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Thomas Udem

Publications and source records attributed to Thomas Udem.

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Carrier Revival in Long Trapped-Ion Chains

For a single trapped ion, the excitation spectrum of a narrow optical transition consists of a Doppler- and recoil-free carrier accompanied by motional sidebands, which are equally spaced by the trap secular frequency and lie under a Doppler-broadened envelope that is shifted by the photon recoil. Outside the Lamb-Dicke regime, the large photon recoil distributes the line strength across many sidebands and suppresses excitation of the carrier. With multiple ions, the motional spectrum becomes dense, and the carrier is further weakened. Here, we predict a counterintuitive revival effect: increasing the number of ions in a linear chain can restore strong carrier excitation even under trapping conditions far from the single-ion Lamb-Dicke regime. Using a quantum-mechanical model of the excitation dynamics in linear ion chains, we find that sufficiently long chains concentrate the spectrum into the carrier. This effect enables efficient excitation of light ions at short wavelengths. It may also benefit multi-ion optical clocks and mixed-species quantum-logic spectroscopy.

physics.atom-ph

Sub-part-per-trillion test of the Standard Model with atomic hydrogen

Quantum electrodynamics (QED), the first relativistic quantum field theory, describes light-matter interactions at a fundamental level and is one of the pillars of the Standard Model (SM). Through the extraordinary precision of QED, the SM predicts the energy levels of simple systems such as the hydrogen atom with up to 13 significant digits, making hydrogen spectroscopy an ideal test bed. The consistency of physical constants extracted from different transitions in hydrogen using QED, such as the proton charge radius $r_\mathrm{p}$, constitutes a test of the theory. However, values of $r_\mathrm{p}$ from recent measurements of atomic hydrogen are partly discrepant with each other and with a more precise value from spectroscopy of muonic hydrogen. This prevents a test of QED at the level of experimental uncertainties. Here we present a measurement of the 2S-6P transition in atomic hydrogen with sufficient precision to distinguish between the discrepant values of $r_\mathrm{p}$ and enable rigorous testing of QED and the SM overall. Our result $\nu^{}_{\text{2S-6P}}$ = 730,690,248,610.79(48) kHz gives a value of $r_\mathrm{p}$ = 0.8406(15) fm at least 2.5-fold more precise than from other atomic hydrogen determinations and in excellent agreement with the muonic value. The SM prediction of the transition frequency (730,690,248,610.79(23) kHz) is in excellent agreement with our result, testing the SM to 0.7 parts per trillion (ppt) and, specifically, bound-state QED corrections to 0.5 parts per million (ppm), their most precise test so far.

physics.atom-ph

A low repetition rate optical frequency comb

Reducing the pulse repetition rate of an optical frequency comb increases the pulse energy for a given average power. This enhances the efficiency of nonlinear frequency conversion and it facilitates extending the accessible wavelength range, for example into the extreme ultraviolet (XUV). The resulting spectrally dense frequency comb can still be used for precision spectroscopy of narrow atomic or molecular transitions. In this article, we demonstrate a low-noise infrared frequency comb with a repetition rate as low as 40 kHz using a Yb:KYW mode-locked laser, pulse picking, and subsequent amplification. The frequency comb structure is confirmed by generating a beat note with a continuous wave reference laser. A comb mode is actively stabilized to the reference laser, and the integrated rms phase noise from 20 Hz to 20 kHz is measured to be 195 mrad.

physics.optics

Number-Resolved Detection of Dark Ions in Coulomb Crystals

While it is straightforward to count laser-cooled trapped ions by fluorescence imaging, detecting the number of dark ions embedded and sympathetically cooled in a mixed ion crystal is more challenging. We demonstrate a method to track the number of dark ions in real time with single-particle sensitivity. This is achieved by observing discrete steps in the amount of fluorescence emitted from the coolant ions while exciting secular motional resonances of dark ions. By counting the number of fluorescence steps, we can identify the number of dark ions without calibration and without relying on any physical model of the motional excitation. We demonstrate the scheme by detecting H$_2^+$ and H$_3^+$ ions embedded in a Be$^+$ ion Coulomb crystal in a linear radio frequency trap. Our method allows observing the generation and destruction of individual ions simultaneously for different types of ions. Besides high-resolution spectroscopy of dark ions, another application is the detection of chemical reactions in real time with single-particle sensitivity. This is demonstrated in this work.

physics.atom-ph

Motional resonances of three-dimensional dual-species Coulomb crystals

We investigate the motional resonances of dual-species Coulomb crystals comprised of $^9$Be$^+$ and $^{24}$Mg$^+$ ions held in a 4-rod linear Paul trap. Our experimental data and simulations show that the secular motion of such mixed crystals has rich dynamics. Their secular spectra can differ significantly from those of pure ion crystals. We propose a simple model based on mechanical coupling with Coulomb interactions between the two different ion species that explains many features of the secular spectrum. Our findings contribute to a more reliable identification of the ion species in mixed crystals.

physics.atom-ph

Simple phase noise measurement scheme for cavity-stabilized laser systems

We describe a simple method for measuring the residual fast phase noise of a cavity-stabilized laser using the cavity as a reference. The method is based on generating a beat note between the laser output and the strongly filtered light transmitted through the cavity. The beat note can be directly analyzed without requiring further calibration of system parameters. We apply the method to measure the residual phase noise of an external-cavity diode laser (ECDL) locked to a reference cavity and compare the results with an analysis of the in-loop error signal of the feedback system.

physics.optics

A crucial test for astronomical spectrograph calibration with frequency combs

Laser frequency combs (LFCs) are well on their way to becoming the next-generation calibration sources for precision astronomical spectroscopy. This development is considered key in the hunt for low-mass rocky exoplanets around solar-type stars whose discovery with the radial-velocity method requires cm/s Doppler precision. In order to prove such precise calibration with an LFC, it must be compared to another calibrator of at least the same precision. Being the best available spectrograph calibrator, this means comparing it to a second - fully independent - LFC. This test had long been pending, but our installation of two LFCs at the ultra-stable spectrograph HARPS presented the so far unique opportunity for simultaneous calibrations with two separate LFCs. Although limited in time, the test results confirm the 1 cm/s stability that has long been anticipated by the astronomical community.

astro-ph.IM

Deuteron charge radius and Rydberg constant from spectroscopy data in atomic deuterium

We give a pedagogical description of the method to extract the charge radii and Rydberg constant from laser spectroscopy in regular hydrogen (H) and deuterium (D) atoms, that is part of the CODATA least-squares adjustment (LSA) of the fundamental physical constants. We give a deuteron charge radius Rd from D spectroscopy alone of 2.1415(45) fm. This value is independent of the measurements that lead to the proton charge radius, and five times more accurate than the value found in the CODATA Adjustment 10. The improvement is due to the use of a value for the 1S->2S transition in atomic deuterium which can be inferred from published data or found in a PhD thesis.

physics.atom-ph

Real-time dual frequency comb spectroscopy in the near infrared

We use two femtosecond Erbium-doped fiber lasers with slightly different repetition rates to perform a modern type of Fourier transform spectroscopy without moving parts. The measurements are done in real time, and it takes less than 50 microseconds. We work with somewhat different spectral outputs from two Erbium-doped fiber lasers and employ spectral filtering based on a 2f-2f grating setup to select the common spectral region of interest, thereby increasing the signal-to-noise ratio. The interferogram is taken with a 20 cm long gas cell, containing a mixture of acetylene and air at atmospheric pressure, and is fast-Fourier-transformed to obtain the broadband spectral fingerprint of the gas.

physics.optics

Improved Measurement of the Hydrogen 1S - 2S Transition Frequency

We have measured the 1S - 2S transition frequency in atomic hydrogen via two photon spectroscopy on a 5.8 K atomic beam. We obtain $f_{1S-2S} = 2 466 061 413 187 035 (10)$ Hz for the hyperfine centroid. This is a fractional frequency uncertainty of $4.2\times 10^{-15}$ improving the previous measure- ment by our own group [M. Fischer et al., Phys. Rev. Lett. 92, 230802 (2004)] by a factor of 3.3. The probe laser frequency was phase coherently linked to the mobile cesium fountain clock FOM via a frequency comb.

physics.atom-ph

Cavity-enhanced dual-comb spectroscopy

The sensitivity of molecular fingerprinting is dramatically improved when placing the absorbing sample in a high-finesse optical cavity, thanks to the large increase of the effective path-length. As demonstrated recently, when the equidistant lines from a laser frequency comb are simultaneously injected into the cavity over a large spectral range, multiple trace-gases may be identified within a few milliseconds. Analyzing efficiently the light transmitted through the cavity however still remains challenging. Here, a novel approach, cavity-enhanced frequency comb Fourier transform spectroscopy, fully overcomes this difficulty and measures ultrasensitive, broad-bandwidth, high-resolution spectra within a few tens of $μ$s. It could be implemented from the Terahertz to the ultraviolet regions without any need for detector arrays. We recorded, within 18 $μ$s, spectra of the 1.0 $μ$m overtone bands of ammonia spanning 20 nm with 4.5 GHz resolution and a noise-equivalent-absorption at one-second-averaging per spectral element of 3 10^-12 cm^-1Hz^-1/2, thus opening a route to time-resolved spectroscopy of rapidly-evolving single-events.

physics.optics

Laser frequency combs for astronomical observations

A direct measurement of the universe's expansion history could be made by observing in real time the evolution of the cosmological redshift of distant objects. However, this would require measurements of Doppler velocity drifts of about 1 centimeter per second per year, and astronomical spectrographs have not yet been calibrated to this tolerance. We demonstrate the first use of a laser frequency comb for wavelength calibration of an astronomical telescope. Even with a simple analysis, absolute calibration is achieved with an equivalent Doppler precision of approximately 9 meters per second at about 1.5 micrometers - beyond state-of-the-art accuracy. We show that tracking complex, time-varying systematic effects in the spectrograph and detector system is a particular advantage of laser frequency comb calibration. This technique promises an effective means for modeling and removal of such systematic effects to the accuracy required by future experiments to see direct evidence of the universe's putative acceleration.

astro-ph

Cavity Enhanced Optical Vernier Spectroscopy, Broad Band, High Resolution, High Sensitivity

A femtosecond frequency comb provides a vast number of equidistantly spaced narrow band laser modes that can be simultaneously tuned and frequency calibrated with 15 digits accuracy. Our Vernier spectrometer utilizes all of theses modes in a massively parallel manner to rapidly record both absorption and dispersion spectra with a sensitivity that is provided by a high finesse broad band optical resonator and a resolution that is only limited by the frequency comb line width while keeping the required setup simple.

physics.optics