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Thomas Zanon-Willette

Publications and source records attributed to Thomas Zanon-Willette.

13 recordsLinked to original sources

Magic-wavelength matter-wave interferometry with optical clock states

Optical clocks and atom interferometers provide complementary ways to measure time, motion and gravity. Combining these capabilities requires matter-wave beam splitters that manipulate different clock states in the same way, so that optical internal energy becomes a controlled degree of freedom rather than a source of systematic phase shifts. Here we realized a dual matter-wave interferometer operating simultaneously on the two states of the $^{88}$Sr optical clock transition, $^1S_0$ and $^3P_0$. The interferometer is driven by Bragg pulses at the 813 nm magic wavelength, for which the two clock states experience the same optical coupling strength. This realizes a common matter-wave beam splitter for atoms whose internal energies differ by an optical excitation. With a sensitivity of 30 mrad, our measurement is consistent with a zero differential phase shift between the two clock-state Mach-Zehnder interferometers, translating to an absence of state-dependent acceleration in free fall at the level of $10^{-5}$. We further used the same interferometer to measure state-dependent optical dipole forces and determine a tune-out wavelength of the metastable $^3P_0$ state to be 478.95(8) nm. These results establish magic-wavelength clock-state interferometry as a platform for differential force sensing, excited-state polarizability metrology and future quantum-clock tests of gravity.

physics.atom-ph

Ramsey Interferometry in Wigner-Majorana Qudits

Ramsey interferometry estimates a detuning from the phase accumulated between two interaction zones, with a resolution set by the interrogation time $τ$. We propose a single-qudit extension based on Wigner-Majorana (WM) spin-$j$ dynamics, whose internal levels form a multipath interferometer. The enhancement is not generic: ideal $\mathrm{QFT}_D$ and $\sqrt{X_D}$ sequences do not densify the central fringe under the population readouts considered. Instead, in manifolds that realize the WM coupling, it arises from coherences between separated ladder states created and recombined by a single near-resonant drive per Ramsey zone. For the qutrit, preparing the central state of a spin-1 WM manifold and measuring its return probability gives $P_3(Δ)=\cos^2(Δτ)$, versus the qubit $P_2(Δ)=\cos^2(Δτ/2)$. The central fringe is thus compressed twofold at fixed $τ$ and the maximal slope doubled in the ideal limit, with contrast ideally unity. For higher-dimensional WM manifolds (odd and even $D$) the central response sharpens with dimension, but the signal spreads over several channels; we introduce a scalar readout from nearest-neighbor shoulder populations and quantify the resolution-contrast trade-off via the slope $S_D$ and contrast $C_D$. We also study robustness to diagonal phase noise from probe-shift fluctuations: under projector-type common-mode dephasing, the WM readouts are less contrast-sensitive than the qubit readout. The robustness is symmetry-selective, not universal: for linear Zeeman dephasing ($L=J_z$), the large $m$-separation that compresses the fringe also enhances dephasing, so higher-dimensional readouts become more sensitive, not protected. The WM qutrit is thus a practical operating point for enhanced Ramsey spectroscopy at fixed $τ$; higher qudits trade extra slope for reduced contrast.

quant-ph

Dark state role in time-reversal symmetry breaking

We investigate the role of the global driving phase $Φ$ in the dynamics of driven few-level quantum systems, a central setting in coherent control of atomic, molecular, and solid-state platforms. In particular, we focus on systems with closed-loop couplings, where external driving fields induce interference effects that strongly influence population transfer and symmetry properties of time-evolution. While full time-reversal symmetry requires $Φ=0,π$, leading to a real Hamiltonian, we focus on a less restrictive transformation, the phase inversion (or complex conjugation of the Hamiltonian), under which population dynamics can remain symmetric even though coherences generally do not. We show that the presence of a dark (spectator) state is a sufficient condition for this population phase symmetry (P$Φ$S), as it constrains the dynamics to reduced subspaces characterized by SU(2) or open-loop SU(3) evolution. We analyze this mechanism in three- and four-level systems and derive general conditions for P$Φ$S that extend to generic $n$-level configurations, with $n$ even. These findings provide practical guidelines for achieving robust control in quantum systems, with potential applications in quantum information processing and quantum computing.

quant-ph

Experimental realization of a SU(3) color-orbit coupling in an ultracold gas

Spin-orbit interaction couples the spin of a particle to its motion and leads to spin-induced transport phenomena such as spin-Hall effects and Chern insulators. In this work, we extend the concept of internal-external state coupling to higher internal symmetry, exploring features beyond the established spin-orbit regime. We couple suitable resonant laser beams to a gas of ultracold atoms, thereby inducing artificial SU(3) non-Abelian gauge fields that act on a degenerate ground state manifold comprised of three dark states. We demonstrate the inherent all-state connectivity of SU(3) systems by performing targeted geometric transformations. Then, we investigate color-orbit coupling, an extension of SU(2) spin-orbit coupling to SU(3) systems. We reveal a rich dynamical interplay between three distinct oscillation frequencies, which possesses interesting analogies with neutrino oscillations and quark mixing mechanisms. In the future, the system should provide a testbed for exploring topological properties of SU(3) systems.

physics.atom-ph

Bi-color atomic beam slower and magnetic field compensation for ultracold gases

Transversely loaded bidimensional-magneto-optical-traps (2D-MOT) have been recently developed as high flux sources for cold strontium atoms to realize a new generation of compact experimental setups. Here, we discuss on the implementation of a cross-polarized bi-color slower for a strontium atomic beam improving the 2D-MOT loading, and increasing the number of atoms in a final MOT by eleven times. Our slowing scheme addresses simultaneously two excited Zeeman substates of the 88Sr 1S0->1P1 transition at 461 nm. We also realized a 3-axis active feedback control of the magnetic field down to the microgauss regime. Such a compensation is performed thanks to a network of eight magnetic field probes arranged in a cuboid configuration around the atomic cold sample, and a pair of coils in Helmholtz configuration along each of three Cartesian directions. Our active feedback is capable of efficiently suppressing most of the magnetically-induced position fluctuations of the 689~nm intercombination-line MOT.

physics.atom-ph

Harmonic fine tuning and triaxial spatial anisotropy of dressed atomic spins

The addition of a weak oscillating field modifying strongly dressed spins enhances and enriches the system quantum dynamics. Through low-order harmonic mixing the bichromatic driving generates additional rectified static field acting on the spin system. The secondary field allows for a fine tuning of the atomic response and produces effects not accessible with a single dressing field, such as a spatial triaxial anisotropy of the spin coupling constants and acceleration of the spin dynamics. This tuning-dressed configuration introduces an extra handle for the system full engineering for quantum control applications. Tuning amplitude, harmonic content, spatial orientation and phase relation are control parameters. A theoretical analysis, based on perturbative approach, is experimentally validated by applying a bichromatic radiofrequency field to an optically pumped Cs atomic vapour. We measure the resonance shifts produced by tuning fields up to the third harmonic.

quant-ph

Generalized hyper-Ramsey resonance with spinors

The generalized hyper-Ramsey resonance formula originally published in Phys. Rev. A vol 92, 023416 (2015) is derived using a Cayley-Klein spinor parametrization. The shape of the interferometric resonance and the associated composite phase-shift are reformulated including all individual laser pulse parameters. Potential robustness of signal contrast and phase-shift of the wave-function fringe pattern can now be arbitrarily explored tracking any shape distortion due to systematic effects from the probe laser. An exact and simple analytical expression describing a Ramsey's method of separated composite oscillating laser fields with quantum state control allows us to accurately simulate all recent clock interrogation protocols under various pulse defects.

physics.atom-ph

Progress and perspectives on composite laser-pulses spectroscopy for high-accuracy optical clocks

Probing an atomic resonance without disturbing it is an ubiquitous issue in physics. This problem is critical in high-accuracy spectroscopy or for the next generation of atomic optical clocks. Ultra-high resolution frequency metrology requires sophisticated interrogation schemes and robust protocols handling pulse length errors and residual frequency detuning offsets . This review reports recent progress and perspective in such schemes, using sequences of composite laser-pulses tailored in pulse duration, frequency and phase, inspired by NMR techniques and quantum information processing. After a short presentation of Rabi technique and NMR-like composite pulses allowing efficient compensation of electromagnetic field perturbations to achieve robust population transfers, composite laser-pulses are investigated within Ramsey's method of separated oscillating fields in order to generate non-linear compensation of probe-induced frequency shifts. Laser-pulses protocols such as Hyper-Ramsey (HR), Modified Hyper-Ramsey (MHR), Generalized Hyper-Ramsey (GHR) and hybrid schemes are reviewed. These techniques provide excellent protection against both probe induced light-shift perturbations and laser intensity variations. More sophisticated schemes generating synthetic frequency-shifts are presented. They allow to reduce or completely eliminate imperfect correction of probe-induced frequency-shifts even in presence of decoherence due to the laser line-width. Finally, two universal protocols are presented which provide complete elimination of probe-induced frequency shifts in the general case where both decoherence and relaxation dissipation effects are present by using exact analytic expressions for phase-shifts and the clock frequency detuning. These techniques might be applied to atomic, molecular and nuclear frequency metrology, mass spectrometry as well as precision spectroscopy.

physics.atom-ph

First pressure shift measurement of ozone molecular lines at 9.54 $μ$m using a tunable quantum cascade laser

Using a free-running distributed-feedback quantum cascade laser (QCL) emitting at 9.54 $μ$m, the pressure shift parameters of four intense rovibrational transitions in the $ν_3$ fundamental band of ozone induced by oxygen (O$_2$), air and the noble gases helium (He), argon (Ar), and xenon (Xe) are obtained by employing second harmonic detection. The experimental analysis comprises a full uncertainty budget and provides line shift data which are traceable to SI. The high density of transitions in the $ν_3$ spectral region of ozone make this region particularly difficult to study with more commonly used techniques such as Fourier transform spectroscopy. The comparatively high spectral resolution of the QCL in the MHz range, on the contrary, allows to measure molecular shifts at relatively low pressures (from 2 to 70 hPa), thus reducing the impact of spectral congestion due to pressure broadening of molecular lines. The comparison of our results with published data shows that presently recommended values for the pressure shift are too low in this region. This observation is corroborated by semi-classical calculations using the Robert-Bonamy formalism. A slight negative $J$ dependence, already observed in other ozone vibrational bands, is predicted. Systematic use of our technique could be very useful to support this hypothesis and to make up for the lack of shift parameters for ozone $ν_3$ transitions in molecular spectral databases. A subsequent stabilization of the QCL onto an optical frequency comb will open up possibilities to perform metrological measurements of Doppler-free molecular lines.

physics.atom-ph

Probe light-shift elimination in Generalized Hyper-Ramsey quantum clocks

We present a new interrogation scheme for the next generation of quantum clocks to suppress frequency-shifts induced by laser probing fields themselves based on Generalized Hyper-Ramsey resonances. Sequences of composite laser pulses with specific selection of phases, frequency detunings and durations are combined to generate a very efficient and robust frequency locking signal with almost a perfect elimination of the light-shift from off resonant states and to decouple the unperturbed frequency measurement from the laser's intensity. The frequency lock point generated from synthesized error signals using either $π/4$ or $3π/4$ laser phase-steps during the intermediate pulse is tightly protected against large laser pulse area variations and errors in potentially applied frequency shift compensations. Quantum clocks based on weakly allowed or completely forbidden optical transitions in atoms, ions, molecules and nuclei will benefit from these hyper-stable laser frequency stabilization schemes to reach relative accuracies below the 10$^{-18}$ level.

physics.atom-ph

Continued fraction analysis of dressed systems: application to periodically driven optical lattices

Radio-frequency quantum engineering of spins is based on the dressing by a non resonant electromagnetic field. Radio-frequency dressing occurs also for the motion of particles, electrons or ultracold atoms, within a periodic spatial potential. The dressing, producing a renormalisation and also a freeze of the system energy, is described by different approaches, dressed atom, magnetic resonance semiclassical treatment, continued fraction solution of the Schrödinger equation. A comparison between those solutions points out that the semiclassical treatment, to be denoted as the $S$-solution, represents the most convenient tool to evaluate the tunneling renormalization of ultracold atoms.

physics.atom-ph

Magic radio-frequency dressing of nuclear spins in high-accuracy optical clocks

A Zeeman-insensitive optical clock atomic transition is engineered when nuclear spins are dressed by a non resonant radio-frequency field. For fermionic species as $^{87}$Sr, $^{171}$Yb, and $^{199}$Hg, particular ratios between the radiofrequency driving amplitude and frequency lead to "magic" magnetic values where a net cancelation of the Zeeman clock shift and a complete reduction of first order magnetic variations are produced within a relative uncertainty below the $10^{-18}$ level. An Autler-Townes continued fraction describing a semi-classical radio-frequency dressed spin is numerically computed and compared to an analytical quantum description including higher order magnetic field corrections to the dressed energies.

physics.atom-ph

Nuclear Spin Effects in Optical Lattice Clocks

We present a detailed experimental and theoretical study of the effect of nuclear spin on the performance of optical lattice clocks. With a state-mixing theory including spin-orbit and hyperfine interactions, we describe the origin of the $^1S_0$-$^3P_0$ clock transition and the differential g-factor between the two clock states for alkaline-earth(-like) atoms, using $^{87}$Sr as an example. Clock frequency shifts due to magnetic and optical fields are discussed with an emphasis on those relating to nuclear structure. An experimental determination of the differential g-factor in $^{87}$Sr is performed and is in good agreement with theory. The magnitude of the tensor light shift on the clock states is also explored experimentally. State specific measurements with controlled nuclear spin polarization are discussed as a method to reduce the nuclear spin-related systematic effects to below 10$^{-17}$ in lattice clocks.

physics.atom-ph