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Thomas L. Howarth

Publications and source records attributed to Thomas L. Howarth.

6 recordsLinked to original sources

Unified scaling and shape laws for turbulent premixed methane and hydrogen jet flames

The scaling of turbulent premixed flames is typically described by correlations derived for unity-Lewis-number fuels. However, their validity for hydrogen (H$_{2}$) remains uncertain due to the thermodiffusive effects associated with its low Lewis number. In this study, turbulent premixed H$_{2}$ and methane (CH$_{4}$) jet flames are systematically compared over a wide range of operating conditions. Experiments were conducted for Reynolds numbers between 5000 and 60000 and effective Karlovitz numbers spanning 3-368. Flame structure and global flame geometry were characterized using spatially resolved OH$^{*}$ chemiluminescence imaging, allowing consistent comparison between the two fuels across different turbulence intensities. The results are interpreted via a unified framework that incorporates two thermodynamic- and fuel-dependent parameters: a flame speed factor, $\alpha$, representing the enhancement of local burning rates, and a shape factor, $\gamma$, describing the scaling of mean flame geometry. Despite significant fuel-specific thermodiffusive effects associated with preferential diffusion and intrinsic reactivity, which lead H$_{2}$ flames to exhibit enhanced sensitivity to turbulence and more compact flame configurations, both H$_{2}$ and CH$_{4}$ flames are found to exhibit robust and consistent turbulent scaling behavior when analysed within the proposed unified framework. The resulting correlations provide a generalised description of turbulent burning velocity and flame structure, demonstrating that key turbulence-chemistry interactions can be captured within a common model across fuels with widely different Lewis numbers. Overall, the dataset spans multiple turbulence regimes and flame geometries for both fuels, providing a valuable experimental benchmark for the validation of turbulent combustion models across different regimes.

physics.flu-dyn

Fourier extensions for matrix-function block encodings with error-independent subnormalization bounds

Block encodings of non-unitary matrix functions are central to quantum numerical linear algebra. Hamiltonian simulation is a natural input model for Hermitian matrices, but accurate block encodings often incur large subnormalization. We decouple the accuracy from the subnormalization by formulating the matrix-function block encoding as a Fourier-extension approximation problem, yielding a linear combination of unitaries for Hermitian matrix inputs. Fourier extensions approximate non-periodic functions by a Fourier series on a larger periodic domain, creating redundant coefficients that can be optimized for their absolute sum, and hence subnormalization. The coefficients may be chosen for optimal subnormalization with algebraic convergence, by tuning the subnormalization bound for increasing rates of exponential convergence, or by Sobolev-regularized fitting to accommodate more general spectral sets. Fourier-extension block encodings apply to eigenvalue transforms of Hermitian matrices, or to odd singular-value transforms of general matrices, including as a quantum linear systems algorithm.

quant-ph

Role of enthalpy transport in laminar premixed hydrogen flames at atmospheric and elevated pressures

This work discusses the role of diffusive enthalpy transport in relation to the origin of thermodiffusive instability and the resulting enhanced reactivity. Thermodiffusive effects in premixed hydrogen flames are typically explained and modelled via local equivalence ratio fluctuations. However, it is reiterated here that the imbalance between species and thermal diffusion (differential diffusion), rather than local species-to-species diffusive imbalances (preferential diffusion) is the leading-order effect. Reactant (H$_2$), product (H$_2$O) and intermediate (H) species are demonstrated to all play a role in the transport of enthalpy through an analysis of enthalpy flux divergence terms in unstretched flames. Premixed counterflow flames at various strain rates and pressures are then analysed to demonstrate that enhanced reactivity originates from a combination of enthalpy transport and the broadness of the reaction zone relative to the thickness of the flame. Effects resulting from key pressure fall-off reactions are also discussed to determine the importance of detailed chemistry, and the usage of Zeldovich number. Finally, two-dimensional planar flames are simulated and analysed to demonstrate the role of curvature in addition to strain rate, and the implications of the findings in blends and turbulent flames are discussed.

physics.flu-dyn

Effects of Intrinsic Flame Instabilities on Nitrogen Oxide Formation in Laminar Premixed Ammonia/Hydrogen/Air Flames

This study investigates the characteristics of nitrogen oxide (NO) formation in two-dimensional (2D) laminar premixed ammonia/hydrogen/air flames and the impact of thermodiffusively driven intrinsic flame instabilities (IFIs). To this end, a set of three highly resolved direct numerical simulations (DNS) at lean ambient conditions and varying hydrogen fraction in the fuel blend are conducted. The analysis of these DNS reveals a significant increase of NO formation in positively curved regions of the flame, particularly for lower hydrogen fuel fractions, while negatively curved areas exhibit reduced NO concentrations. However, despite the strong variations of local mass fractions of NO in the flame sheet, the mean mass fraction in the post-flame region remains close to the solution from a one-dimensional flame. Through a representative flame segment analysis of positively curved, negatively curved, and flat regions, key reactions contributing to NO formation are determined, with the HNO pathway being the predominant production and the deNOx pathway being the predominant consumption pathway across all cases. Thermal NO plays no significant role in the considered cases. Generally, the peaks of NO production shift to lower values of progress variable in the negatively curved regions, leading to an annihilation of the production and consumption terms in the low hydrogen fuel fraction case. The decrease of NO production is found to be mainly driven by changes of the radical concentrations, rather than changes of the temperature-dependent reaction rate coefficients.

physics.flu-dyn

Comprehensive linear stability analysis for intrinsic instabilities in premixed ammonia/hydrogen/air flames

Two-dimensional direct numerical simulations of planar laminar premixed ammonia/hydrogen/air flames are conducted for a wide range of equivalence ratios, hydrogen ($\rm H_2$) fractions in the fuel blend, pressures, and unburned temperatures to study intrinsic flame instabilities (IFIs) in the linear regime. For stoichiometric and lean mixtures at ambient conditions, a non-monotonic behavior of thermo-diffusive instabilities with increasing ($\rm H_2$) fraction is observed. Strongest instabilities occur for molar ($\rm H_2$) fractions of 40%. The analysis shows that this behavior is linked to the joint effect of variations of the effective Lewis number and Zeldovich number. IFIs in ammonia/hydrogen blends further show a non-monotonic trend with respect to pressure, which is found to be linked to the chemistry of the hydroperoxyl radical $\rm HO_2$. The addition of $\rm NH_3$ opens new reaction pathways for the consumption of $\rm HO_2$ resulting in a chain carrying behavior in contrast to its chain terminating nature in pure $\rm H_2$/air flames. Theoretically derived dispersion relations can predict the non-monotonic behavior for lean conditions. However, these are found to be sensitive to the different methods for evaluating the Zeldovich number available in the literature.

physics.flu-dyn

Direct numerical simulation of a high-pressure hydrogen micromix combustor: flame structure and stabilisation mechanism

A high-pressure hydrogen micromix combustor has been investigated using direct numerical simulation with detailed chemistry to examine the flame structure and stabilisation mechanism. The configuration of the combustor was based on the design by Schefer [1], using numerical periodicity to mimic a large square array. A precursor simulation of an opposed jet-in-crossflow was first conducted to generate appropriate partially-premixed inflow boundary conditions for the subsequent reacting simulation. The resulting flame can be described as a predominantly-lean inhomogeneously-premixed lifted jet flame. Five main zones were identified: a jet mixing region, a core flame, a peripheral flame, a recirculation zone, and combustion products. The core flame, situated over the jet mixing region, was found to burn as a thin reaction front, responsible for over 85% of the total fuel consumption. The peripheral flame shrouded the core flame, had low mean flow with high turbulence, and burned at very lean conditions (in the distributed burning regime). It was shown that turbulent premixed flame propagation was an order-of-magnitude too slow to stabilise the flame at these conditions. Stabilisation was identified to be due to ignition events resulting from turbulent mixing of fuel from the jet into mean recirculation of very lean hot products. Ignition events were found to correlate with shear-driven Kelvin-Helmholtz vortices, and increased in likelihood with streamwise distance. At the flame base, isolated events were observed, which developed into rapidly burning flame kernels that were blown downstream. Further downstream, near-simultaneous spatially-distributed ignition events were observed, which appeared more like ignition sheets. The paper concludes with a broader discussion that considers generalising from the conditions considered here.

physics.flu-dyn