arXiv subjects

Thomas Weiss

Publications and source records attributed to Thomas Weiss.

30 records · Page 2Linked to original sources

arXiv2021

Watching a Single Fluorophore Molecule Walk into a Plasmonic Hotspot

Plasmonic nanoantennas allow for enhancing the spontaneous emission, altering the emission polarization, and shaping the radiation pattern of quantum emitters. A critical challenge for the experimental realizations is positioning a single emitter into the hotspot of a plasmonic antenna with nanoscale accuracy. We demonstrate a dynamic light-matter interaction nanosystem enabled by the DNA origami technique. A single fluorophore molecule can autonomously and unidirectionally walk into the hotspot of a plasmonic nanoantenna along a designated origami track. Successive fluorescence intensity increase and lifetime reduction are in situ monitored using single-molecule fluorescence spectroscopy, while the fluorophore walker gradually approaches and eventually enters the plasmonic hotspot. Our scheme offers a dynamic platform, which can be used to develop functional materials, investigate intriguing light-matter interaction phenomena, and serve as prototype system for examining theoretical models.

physics.optics↗

arXiv2021

Gold nanocrystal-mediated sliding of doublet DNA origami filaments

Sliding is one of the fundamental mechanical movements in machinery. In macroscopic systems, double-rack pinion machines employ gears to slide two linear tracks along opposite directions. In microscopic systems, kinesin-5 proteins crosslink and slide apart antiparallel microtubules, promoting spindle bipolarity and elongation during mitosis. Here we demonstrate an artificial nanoscopic analog, in which gold nanocrystals can mediate coordinated sliding of two antiparallel DNA origami filaments powered by DNA fuels. Stepwise and reversible sliding along opposite directions is in situ monitored and confirmed using fluorescence spectroscopy. A theoretical model including different energy transfer mechanisms is developed to understand the observed fluorescence dynamics. We further show that such sliding can also take place in the presence of multiple DNA sidelocks that are introduced to inhibit the relative movements. Our work enriches the toolbox of DNA-based nanomachinery, taking one step further toward the vision of molecular nanofactories.

physics.bio-ph↗

arXiv2021

DNA-assembled nanoarchitectures with multiple components in regulated and coordinated motion

Coordinating functional parts to operate in concert is essential for machinery. In gear trains, meshed gears are compactly interlocked, working together to impose rotation or translation. In photosynthetic systems, a variety of biological entities in the thylakoid membrane interact with each other, converting light energy into chemical energy. However, coordinating individual parts to carry out regulated and coordinated motion within an artificial nanoarchitecture poses challenges, owing to the requisite control on the nanoscale. Here, we demonstrate DNA-directed nanosystems, which comprise hierarchically-assembled DNA origami filaments, fluorophores, and gold nanocrystals. These individual building blocks can execute independent, synchronous, or joint motion upon external inputs. These are optically monitored in situ using fluorescence spectroscopy, taking advantage of the sensitive distance-dependent interactions between the gold nanocrystals and fluorophores positioned on the DNA origami. Our work leverages the complexity of DNA-based artificial nanosystems with tailored dynamic functionality, representing a viable route towards technomimetic nanomachinery.

physics.bio-ph↗

arXiv2021

Near surface defects: Cause of deficit between internal and external open-circuit voltage in solar cells

The presence of interface recombination in a complex multilayered thin-film solar structure causes a disparity between the internal open-circuit voltage (VOC,in), measured by photoluminescence, and the external open-circuit voltage (VOC,ex) i.e. an additional VOC deficit. Higher VOC,ex value aim require a comprehensive understanding of connection between VOC deficit and interface recombination. Here, a deep near-surface defect model at the absorber/buffer interface is developed for copper indium di-selenide solar cells grown under Cu excess conditions to explain the disparity between VOC,in and VOC,ex.. The model is based on experimental analysis of admittance spectroscopy and deep-level transient spectroscopy, which show the signature of deep acceptor defect. Further, temperature-dependent current-voltage measurements confirm the presence of near surface defects as the cause of interface recombination. The numerical simulations show strong decrease in the local VOC,in near the absorber/buffer interface leading to a VOC deficit in the device. This loss mechanism leads to interface recombination without a reduced interface bandgap or Fermi level pinning. Further, these findings demonstrate that the VOC,in measurements alone can be inconclusive and might conceal the information on interface recombination pathways, establishing the need for complementary techniques like temperature dependent current voltage measurements to identify the cause of interface recombination in the devices.

cond-mat.mtrl-sci↗

arXiv2020

All-dielectric silicon metalens for two-dimensional particle manipulation in optical tweezers

Dynamic control of compact chip-scale contactless manipulation of particles for bioscience applications remains a challenging endeavor, which is restrained by the balance between trapping efficiency and scalable apparatus. Metasurfaces offer the implementation of feasible optical tweezers on a planar platform for shaping the exerted optical force by a microscale-integrated device. Here, we design and experimentally demonstrate a highly efficient silicon-based metalens for two-dimensional optical trapping in the near-infrared. Our metalens concept is based on the Pancharatnam-Berry phase, which enables the device for polarization-sensitive particle manipulation. Our optical trapping setup is capable of adjusting the position of both the metasurface lens and the particle chamber freely in three directions, which offers great freedom for optical trap adjustment and alignment. Two-dimensional (2D) particle manipulation is done with a relatively low numerical aperture metalens ($NA_{ML}=0.6$). We experimentally demonstrate both 2D polarization sensitive drag and drop manipulation of polystyrene particles suspended in water and transfer of angular orbital momentum to these particles with a single tailored beam. Our work may open new possibilities for lab-on-a-chip optical trapping for bioscience applications and micro to nanoscale optical tweezers.

physics.optics↗

arXiv2019

Metasurface interferometry towards quantum sensors

Optical metasurfaces open new avenues for precise wavefront control of light for integrated quantum technology. Here, we demonstrate a hybrid integrated quantum photonic system that is capable to entangle and disentangle two-photon spin states at a dielectric metasurface. By interfering single-photon pairs at a nanostructured dielectric metasurface, a path-entangled two-photon NOON state with circular polarization is generated that exhibits a quantum HOM interference visibility of 86 $\pm$ 4%. Furthermore, we demonstrate nonclassicality and phase sensitivity in a metasurface-based interferometer with a fringe visibility of 86.8 $\pm$ 1.1 % in the coincidence counts. This high visibility proves the metasurface-induced path entanglement inside the interferometer. Our findings provide a promising way to hybrid-integrated quantum technology with high-dimensional functionalities in various applications like imaging, sensing, and computing.

physics.optics↗

arXiv2019

Multichannel vectorial holographic display and encryption

Since its invention, holography has emerged as a powerful tool to fully reconstruct the wavefronts of light including all the fundamental properties (amplitude, phase, polarization, wave vector, and frequency). For exploring the full capability for information storage/display and enhancing the encryption security of metasurface holograms, smart multiplexing techniques together with suitable metasurface designs are highly demanded. Here, we integrate multiple polarization manipulation channels for various spatial phase profiles into a single birefringent vectorial hologram by completely avoiding unwanted cross-talk. Multiple independent target phase profiles with quantified phase relations that can process significantly different information in different polarization states are realized within a single metasurface. For our metasurface holograms, we demonstrate high fidelity, large efficiency, broadband operation, and a total of twelve polarization channels. Such multichannel polarization multiplexing can be used for dynamic vectorial holographic display and can provide triple protection for optical security. The concept is appealing for applications of arbitrary spin to angular momentum conversion and various phase modulation/beam shaping elements.

physics.optics↗

arXiv2019

First-order perturbation theory for material changes in the surrounding of open optical resonators

The single-mode approximation of the resonant state expansion has proven to give accurate first-order approximations of resonance shifts and linewidth changes when modifying the material properties inside open optical resonators. Here, we extend this first-order perturbation theory to modifications of the material properties in the surrounding medium. As a side product of our derivations, we retrieve the already known analytical normalization condition for resonant states. We apply our theory to two example systems: A metallic nanosphere and a one-dimensional photonic crystal slab.

physics.optics↗

arXiv2017

Reflected Brownian motions in the KPZ universality class

This book presents a detailed study of a system of interacting Brownian motions in one dimension. The interaction is point-like such that the $n$-th Brownian motion is reflected from the Brownian motion with label $n-1$. This model belongs to the Kardar-Parisi-Zhang (KPZ) universality class. In fact, because of the singular interaction, many universal properties can be established with rigor. They depend on the choice of initial conditions. Discussion addresses packed and periodic initial conditions, stationary initial conditions, and mixtures thereof. The suitably scaled spatial process will be proven to converge to an Airy process in the long time limit. A chapter on determinantal random fields and another one on Airy processes are added to have the notes self-contained. This book serves as an introduction to the KPZ universality class, illustrating the main concepts by means of a single model only. It will be of interest to readers from interacting diffusion processes and non-equilibrium statistical mechanics.

math-ph↗

arXiv2015

Scaling limit for Brownian motions with one-sided collisions

We consider Brownian motions with one-sided collisions, meaning that each particle is reflected at its right neighbour. For a finite number of particles a Schütz-type formula is derived for the transition probability. We investigate an infinite system with periodic initial configuration, that is, particles are located at the integer lattice at time zero. The joint distribution of the positions of a finite subset of particles is expressed as a Fredholm determinant with a kernel defining a signed determinantal point process. In the appropriate large time scaling limit, the fluctuations in the particle positions are described by the Airy$_1$ process.

math-ph↗

arXiv2015

Polarization control of quantum dot emission by chiral photonic crystal slabs

We investigate theoretically the polarization properties of the quantum dot's optical emission from chiral photonic crystal structures made of achiral materials in the absence of external magnetic field at room temperature. The mirror symmetry of the local electromagnetic field is broken in this system due to the decreased symmetry of the chiral modulated layer. As a result, the radiation of randomly polarized quantum dots normal to the structure becomes partially circularly polarized. The sign and degree of circular polarization are determined by the geometry of the chiral modulated structure and depend on the radiation frequency. A degree of circular polarization up to 99% can be achieved for randomly distributed quantum dots, and can be close to 100% for some single quantum dots.

physics.optics↗

arXiv2015

Brownian Motions with One-Sided Collisions: The Stationary Case

We consider an infinite system of Brownian motions which interact through a given Brownian motion being reflected from its left neighbor. Earlier we studied this system for deterministic periodic initial configurations. In this contribution we consider initial configurations distributed according to a Poisson point process with constant intensity, which makes the process space-time stationary. We prove convergence to the Airy process for stationary the case. As a byproduct we obtain a novel representation of the finite-dimensional distributions of this process. Our method differs from the one used for the TASEP and the KPZ equation by removing the initial step only after the limit $t\to\infty$. This leads to a new universal cross-over process.

math-ph↗