxation time approximation. Surprisingly, its use in intense laser physics results in a pronounced failure, because ionization {is highly overestimated.} Here, this shortcoming is corrected by developing a strong field model in which the many-body environment is represented by a heat bath. Our model reveals that ionization enhancement and suppression by several orders of magnitude are still possible, however only in more extreme parameter regimes. Our approach allows the integration of many-body physics into intense laser dynamics with minimal computational and mathematical complexity, thus facilitating the identification of novel effects in strong-field physics and attosecond {science}.

physics.optics↗

arXiv2024

Photon bunching in high-harmonic emission controlled by quantum light

Attosecond spectroscopy comprises several techniques to probe matter through electrons and photons. One frontier of attosecond methods is to reveal complex phenomena arising from quantum-mechanical correlations in the matter system, in the photon fields and among them. Recent theories have laid the groundwork for understanding how quantum-optical properties affect high-field photonics, such as strong-field ionization and acceleration of electrons in quantum-optical fields, and how entanglement between the field modes arises during the interaction. Here we demonstrate a new experimental approach that transduces some properties of a quantum-optical state through a strong-field nonlinearity. We perturb high-harmonic emission from a semiconductor with a bright squeezed vacuum field resulting in the emission of sidebands of the high-harmonics with super-Poissonian statistics, indicating that the emitted photons are bunched. Our results suggest that perturbing strong-field dynamics with quantum-optical states is a viable way to coherently control the generation of these states at short wavelengths, such as extreme ultraviolet or soft X-rays. Quantum correlations will be instrumental to advance attosecond spectroscopy and imaging beyond the classical limits.

quant-ph↗

arXiv2024

Table-Top Tunable Chiral Photonic Emitter

The increasing interest in chiral light stems from its spiral trajectory along the propagation direction, facilitating the interaction between different polarization states of light and matter. Despite tremendous achievements in chiral light-related research, the generation and control of chiral pulse have presented enduring challenges, especially at the terahertz and ultraviolet spectral ranges, due to the lack of suitable optical elements for effective pulse manipulation. Conventionally, chiral light can be obtained from intricate optical systems, by an external magnetic field, or by metamaterials, which necessitate sophisticated optical configurations. Here, we propose a versatile tunable chiral emitter, composed of only two planar Weyl semimetals slabs, addressing the challenges in both spectral ranges. Our results open the way to a compact tunable chiral emitter platform in both terahertz and ultra-violet frequency ranges. This advancement holds the potential to serve as the cornerstone for integrated chiral photonics.

physics.optics↗

arXiv2020

Wannier quasi-classical approach to high harmonic generation in semiconductors

We develop a quasi-classical theory of high harmonic generation in semiconductors based on an interband current that has been transformed from Bloch to Wannier basis. The Wannier quasi-classical approach reveals a complete picture of the mechanisms shaping high harmonic generation, such that quantitative agreement with full quantum calculations is obtained. The intuitive picture revealed by quasi-classical wavepacket propagation will be helpful in the interpretation and design of high harmonic and attosecond experiments. Beyond that, the capacity to quantitatively model quantum dynamics with classical trajectories should prove useful for a wider spectrum of condensed matter research, including coherent control, transport theory, and strong field physics.

cond-mat.mes-hall↗

arXiv2018

Multi-Band Petahertz Currents Resolved via High Harmonic Generation Spectroscopy

Strong field driven electric currents in condensed matter systems open new frontiers in petahertz electronics. In this regime new challenges arise as the role of the band structure and the quantum nature of electron-hole dynamics have yet to be resolved. Here we reveal the underlying attosecond dynamics that dictates the temporal evolution of carriers in multi-band solid state systems, via high harmonic generation (HHG) spectroscopy. We demonstrate that when the electron-hole relative velocity approaches zero, enhanced quantum interference leads to the appearance of spectral caustics in the HHG spectrum. Introducing the role of the dynamical joint density of states (JDOS) we identify its direct mapping into the spectrum, exhibiting singularities at the spectral caustics. By probing these singularities, we visualize the structure of multiple unpopulated high conduction bands. Our results open a new path in the control and study of attosecond quasi-particle interactions within the field dressed band structure of crystals.

physics.optics↗

arXiv2017

Explicit formulation of second and third order optical nonlinearity in the FDTD framework

The finite-difference time-domain (FDTD) method is a flexible and powerful technique for rigorously solving Maxwell's equations. However, three-dimensional optical nonlinearity in current commercial and research FDTD softwares requires solving iteratively an implicit form of Maxwell's equations over the entire numerical space and at each time step. Reaching numerical convergence demands significant computational resources and practical implementation often requires major modifications to the core FDTD engine. In this paper, we present an explicit method to include second and third order optical nonlinearity in the FDTD framework based on a nonlinear generalization of the Lorentz dispersion model. A formal derivation of the nonlinear Lorentz dispersion equation is equally provided, starting from the quantum mechanical equations describing nonlinear optics in the two-level approximation. With the proposed approach, numerical integration of optical nonlinearity and dispersion in FDTD is intuitive, transparent, and fully explicit. A strong-field formulation is also proposed, which opens an interesting avenue for FDTD-based modelling of the extreme nonlinear optics phenomena involved in laser filamentation and femtosecond micromachining of dielectrics.

physics.optics↗

arXiv2015

MeV femtosecond electron pulses from direct-field acceleration in low density atomic gases

Using three-dimensional particle-in-cell simulations, we show that few-MeV electrons can be produced by focusing tightly few-cycle radially-polarized laser pulses in a low-density atomic gas. In particular, it is observed that for the few-TW laser power needed to reach relativistic electron energies, longitudinal attosecond microbunching occurs naturally, resulting in femtosecond structures with high-contrast attosecond density modulations. The three-dimensional particle-in-cell simulations show that in the relativistic regime the leading pulse of these attosecond substructures survives to propagation over extended distances, suggesting that it could be delivered to a distant target, with the help of a properly designed transport beamline.

physics.optics↗

arXiv2015

Saturable Lorentz model for fully explicit three-dimensional modeling of nonlinear optics

Inclusion of the instantaneous Kerr nonlinearity in the FDTD framework leads to implicit equations that have to be solved iteratively. In principle, explicit integration can be achieved with the use of anharmonic oscillator equations, but it tends to be unstable and inappropriate for studying strong-field phenomena like laser filamentation. In this paper, we show that nonlinear susceptibility can be provided instead by a harmonic oscillator driven by a nonlinear force, chosen in a way to reproduce the polarization obtained from the solution of the quantum mechanical two level equations. The resulting saturable, nonlinearly-driven, harmonic oscillator model reproduces quantitatively the quantum mechanical solutions of harmonic generation in the under-resonant limit, up to the 9th harmonic. Finally, we demonstrate that fully explicit leapfrog integration of the saturable harmonic oscillator is stable, even for the intense laser fields that characterize laser filamentation and high harmonic generation.

physics.optics↗

arXiv2013

Femtosecond 240-keV electron pulses from direct laser acceleration in a low-density gas

We propose a simple laser-driven electron acceleration scheme based on tightly focused radially polarized laser pulses for the production of femtosecond electron bunches with energies in the few-hundreds-of-keV range. In this method, the electrons are accelerated forward in the focal volume by the longitudinal electric field component of the laser pulse. Three-dimensional test-particle and particle-in-cell simulations reveal the feasibility of generating well-collimated electron bunches with an energy spread of 5% and a temporal duration of the order of 1 fs. These results offer a route towards unprecedented time resolution in ultrafast electron diffraction experiments.

physics.acc-ph↗

arXiv2013

Quantum Breathing Mode of Trapped Systems in One and Two Dimensions

We investigate the quantum breathing mode (monopole oscillation) of trapped fermionic particles with Coulomb and dipole interaction in one and two dimensions. This collective oscillation has been shown to reveal detailed information on the many-particle state of interacting trapped systems and is thus a sensitive diagnostics for a variety of finite systems, including cold atomic and molecular gases in traps and optical lattics, electrons in metal clusters and in quantum confined semiconductor structures or nanoplasmas. An improved sum rule formalism allows us to accurately determine the breathing frequencies from the ground state of the system, avoiding complicated time-dependent simulations. In combination with the Hartree-Fock and the Thomas-Fermi approximations this enables us to extend the calculations to large particle numbers $N$ on the order of several million. Tracing the breathing frequency to large $N$ as a function of the coupling parameter of the system reveals a surprising difference of the asymptotic behavior of one-dimensional and two-dimensional harmonically trapped Coulomb systems.

quant-ph↗

arXiv2012

Dynamical Magnetic and Nuclear Polarization in Complex Spin Systems: Semi-magnetic II-VI Quantum Dots

Dynamical magnetic and nuclear polarization in complex spin systems is discussed on the example of transfer of spin from exciton to the central spin of magnetic impurity in a quantum dot in the presence of a finite number of nuclear spins. The exciton is described in terms of the electron and heavy hole spins interacting via exchange interaction with magnetic impurity, via hypeprfine interaction with a finite number of nuclear spins and via dipole interaction with photons. The time-evolution of the exciton, magnetic impurity and nuclear spins is calculated exactly between quantum jumps corresponding to exciton radiative recombination. The collapse of the wavefunction and the refilling of the quantum dot with new spin polarized exciton is shown to lead to build up of magnetization of the magnetic impurity as well as nuclear spin polarization. The competition between electron spin transfer to magnetic impurity and to nuclear spins simultaneous with the creation of dark excitons is elucidated. The technique presented here opens up the possibility of studying optically induced Dynamical Magnetic and Nuclear Polarization in Complex Spin Systems.

cond-mat.mes-hall↗

arXiv2012

Spin textures in strongly coupled electron spin and magnetic or nuclear spin systems in quantum dots

Controlling electron spins strongly coupled to magnetic and nuclear spins in solid state systems is an important challenege in the field of spintronics and quantum computation. We show here that electron droplets with no net spin in semiconductor quantum dots strongly coupled with magnetic ion/nuclear spin systems break down at low temperature and form a non-trivial anti-ferromagnetic spatially ordered spin-texture of magneto-polarons. The spatially ordered combined electron-magnetic ion spin-texture, associated with spontaneous symmetry-breaking in the parity of electronic charge density and magnetization of magnetic ions, emerge from both ab-initio density functional approach to the electronic system coupled with mean-field approximation for the magnetic/nuclear spin system and fully mircoscopic exact diagonalization of small systems. The predicted phase diagram determines the critical temperature as a function of coupling strength and identifies possible phases of the strongly coupled spin system. This prediction may arrest fluctuations in spin system and open the way to control, manipulate and prepare magnetic and nuclear spin ensembles in semiconductor nanostructures.

cond-mat.mes-hall↗

arXiv2012

Multiscale QM/MM Molecular Dynamics Study on the First Steps of Guanine-Damage by Free Hydroxyl Radicals in Solution

Understanding the damage of DNA bases from hydrogen abstraction by free OH radicals is of particular importance to reveal the effect of hydroxyl radicals produced by the secondary effect of radiation. Previous studies address the problem with truncated DNA bases as ab-initio quantum simulation required to study such electronic spin dependent processes are computationally expensive. Here, for the first time, we employ a multiscale and hybrid Quantum-Mechanical-Molecular-Mechanical simulation to study the interaction of OH radicals with guanine-deoxyribose-phosphate DNA molecular unit in the presence of water where all the water molecules and the deoxyribose-phosphate fragment are treated with the simplistic classical Molecular-Mechanical scheme. Our result illustrates that the presence of water strongly alters the hydrogen-abstraction reaction as the hydrogen bonding of OH radicals with water restricts the relative orientation of the OH-radicals with respective to the the DNA base (here guanine). This results in an angular anisotropy in the chemical pathway and a lower efficiency in the hydrogen abstraction mechanisms than previously anticipated for identical system in vacuum. The method can easily be extended to single and double stranded DNA without any appreciable computational cost as these molecular units can be treated in the classical subsystem as has been demonstrated here.

physics.comp-ph↗