arXiv subjects

Thomas Volz

Publications and source records attributed to Thomas Volz.

At least 19 recordsLinked to original sources

arXiv2026

Industry-ready spin-photon interfaces for hybrid photonic quantum computing

Hybrid photonic quantum computers, combining stationary matter qubits and flying photonic qubits, offer an intrinsically networked and resource-efficient route to large-scale, error-corrected quantum computation. Their core components are cavity-coupled matter qubits that act as light--matter interfaces, enabling: high-efficiency on-demand single-photon generation, stable near-unity photon indistinguishability and spin--multi-photon entanglement. Semiconductor quantum dots in microcavities are a leading platform for realizing such devices. Yet reaching the performance, reproducibility and spin-coherence thresholds for large-scale error correction remains a major challenge requiring industrial fabrication and control. Here we report thousands of monolithic semiconductor quantum-dot devices fabricated using a III--V pilot production-line process compatible with large-scale deployment. Systematic control of source parameters yields state-of-the-art efficiency and supports a path to optical losses below fault-tolerance thresholds. Using field-quadrature state reconstruction as a stringent joint test of efficiency and indistinguishability, we observe near-unity photon quantum purity stable over tens of minutes and a record single-photon Wigner-function negativity. We further demonstrate seven-partite spin--multi-photon entanglement and spin coherence extendable to microsecond timescales in the low-magnetic-field regime. Finally, photons from distant sources are as indistinguishable as photons emitted successively by a single source. These results establish foundry-compatible III--V quantum dots as a scalable platform for hybrid photonic quantum computing.

quant-ph↗

arXiv2025

Coupling 4H-Silicon Carbide spins to a microwave resonator at milli-Kelvin temperature

Coupling microwave cavity modes with spin qubit transitions is crucial for enabling efficient qubit readout and control, long-distance qubit coupling, quantum memory implementation, and entanglement generation. We experimentally observe the coupling of different spin qubit transitions in Silicon Carbide (SiC) material to a 3D microwave (MW resonator mode around 12.6~GHz at a temperature of 10~mK. Tuning the spin resonances across the cavity resonance via magnetic-field sweeps, we perform MW cavity transmission measurements. We observe spin transitions of different spin defects that are detuned from each other by around 60-70~MHz. By optically exciting the SiC sample placed in the MW cavity with an 810~nm laser, we observe the coupling of an additional spin resonance to the MW cavity, also detuned by around 60-70 MHz from the centre resonance. We perform complementary confocal optical spectroscopy as a function of temperature from 4~K to 200~K. Combining the confocal spectroscopy results and a detailed analysis of the MW-resonator-based experiments, we attribute the spin resonances to three different paramagnetic defects: positively-charged carbon antisite vacancy pair (CAV$^+$), and the negatively-charged silicon vacancy spins located at two different lattice sites, namely V$_1$ and V$_2$ spins. The V$_1$ and V$_2$ lines in SiC are interesting qubit transitions since they are known to be robust to decoherence. Additionally, the CAV$^+$-transition is known to be a bright single-photon source. Consequently, the demonstration of the joint coupling of these spin qubits to a MW cavity mode could lead to interesting new modalities: The microwave cavity could act as an information bus and mediate long-range coupling between the spins, with potential applications in quantum computing and quantum communication, which is an attractive proposition in a CMOS-compatible material such as SiC.

quant-ph↗

arXiv2024

Efficient fiber-pigtailed source of indistinguishable single photons

Semiconductor quantum dots in microcavities are an excellent platform for the efficient generation of indistinguishable single photons. However, their use in a wide range of quantum technologies requires their controlled fabrication and integration in compact closed-cycle cryocoolers, with a key challenge being the efficient and stable extraction of the single photons into a single-mode fiber. Here we report on a novel method for fiber-pigtailing of deterministically fabricated single-photon sources. Our technique allows for nanometer-scale alignment accuracy between the source and a fiber, alignment that persists all the way from room temperature to 2.4 K. We demonstrate high performance of the device under near-resonant optical excitation with g$^{(2)}$(0) = 1.3 %, a photon indistinguishability of 97.5 % and a fibered brightness of 20.8 %. We show that the indistinguishability and single-photon rate are stable for over ten hours of continuous operation in a single cooldown. We further confirm that the device performance is not degraded by nine successive cooldown-warmup cycles.

quant-ph↗

arXiv2024

Three-Dimensional and Selective Displacement Sensing of a Levitated Nanoparticle via Spatial Mode Decomposition

We propose and experimentally demonstrate a novel detection method that significantly improves the precision of real-time measurement of the three-dimensional displacement of a levitated dipolar scatterer. Our technique relies on spatial mode sorting of the light scattered by the levitated object, allowing us to selectively extract the position information of all translational degrees of freedom with minimal losses. To this end, we collect all the light back-scattered from a levitated nanoparticle using a parabolic mirror and couple it into a spatial mode sorter. We measure displacement sensitivities ($\sqrt{S_{\mathrm{imp}, x}}, \sqrt{S_{\mathrm{imp}, y}}, \sqrt{S_{\mathrm{imp}, z}}$) $=$ (1.7, 2.4, 1.0) $\times$ $10^{-14}$ m/$\sqrt{\mathrm{Hz}}$ below the zero-point motion ($x_{\mathrm{zpm}}, y_{\mathrm{zpm}}, z_{\mathrm{zpm}}$) $=$ (2.2, 2.4, 1.6) $\times$ $10^{-12}$ m of the levitated particle considered here. In the regime where environmental decoherence is not limited by gas collision we estimate that our method can reach measurement efficiencies of $(\eta_{^{\mathrm{tot}}}^{_{x}}, \eta_{^{\mathrm{tot}}}^{_{y}}, \eta_{^{\mathrm{tot}}}^{_{z}}) = (0.13, 0.18, 0.33) > 1/9$, which would enable the 3D motional quantum ground state of a levitated optomechanical system.

physics.optics↗

arXiv2023

Coupling nitrogen-vacancy centre spins in diamond to a grape dimer

Two grapes irradiated inside a microwave (MW) oven typically produce a series of sparks and can ignite a violent plasma. The underlying cause of the plasma has been attributed to the formation of morphological-dependent resonances (MDRs) in the aqueous dielectric dimers that lead to the generation of a strong evanescent MW hotspot between them. Previous experiments have focused on the electric-field component of the field as the driving force behind the plasma ignition. Here we couple an ensemble of nitrogen-vacancy (NV) spins in nanodiamonds (NDs) to the magnetic-field component of the dimer MW field. We demonstrate the efficient coupling of the NV spins to the MW magnetic-field hotspot formed between the grape dimers using Optically Detected Magnetic Resonance (ODMR). The ODMR measurements are performed by coupling NV spins in NDs to the evanescent MW fields of a copper wire. When placing a pair of grapes around the NDs and matching the ND position with the expected magnetic-field hotspot, we see an enhancement in the ODMR contrast by more than a factor of two compared to the measurements without grapes. Using finite-element modelling, we attribute our experimental observation of the field enhancement to the MW hotspot formation between the grape dimers. The present study not only validates previous work on understanding grape-dimer resonator geometries, but it also opens up a new avenue for exploring novel MW resonator designs for quantum technologies.

quant-ph↗

arXiv2023

Inert shell coating for enhanced laser refrigeration of nanoparticles: application in levitated optomechanics

We report on a study exploring the design of nanoparticles that can enhance their laser refrigeration efficiency for applications in levitated optomechanics. In particular, we developed lanthanide-doped nanocrystals with an inert shell coating and compared their performance with bare nanocrystals. While optically levitated, we studied the refrigeration of both types of nanoparticles while varying the pressure. We found that the core-shell design shows an improvement in the minimum final temperature: a fourth of the core-shell nanoparticles showed a significant cooling compared to almost none of the bare nanoparticles. Furthermore, we measured a core-shell nanoparticle cooling down to a temperature of 147 K at 26 mbar in the underdamped regime. Our study is a first step towards engineering nanoparticles that are suitable for achieving absolute (centre-of-mass and internal temperature) cooling in levitation, opening new avenues for force sensing and the realization of macroscopic quantum superpositions.

physics.optics↗

arXiv2022

Probing many-body correlations using quantum-cascade correlation spectroscopy

The radiative quantum cascade, i.e. the consecutive emission of photons from a ladder of energy levels, is of fundamental importance in quantum optics. For example, the two-photon cascaded emission from calcium atoms was used in pioneering experiments to test Bell inequalities. In solid-state quantum optics, the radiative biexciton-exciton cascade has proven useful to generate entangled-photon pairs. More recently, correlations and entanglement of microwave photons emitted from a two-photon cascaded process were measured using superconducting circuits. All these experiments rely on the highly non-linear nature of the underlying energy ladder, enabling direct excitation and probing of specific single-photon transitions. Here, we use exciton polaritons to explore the cascaded emission of photons in the regime where individual transitions of the ladder are not resolved, a regime that has not been addressed so far. We excite a polariton quantum cascade by off-resonant laser excitation and probe the emitted luminescence using a combination of spectral filtering and correlation spectroscopy. Remarkably, the measured photon-photon correlations exhibit a strong dependence on the polariton energy, and therefore on the underlying polaritonic interaction strength, with clear signatures from two- and three-body Feshbach resonances. Our experiment establishes photon-cascade correlation spectroscopy as a highly sensitive tool to provide valuable information about the underlying quantum properties of novel semiconductor materials and we predict its usefulness in view of studying many-body quantum phenomena.

quant-ph↗

arXiv2022

Structural and optical properties of micro-diamonds with SiV- color centers

Isolated, micro-meter sized diamonds are grown by micro-wave plasma chemical vapour deposition technique on Si(001) substrates. Each diamond is uniquely identified by markers milled in the Si substrate by Ga+ focused ion beam. The morphology and micrograin structure analysis indicates that the diamonds are icosahedral or bi-crystals. Icosahedral diamonds have higher (up to $\sigma_\mathrm{h}$ = 2.3 GPa), and wider distribution ($\Delta\sigma_\mathrm{h}$ = 4.47 GPa) of hydrostatic stress built up at the microcrystal grain boundaries, compared to the other crystals. The number and spectral shape of SiV- color centers incorporated in the micro-diamonds is analysed, and estimated by means of temperature dependent photoluminescence measurements, and Montecarlo simulations. The Montecarlo simulations indicate that the number of SiV- color centers is a few thousand per micro-diamond.

cond-mat.mtrl-sci↗

arXiv2022

Roadmap for Optical Tweezers

Optical tweezers are tools made of light that enable contactless pushing, trapping, and manipulation of objects ranging from atoms to space light sails. Since the pioneering work by Arthur Ashkin in the 1970s, optical tweezers have evolved into sophisticated instruments and have been employed in a broad range of applications in life sciences, physics, and engineering. These include accurate force and torque measurement at the femtonewton level, microrheology of complex fluids, single micro- and nanoparticle spectroscopy, single-cell analysis, and statistical-physics experiments. This roadmap provides insights into current investigations involving optical forces and optical tweezers from their theoretical foundations to designs and setups. It also offers perspectives for applications to a wide range of research fields, from biophysics to space exploration.

physics.optics↗

arXiv2021

Modified coherence of quantum spins in a damped pure-dephasing model

We consider a spin-$j$ particle coupled to a structured bath of bosonic modes that decay into thermal baths. We obtain an analytic expression for the reduced spin state and use it to investigate non-Markovian spin dynamics. In the heavily overdamped regime, spin coherences are preserved due to a quantum Zeno affect. We extend the solution to two spins and include coupling between the modes, which can be leveraged for preservation of the symmetric spin subspace. For many spins, we find that inter-mode coupling gives rise to a privileged symmetric mode gapped from the other modes. This provides a handle to selectively address that privileged mode for quantum control of the collective spin. Finally, we show that our solution applies to defects in solid-state systems, such as NV$^{-}$ centres in diamond.

quant-ph↗

arXiv2021

Absorptive laser threshold magnetometry: combining visible diamond Raman lasers and nitrogen-vacancy centres

We propose a high-sensitivity magnetometry scheme based on a diamond Raman laser with visible pump absorption by an ensemble of coherently microwave driven negatively charged nitrogen-vacancy centres (NV) in the same diamond crystal. The NV centres' absorption and emission are spin-dependent. We show how the varying absorption of the NV centres changes the Raman laser output. A shift in the diamond Raman laser threshold and output occurs with the external magnetic-field and microwave driving. We develop a theoretical framework including steady-state solutions to describe the effects of coherently driven NV centres in a diamond Raman laser. We discuss that such a laser working at the threshold can be employed for magnetic-field sensing. In contrast to previous studies on NV magnetometry with visible laser absorption, the laser threshold magnetometry method is expected to have low technical noise, due to low background light in the measurement signal. For magnetic-field sensing, we project a shot-noise limited DC sensitivity of a few $\mathrm{pT}/\sqrt{\mathrm{Hz}}$ in a well-calibrated cavity with realistic parameters. This sensor employs the broad visible absorption of NV centres and unlike previous laser threshold magnetometry proposals it does not rely on active NV centre lasing or an infrared laser medium at the specific wavelength of the NV centre's infrared absorption line.

quant-ph↗

arXiv2020

Exciton-exciton interaction beyond the hydrogenic picture in a MoSe$_2$ monolayer in the strong light-matter coupling regime

In transition metal dichalcogenides layers of atomic scale thickness, the electron-hole Coulomb interaction potential is strongly influenced by the sharp discontinuity of the dielectric function across the layer plane. This feature results in peculiar non-hydrogenic excitonic states, in which exciton-mediated optical nonlinearities are predicted to be enhanced as compared to their hydrogenic counterpart. To demonstrate this enhancement, we performed optical transmission spectroscopy of a MoSe$_2$ monolayer placed in the strong coupling regime with the mode of an optical microcavity, and analyzed the results quantitatively with a nonlinear input-output theory. We find an enhancement of both the exciton-exciton interaction and of the excitonic fermionic saturation with respect to realistic values expected in the hydrogenic picture. Such results demonstrate that unconventional excitons in MoSe$_2$ are highly favourable for the implementation of large exciton-mediated optical nonlinearities, potentially working up to room temperature.

cond-mat.mes-hall↗

arXiv2019

Amplification by stimulated emission of nitrogen vacancy centres in a diamond-loaded fibre cavity

Laser-threshold magetometry using the negatively charged nitrogen-vacancy (NV-) centre in diamond as a gain medium has been proposed as a technique to dramatically enhance the sensitivity of room-temperature magnetometry. We experimentally explore a diamond-loaded open tunable fibre-cavity system as a potential contender for the realization of lasing with NV- centres. We observe amplification of the transmission of a cavity-resonant seed laser at 721 nm when the cavity is pumped at 532 nm, and attribute this to stimulated emission. Changes in the intensity of spontaneously emitted photons accompany the amplification, and a qualitative model including stimulated emission and ionisation dynamics of the NV- centre captures the dynamics in the experiment very well. These results highlight important considerations in the realization of an NV- laser in diamond.

quant-ph↗

arXiv2019

Geometric pathway to scalable quantum sensing

Entangled resources enable quantum sensing that achieves Heisenberg scaling, a quadratic improvement on the standard quantum limit, but preparing large scale entangled states is challenging in the presence of decoherence. We present a quantum control strategy using highly nonlinear geometric phase gates for preparing entangled states on spin ensembles which can be used for practical precision metrology. The method uses a dispersive coupling of $N$ spins to a common bosonic mode and does not require addressability, special detunings, or interactions between the spins. Using a control sequence that executes Grover's algorithm on a subspace of permutationally symmetric states, a target entangled resource state can be prepared using $O(N^{5/4})$ geometric phase gates. The geometrically closed path of the control operations ensures the gates are insensitive to the initial state of the mode and the sequence has built-in dynamical decoupling providing resilience to dephasing errors.

quant-ph↗

arXiv2019

Ensemble-induced strong light-matter coupling of a single quantum emitter

We discuss a technique to strongly couple a single target quantum emitter to a cavity mode, which is enabled by virtual excitations of a nearby mesoscopic ensemble of emitters. A collective coupling of the latter to both the cavity and the target emitter induces strong photon non-linearities in addition to polariton formation, in contrast to common schemes for ensemble strong coupling. We demonstrate that strong coupling at the level of a single emitter can be engineered via coherent and dissipative dipolar interactions with the ensemble, and provide realistic parameters for a possible implementation with SiV$^{-}$ defects in diamond. Our scheme can find applications, amongst others, in quantum information processing or in the field of cavity-assisted quantum chemistry.

quant-ph↗

arXiv2018

Bayesian estimation of switching rates for blinking emitters

Single quantum light-emitters are valuable resources for engineered quantum systems. They can function as robust single-photon generators, allow optical control of single spins, provide readout capabilities for atomic-scale sensors, and provide interfaces between stationary and flying qubits. Environmental factors can lead to single emitters exhibiting "blinking", whereby the fluorescence level switches between on and off states. Detailed characterisation of this blinking behaviour including determining the switching rates is often a powerful way to gain understanding about the underlying physical mechanisms. While simple thresholds can be used to identify the on and off intervals and thus extract the rates from the time-series of counts for bright emitters with low background noise, such approaches become difficult for emitters fluorescing at low levels, high noise, or switching at fast rates. We develop a Bayesian approach capable of inferring switching rates directly from the time-series. This is able to deal with high levels of noise and fast switching in fluorescence traces. Moreover, the Bayesian inference also yields a robust picture of the parameter uncertainties, providing a benefit also for bright emitters in low-noise settings. The technique can be adapted to identify the underlying states as well as extracting the rates of switching. Finally, our method is applicable to a broad range of systems that show behaviour analogous to a single blinking emitter.

quant-ph↗

arXiv2017

Quantum-correlated photons from semiconductor cavity polaritons

Over the past decade, exciton-polaritons in semiconductor microcavities have attracted a great deal of interest as a driven-dissipative quantum fluid. These systems offer themselves as a versatile platform for performing Hamiltonian simulations with light, as well as for experimentally realizing nontrivial out-of-equilibrium phase transitions. In addition, polaritons exhibit a sizeable mutual interaction strength that opens up a whole range of possibilities in the context of quantum state generation. While squeezed light emission from polaritons has been reported previously, the granular nature of polaritons has not been observed to date. The latter capability is particularly attractive for realizing strongly correlated many-body quantum states of light on scalable arrays of coupled cavities. Here we demonstrate that by optically confining polaritons to a very small effective mode volume, one can reach the weak blockade regime, in which the nonlinearity turns strong enough to become significant at the few particle level, and thus produce a non-negligible antibunching in the emitted photons statistics. Our results act as a door opener for accessing the newly emerging field of quantum polaritonics, and as a proof of principle that optically confined exciton-polaritons can be considered as a realistic, new strategy to generate single photons.

cond-mat.mes-hall↗

arXiv2016

Observation of room-temperature spontaneous superradiance from single diamond nanocrystals

We report the observation of room-temperature superradiance from single, highly luminescent diamond nanocrystals with spatial dimensions much smaller than the wavelength of light, and each containing a large number (~10^3) of embedded nitrogen-vacancy (NV) centres. After excitation of the nanodiamonds with an off-resonant, green laser pulse, we observe i) ultrafast radiative lifetimes down to ~ 1 ns, and ii) super-Poissonian photon bunching in the autocorrelation function of the light emitted from the fastest nanodiamonds. We explain our findings with a detailed theoretical model based on collective Dicke states and well-known properties of NV centres. Using a minimal set of fit parameters, the model captures both the wide range of different lifetimes and the nontrivial photon correlations found in the experiments. The results pave the way towards a systematic study of superradiance in a well controlled, solid-state quantum system at room temperature. Ultimately, quantum engineering of superradiance in diamond has the potential for advancing applications in quantum sensing, energy harvesting, and efficient photon detection.

quant-ph↗