arXiv subjects

Thomas E. Murphy

Publications and source records attributed to Thomas E. Murphy.

34 records · Page 2Linked to original sources

arXiv2016

Mid-infrared time-resolved photoconduction in black phosphorus

Black phosphorus has attracted interest as a material for use in optoelectronic devices due to many favorable properties such as a high carrier mobility, field-effect, and a direct bandgap that can range from 0.3 eV in its bulk crystalline form to 2 eV for a single atomic layer. The low bandgap energy for bulk black phosphorus allows for direct transition photoabsorption that enables detection of light out to mid-infrared frequencies. In this work we characterize the room temperature optical response of a black phosphorus photoconductive detector at wavelengths ranging from 1.56 $μ$m to 3.75 $μ$m. Pulsed autocorrelation measurements in the near-infrared regime reveal a strong, sub-linear photocurrent nonlinearity with a response time of 1 ns, indicating that gigahertz electrical bandwidth is feasible. Time resolved photoconduction measurements covering near- and mid-infrared frequencies show a fast 65 ps rise time, followed by a carrier relaxation with a time scale that matches the intrinsic limit determined by autocorrelation. The sublinear photoresponse is shown to be caused by a reduction in the carrier relaxation time as more energy is absorbed in the black phosphorus flake and is well described by a carrier recombination model that is nonlinear with excess carrier density. The device exhibits a measured noise-equivalent power of 530 pW/$\sqrt{\text{Hz}}$ which is the expected value for Johnson noise limited performance. The fast and sensitive room temperature photoresponse demonstrates that black phosphorus is a promising new material for mid-infrared optoelectronics.

cond-mat.mtrl-sci↗

arXiv2016

Experimental observation of chimera and cluster states in a minimal globally coupled network

A "chimera state" is a dynamical pattern that occurs in a network of coupled identical oscillators when the symmetry of the oscillator population is broken into synchronous and asynchronous parts. We report the experimental observation of chimera and cluster states in a network of four globally coupled chaotic opto-electronic oscillators. This is the minimal network that can support chimera states, and our study provides new insight into the fundamental mechanisms underlying their formation. We use a unified approach to determine the stability of all the observed partially synchronous patterns, highlighting the close relationship between chimera and cluster states as belonging to the broader phenomenon of partial synchronization. Our approach is general in terms of network size and connectivity. We also find that chimera states often appear in regions of multistability between global, cluster, and desynchronized states.

nlin.CD↗

arXiv2015

Terahertz Nonlinearity in Graphene Plasmons

Sub-wavelength graphene structures support localized plasmonic resonances in the terahertz and mid-infrared spectral regimes. The strong field confinement at the resonant frequency is predicted to significantly enhance the light-graphene interaction, which could enable nonlinear optics at low intensity in atomically thin, sub-wavelength devices. To date, the nonlinear response of graphene plasmons and their energy loss dynamics have not been experimentally studied. We measure and theoretically model the terahertz nonlinear response and energy relaxation dynamics of plasmons in graphene nanoribbons. We employ a THz pump-THz probe technique at the plasmon frequency and observe a strong saturation of plasmon absorption followed by a 10 ps relaxation time. The observed nonlinearity is enhanced by two orders of magnitude compared to unpatterned graphene with no plasmon resonance. We further present a thermal model for the nonlinear plasmonic absorption that supports the experimental results.

physics.optics↗

arXiv2015

Complete Characterization of Stability of Cluster Synchronization in Complex Dynamical Networks

Synchronization is an important and prevalent phenomenon in natural and engineered systems. In many dynamical networks, the coupling is balanced or adjusted in order to admit global synchronization, a condition called Laplacian coupling. Many networks exhibit incomplete synchronization, where two or more clusters of synchronization persist, and computational group theory has recently proved to be valuable in discovering these cluster states based upon the topology of the network. In the important case of Laplacian coupling, additional synchronization patterns can exist that would not be predicted from the group theory analysis alone. The understanding of how and when clusters form, merge, and persist is essential for understanding collective dynamics, synchronization, and failure mechanisms of complex networks such as electric power grids, distributed control networks, and autonomous swarming vehicles. We describe here a method to find and analyze all of the possible cluster synchronization patterns in a Laplacian-coupled network, by applying methods of computational group theory to dynamically-equivalent networks. We present a general technique to evaluate the stability of each of the dynamically valid cluster synchronization patterns. Our results are validated in an electro-optic experiment on a 5 node network that confirms the synchronization patterns predicted by the theory.

nlin.CD↗

arXiv2015

Harvesting entropy and quantifying the transition from noise to chaos in a photon-counting feedback loop

Some physical processes, including the intensity fluctuations of a chaotic laser, the detection of single photons, and the Brownian motion of a microscopic particle in a fluid are unpredictable, at least on long timescales. This unpredictability can be due to a variety of physical mechanisms, but it is quantified by an entropy rate. This rate describes how quickly a system produces new and random information, is fundamentally important in statistical mechanics and practically important for random number generation. We experimentally study entropy generation and the emergence of deterministic chaotic dynamics from discrete noise in a system that applies feedback to a weak optical signal at the single-photon level. We show that the dynamics qualitatively change from shot noise to chaos as the photon rate increases, and that the entropy rate can reflect either the deterministic or noisy aspects of the system depending on the sampling rate and resolution.

nlin.CD↗

arXiv2015

Hybrid Metal-Graphene Plasmons for Tunable Terahertz Technology

Among its many outstanding properties, graphene supports terahertz surface plasma waves -- sub-wavelength charge density oscillations connected with electromagnetic fields that are tightly localized near the surface[1,2]. When these waves are confined to finite-sized graphene, plasmon resonances emerge that are characterized by alternating charge accumulation at the opposing edges of the graphene. The resonant frequency of such a structure depends on both the size and the surface charge density, and can be electrically tuned throughout the terahertz range by applying a gate voltage[3,4]. The promise of tunable graphene THz plasmonics has yet to be fulfilled, however, because most proposed optoelectronic devices including detectors, filters, and modulators[5-10] desire near total modulation of the absorption or transmission, and require electrical contacts to the graphene -- constraints that are difficult to meet using existing plasmonic structures. We report here a new class of plasmon resonance that occurs in a hybrid graphene-metal structure. The sub-wavelength metal contacts form a capacitive grid for accumulating charge, while the narrow interleaved graphene channels, to first order, serves as a tunable inductive medium, thereby forming a structure that is resonantly-matched to an incident terahertz wave. We experimentally demonstrate resonant absorption near the theoretical maximum in readily-available, large-area graphene, ideal for THz detectors and tunable absorbers. We further predict that the use of high mobility graphene will allow resonant THz transmission near 100%, realizing a tunable THz filter or modulator. The structure is strongly coupled to incident THz radiation, and solves a fundamental problem of how to incorporate a tunable plasmonic channel into a device with electrical contacts.

cond-mat.mes-hall↗

arXiv2015

Carrier Dynamics and Transient Photobleaching in Thin Layers of Black Phosphorus

We present polarization-resolved transient transmission measurements on multi-layer black phosphorus. Background free two-color pump-probe spectroscopy measurements are carried out on mechanically exfoliated black phosphorus flakes that have been transferred to a large-bandgap, silicon carbide substrate. The blue-shifted pump pulse (780 nm) induces an increased transmission of the probe pulse (1560 nm) over a time scale commensurate with the measurement resolution (hundreds of fs). After the initial pump-induced transparency, the sign of the transient flips and a slower enhanced absorption is observed. This extended absorption is characterized by two relaxation time scales of 180 ps and 1.3 ns. The saturation peak is attributed to Pauli blocking while the extended absorption is ascribed to a Drude response of the pump-induced carriers. The anisotropic carrier mobility in the black phosphorus leads to different weights of the Drude absorption, depending on the probe polarization, which is readily observed in the amplitude of the pump-probe signals.

cond-mat.mtrl-sci↗

arXiv2015

Terahertz nonlinear conduction and absorption saturation in silicon waveguides

We employ a silicon dielectric waveguide to confine and concentrate terahertz pulses, and observe that the absorption saturates under strong terahertz fields. By comparing the response between lightly-doped and intrinsic silicon waveguides, we confirm the role of hot carriers in this saturable absorption. We introduce a nonlinear dynamical model of Drude conductivity that, when incorporated into a wave propagation equation, accurately reproduces the observations and elucidates the physical mechanisms underlying this nonlinear effect. The results are numerically confirmed by Monte Carlo simulations of the Boltzmann transport equation, coupled with split-step nonlinear wave propagation.

cond-mat.mtrl-sci↗

arXiv2014

Sensitive Room-Temperature Terahertz Detection via Photothermoelectric Effect in Graphene

Terahertz (THz) radiation has uses from security to medicine; however, sensitive room-temperature detection of THz is notoriously difficult. The hot-electron photothermoelectric effect in graphene is a promising detection mechanism: photoexcited carriers rapidly thermalize due to strong electron-electron interactions, but lose energy to the lattice more slowly. The electron temperature gradient drives electron diffusion, and asymmetry due to local gating or dissimilar contact metals produces a net current via the thermoelectric effect. Here we demonstrate a graphene thermoelectric THz photodetector with sensitivity exceeding 10 V/W (700 V/W) at room temperature and noise equivalent power less than 1100 pW/Hz^1/2 (20 pW/Hz^1/2), referenced to the incident (absorbed) power. This implies a performance which is competitive with the best room-temperature THz detectors for an optimally coupled device, while time-resolved measurements indicate that our graphene detector is eight to nine orders of magnitude faster than those. A simple model of the response, including contact asymmetries (resistance, work function and Fermi-energy pinning) reproduces the qualitative features of the data, and indicates that orders-of-magnitude sensitivity improvements are possible.

cond-mat.mes-hall↗

arXiv2013

Symmetries, Cluster Synchronization, and Isolated Desynchronization in Complex Networks

Synchronization is of central importance in power distribution, telecommunication, neuronal, and biological networks. Many networks are observed to produce patterns of synchronized clusters, but it has been difficult to predict these clusters or understand the conditions under which they form, except for in the simplest of networks. In this article, we shed light on the intimate connection between network symmetry and cluster synchronization. We introduce general techniques that use network symmetries to reveal the patterns of synchronized clusters and determine the conditions under which they persist. The connection between symmetry and cluster synchronization is experimentally explored using an electro-optic network. We experimentally observe and theoretically predict a surprising phenomenon in which some clusters lose synchrony while leaving others synchronized. The results could guide the design of new power grid systems or lead to new understanding of the dynamical behavior of networks ranging from neural to social.

nlin.CD↗

arXiv2013

Experimental Observations of Group Synchrony in a System of Chaotic Optoelectronic Oscillators

We experimentally demonstrate group synchrony in a network of four nonlinear optoelectronic oscillators with time-delayed coupling. We divide the nodes into two groups of two each, by giving each group different parameters and by enabling only inter-group coupling. When coupled in this fashion, the two groups display different dynamics, with no isochronal synchrony between them, but the nodes in a single group are isochronally synchronized, even though there is no intra-group coupling. We compare experimental behavior with theoretical and numerical results.

nlin.CD↗

arXiv2011

Robustness of Optimal Synchronization in Real Networks

Experimental studies of synchronization properties on networks with controlled connection topology can provide powerful insights into the physics of complex networks. Here, we report experimental results on the influence of connection topology on synchronization in fiber-optic networks of chaotic optoelectronic oscillators. We find that the recently predicted non-monotonic, cusp-like synchronization landscape manifests itself in the rate of convergence to the synchronous state. We also observe that networks with the same number of nodes, same number of links, and identical eigenvalues of the coupling matrix can exhibit fundamentally different approaches to synchronization. This previously unnoticed difference is determined by the degeneracy of associated eigenvectors in the presence of noise and mismatches encountered in real-world conditions.

nlin.CD↗

arXiv2010

Dynamic synchronization of a time-evolving optical network of chaotic oscillators

We present and experimentally demonstrate a technique for achieving and maintaining a global state of identical synchrony of an arbitrary network of chaotic oscillators even when the coupling strengths are unknown and time-varying. At each node an adaptive synchronization algorithm dynamically estimates the current strength of the net coupling signal to that node. We experimentally demonstrate this scheme in a network of three bidirectionally coupled chaotic optoelectronic feedback loops and we present numerical simulations showing its application in larger networks. The stability of the synchronous state for arbitrary coupling topologies is analyzed via a master stability function approach.

nlin.CD↗

arXiv2009

Adaptive synchronization of coupled chaotic oscillators

We experimentally demonstrate and numerically simulate a new adaptive method to maintain synchronization between coupled nonlinear chaotic oscillators, when the coupling between the systems is unknown and time-varying (e.g., due to environmental parameter drift). The technique is applied to optoelectronic feedback loops exhibiting high dimensional chaotic dynamics. In addition to keeping the two systems isochronally synchronized in the presence of a priori unknown time-varying coupling strength, the technique provides an estimate of the time-varying coupling.

nlin.CD↗

arXiv2009

Complex Dynamics and Synchronization of Delayed-Feedback Nonlinear Oscillators

We describe a flexible and modular delayed-feedback nonlinear oscillator that is capable of generating a wide range of dynamical behaviours, from periodic oscillations to high-dimensional chaos. The oscillator uses electrooptic modulation and fibre-optic transmission, with feedback and filtering implemented through real-time digital-signal processing. We consider two such oscillators that are coupled to one another, and we identify the conditions under which they will synchronize. By examining the rates of divergence or convergence between two coupled oscillators, we quantify the maximum Lyapunov exponents or transverse Lyapunov exponents of the system, and we present an experimental method to determine these rates that does not require a mathematical model of the system. Finally, we demonstrate a new adaptive control method that keeps two oscillators synchronized even when the coupling between them is changing unpredictably.

nlin.CD↗

arXiv2008

Using Synchronization for Prediction of High-Dimensional Chaotic Dynamics

We experimentally observe the nonlinear dynamics of an optoelectronic time-delayed feedback loop designed for chaotic communication using commercial fiber optic links, and we simulate the system using delay differential equations. We show that synchronization of a numerical model to experimental measurements provides a new way to assimilate data and forecast the future of this time-delayed high-dimensional system. For this system, which has a feedback time delay of 22 ns, we show that one can predict the time series for up to several delay periods, when the dynamics is about 15 dimensional.

nlin.CD↗