arXiv subjects

Thomas Südmeyer

Publications and source records attributed to Thomas Südmeyer.

11 recordsLinked to original sources

arXiv2026

Free-Running Ring Quantum Cascade Laser with 50 kHz Linewidth

We report on the noise characterization of a free-running ring quantum cascade laser resonator emitting a single frequency mode around 7.7 $μ$m. Using a gas cell filled with N$_2$O as a frequency-to-voltage discriminator, we measured the frequency noise power spectral density of the laser from which we extracted its linewidth. The results show a full width at half maximum close to 50 kHz at 1 s integration time, which represents at least a sixfold improvement compared to state-of-the-art quantum cascade lasers operating in a spectral region above 7 $μ$m. We also demonstrate that such lasers can be efficiently used for frequency modulation spectroscopy, which opens up new possibilities for high resolution metrology and spectroscopic applications in the mid-infrared.

physics.optics↗

arXiv2025

Ion-Beam-Sputtered Mid-Infrared Coatings for Hybrid Supermirrors

We report on the development of low-loss ion-beam-sputtered (IBS) mid-infrared coatings for hybrid supermirrors. Two highly reflective designs were realized: HR1, a 4-period a-Si/SiO$_2$ DBR with an Al$_2$O$_3$ bonding layer, and HR2, a 6-period a-Si/Ta$_2$O$_5$ DBR with an a-Si terminating layer for bonding. Combined with a GaAs/AlGaAs crystalline mirror, HR2-based hybrids yielded a total loss of 9.3 ppm and excess loss of 6.8 ppm at 4.45 $μ$m, with cavity finesse up to 396000. For the first time, we used IBS-deposited a-Si directly as a bonding layer, verified its sub-angstrom roughness, and demonstrated excellent performance. This establishes a clear path toward scalable coatings for longer mid-infrared wavelengths, building on prior results in Nat. Commun. 14, 7846 (2023).

physics.optics↗

arXiv2025

Non-resonant Optical Injection Locking in Quantum Cascade Laser Frequency Combs

Optical injection locking of the repetition frequency of a quantum cascade laser frequency comb is demonstrated using an intensity modulated near-infrared light at 1.55 $μ$m illuminating the front facet of the laser. Compared to the traditional electrical modulation approach, the introduced technique presents benefits from several perspectives such as the availability of mature and high bandwidth equipment in the near-infrared, circumvent the need of dedicated electronic components for the quantum cascade laser, and allows a direct link between the near and mid-infrared for amplitude to frequency modulation. We show that this stabilization scheme, used with moderate near-infrared power of a few milliwatts, allows for a strong reduction of the frequency noise. We also perform a full characterization of the mechanism and evidence that the locking range follows Adler's law. A comparison of our results with those in recent literature indicates that the optical approach leads to better performance compared to the traditional method, which we expect to benefit mid-infrared spectroscopy and metrological applications.

physics.optics↗

arXiv2024

Low Phase Noise, Record-High Power Optical Parametric Oscillator Tunable from 2.7-4.7 μm for Metrology Applications

Within the domain of optical frequency comb systems operating in the mid-infrared, extensive exploration has been undertaken regarding critical parameters such as stabilization, coherence, or spectral tunability. Despite this, certain essential parameters remain inadequately addressed, particularly concerning the light source prerequisites for advanced spectroscopy techniques operating in the 3-5 $μ$m spectral region. Specifically, the necessity for high simultaneous stability of average power, spectral shape, and temporal properties, alongside requirements for excellent beam quality and high powers of several Watts, emerges for applications like cavity-enhanced Doppler-free saturation spectroscopy. Existing systems fall short of meeting these rigorous criteria. This study delves into the metrology aspects of an optical parametric oscillator system, with a particular emphasis on its suitability for powerhungry metrology applications. Notably, the highest average power reported in the 3-5 $μ$m region, reaching 10.3W for the idler output at 3.1 $μ$m, is achieved. Additionally, new aspects, like the analysis of idler phase noise and beam quality and the onset of higher order modes are discussed. These findings represent a significant advancement towards the realization of highly-stable, metrologygrade frequency combs in the mid-infrared, thereby facilitating precision spectroscopy techniques previously constrained by light source average powers and quality limitations.

physics.optics↗

arXiv2023

Coherence analysis of tightly locked mid-infrared quantum cascade laser frequency combs

Frequency combs are powerful tools for many applications and high performances are achieved by stabilizing these lasers. For operation in the mid-infrared, quantum cascade lasers (QCL) are ideal candidates as they present numerous advantages. However, stabilized QCL-combs lack of a detailed characterization of their noise properties due to the sensitivity limits of current analyzing techniques. To overcome these challenges, we developed what we believe to be the first tightly locked dual QCL-comb system. Its use is twofold. First, phase noise analysis of the dual-comb signal shows residual phase noise below 600 mrad for all comb lines, and we characterize the comb coherence as well as the performances of the repetition frequency locking mechanism. Second, we demonstrate coherent averaging with a $7 \times 10^5$ Hz$^{1/2}$ figure-of-merit system, which is compatible with high precision spectroscopy.

physics.optics↗

arXiv2023

Coherent Control of Mid-Infrared Frequency Comb by Optical Injection of Near-Infrared Light

We demonstrate the use of a low power near-infrared laser illuminating the front facet of a quantum cascade laser (QCL) as an optical actuator for the coherent control of a mid-infrared frequency comb. We show that by appropriate current control of the QCL comb and intensity modulation of the near-infrared laser, a tight phase lock of a comb line to a distributed feedback laser is possible with 2 MHz of locking bandwidth and 200 mrad of residual phase noise. A characterization of the whole scheme is provided showing the limits of the electrical actuation which we bypassed using the optical actuation. Both comb degrees of freedom can be locked by performing electrical injection locking of the repetition rate in parallel. However, we show that the QCL acts as a fast near-infrared light detector such that injection locking can also be achieved through modulation of the near-infrared light. These results on the coherent control of a quantum cascade laser frequency comb are particularly interesting for coherent averaging in dual-comb spectroscopy and for mid-infrared frequency comb applications requiring high spectral purity.

physics.optics↗

arXiv2022

High-Resolution Quantum Cascade Laser Dual-Comb Spectroscopy in the Mid-Infrared with Absolute Frequency Referencing

Quantum cascade laser (QCL) frequency combs have revolutionized mid-infrared (MIR) spectroscopy by their high brightness and fast temporal resolution, and are a promising technology for fully-integrated and cost-effective sensors. As for other integrated comb sources such as micro-combs and interband cascade laser, QCLs have a comb spacing of several GHz, which is adequate for measurements of wide absorbing structures, typically found in liquid or solid samples. However, high-resolution gas-phase spectra require spectral interleaving and frequency calibration. We developed a frequency calibration scheme for fast interleaved measurements with combs featuring multi-GHz spacing. We then demonstrate dual-comb spectroscopy with 600 kHz accuracy in single-shot 54-ms measurements over 40 cm$^{-1}$ using two QCLs at 7.8 $\mathrmμ$m. This work is an important contribution towards fast fingerprinting of complex molecular mixtures in the MIR. Moreover, the calibration scheme could be used with micro-combs for spectroscopy and ranging, both in comb-swept and comb-calibrated setups.

physics.optics↗

arXiv2022

Synchronization of frequency combs by optical injection

Optical frequency combs based on semiconductor lasers are a promising technology for monolithic integration of dual-comb spectrometers. However, the stabilization of the offset frequency fceo remains a challenging feat due the lack of octave-spanning spectra. In a dual-comb configuration, the uncorrelated jitter of the offset frequencies leads to a non-periodic signal resulting in broadened beatnotes with a limited signal-to-noise ratio (SNR). Hence, expensive data acquisition schemes and complex signal processing are currently required. Here, we show that the offset frequencies of two frequency combs can be synchronized by optical injection locking, which allows full phase-stabilization when combined with electrical injection. A single comb line isolated via an optical Vernier filter serves as Master oscillator for injection locking. The resulting dual-comb signal is periodic and stable over thousands of periods. This enables coherent averaging using analog electronics, which increases the SNR and reduces the data size by one and three orders of magnitude, respectively. The presented method will enable fully phase-stabilized dual-comb spectrometers by leveraging on integrated optical filters and provides access for measuring and stabilizing fceo.

physics.optics↗

arXiv2021

Centimeter-scale propagation of optical surface waves at visible wavelengths

Guiding and confining light at interfaces is crucial for applications involving light-matter interactions such as surface spectroscopy, nonlinear optics, and quantum information technology. While dielectric surface waves offer promising perspectives for strong light confinement at non-absorbing interfaces, their capacity has not yet been widely explored. Here, we focus on the propagation properties of optical modes supported at the free surface of a one-dimensional photonic crystal. The contributions of intrinsic and extrinsic loss mechanisms are investigated. Structures optimized to support long propagating optical surface waves are designed and fabricated. We experimentally demonstrate, for the first time, the existence of optical surface waves capable of propagating over centimeter-scale distances in the visible spectral range. Our results open new perspectives for the use of optical surface waves in integrated optics and enhanced light-matter interactions.

physics.optics↗

arXiv2021

A Kerr Polarization Controller

Kerr-effect-induced changes of the polarization state of light are well known in pulsed laser systems. An example is nonlinear polarization rotation, which is critical to the operation of many types of mode-locked lasers. Here, we demonstrate that the Kerr effect in a high-finesse Fabry-Pérot resonator can be utilized to control the polarization of a continuous wave laser. It is shown that a linearly-polarized input field is converted into a left- or right-circularly-polarized field, controlled via the optical power. The observations are explained by Kerr-nonlinearity induced symmetry breaking, which splits the resonance frequencies of degenerate modes with opposite polarization handedness in an otherwise symmetric resonator. The all-optical polarization control is demonstrated at threshold powers down to 7 mW. The physical principle of such Kerr effect-based polarization controllers is generic to high-Q Kerr-nonlinear resonators and could also be implemented in photonic integrated circuits. Beyond polarization control, the spontaneous symmetry breaking of polarization states could be used for polarization filters or highly sensitive polarization sensors when operated close to the symmetry-breaking point.

physics.optics↗

arXiv2019

Ultralow-Noise Photonic Microwave Synthesis using a Soliton Microcomb-based Transfer Oscillator

The synthesis of ultralow-noise microwaves is of both scientific and technological relevance for timing, metrology, communications and radio-astronomy. Today, the lowest reported phase noise signals are obtained via optical frequency-division using mode-locked laser frequency combs. Nonetheless, this technique ideally requires high repetition rates and tight comb stabilisation. Here, a soliton microcomb with a 14 GHz repetition rate is generated with an ultra-stable pump laser and used to derive an ultralow-noise microwave reference signal, with an absolute phase noise level below -60 dBc/Hz at 1 Hz offset frequency and -135 dBc/Hz at 10 kHz. This is achieved using a transfer oscillator approach, where the free-running microcomb noise (which is carefully studied and minimised) is cancelled via a combination of electronic division and mixing. Although this proof-of-principle uses an auxiliary comb for detecting the microcomb's offset frequency, we highlight the prospects of this method with future self-referenced integrated microcombs and electro-optic combs, that would allow for ultralow-noise microwave and sub-terahertz signal generators.

physics.app-ph↗