arXiv subjects

Thomas Chalopin

Publications and source records attributed to Thomas Chalopin.

16 recordsLinked to original sources

arXiv2026

Universal scaling of fluctuations and correlations across the superfluid transition

The critical behavior of a system near a continuous phase transition is commonly characterized by power laws and a set of universal critical exponents. Yet universality at phase transitions has even more fundamental manifestations. It dictates that all observables follow universal scaling functions, which may extend beyond simple power laws. Furthermore, microscopic details are captured entirely by only two system-specific scale factors, that rescale any measured quantity onto its universal form. In this work, we report the experimental validation of this prediction in ultracold lattice Bose gases undergoing the superfluid transition. We extract the scale factors by collapsing the order-parameter cumulants measured at varying entropies. We show that these factors specify scaling functions governing both the order-parameter distribution and two-point correlations. By measuring these scaling functions, we also determine three critical exponents $\beta$, $\gamma$ and $\nu$. Our results provide an experimental demonstration that universal scaling is simultaneously obeyed by multiple observables in a quantum many-body system.

cond-mat.quant-gas↗

arXiv2026

Emergence of spin entanglement with the pseudogap onset in the Fermi-Hubbard model

Despite decades of intense theoretical and experimental investigation, the two-dimensional Fermi-Hubbard model still resists a complete microscopic understanding. Conventional approaches typically probe global observables and locally resolved correlation functions. Here, we develop a complementary perspective based on the measurement of entanglement. Using both an ultracold-atom quantum simulator and numerical simulations based on the dynamical vertex approximation, we find that entanglement is closely tied to the onset of the enigmatic pseudogap regime: spin-singlet entanglement emerges only as the pseudogap sets in and, in contrast to classical correlations, remains confined to nearest-neighbour sites in this regime. Our results, therefore, disfavour purely classical-fluctuation theories of the pseudogap and constrain microscopic models to those that develop nearest-neighbour spin-singlet entanglement at the pseudogap onset.

cond-mat.str-el↗

arXiv2026

Observation of emergent scaling of spin-charge correlations at the onset of the pseudogap

In strongly correlated materials, interacting electrons are entangled and form collective quantum states, resulting in rich low-temperature phase diagrams. Notable examples include cuprate superconductors, in which superconductivity emerges at low doping out of an unusual "pseudogap" metallic state above the critical temperature. The Fermi-Hubbard model, describing a wide range of phenomena associated with strong electron correlations, still offers major computational challenges despite its simple formulation. In this context, ultracold atoms quantum simulators have provided invaluable insights into the microscopic nature of correlated quantum states. Here, we use a quantum gas microscope Fermi-Hubbard simulator to explore a wide range of dopings and temperatures in a regime where a pseudogap is known to develop. By measuring multi-point correlation functions up to fifth order, we uncover a novel universal scaling behaviour in magnetic and higher-order spin-charge correlations characterised by a doping-dependent temperature scale. Accurate comparisons with determinant Quantum Monte Carlo and Minimally Entangled Typical Thermal States simulations confirm that this temperature scale is comparable to the pseudogap temperature T*. Our quantitative findings reveal a novel qualitative behaviour of magnetic properties and spin-charge correlations in an emergent pseudogap and pave the way towards the exploration of charge pairing and collective phenomena expected at lower temperatures.

cond-mat.str-el↗

arXiv2025

Connected correlations in cold atom experiments

The recent development of single-atom-resolved probes has made full counting statistics measurements accessible in quantum gas experiments. This capability provides access to high-order moments of physical observables, from which cumulants, or equivalently connected correlations, can be precisely determined. Through a selection of recent cold atom experiments, this article illustrates the significance of connected correlations in characterizing ensembles of interacting quantum particles. First, non-zero connected correlations of order n > 2 unambiguously identify non-Gaussian quantum states. Second, connected correlations of order n identify clusters made of n elements whose statistical properties are irreducible to combinations of smaller clusters. The ability to identify such multi-particle clusters offers a an interesting perspective on strongly correlated quantum states of matter at the microscopic scale.

cond-mat.quant-gas↗

arXiv2025

Observation of universal non-Gaussian statistics of the order parameter across a continuous phase transition

Second-order phase transitions are characterised by critical scaling and universality. The singular behaviour of thermodynamic quantities at the transition, in particular, is determined by critical exponents of the universality class of the transition. However, critical properties are also characterised by the probability distribution of the order parameter across the transition, where non-Gaussian statistics are expected, but remain largely unexplored. Here, making use of single-atom-resolved detection in momentum space, we measure the full probability distribution of the order-parameter amplitude across a continuous phase transition in an interacting lattice Bose gas. We find that fluctuations are captured by an effective potential -- reconstructed from the measured probability distribution by analogy with Landau theory -- displaying a non-trivial minimum in the superfluid (ordered) phase, which vanishes at the transition point. Additionally, we observe non-Gaussian statistics of the order parameter near the transition, distinguished by non-zero high-order cumulants undergoing abrupt sign changes. We show numerically that these sign changes of the cumulants obey critical scaling in homogeneous systems, and that their experimental behaviour is not reproduced by classical models, whereas it is captured by a low-temperature quantum model. Our results underscore the crucial role of order parameter statistics in probing critical phenomena and universality.

cond-mat.quant-gas↗

arXiv2025

High-fidelity collisional quantum gates with fermionic atoms

Quantum simulations of electronic structure and strongly correlated quantum phases are widely regarded as among the most promising applications of quantum computing. These computations naturally benefit from native fermionic encodings, which intrinsically restrict the Hilbert space to physical states consistent with fermionic statistics and conservation laws like particle number and magnetization independent of gate errors. While ultracold atoms in optical lattices are established as powerful analog simulators of strongly correlated fermionic matter, neutral-atom platforms have concurrently emerged as versatile, scalable architectures for spin-based digital quantum computation. Unifying these capabilities requires high-fidelity gates that preserve motional degrees of freedom of fermionic atoms, paving the way for a new generation of programmable fermionic quantum processors. Here we demonstrate collisional entangling gates with fidelities up to 99.75(6)% and Bell state lifetimes exceeding $10\,s$, realized via controlled interactions of fermionic atoms in an optical superlattice. Using quantum gas microscopy, we microscopically characterize spin-exchange and pair-tunneling gates, and realize a robust, composite pair-exchange gate, a fundamental primitive for quantum chemistry simulations. Our results establish controlled collisions in optical lattices as a competitive and complementary approach to high entangling gate fidelities in neutral-atom quantum computers. When embedded within a fermionic architecture, this capability enables the preparation of complex quantum states and advanced readout protocols for a new class of scalable analog-digital hybrid quantum simulators. Combined with local addressing, these gates mark a crucial step towards a fully digital fermionic quantum computer based on the controlled motion and entanglement of fermionic neutral atoms.

cond-mat.quant-gas↗

arXiv2024

Local control and mixed dimensions: Exploring high-temperature superconductivity in optical lattices

The simulation of high-temperature superconducting materials by implementing strongly correlated fermionic models in optical lattices is one of the major objectives in the field of analog quantum simulation. Here we show that local control and optical bilayer capabilities combined with spatially resolved measurements create a versatile toolbox to study fundamental properties of both nickelate and cuprate high-temperature superconductors. On the one hand, we present a scheme to implement a mixed-dimensional (mixD) bilayer model that has been proposed to capture the essential pairing physics of pressurized bilayer nickelates. This allows for the long-sought realization of a state with long-range superconducting order in current lattice quantum simulation machines. In particular, we show how coherent pairing correlations can be accessed in a partially particle-hole transformed and rotated basis. On the other hand, we demonstrate that control of local gates enables the observation of $d$-wave pairing order in the two-dimensional (single-layer) repulsive Fermi-Hubbard model through the simulation of a system with attractive interactions. Lastly, we introduce a scheme to measure momentum-resolved dopant densities, providing access to observables complementary to solid-state experiments -- which is of particular interest for future studies of the enigmatic pseudogap phase appearing in cuprates.

cond-mat.quant-gas↗

arXiv2024

Optical superlattice for engineering Hubbard couplings in quantum simulation

Quantum simulations of Hubbard models with ultracold atoms rely on the exceptional control of coherent motion provided by optical lattices. Here we demonstrate enhanced tunability using an optical superlattice in a fermionic quantum gas microscope. With our phase-stable bichromatic design, we achieve a precise control of tunneling and tilt throughout the lattice, as evidenced by long-lived coherent double-well oscillations and next-nearest-neighbor quantum walks in a staggered configuration. We furthermore present correlated quantum walks of two particles initiated through a resonant pair-breaking mechanism. Finally, we engineer tunable spin couplings through local offsets and create a spin ladder with ferromagnetic and antiferromagnetic couplings along the rungs and legs, respectively. Our work underscores the high potential of optical superlattices for engineering, simulating, and detecting strongly correlated many-body quantum states.

cond-mat.quant-gas↗

arXiv2023

Formation of stripes in a mixed-dimensional cold-atom Fermi-Hubbard system

The relation between d-wave superconductivity and stripes is fundamental to the understanding of ordered phases in cuprates. While experimentally both phases are found in close proximity, numerical studies on the related Fermi-Hubbard model have long been investigating whether stripes precede, compete or coexist with superconductivity. Such stripes are characterised by interleaved charge and spin density wave ordering where fluctuating lines of dopants separate domains of opposite antiferromagnetic order. Here we show first signatures of stripes in a cold-atom Fermi-Hubbard quantum simulator. By engineering a mixed-dimensional system, we increase their typical energy scales to the spin exchange energy, enabling us to access the interesting crossover temperature regime where stripes begin to form. We observe extended, attractive correlations between hole dopants and find an increased probability to form larger structures akin to stripes. In the spin sector, we study correlation functions up to third order and find results consistent with stripe formation. These higher-order correlation measurements pave the way towards an improved microscopic understanding of the emergent properties of stripes and their relation to other competing phases. More generally, our approach has direct relevance for newly discovered high-temperature superconducting materials in which mixed dimensions play an essential role.

cond-mat.quant-gas↗

arXiv2022

Magnetically mediated hole pairing in fermionic ladders of ultracold atoms

Pairing of mobile charge carriers in doped antiferromagnets plays a key role in the emergence of unconventional superconductivity. In these strongly correlated materials, the pairing mechanism is often assumed to be mediated by magnetic correlations, in contrast to phonon-mediated interactions in conventional superconductors. A precise understanding of the underlying mechanism in real materials is, however, still lacking, and has been driving experimental and theoretical research for the past 40 years. Early theoretical studies established the emergence of binding among dopants in ladder systems, where idealised theoretical toy models played an instrumental role in the elucidation of pairing, despite repulsive interactions. Here, we realise this long-standing theoretical prediction and report on the observation of hole pairing due to magnetic correlations in a quantum gas microscope setting. By engineering doped antiferromagnetic ladders with mixed-dimensional couplings we suppress Pauli blocking of holes at short length scales. This results in a drastic increase in binding energy and decrease in pair size, enabling us to observe pairs of holes predominantly occupying the same rung of the ladder. We find a hole-hole binding energy on the order of the superexchange energy, and, upon increased doping, we observe spatial structures in the pair distribution, indicating repulsion between bound hole pairs. By engineering a configuration in which binding is strongly enhanced, we delineate a novel strategy to increase the critical temperature for superconductivity.

cond-mat.quant-gas↗

arXiv2021

Realising the Symmetry-Protected Haldane Phase in Fermi-Hubbard Ladders

Topology in quantum many-body systems has profoundly changed our understanding of quantum phases of matter. The paradigmatic model that has played an instrumental role in elucidating these effects is the antiferromagnetic spin-1 Haldane chain. Its ground state is a disordered state, with symmetry-protected fourfold-degenerate edge states due to fractional spin excitations. In the bulk, it is characterised by vanishing two-point spin correlations, gapped excitations, and a characteristic non-local order parameter. More recently it was understood that the Haldane chain forms a specific example of a more general classification scheme of symmetry protected topological (SPT) phases of matter that is based on ideas connecting to quantum information and entanglement. Here, we realise such a topological Haldane phase with Fermi-Hubbard ladders in an ultracold-atom quantum simulator. We directly reveal both edge and bulk properties of the system through the use of single-site and particle-resolved measurements as well as non-local correlation functions. Continuously changing the Hubbard interaction strength of the system allows us to investigate the robustness of the phase to charge (density) fluctuations far from the regime of the Heisenberg model employing a novel correlator.

cond-mat.quant-gas↗

arXiv2021

Probing chiral edge dynamics and bulk topology of a synthetic Hall system

Quantum Hall systems are characterized by the quantization of the Hall conductance -- a bulk property rooted in the topological structure of the underlying quantum states. In condensed matter devices, material imperfections hinder a direct connection to simple topological models. Artificial systems, such as photonic platforms or cold atomic gases, open novel possibilities by enabling specific probes of topology or flexible manipulation e.g. using synthetic dimensions. However, the relevance of topological properties requires the notion of a bulk, which was missing in previous works using synthetic dimensions of limited sizes. Here, we realize a quantum Hall system using ultracold dysprosium atoms, in a two-dimensional geometry formed by one spatial dimension and one synthetic dimension encoded in the atomic spin $J=8$. We demonstrate that the large number of magnetic sublevels leads to distinct bulk and edge behaviors. Furthermore, we measure the Hall drift and reconstruct the local Chern marker, an observable that has remained, so far, experimentally inaccessible. In the center of the synthetic dimension -- a bulk of 11 states out of 17 -- the Chern marker reaches 98(5)\% of the quantized value expected for a topological system. Our findings pave the way towards the realization of topological many-body phases.

cond-mat.quant-gas↗

arXiv2019

Probing quantum criticality and symmetry breaking at the microscopic level

We report on an experimental study of the Lipkin-Meshkov-Glick model of quantum spins interacting at infinite range in a transverse magnetic field, which exhibits a ferromagnetic phase transition in the thermodynamic limit. We use Dysprosium atoms of electronic spin $J=8$, subjected to a quadratic Zeeman light shift, to simulate $2J=16$ interacting spins $1/2$. We probe the system microscopically using single magnetic sublevel resolution, giving access to the spin projection parity, which is the collective observable characterizing the underlying $\mathbb{Z}_2$ symmetry. We measure the thermodynamic properties and dynamical response of the system, and study the quantum critical behavior around the transition point. In the ferromagnetic phase, we achieve coherent tunneling between symmetry-broken states, and test the link between symmetry breaking and the appearance of a finite order parameter.

cond-mat.quant-gas↗

arXiv2019

Enhanced magnetic sensitivity with non-gaussian quantum fluctuations

The precision of a quantum sensor can overcome its classical counterpart when its constituents are entangled. In gaussian squeezed states, quantum correlations lead to a reduction of the quantum projection noise below the shot noise limit. However, the most sensitive states involve complex non-gaussian quantum fluctuations, making the required measurement protocol challenging. Here we measure the sensitivity of non-classical states of the electronic spin $J = 8$ of dysprosium atoms, created using light-induced non-linear spin coupling. Magnetic sublevel resolution enables us to reach the optimal sensitivity of non-gaussian (oversqueezed) states, well above the capability of squeezed states and about half the Heisenberg limit.

cond-mat.quant-gas↗

arXiv2018

Anisotropic light-shift and magic-polarization of the intercombination line of Dysprosium atoms in a far-detuned dipole trap

We characterize the anisotropic differential ac-Stark shift for the Dy $626$ nm intercombination transition, induced in a far-detuned $1070$ nm optical dipole trap, and observe the existence of a "magic polarization" for which the polarizabilities of the ground and excited states are equal. From our measurements we extract both the scalar and tensorial components of the dynamic dipole polarizability for the excited state, $α_E^\text{s} = 188 (12)\,α_\text{0}$ and $α_E^\text{t} = 34 (12)\,α_\text{0}$, respectively, where $α_\text{0}$ is the atomic unit for the electric polarizability. We also provide a theoretical model allowing us to predict the excited state polarizability and find qualitative agreement with our observations. Furthermore, we utilize our findings to optimize the efficiency of Doppler cooling of a trapped gas, by controlling the sign and magnitude of the inhomogeneous broadening of the optical transition. The resulting initial gain of the collisional rate allows us, after forced evaporation cooling, to produce a quasi-pure Bose-Einstein condensate of $^{162}$Dy with $3\times 10^4$ atoms.

cond-mat.quant-gas↗

arXiv2018

Quantum-enhanced sensing using non-classical spin states of a highly magnetic atom

Coherent superposition states of a mesoscopic quantum object play a major role in our understanding of the quantum to classical boundary, as well as in quantum-enhanced metrology and computing. However, their practical realization and manipulation remains challenging, requiring a high degree of control of the system and its coupling to the environment. Here, we use dysprosium atoms - the most magnetic element in its ground state - to realize coherent superpositions between electronic spin states of opposite orientation, with a mesoscopic spin size J=8. We drive coherent spin states to quantum superpositions using non-linear light-spin interactions, observing a series of collapses and revivals of quantum coherence. These states feature highly non-classical behavior, with a sensitivity to magnetic fields enhanced by a factor 13.9(1.1) compared to coherent spin states - close to the Heisenberg limit 2J=16 - and an intrinsic fragility to environmental noise.

quant-ph↗