arXiv subjects

Thomas Pertsch

Publications and source records attributed to Thomas Pertsch.

At least 55 records · Page 3Linked to original sources

arXiv2022

Nonlinear quantum spectroscopy with Parity-Time symmetric integrated circuits

We propose a novel quantum nonlinear interferometer design that incorporates a passive PT symmetric coupler sandwiched between two nonlinear sections where signal-idler photon pairs are generated. The PT-symmetry enables efficient coupling of the longer-wavelength idler photons and facilitates the sensing of losses in the second waveguide exposed to analyte under investigation, whose absorption can be inferred by measuring only the signal intensity at a shorter wavelength where efficient detectors are readily available. Remarkably, we identify a new phenomenon of sharp signal intensity fringe shift at critical idler loss values, which is distinct from the previously studied PT-symmetry breaking. We discuss how such unconventional properties arising from quantum interference can provide a route to enhancing the sensing of analytes and facilitate broadband spectroscopy applications in integrated photonic platforms.

physics.optics↗

arXiv2022

Group index matched frequency conversion in lithium niobate on insulator waveguides

Sources of spectrally engineered photonic states are a key resource in several quantum technologies. Of particular importance are the so-called factorizable biphoton states which possess no spectral entanglement and hence, are ideal for heralded generation of high-purity single photons. An essential prerequisite for generating these states through nonlinear frequency conversion is the control over the group indices of the photonic modes of the source. Here, we show that thin-film lithium niobate on insulator (LNOI) is an excellent platform for this purpose. We design and fabricate periodically poled ridge waveguides in LNOI to demonstrate group index engineering of its guided photonic modes and harness this control to experimentally realize on-chip group index matched type-II sum-frequency generation (SFG) and photon-pair creation through spontaneous parametric down-conversion (SPDC). Also, we numerically study the role of the top cladding layer in tuning the dispersion properties of the ridge waveguide structures and reveal a distinctive difference between the air and silica-clad designs which are currently among the two most common device cladding configurations in LNOI. We expect that these results will be relevant for various classical and quantum applications where dispersion control is crucial in tailoring the nonlinear response of the LNOI-based devices.

physics.optics↗

arXiv2022

Equivalence of reflection paths of light and Feynman paths in stacked metasurfaces

We show the existence of virtual polarization states during the interaction of modes in metasurface stacks. In support of our findings we experimentally realize a metasurface stack, consisting of an isotropic layer of nano-patches and an anisotropic layer of nano-wires. Utilizing an analogy to the interaction of electrons at junctions in mesoscopic electron transport via Feynman paths, we present a semi-analytical description of the modal interaction inside this stack. We then derive a series of all possible reflection paths light can take inside the metasurface stack.

physics.optics↗

arXiv2021

Material-specific high-resolution table-top extreme ultraviolet microscopy

Microscopy with extreme ultraviolet (EUV) radiation holds promise for high-resolution imaging with excellent material contrast, due to the short wavelength and numerous element-specific absorption edges available in this spectral range. At the same time, EUV radiation has significantly larger penetration depths than electrons. It thus enables a nano-scale view into complex three-dimensional structures that are important for material science, semiconductor metrology, and next-generation nano-devices. Here, we present high-resolution and material-specific microscopy at 13.5 nm wavelength. We combine a highly stable, high photon-flux, table-top EUV source with an interferometrically stabilized ptychography setup. By utilizing structured EUV illumination, we overcome the limitations of conventional EUV focusing optics and demonstrate high-resolution microscopy at a half-pitch lateral resolution of 16 nm. Moreover, we propose mixed-state orthogonal probe relaxation ptychography, enabling robust phase-contrast imaging over wide fields of view and long acquisition times. In this way, the complex transmission of an integrated circuit is precisely reconstructed, allowing for the classification of the material composition of mesoscopic semiconductor systems.

physics.optics↗

arXiv2021

Mid-Infrared Photon-Pair Generation in AgGaS$_2$

We demonstrate non-degenerate photon-pair generation by spontaneous parametric down conversion in a silver gallium sulfide AgGaS$_2$ crystal. By tuning the pump wavelength, we achieve phase matching over a large spectral range. This allows to generate idler photons in the mid-infrared spectral range above 6 $μm$ wavelength with corresponding signal photons in the visible. Also, we show photon pair generation with broad spectral bandwidth. These results are a valuable step towards the development of quantum imaging and sensing techniques in the mid-infrared.

physics.optics↗

arXiv2021

In-fiber second-harmonic generation with embedded two-dimensional materials

Silica-based optical fibers are a workhorse of nonlinear optics. They have been used to demonstrate nonlinear phenomena such as solitons and self-phase modulation. Since the introduction of the photonic crystal fiber, they have found many exciting applications, such as supercontinuum white light sources and third-harmonic generation, among others. They stand out by their low loss, large interaction length, and the ability to engineer its dispersive properties, which compensate for the small chi(3) nonlinear coefficient. However, they have one fundamental limitation: due to the amorphous nature of silica, they do not exhibit second-order nonlinearity, except for minor contributions from surfaces. Here, we demonstrate significant second-harmonic generation in functionalized optical fibers with a monolayer of highly nonlinear MoS2 deposited on the fiber guiding core. The demonstration is carried out in a 3.5 mm short piece of exposed core fiber, which was functionalized in a scalable process CVD-based process, without a manual transfer step. This approach is scalable and can be generalized to other transition metal dichalcogenides and other waveguide systems. We achieve an enhancement of more than 1000x over a reference sample of equal length. Our simple proof-of-principle demonstration does not rely on either phase matching to fundamental modes, or ordered growth of monolayer crystals, suggesting that pathways for further improvement are within reach. Our results do not just demonstrate a new path towards efficient in-fiber SHG-sources, instead, they establish a platform with a new route to chi(2)-based nonlinear fiber optics, optoelectronics, and photonics platforms, integrated optical architectures, and active fiber networks.

physics.optics↗

arXiv2021

Metasurface-Assisted Quantum Ghost Discrimination of Polarization Objects

We develop a concept of metasurface-assisted ghost imaging for non-local discrimination between a set of polarization objects. The specially designed metasurfaces are incorporated in the imaging system to perform parallel state transformations in general elliptical bases of quantum-entangled or classically-correlated photons. Then, only four or fewer correlation measurements between multiple metasurface outputs and a simple polarization-insensitive bucket detector after the object can allow for the identification of fully or partially transparent polarization elements and their arbitrary orientation angles. We rigorously establish that entangled photon states offer a fundamental advantage compared to classical correlations for a broad class of objects. The approach can find applications for real-time and low-light imaging across diverse spectral regions in dynamic environments.

quant-ph↗

arXiv2021

Spontaneous Parametric Down-Conversion from Resonant Metasurfaces

All-dielectric optical metasurfaces are a workhorse in nano-optics due to both their ability to manipulate light in different degrees of freedom and their excellent performance at light frequency conversion. Here, we demonstrate first-time generation of photon pairs via spontaneous parametric-down conversion in lithium niobate quantum optical metasurfaces with electric and magnetic Mie-like resonances at various wavelengths. By engineering the quantum optical metasurface, we tailor the photon-pair spectrum in a controlled way. Within a narrow bandwidth around the resonance, the rate of pair production is enhanced up to two orders of magnitude compared to an unpatterned film of the same thickness and material. These results enable flat-optics sources of entangled photons -- a new promising platform for quantum optics experiments.

physics.optics↗

arXiv2020

Broadband holography-assisted coherent imaging -- towards attosecond imaging at the nanoscale

In recent years nanoscale coherent imaging has emerged as an indispensable imaging modality allowing to surpass the resolution limit given by classical imaging optics. At the same time, attosecond science has experienced enormous progress and has revealed the ultrafast dynamics in atoms, molecules, and complex materials. Combining attosecond temporal resolution of pump-probe experiments with nanometer spatial resolution would allow studying ultrafast dynamics on the smallest spatio-temporal scales but has not been demonstrated yet. Unfortunately, the large bandwidth of attosecond pulses usually hinders high-resolution coherent imaging. Here we present a robust holography-enhanced coherent imaging method, which allows combining high quality and high spatial resolution coherent imaging with a large spectral bandwidth. By implementing our method at a high harmonic source we demonstrate, for the first time, a spatial resolution of 34 nm (2.5 λ) in combination with a spectral bandwidth supporting a Fourier limited pulse duration of only 380 as. The method is single-shot capable, additionally retrieves the spectrum from the measured diffraction pattern, and is thus immune against shot-to-shot fluctuations. This paves the way for an ultrafast view on nanoscale dynamics e.g. ultrafast charge transfer or ultrafast spin currents being relevant for Petahertz electronics and future data storage.

physics.optics↗

arXiv2020

Scalable functionalization of optical fibers using atomically thin semiconductors

Atomically thin transition metal dichalcogenides are highly promising for integrated optoelectronic and photonic systems due to their exciton-driven linear and nonlinear interaction with light. Integrating them into optical fibers yields novel opportunities in optical communication, remote sensing, and all-fiber optoelectronics. However, scalable and reproducible deposition of high quality monolayers on optical fibers is a challenge. Here, we report the chemical vapor deposition of monolayer MoS2 and WS2 crystals on the core of microstructured exposed core optical fibers and their interaction with the fibers' guided modes. We demonstrate two distinct application possibilities of 2D-functionalized waveguides to exemplify their potential. First, we simultaneously excite and collect excitonic 2D material photoluminescence with the fiber modes, opening a novel route to remote sensing. Then we show that third harmonic generation is modified by the highly localized nonlinear polarization of the monolayers, yielding a new avenue to tailor nonlinear optical processes in fibers. We anticipate that our results may lead to significant advances in optical fiber based technologies.

physics.app-ph↗

arXiv2020

A fully automated dual-tip scanning near-field optical microscope for localized optical excitation and detection in the visible and near-infrared

Near-field optical microscopes with two independent tips for simultaneous excitation and detection can be essential tools for studying localized optical phenomena on the subwavelength scale. Here, we report on the implementation of a fully automated and robust dual-tip scanning near-field optical microscope (SNOM), in which the excitation tip is stationary, while the detection tip automatically scans the surrounding area. To monitor and control the distance between the two probes, mechanical interactions due to shear forces are used. We experimentally investigate suitable scan parameters and find that the automated dual-tip SNOM can operate stably for a wide range of parameters. To demonstrate the potential of the automated dual-tip SNOM, we characterize the propagation of surface plasmon polaritons on a gold film for visible and near-infrared wavelengths. The good agreement of the measurements with numerical simulations verifies the capability of the dual-tip SNOM for the near-field characterization of localized optical phenomena.

physics.ins-det↗

arXiv2020

Spectral mapping of polarization-correlated photon-pair sources using quantum-classical correspondence

Direct spectral characterization of a quantum photon-pair source usually involves cumbersome, costly, and time-consuming detection issues. In this study, we experimentally characterize the spectral properties of a type-II phase-matched spontaneous parametric down-conversion (SPDC) source based on a titanium-diffused periodically poled lithium niobate (Ti:PPLN) waveguide. The characterization of the spectral information of the generated cross-polarized photon pairs is of importance for the use of such sources in applications including quantum information and communication. We demonstrate that the joint spectral intensity of the cross-polarized photon-pair source can be fully reconstructed using the quantum-classical correspondence through classical sum-frequency generation (SFG) measurements. This technique, which uses a much less complex detection system for visible light, opens the possibility of fast monitoring and control of the quantum state of (polarization-correlated) photon-pair sources to facilitate the realization of a stable and high-usability quantum source.

quant-ph↗

arXiv2020

Discrete dispersion scan setup for measuring few-cycle laser pulses in the mid-infrared

In this work, we demonstrate a discrete dispersion scan scheme using a low number of flat windows to vary the dispersion of laser pulses in discrete steps. Monte Carlo simulations indicate that the pulse duration can be retrieved accurately with less than 10 dispersion steps, which we verify experimentally by measuring few-cycle pulses and material dispersion curves at 3 and 10 micrometer wavelength. This minimal measuring scheme using only five optical components without the need for high-precision positioners and interferometric alignment can be readily implemented in many wavelength ranges and situations.

physics.optics↗

arXiv2020

Color filter arrays based on dielectric metasurface elements

Digital imaging has been steadily improving over the past decades and we are moving towards a wide use of multi- and hyperspectral cameras. A key component of such imaging systems are color filter arrays, which define the spectrum of light detected by each camera pixel. Hence, it is essential to develop a variable, robust and scalable way for controlling the transmission of light. Nanostructured surfaces, also known as metasurfaces, offer a promising solution as their transmission spectra can be controlled by shaping the wavelength-dependent scattering properties of their constituting elements. Here we present, metasurfaces based on silicon nanodisks, which provide filter functions with amplitudes reaching 70-90% of transmission, and well suitable for RGB and CMY color filter arrays, the initial stage towards the further development of hyperspectral filters. We suggest and discuss possible ways to expand the color gamut and improve the color values of such optical filters.

physics.optics↗

arXiv2020

Direct and High-Throughput Fabrication of Mie-Resonant Metasurfaces via Single-Pulse Laser Interference

High-index dielectric metasurfaces featuring Mie-type electric and magnetic resonances have been of a great interest in a variety of applications such as imaging, sensing, photovoltaics and others, which led to the necessity of an efficient large-scale fabrication technique. To address this, here we demonstrate the use of single-pulse laser interference for direct patterning of an amorphous silicon film into an array of Mie resonators. The proposed technique is based on laser-interference-induced dewetting. A precise control of the laser pulse energy enables the fabrication of ordered dielectric metasurfaces in areas spanning tens of micrometers and consisting of thousands of hemispherical nanoparticles with a single laser shot. The fabricated nanoparticles exhibit a wavelength-dependent optical response with a strong electric dipole signature. Variation of the pre-deposited silicon film thickness allows tailoring of the resonances in the targeted visible and infrared spectral ranges. Such direct and high-throughput fabrication paves the way towards a simple realization of spatially invariant metasurface-based devices.

physics.optics↗

arXiv2019

Laser-Induced Spatially-Selective Tailoring of High-Index Dielectric Metasurfaces

Optically resonant high-index dielectric metasurfaces featuring Mie-type electric and magnetic resonances are usually fabricated by means of planar technologies, which limit the degrees of freedom in tunability and scalability of the fabricated systems. Therefore, we propose a complimentary post-processing technique based on ultrashort ($\leq$ 10 ps) laser pulses. The process involves thermal effects: crystallization and reshaping, while the heat is localized by a high-precision positioning of the focused laser beam. Moreover, for the first time, the resonant behavior of dielectric metasurface elements is exploited to engineer a specific absorption profile, which leads to a spatially-selective heating and a customized modification. Such technique has a potential to reduce the complexity in the fabrication of non-uniform metasurface-based optical elements. Two distinct cases, a spatial pixelation of a large-scale metasurface and a height modification of metasurface elements, are explicitly demonstrated.

physics.optics↗

arXiv2018

Sub-micrometer Nanostructure-based RGB Filters for CMOS Image Sensors

Digital color imaging relies on spectral filters on top of a pixelated sensor, such as a CMOS image sensor. An important parameter of imaging devices is their resolution, which depends on the size of the pixels. For many applications, a high resolution is desirable, consequently requiring small spectral filters. Dielectric nanostructures, due to their resonant behavior and its tunability, offer the possibility to be assembled into flexible and miniature spectral filters, which could potentially replace conventional pigmented and dye-based color filters. In this paper, we demonstrate the generation of transmissive structural colors based on uniform-height amorphous silicon nanostructures. We optimize the structures for the primary RGB colors and report the construction of sub-micrometer RGB filter arrays for a pixel size down to 0.5 μm.

physics.optics↗

arXiv2018

All-dielectric resonant meta-optics goes active

All-dielectric resonant nanophotonics is a rapidly developing research field driven by its exceptional application potential for low-loss nanoscale metadevices. The tight confinement of the local electromagnetic fields and interferences in resonant photonic nanostructures can boost many optical effects, thus offering novel opportunities for the subwavelength control of light-matter-interactions. Active, light-emitting nanoscale structures are of particular interest, as they offer unique opportunities for novel types of light sources and nanolasers. Here, we review the latest advances in this recently emerged and rapidly growing field of active dielectric resonant nanophotonics enabled by dipolar and multipolar Mie-type resonances. More specifically, we discuss how to employ dielectric nanostructures for the resonant control of emission from quantum dots, two-dimensional transition metal dichalcogenides, and halide perovskites. We also foresee various future research directions and applications of active all-dielectric resonant nanostructures including but not limited to lasing in topologically robust systems, light-matter interactions beyond the electric dipole limit, light-emitting surfaces, and tunable active metadevices.

physics.optics↗